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At least 847 records · Page 47

Updates to the Regional Seismic Travel Time (RSTT) Model: 1. Tomography

Abstract A function of global monitoring of nuclear explosions is the development of Earth models for predicting seismic travel times for more accurate calculation of event locations. Most monitoring agencies rely on fast, distance-dependent one-dimensional (1D) Earth models to calculate seismic event locations quickly and in near real-time. RSTT (Regional Seismic Travel Time) is a seismic velocity model and computer software package that captures the major effects of three-dimensional crust and upper mantle structure on regional seismic travel times, while still allowing for fast prediction speed (milliseconds). We describe updates to the RSTT model using a refined data set of regional phases (i.e., Pn, Pg, Sn, Lg) using the Bayesloc relative relocation algorithm. The tomographic inversion shown here acts to refine the previous RSTT public model ( rstt201404um ) and displays significant features related to areas of global tectonic complexity as well as further reduction in arrival residual values. Validation of the updated RSTT model demonstrates significant reduction in median epicenter mislocation (15.3 km) using all regional phases compared to the iasp91 1D model (22.1 km) as well as to the current station correction approach used at the Comprehensive Nuclear-Test-Ban Treaty Organization International Data Centre (18.9 km).

58 GEOSCIENCES↗

Nuclear two point correlation functions on a quantum computer

The calculation of dynamic response functions is expected to be an early application benefiting from rapidly developing quantum hardware resources. The ability to calculate real-time quantities of strongly correlated quantum systems is one of the most exciting applications that can easily reach beyond the capabilities of traditional classical hardware. Response functions of fermionic systems at moderate momenta and energies corresponding roughly to the Fermi energy of the system are a potential early application because the relevant operators are nearly local, and the energies can be resolved in moderately short real time, reducing the spatial resolution and gate depth required. This is particularly the case in quasielastic electron and neutrino scattering from nuclei, a topic of great interest in the nuclear and particle physics communities and directly related to experiments designed to probe neutrino properties. In this paper we use current quantum hardware and error mitigation protocols to calculate response functions for a highly simplified nuclear model through calculations of a 2-point real time correlation function for a modified Fermi-Hubbard model in two dimensions with three distinguishable nucleons on four lattice sites.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Thermochemistry of Aerospace Materials

The reliability and development of aerospace materials in extreme environments relies on a comprehensive understanding of their thermochemical properties. Such properties are commonly used for equilibrium phase stability calculations of interactions with corrosive environments at very high temperatures. These calculations can lead to in-depth understanding of degradation mechanisms in both coatings and components for applications such as nuclear thermal propulsion and gas turbine engines, both of which are part of NASA’s current R&D focus for improving propulsion systems for aerospace missions. The first part of this talk summarizes and discuss our current thermochemical calculations of the behavior of ceramic-ceramic (cercer) UN-based fuels and their coating systems during nuclear thermal rocket operation. The second part of the talk summarizes and discuss the energetics of reactions of ceramic coating materials and their binary oxide components with silicate melts measured by high temperature reaction calorimetry.

Nuclear Thermal propulsion↗

Feasibility of Pulsed Current Technology for Removing Bulk Carbon from TRISO-based Fuels

The work described in this report has evaluated the technical feasibility of maturing the pulsed current technology and its full-scale application to processing TRISO used nuclear fuel. No insurmountable technological or safety barriers were identified to successfully maturing the technology to the fourth TRL, which was considered appropriate for a DOE-NE program. The authors recommend DOE-NE’s Nuclear Fuel Cycle and Supply Chain Office should pursue the technology on that basis. In the immediate future, the authors recommend DOE-NE’s Nuclear Fuel Cycle and Supply Chain Office should acquire non-radioactive surrogate and natural uranium TRISO compacts and pebbles as they become available from commercial vendors. These surrogates could then be used to mature the pulsed current technology.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Evaluation of Physical Security Risk for Potential Implementation of FLEX using Dynamic Simulation Methods

