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At least 847 records · Page 47

Emitted radiation characteristics of plutonium dioxide radioisotope thermoelectric generators

The nuclear and emitted radiation characteristics of the radioisotope elements and impurities in commercial grade plutonium dioxide are presented in detail. The development of the methods of analysis are presented. Radioisotope thermoelectric generators (RTG) of 1575, 3468 and 5679 thermal watts are characterized with respect to neutron and gamma photon source strength as well as spatial and number flux distribution. The results are presented as a function of detector position and light element contamination concentration for fuel age ranging from 'fresh' to 18 years. The data may be used to obtain results for given O-18 and Pu-236 concentrations. The neutron and gamma photon flux and dose calculations compare favorably with reported experimental values for SNAP-27.

Gingo, P. J.↗

An Artificial Neural Network System for Photon-Based Active Interrogation Applications

Active interrogation (AI) is a promising technique to detect shielded special nuclear materials (SNMs). At the University of Michigan, we are developing a photon-based AI system that uses bremsstrahlung radiation from an electron linear accelerator (linac) as an ionizing source and stilbene organic scintillating detectors for neutron detection. Stilbene scintillators are sensitive to fast neutrons and photons and have excellent pulse shape discrimination (PSD) capabilities. The traditional charge integration (CI) method commonly used for PSD analysis eliminates piled-up pulses and relies on a particle discrimination line to separate neutrons and photons. The presence of the intense photon flux during AI creates a significant number of piled-up events in the stilbene scintillator, thereby posing a great challenge to the traditional CI method. Identifying true single neutron pulses becomes challenging due to the presence of a pile-up cloud and overlapping neutron, photon and pile-up clouds in the PSD analysis. To mitigate the effect of pulse pile up and identify true single neutron pulses from stilbene scintillators, an artificial neural network (ANN) system is developed. The developed ANN system identifies single neutron pulses and neutron-photon combinations from piled-up events. The results obtained from a 252Cf measurement in the presence of the intense photon flux show that the developed ANN system outperforms the traditional CI method. Since many piled-up events lie above the particle discrimination line, they get misclassified as neutrons by the traditional CI method resulting in 25% overestimation of the net neutron count rate during the linac pulse. The overall net neutron count rate (single and restored neutrons) during the linac pulse, estimated by the ANN system is 60% of the ground truth. Energy spectroscopy of the ANN attributed single neutron pulses further provides evidence on the detection of prompt fission neutrons from the 252Cf fission source.

42 ENGINEERING↗

Efficient loading of reduced data ensembles produced at ORNL SNS/HFIR neutron time-of-flight facilities

We present algorithmic improvements to the loading operations of certain reduced data ensembles produced from neutron scattering experiments at Oak Ridge National Laboratory (ORNL) facilities. Ensembles from multiple measurements are required to cover a wide range of the phase space of a sample material of interest. They are stored using the standard NeXus schema on individual HDF5 files. This makes it a scalability challenge, as the number of experiments stored increases in a single ensemble file. The present work follows up on our previous efforts on data management algorithms, to address identified input output (I/O) bottlenecks in Mantid, an open-source data analysis framework used across several neutron science facilities around the world. We reuse an in-memory binary-tree metadata index that resembles data access patterns, to provide a scalable search and extraction mechanism. In addition, several memory operations are refactored and optimized for the current common use cases, ranging most frequently from 10 to 180, and up to 360 separate measurement configurations. Results from this work show consistent speed ups in wall-clock time on the Mantid LoadMD routine, ranging from 19% to 23% on average, on ORNL production computing systems. The latter depends on the complexity of the targeted instrument-specific data and the system I/O and compute variability for the shared computational resources available to users of ORNL’s Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR) instruments. Nevertheless, we continue to highlight the need for more research to address reduction challenges as experimental data volumes, user time and processing costs increase.

