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At least 847 records · Page 47

Assessing Fuel Cycle Options for Elysium Molten Chloride Salt Fast Reactor from Spent Nuclear Fuel, Plutonium, and Depleted Uranium (Final CRADA Report)

Argonne National Laboratory performed calculations in order to determine the viability of various mode of operation and operating conditions for the reactor designed by Elysium Industry. The reactor description, operating conditions, startup fuel composition, and other relevant information were provided by Elysium to Argonne. The tools currently available at Argonne were used to perform the calculations and provide an assessment for the various cases agreed upon. The results were shared with Elysium.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fission Product Mass Yields in Uranium-233 and Plutonium-239 from Fast-Neutron-Induced Fission

Precise knowledge of nuclear fission is a critical component for nuclear energy and stockpile stewardship research. Despite having been discovered over 80 years ago, fission is not fully described by a predictive theory, so thorough and accurate nuclear data libraries are necessary. These libraries provide information about the fission process in studied isotopes that is used in scientific and engineering models.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A Robust Assessment of High-Precision Plutonium Isotopic Analysis by Thermal Ionization Mass Spectrometry [Slides]

TIMS at SRNL • SRNL consolidated analytical laboratories and services into one area – loss of TIMS capability during relocation. • SRNL installed a new Thermo Scientific TRITON Plus TIMS in our Category II Nuclear Facility to re-establish the lab’s TIMS capabilities in Feb. 2024. • Allows for handling, preparation, purification, and analysis of high-level radiological materials within a single location • Pu and U isotopic composition and assay measurement qualification have been priority since installation. • Once the instrument has been qualified, this capability will support internal and external customers.

07 ISOTOPE AND RADIATION SOURCES↗

Production of NBL PO plutonium isotopic standards CRM 136A, CRM 137A, and CRM 138A

Lawrence Livermore National Laboratory (LLNL) produced approximately 1 mg units of purified Pu from the parent New Brunswick Laboratory (NBL) certified reference materials (CRM) 137, 136 and 138 isotopic standards for the NBL Program Office (NBL PO) as detailed in the revised project plan. As stated in the plan, three representative units of each material were dispensed at the same time to be characterized at LLNL and provide informational values for the quantity of Pu and progeny nuclides in each unit. NBL PO intends to collect and evaluate isotopic measurement data from multiple laboratories and certify these materials as new isotopic standards C137A, C136A, and C138A, respectively. Soon after production eleven units of each analytical standard were shipped to other analytical laboratories for the certification effort, and 121, 119, and 119 units of C137A, C136A and C138A, respectively were shipped to Mickey Finch at Y12 NBL distribution center in November 2024 (30-gallon drum, TID 003777 PRL 7000005043). Residual purified Pu from the effort is being stored indefinitely in B332 at LLNL. Detailed methods can be found in the production plan, and this report describes and documents aspects of the production effort that are not in or were modified from the original production plan.

and nuclear chemistry↗

Lilith: An Enduring Plutonium Critical Assembly [Slides]

A design of an enduring Pu critical assembly has been produced. This is very important to DOE/NNSA missions. This assembly would result in advances/improvements in nuclear data validation, analytical methods validation, dosimetry, reactor kinetics, materials, and more.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