The requirements for United States nuclear power plants to maintain a large onsite physical security force contribute to their large operational costs. The cost of maintaining the current physical security posture is approximately 10% of the overall operation and maintenance budget for commercial nuclear power plants. The goal of the Light Water Reactor Sustainability Program Physical Security Pathway is to develop tools, methods, and technologies and provide the technical basis for an optimized physical security posture. This pathway will analyze and minimize the conservatisms built into current security postures in order to reduce security costs while still ensuring adequate security and operational safety. The research performed at Idaho National Laboratory within this pathway has successfully developed a dynamic force-on-force (FOF) modeling framework using various computer simulation tools and integrated them with the dynamic assessment Event Modeling Risk Assessment using Linked Diagrams (EMRALD) tool. This document provides an overview of lessons learned in applying a dynamic computational framework that links results from a commercially available FOF simulation tool, a commercially available thermal-hydraulic tool, and EMRALD to an operating commercial nuclear power plant. This process of including plant procedures and multiple analysis results is being called Modeling and Analysis for Safety Security using Dynamic EMRALD Framework. Previous reports described how a user could integrate their plant-specific FOF models with the dynamic simulation tool EMRALD, model operator actions, integrate with probabilistic risk assessment tools, such as Computer Aided Fault Tree Analysis System or Systems Analysis Programs for Hands-on Integrated Reliability Evaluations, and with thermal-hydraulic tools, such as RELAP-5. Previous reports applied various combinations of available simulations codes with EMRALD using generic plant models to demonstrate how to perform the analysis. This report documents the results of applying the dynamic computational framework to an actual nuclear facility using their security scenarios and timelines. The purpose of this study was to verify that results achieved using generic models are similar to actual plant results and to refine our guidance of the use of the framework. Such an assessment enables further analysis, such as what-if scenarios and staff-reduction evaluation, thereby optimizing physical security at plants. NOTE: The work performed in this report is based on a generic EMRALD model with actual plant data used for the analysis. However, only the generic model and general results of the analysis are in the report. No plant’s sensitive information is discussed in this report. The discussion shows examples of insights that can be obtained from the MASS-DEF methodology.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

MECHANISTIC MULTIPHYSICS MODELING OF CLADDING RUPTURE IN NUCLEAR FUEL RODS DURING LOSS-OF-COOLANT ACCIDENT CONDITIONS

The Loss of Coolant Accident (LOCA) is a design basis accident that is included as part of the safety analysis of nuclear power plants. As the nuclear industry desires to increase the cycle length and discharge burnup of existing nuclear power plants they must demonstrate safe operation during a LOCA on high burnup fuel. During a LOCA transient on high burnup fuel rods, the rods may undergo a process known as fuel fragmentation, relocation, and dispersal (FFRD). To permit dispersal, the cladding encapsulating the fuel must rupture with an opening size large enough to allow the fragmented fuel particles to release. Current licensing tools used by industry and the United States Nuclear Regulatory Commission are limited in geometric fidelity and materials that can be analyzed. These simulation tools generally employ a quasi-two-dimensional (1.5D or Layered1D) or 2D-RZ axisymmetric geometric representations exclusively. While a valid approach under some instances, there are times when important physics have an asymmetric behavior in the fuel rod. Examples include fuel fragmentation, thermal-hydraulic boundary conditions, and cladding rupture, all of which are important for LOCA analysis. As industry pursues burnup extensions it must be demonstrated that fuel dispersal can be mitigated or eliminated. To do this, an understanding of the rupture opening after cladding failure is required. This work presents the development of a model for predicting the size and location of the rupture opening in failed fuel rods during LOCA conditions using advanced modeling and simulation tools. In order to supply the rupture model with appropriate boundary conditions, improvements to fuel fragmentation, axial relocation and oxidation modeling were required. First, the eXtended Finite Element Method (XFEM) is used to mechanistically predict the number of fuel fragments that form due to material strength randomization, criteria for strength randomization, mesh density, power ramping rates and irradiation effects. These predictions with associated uncertainty were compared to empirical correlations developed for UO2 verifying that they can be used with increased confidence in subsequent axial relocation analyses. Secondly, a new first-of-its-kind Layered2D computational framework was developed that provides the ability to apply azimuthally varying boundary conditions while providing discrete layers to track fuel movement during the LOCA. An existing fuel axial relocation model developed for Layered1D was extended to work within the Layered2D framework. A large sensitivity study was performed on the initial version of the model to identify modeling parameters of particular importance, with the emissivity used for radiation after blowdown being the primary source of uncertainty. Then, a simplistic approach to incorporate mechanical degradation of the cladding due to oxidation was also developed to investigate the impact of reduced cladding thickness on predictions of the time to failure of cladding tubes. It was found that the cladding will typically rupture prior to a reduction in thickness that is sufficient to impact the rupture behavior. A model was then developed for predicting cladding rupture that transfers the cladding surface temperatures, rod internal and external pressures, fast neutron fluence, and fast neutron flux from a more detailed Layered1D, Layered2D, or 2D-RZ analysis to a 3D cladding only analysis. Comparisons of the rupture model to a few experiments indicate reasonable predictions. The rupture model was then applied to two accident tolerant fuel concepts (FeCrAl and Cr-coated Zircaloy) where it predicted that both ATF concepts would have smaller rupture openings and delayed rupture times than the standard Zircaloy-4 cladding material under identical loading conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