Godoy, William↗

Post-Irradiation Evaluation of Eurofer97 Fracture Toughness Using Miniature Multinotch Bend Bar Specimens

In this study, we performed fracture toughness characterization of ten neutron-irradiated Eurofer97 variants using precracked miniature multi-notch bend bar (M4CVN) specimens based on the Master Curve method in the ASTM E1921 standard. The neutron irradiation was performed in the flux trap position of the High Flux Isotope Reactor (HFIR) of the Oak Ridge National Laboratory (ORNL) with the nominal irradiation temperature of 300°C and irradiation dose of 2.5 displacements per atom (dpa). Depending on the irradiation temperature and materials, we observed different degrees of irradiation hardening and embrittlement for ten Eurofer97 variants. The upper shift in the Master Curve reference temperature T0Q vs. the increase in Vickers microhardness values showed a liner relationship for only a few materials indicating different irradiation responses of the Eurofer97 variants.

Chen, Xiang↗

The First Neptunium Dioxide Neutron Diffraction Experiment at HFIR

Here we present the first neutron diffraction experiment of a 50 mg sample of neptunium(IV) dioxide (NpO 2 ) powder at the High Flux Isotope Reactor (HFIR) using the wide-angle neutron diffractometer (WAND 2 ) HB-2C. We also provide a brief literature survey to pinpoint gaps in the crystal, electronic, and magnetic structure of NpO 2 to determine the optimum experiment to be pursued in the next HFIR user proposal cycle. Characterizing actinide materials with neutron diffraction, inelastic scattering, neutron imaging, polarized neutron studies, and small-angle neutron scattering techniques will increase our understanding of 5f electron behavior and elucidate atomic and magnetic structural properties. This strategy will help fill gaps in the literature and provide theoretical physicists with the data needed to build physical and chemical models to guide and validate computational methods. These methods may be used for predicting structural and chemical features of actinide-based materials. This proof-of-principle effort begins to uncover how to advance actinide science and technology at Oak Ridge National Laboratory (ORNL) using neutron capabilities. This effort has already sparked collaborative discussions between researchers outside the Radioisotope Science and Technology Division, including theoretical physicists from the Nuclear Nonproliferation Division and beamline scientists in the Neutron Scattering Division. We intend to continue pursuing neutron experiments and develop a scientific strategy focused on studying transuranium elements (e.g., Np, Pu, Am, and Cm) using the advanced neutron capabilities at ORNL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dynamic friction and wear of a solid film lubricant during radiation exposure in a nuclear reactor

The effect of nuclear reactor radiation on the performance of a solid film lubricant was studied. The film consisted of molybdenum disulfide and graphite in a sodium silicate binder. Radiation levels of fast neutrons (E or = 1 MeV) were fluxed up to 3.5 times 10 to the 12th power n/sq cm-sec (intensity) and fluences up to 2 times 10 to the 18th power n/sq cm (total exposure). Coating wear lives were much shorter and friction coefficients higher in a high flux region of the reactor than in a low flux region. The amount of total exposure did not affect lubrication behavior as severely as the radiation intensity during sliding.

Jacobson, T. P.↗

Uranium in NIMROC standard igneous rock samples

Results are reported for analysis of the uranium in multiple samples of each of six igneous-rock standards (dunite, granite, lujavrite, norite, pyroxenite, and syenite) prepared as geochemical reference standards for elemental and isotopic compositions. Powdered rock samples were examined by measuring delayed neutron emission after irradiation with a flux of the order of 10 to the 13th power neutrons/sq cm per sec in a nuclear reactor. The measurements are shown to compare quite favorably with previous uranium determinations for other standard rock samples.

Rowe, M. W.↗

Mass resolution optimization in a large isotopic composition experiment

A range-energy experiment was built to measure the isotopic composition of galactic cosmic rays. An enrichment of neutron rich isotopes, 22Ne and (25Mg + 26Mg) in particular, when compared to the solar composition is shown. A rich statistics measurement of these and other neutron-rich isotopes in the galactic flux yields information to the source of these particles. A computer simulation of the experiment was used to estimate the instrument resolution. The Cherenkov detector light collection efficiency, was calculated. Absorption of light in the radiator was considered to determine the optimum Cherenkov medium thickness. The experiment will determine the isotopic composition for the elements neon through argon in the energy range 300 to 800 MeV per nucleon.