An Approach to Automate tools for the Risk Assessment of Digital Instrumentation and Control Systems

Reliable digital instrumentation and control systems (DI&C) are integral for sustaining the continued operation of nuclear power plants. These systems ensure that nuclear reactors operate safely, efficiently, and within regulatory requirements. Yet, the cost of designing and licensing new nuclear DI&C can be prohibitively expensive. Under the U.S. Department of Energy Light Water Reactor Sustainability Program, Idaho National Laboratory has developed a framework for supporting the risk-informed design of DI&C systems by offering methods to support the identification, quantification, and evaluation of risks for various DI&C design architectures. The framework indicates potential software failure modes and provides pathways for quantifying the potential for these software failures, including common cause failures. Using the framework’s systematic approach, challenges for assessing risks within new and existing nuclear DI&C systems can be reduced. Nevertheless, the current framework can be further improved using the convenience of automation. This paper introduces the development of Software for the Hazard Identification and Evaluation of Digital Systems (SHIELDS). SHIELDS is an engineering software package that enables the identification, elimination, and mitigation of potential risks and reduces the burden of deploying reliable DI&C systems. This work introduces plans and techniques to digitize and improve the manual risk assessment modules of the framework. These improvements will save time and increase the repeatability and usability of the framework, making it more accessible to a wider range of users. Ultimately, this introduces SHIELDS and how its modules support efficient development of safe and reliable DI&C systems.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

First Phase Consensus Roadmap for Development of Condition-Based Cable Reliability Assurance

The objective of this work was to develop a first phase consensus roadmap for condition-based qualification (CBQ) of electrical cables. With CBQ, qualification of Class 1E electrical cables moves from a time-based approach to a condition-based approach, which is anticipated to be safer in terms of reliability and conservatism, and more cost effective in the long run. However, due to barriers, the CBQ approach has not yet been adopted by U.S. nuclear power plants (NPPs). Based upon a review of current work evaluating CBQ, the limitation of available condition monitoring technology seems to be the largest barrier. The importance of condition monitoring, or more specifically selecting appropriate condition indicators, during CBQ cannot be understated. However, selecting appropriate condition indicators is challenged by techniques that are destructive and only evaluate cable degradation locally. Further, arguably, no one identified condition indicator fully establishes cable condition. Thus, additional work is necessary to evaluate potential condition indicators towards CBQ. In addition to the requirements of IEC/IEEE Std. 60780-323, ideal condition indicators should include a) both destructive and non-destructive approaches, b) both local and global measurements, c) real-time (i.e., online) monitoring that trends with degradation, d) enable correlation with qualified levels of degradation, and e) be established within a repository of condition indicators with applicable materials and/or components and their acceptance criteria. Additional work is needed in development of technology and methodology prior to adoption of CBQ, especially for extending qualified life of installed components. Education and early experience by the industry and regulators will be required for this change in approach as an alternative to re-analysis. A series of workshops that bring together stakeholders to identify and address gaps will be needed. The longstanding cooperative working group of cable researchers from the U.S. Department of Energy, the Electric Power Research Institute, and the Nuclear Regulatory Commission forms a valuable starting point for development of a consensus roadmap to condition-based qualification approach as a viable options for qualification of cable systems in U.S. light water reactors.

42 ENGINEERING↗

Structural Materials and Fuels for Space Power Plants

A fission reactor combined with Stirling convertor power generation is one promising candidate in on-going Fission Surface Power (FSP) studies for future lunar and Martian bases. There are many challenges for designing and qualifying space-rated nuclear power plants. In order to have an affordable and sustainable program, NASA and DOE designers want to build upon the extensive foundation in nuclear fuels and structural materials. This talk will outline the current Fission Surface Power program and outline baseline design options for a lunar power plant with an emphasis on materials challenges. NASA first organized an Affordable Fission Surface Power System Study Team to establish a reference design that could be scrutinized for technical and fiscal feasibility. Previous papers and presentations have discussed this study process in detail. Considerations for the reference design included that no significant nuclear technology, fuels, or material development were required for near term use. The desire was to build upon terrestrial-derived reactor technology including conventional fuels and materials. Here we will present an overview of the reference design, Figure 1, and examine the materials choices. The system definition included analysis and recommendations for power level and life, plant configuration, shielding approach, reactor type, and power conversion type. It is important to note that this is just one concept undergoing refinement. The design team, however, understands that materials selection and improvement must be an integral part of the system development.

Bowman, Cheryl↗

Survey of Advanced Generation IV Reactor Parameters for Integrated Energy System Modeling Capabilities

This paper is to categorize and characterize advanced Generation IV nuclear reactors that are not water based according to the key parameters for the Integrated Energy Systems (IES) project[1]. A key goal of the IES project is to assess the economic viability of including an advanced nuclear reactor into an IES. The landscape of advanced reactors is heterogeneous: several unique designs with different heat profiles are currently being studied and designed. This report provides a high-level perspective of advanced reactor concepts, including primary loop nuclear output temperatures and operation schemes that could affect secondary side power production or storage. For example, this report addresses the type of thermodynamic system (Brayton, supercritical CO 2 [S-CO 2 ], etc.) and the various pressures and temperatures on the secondary side that are expected to be provided by the various primary side reactor types. Based on these characteristics, it may be possible to determine which type of nuclear power plant could be the most economical for analysis in the IES framework for power production coupled with energy storage and waste heat utilization. The results of this effort will serve as input for model development of various secondary side components, concentrating on off-the-shelf capabilities for current and near future secondary side power generation and heat rejection as simulated in TRANSFORM. Generic models can be created which are agnostic of the nuclear energy supply without violating intellectual property rights of the developer. These models can be used to make informed decisions on the economics of integrating various energy system components with nuclear plant designs. Once complete, conclusions may be drawn regarding (1) the economics, efficiency, and reliability of certain nuclear reactors, (2) certain industry processes and energy storage systems, and (3) prioritization of certain reactor types with the studied industry types.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Passive Temperature Sensors for Nuclear Applications

Thermocouples are generally used to provide real-time temperature indications in instrumented tests performed at material and test reactors. Passive temperature monitors, such as Silicon Carbide (SiC) and melt wires, may be included in such tests as an independent technique of detecting peak temperatures experienced during irradiation. In less expensive static (drop-in) capsule tests, which have no leads attached for real-time data transmission, melt wires, and SiC temperature monitors (TMs) are essentially the only possibility for peak temperature indication. A melt wire involves placing materials (wires) of a known composition and melting temperature in a test. An inventory is maintained at Material Science Laboratory (MSL) for melt wires ranging in temperatures from 30°C to 1500°C. Unfortunately, melt wires are limited in that it can only detect whether a single temperature is or is not exceeded (melt wire melted or not). SiC TMs, which can also be used to detect peak irradiation temperatures, are advantageous because a single monitor can allow to determine the peak temperature reached within a relatively broad range (100 – 1200°C) resulting in accuracies within ±20°C. Irradiation temperature is determined by measuring a property change after isochronal annealing or during a continuously monitored annealing process using specialized equipment at MSL. Recent research has produced a passive monitor known as sublime temperature monitor. This passive sensor has the capability of recording temperature gradients and pinpointing exactly where a temperature is located along that gradient. Long measurement lengths are achieved with very high accuracy in the location of desired temperature measurements (±2 mm over a 1 m span); however, this sensor has not been deployed in a nuclear reactor. This article will focus only on passive temperature sensors currently being researched and implemented under the Advanced Sensors and Instrumentation (ASI) program at Idaho National Laboratory (INL).