Esposito, J. A.↗

Evidence of circumstellar matter surrounding the Hercules X-1 system

We analyze data from two eclipse ingresses of Her X-1 observed with Ginga on 1989 April 30 and May 19. These observations occur, respectively, during the MAIN HIGH and SHORT HIGH states in the 35 day modulation of Her X-1 intensity. We find significant residual X-ray flux during eclipse, with a gradual decrease in flux following the occultation of the neutron star by the atmosphere of HZ Her. During the central part of the eclipse the count rate becomes nearly constant, at 0.5 mCrab in the energy range 1.7-36.8 keV. From a spectral analysis of the residual emission during the total eclipse of the central source in the MAIN HIGH state, we determine the energy spectral index, alpha = 0.8, similar to that before eclipse. A remarkable feature of the eclipse spectrum is that it does not show a significant iron line feature in contrast to massive wind-fed pulsars, such as Vela X-1 and Cen X-3. From a timing analysis of the same eclipse data, we show that there are no pulses. These results imply that the emission comes from the scattering of continuum X-rays by material in a region considerably larger than the companion star. An extended accretion disk corona may be responsible for this scattering. However, partial eclipse of an extended accretion disk corona may be responsible for this scattering. However, partial eclipse of an extended accretion disk corona is insufficient to account for the count rates in mid-eclipse, when known parameters of the binary system are used. Based on the present results, we suggest that scattering occurs not only in the accretion disk corona but also in the circumstellar matter surrounding the system of Her X-1/HZ Her.

Choi, C. S.↗

Evidence of Circumstellar Matter Surrounding the Hercules X-1 System

We analyze data from two eclipse ingresses of Her X-1 observed with Ginga on 1989 April 30 and May 19. These observations occur, respectively, during the MAIN HIGH and SHORT HIGH states in the 35 day modulation of Her X-1 intensity. We find significant residual X-ray flux during eclipse, with a gradual decrease in flux following the occultation of the neutron star by the atmosphere of HZ Her. During the central part of the eclipse the count rate becomes nearly constant, at 0.5 mcrab in the energy range 1.7-36.8 keV. From a spec- tral analysis of the residual emission during the total eclipse of the central source in the MAIN MGH state, we determine the energy spectral index, alpha = 0.8, similar to that before eclipse. A remarkable feature of the eclipse spectrum is that it does not show a significant iron line feature in contrast to massive wind-fed pulsars, such as Vela X-1 and Cen X-3. From a timing analysis of the same eclipse data, we show that there are no pulses. These results imply that the emission comes from the scattering of continuum X-rays by material in a region considerably larger than the companion star. An extended accretion disk corona may be responsible for this scattering. However, partial eclipse of an extended accretion disk corona is insufficient to account for the count rates in mid-eclipse, when known parameters of the binary system are used. Based on the present results, we suggest that scattering occurs not only in the accretion disk corona but also in the circumstellar matter surrounding the system of Her X-1/HZ Her.

Choi, C. S.↗

The Projection of Space Radiation Environments with a Solar Cycle Statistical Model

A solar cycle statistical model has been developed to project sunspot numbers which represent the variations in the space radiation environment. The resultant projection of sunspot numbers in near future were coupled to space-related quantities of interest in radiation protection, such as the galactic cosmic radiation (GCR) deceleration potential (f) and the mean occurrence frequency of solar particle event (SPE). Future GCR fluxes have been derived from a predictive model, in which GCR temporal dependence represented by f was derived from GCR flux and ground-based Climax neutron monitor rate measurements over the last four decades. Results showed that the point dose equivalent inside a typical spacecraft in interplanetary radiation fields was influenced by solar modulation up to a factor of three. One important characteristic of sporadic SPEs is their mean frequency of occurrence, which is dependent on solar activity. Projections of future mean frequency of SPE occurrence were estimated from a power law function of sunspot number. Furthermore, the cumulative probabilities of SPE during short-period missions were defined with the continuous database of proton fluences of SPE. The analytic representation of energy spectra of SPE was constructed by the Weibull distribution for different event sizes. The representative exposure level at each event size was estimated for the guideline of protection systems for astronauts during future space exploration missions.