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Density functional theory calculations of the mixing enthalpy of ternary uranium carbide compounds

The high melting point of uranium-zirconium carbides (U,Zr)C makes them an ideal fuel for nuclear thermal propulsion (NTP) reactors. Gaps remain in the current understanding of the U-Zr-C system due to the difficulty of conducting thermodynamic experiments at NTP operation conditions. Density functional theory calculations using the Hubbard U model (DFT+U) were performed using orbital matrix occupation (OMC) to obtain the mixing enthalpy for UC and ZrC for (U,Zr)C ternary compounds. Similarly, DFT+U calculations were also carried out for the (U,Nb)C and (U,Ta)C systems. In conclusion, the DFT results are envisioned to be used in thermodynamic assessments of the uranium carbide systems based on the CALPHAD approach to supplement the lack of experimental data for the mixing thermodynamics.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Survey of Proposed Standards and Regulations for Artificial Intelligence

Over the last decade, the interest in machine learning and artificial intelligence (A.I) has grown exponentially. Researchers across several industries have explored and proposed uses of machine learning that have the potential to exponentially improve automation, efficiency, etc. The nuclear industry is no exception, with several studies exploring applications in almost every aspect of the field. However, these developments have brought forth a number of concerns. Government officials, industry leaders and many others have called for new regulations to govern the development and implementation of A.I systems. In order for machine learning and A.I to be viable for nuclear applications, there will need to be great regulatory oversight. The purpose of this study is to examine current and proposed regulations that relate to machine learning and provide recommendations for future regulations, specifically for nuclear applications.

99 GENERAL AND MISCELLANEOUS↗

Safeguarding Commercial Breed and Burn Sodium-Cooled Fast Reactors

A new class of reactors is under development in the United States. These new reactor designs use fast neutron spectra and rely on fuel technology advancements to reach fleet-wide operating conditions where neither enrichment nor reprocessing fuel are required to sustain or grow the fleet. Achieving this level of operation requires nuclear fuel that can remain in the reactor environment for much longer than current limits. The transfer of irradiated fuel is also required as the initial fissile source for new and replacement reactors. This class of reactors is known as breed and burn reactors and can be deployed as a fleet whereby the transfer of fuel is used to power subsequent generations of reactors. The use of breed and burn reactors reduces, and potentially eliminates, the need for enrichment and reprocessing to sustain a reactor fleet. Currently, enrichment and reprocessing plants require extremely complicated safeguards implementation and offer States diversion pathways for indirect use material. By eliminating the need for these facilities, a nuclear power fleet based on the BREED AND BURN reactor concept has the potential to indirectly reduce the burden on IAEA safeguards. However, this complex dynamic system does pose new safeguards challenges that are explored further in this report.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Physical and thermal property changes under uniform oxidation in nuclear graphite

Material property changes of fine- and medium-grain nuclear graphite grades were measured after subjection to uniform oxidation. The cores of high temperature reactors are composed of large nuclear graphite block components. Here, these large core components are designed to provide neutron moderation and reflection, create a large thermal sink to assist in operational control, and form the solid core structure containing the nuclear fuel, coolant channels, and the safety critical channels for control rod insertion. Oxidation is a principle degradation mechanism affecting all aspects of the nuclear graphite component functions. This study addresses the underlying physical property changes of nuclear-graphite components for oxidized mass loss ranges beyond the current recommended ASME code rule limits to ensure structural integrity within the graphite components (a maximum mass loss = 10%).

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Summary of Structural Material Modeling Development for the NEAMS Program in Fiscal Year 2020

This report summarizes work performed during Fiscal Year (FY) 2020 at Idaho National Laboratory (INL) for the U.S. Department of Energy?s Nuclear Engineering Advanced Modeling and Simulation (NEAMS) program for the Structural Materials and Chemistry Technical Area in the work package entitled "MS- 20IN050104 - Structural Materials - INL." The Structural Materials and Chemistry Technical Area is a relatively new component of the NEAMS program, and is currently focusing on developing simulation capabilities to support the deployment of nuclear energy in the areas of molten salt reactor chemistry, light water reactor (LWR) structural material degradation, and structural material behavior for advanced reactor applications. INL performed work for to advance capabilities for simulation of structural material behavior in both LWR and advanced reactor applications in the work described here.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Electrochemical Manipulation and Radiolytic Evaluation of Organic Phase Neptunium

Presentation for Seed LDRD proposal presentation: This Seed LDRD research proposes to test an innovative approach to precisely control the oxidation state distribution of neptunium (Np) under used nuclear fuel (UNF) reprocessing conditions using novel electrochemical methods. Current UNF reprocessing technologies are not financially viable in the US, requiring significant scientific and technological innovation to improve cost efficiency. Reducing the number of process cycles is one avenue for increasing cost efficiency, of which resolving the challenge associated with isolating Np is critical. Under envisioned process conditions, Np is present in a mixture of extractable (Np(IV) and Np(VI)) and inextractable (Np(V)) oxidation states, the distribution of which is dependent on several factors, including ionizing radiation dose, that change throughout a reprocessing scheme. Consequently, Np unintentionally partitions into various UNF reprocessing phases and product streams, ultimately increasing the number of process cycles to isolate UNF components. Here, we propose to employ novel, high surface area, optically transparent, Ligand Modified tin-doped indium oxide Electrodes (LMES). These LMEs bind Np, and therefore enable concurrent generation and spectroscopic characterization of Np oxidation states in organic solutions. These proof-of-concept experiments will: (i) facilitate optimization of the proposed electrochemical system conditions for Np oxidation state manipulation; (ii) identify the accessible electrochemical window for Np complexes in the organic phase; (iii) report characteristic optical spectra for each accessible complexed Np oxidation state; and (iv) determine the lifetime and partitioning of a given atypical Np oxidation state in the organic phase in the presence and absence of ionizing radiation fields. The data gathered by this Seed LDRD will provide support for the design of an electrochemical process concept for the precise manipulation of Np oxidation states in UNF reprocessing solvent systems, with the intention of providing advanced control over Np mass transfer, and thus greater process efficiency and economy.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Thermonuclear neutron emission from a sheared-flow stabilized Z-pinch

We report the fusion Z-pinch experiment (FuZE) is a sheared-flow stabilized Z-pinch designed to study the effects of flow stabilization on deuterium plasmas with densities and temperatures high enough to drive nuclear fusion reactions. Results from FuZE show high pinch currents and neutron emission durations thousands of times longer than instability growth times. While these results are consistent with thermonuclear neutron emission, energetically resolved neutron measurements are a stronger constraint on the origin of the fusion production. This stems from the strong anisotropy in energy created in beam-target fusion, compared to the relatively isotropic emission in thermonuclear fusion. In dense Z-pinch plasmas, a potential and undesirable cause of beam-target fusion reactions is the presence of fast-growing, “sausage” instabilities. This work introduces a new method for characterizing beam instabilities by recording individual neutron interactions in plastic scintillator detectors positioned at two different angles around the device chamber. Histograms of the pulse-integral spectra from the two locations are compared using detailed Monte Carlo simulations. These models infer the deuteron beam energy based on differences in the measured neutron spectra at the two angles, thereby discriminating beam-target from thermonuclear production. An analysis of neutron emission profiles from FuZE precludes the presence of deuteron beams with energies greater than 4.65 keV with a statistical uncertainty of 4.15 keV and a systematic uncertainty of 0.53 keV. This analysis demonstrates that axial, beam-target fusion reactions are not the dominant source of neutron emission from FuZE. These data are promising for scaling FuZE up to fusion reactor conditions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