Kim, Myung-Hee↗

Iron K photons from weakly magnetized neutron stars in X-ray binaries

The emission of iron K photons by the continuum X-ray source and the neutron star surface is considered. It is shown that the continuum sources of X-ray binaries produce negligible amounts of iron K photons because nearly all iron atoms in the continuum source are fully stripped due to the intense X-ray fluxes. In contrast, the atmosphere of the neutron star in an X-ray binary might be an important source of iron K photons (photon energy about 6.5 keV) because it is bombarded by a large number of hard X-rays capable of photo-ejecting K-shell electrons from iron atoms. Information is discussed concerning the magnetic field strength, the gravitational potential at the neutron star surface, and the direction of the magnetic dipole axis which are obtainable from the observations of K photons of the neutron star atmosphere.

Bai, T.↗

Preliminary neutronic analysis of a cavity test reactor

A reference configuration was calculated for a cavity test reactor to be used for testing the gascore nuclear rocket concept. A thermal flux of 4.1 x 10 to the 14th power neutrons per square centimeter per second in the cavity was provided by a driver fuel loading of 6.4 kg of enriched uranium in MTR fuel elements. The reactor was moderated and cooled by heavy water and reflected with 25.4 cm of beryllium. Power generation of 41.3 MW in the driver fuel is rejected to a heat sink. Design effort was directed toward minimization of driver power while maintaining 2.7 MW in the cavity during a test run. Ancillary data on material reactivity worths, reactivity coefficients, flux spectra, and power distributions are reported.

Whitmarsh, C. L., Jr.↗

Detection of X-ray emission from the PSR 1259-63/SS 2883 binary system

Nonpulsed but variable X-ray emission has been detected from the binary system containing the radio pulsar PSR 1259-63 during two pointed ROSAT observations, taken 5 months apart. This 47.7 ms radio pulsar is in a highly eccentric (epsilon approximately 0.85) binary system with the 10-15 solar mass Be star SS 2883. It is the first radio pulsar found to be in a binary system with a massive main-sequence companion; it is also the most highly eccentric binary system known to contain a neutron star. The level of X-ray flux detected in the ROSAT observations has increased with orbital phase by a factor of at least 10 between 1992 February and 1993 February. The X-ray flux is significantly greater than expected from the Be star's corona and seems likely to originate either from low-level stellar wind accretion onto the neutron star or from the shock between the stellar wind and the relativistic pulsar wind. The system may be the progenitor of the more slowly rotating Be X-ray binary pulsar systems.

Cominsky, Lynn↗

Defect formation and transmutation behaviors in irradiated tungsten under thermal-neutron shielded and mixed spectrum conditions

Here, this study investigates the microstructural evolution of pure tungsten irradiated under thermal-neutron shielded and mixed spectrum conditions in the High Flux Isotope Reactor (HFIR). Four samples were irradiated at temperatures from 570 °C to 1130 °C up to 0.73 dpa. Neutron spectrum significantly influenced the accumulation of transmutation products, with Re+Os content estimated at ∼0.3–0.6% under thermal-neutron shielded conditions and ∼5.2% under the mixed spectrum condition. Irradiation temperature strongly influences tungsten’s microstructure, with dislocation loops and fine voids forming at lower temperatures and only larger voids and Re/Os segregation observed at higher temperature. Under thermal-neutron shielded conditions, dislocation loops and voids were observed at 570 °C and 790 °C. At the highest irradiation temperature (1130 °C), dislocation loops were no longer observed, while larger but less dense voids remained. Re and Os segregation to void surfaces was evident at 790 °C and 1130 °C, though no precipitation was observed. In contrast, under the mixed-spectrum condition, both spherical and needle-like Re/Os-rich precipitates were observed, frequently accompanied by large voids. Dislocation loops were not observed, but loop-like contrast within the precipitates suggests they may have nucleated on pre-existing loops. Irradiation-induced hardening was assessed for the shielded samples at 570 °C and 790 °C. Dispersed barrier hardening (DBH) analysis, based on TEM-resolved defects, revealed that voids were the dominant contributors to hardening, consistent with literature results. A schematic model is proposed to describe defect and precipitate evolution in tungsten under fusion-relevant transmutation-to-dpa conditions.

Dislocation loops↗