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At least 847 records · Page 47

The Readout Electronics of the Mu2e Electromagnetic Calorimeter

The Mu2e electromagnetic calorimeter has been designed to measure ~100 MeV electrons with energy resolution σE/E <10%, time resolution σt < 500ps and position resolution σx < 1cm. The detector is composed of 1348 un-doped CsI crystals coupled to two large area Silicon Photomultipliers (SiPMs). Each SiPM is connected to a Front End Electronics (FEE) chip which hosts the shaping amplifier and the high voltage linear regulator. A group of 20 FEE is controlled by one Mezzanine Board (MB) which transmits the amplified signals to one Digitizer ReAdout Controller board (DiRAC). The DiRAC samples the waveforms at 200 MHz with 12-bit ADCs, packs the data according to the Mu2e custom format and transmits them to the event builder through an optical transceiver. To limit the number of pass-through connectors and the length of the cables, the readout and digitization electronics is located inside the detector cryostat and close to the interaction target. The boards will have to sustain a neutron fluence of about 5x10 10 n/cm 2 @ 1 MeVeq (Si)/y and a Total Ionizing Dose of about 12 krad, while working into a 1T magnetic field and a vacuum of 10 (-4) Torr. This harsh operational environment has made the electronics design challenging and required an extended campaign of tests to select and qualify the employed electronic components. In this paper we report on the board architecture and design, on the qualification of the prototypes, as well as on the results of the first vertical slice test of the Mu2e calorimeter.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Final Report for Grant

This is the final report for this project. The major objectives were to develop full models and standard cells of CMOS silicon photomultipliers (SiPM) for neutron detection applications. Specifically, the research seeks to replace photomultiplier tubes, used in neutron detection applications, with SiPMs containing integrated readout electronics fabricated in standard CMOS processes. The detectors improve on the detection efficiency, readout speed, resolution (sensitivity), and spatial resolution of current systems. In particular, this work involved collaboration with the instrument and detector group at ORNL who build detectors based on discrete commercially available PMTs and SiPMs. The SiPM detectors developed in this work are based on Perimeter Gated Single Photon Avalanche Diodes (PGSPAD). These devices have tunable breakdown voltage which affects other performance characteristics of the detectors. The ability of the detectors to have integrated readout and tune the noise floor and dynamic range in addition to offering a method for non-uniformity compensation in a compact form significantly impacts the imaging research field and includes the nuclear sciences field, circuits and systems field in addition to varied fields such as geography and biology/medicine.

42 ENGINEERING↗

Computational Optimization of 133m Xe Production via Neutron Irradiation in a TRIGA Reactor

Here, the Comprehensive Nuclear-Test-Ban Treaty bans all nuclear tests worldwide. As part of treaty compliance, the concentration of radioactive nuclides in the atmosphere is monitored to detect nuclear weapons tests. Radioactive noble gas fission products, specifically radioxenon, can vent into the atmosphere after a nuclear weapons test, even if the test is well contained underground or underwater. Radioxenon thus serves as a signal for nuclear weapons tests. All atmospheric monitoring systems require samples of radioxenon isotopes for detector calibration, quality control, and certification. Here, we present a novel, improved method for creating samples of 133m Xe via neutron irradiation of 132 Xe in the Washington State University TRIGA reactor. 132 Xe neutron absorption results in either 133 Xe or 133m Xe—thermal neutron absorption results in 133m Xe 12% of the time, while fast neutron absorption (above ~1 MeV) results in 133m Xe ~50% of the time. To optimize the production of 133m Xe via neutron absorption in 132 Xe in the thermal TRIGA reactor, spectral tuning using an irradiation chamber is required to maximize the fraction of fast neutrons being absorbed and minimize the number of thermal neutrons interacting with the 132 Xe. We used MCNP to tally 132 Xe absorptions with the isotopic tally function, flux tallies and neutron attenuation to estimate the number of neutrons reaching the 132 Xe through the irradiation chamber, and the adjoint importance function to improve the source strength estimate. Additionally, we performed a heat transfer analysis for safety considerations. It was determined that the use of a 96% enriched 10 B boron carbide chamber, placed next to the fuel elements in reactor position D8, increases the 133m Xe/ 133 Xe activity ratio from a baseline value of 0.3 to 1.0, a 233% increase. Additionally, it was determined that the alpha heating produced in the boron does not become an unmanageable problem in the Washington State University reactor.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C↗

Final Report on the Phase II Physics Proposal for T-1063: The Accelerator Neutrino Neutron Interaction Experiment (ANNIE)

The goal of ANNIE is to make the first detailed measurement of the number of neutrons produced by neutrinos interacting with nuclei. This measurement is important for understanding the results of previous and planned neutrino experiments, as neutrons carry away energy from the neutrino interactions that must be accounted for in determining the energy and neutrino type. This effort is also focused on using a new photodetector technology and key target material enhancements to enable advanced water-based neutrino detectors. The ANNIE detector has been installed in the Booster Neutrino Beam at Fermilab, which provides a pulsed source of neutrinos in the energy range of 300-1200 MeV, which is relevant for the next generation of neutrino experiments. In 2017-2018 measurements of the neutron background in this beam were made with a partially-instrumented ANNIE detector. These measurements guided our design of the upgraded detector now built. The upgrade has been realized by adding Large Area Picosecond Photodetectors (LAPPDs) for the first time, more conventional photomultiplier tubes (PMTs), as well as adding electronics channels to the existing data acquisition system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Spectator Proton Detection and Reconstruction in Deep Inelastic D(E,EPS) Scattering

A Radial Time Projection Chamber (RTPC) was designed and installed in Jefferson Lab's Hall B as part of the BONuS12 (Barely Off-shell Nucleon Structure) experiment. The goal of BONuS12 is to accurately measure the structure function of the neutron by scattering 11 GeV electrons and detecting them with the CLAS12 spectrometer. Deuterium gas was used as an effective neutron target, and the new RTPC was used to detect low momentum spectator protons. Protons follow a curved path in the 5 Tesla solenoid that is part of CLAS12, ionizing the He-CO2 gas in an annular drift region surrounding the target. These ionization electrons are radially drifted outwards, amplified using cylindrical GEM (Gaseous Electron Multiplication) foils and recorded using readout pads located along the entire outer face of the cylindrical detector. The particle track reconstruction software discussed in detail in this thesis uses the signals from these pads to build tracks, which are reconstructed into the drift region using the arrival times of the signals and the positions of the pads. The proton momentum is measured from the track?s curvature and thus used to extract information about the struck neutron. This thesis introduces the theory of spectator tagging as an effective strategy for measuring neutron structure, by minimizing nuclear effects in the absence of a free neutron target. Along with discussing the many detectors that make up the CLAS12 spectrometer, the RTPC will be covered in detail, along with the tracking software designed to interpret the electronic signals to rebuild the low-momentum particle tracks, and fit them to extract the relevant kinematics. The results of the software, and preliminary analysis will be shown in the final chapter, as well as the discussion of possible improvements which could be made to the tracking software.

Payette, David↗

Simulating and benchmarking neutron total scattering instrumentation from inception of events to reduced and fitted data

In the design and realization of modern neutron scattering instrumentation, particularly when designing beamline concepts from the ground up, it is desirable to fully benchmark against realistically simulated data. This is especially true for total scattering beamlines, where the future deliverable data is to be analysed in both reciprocal- and real-space representations, and needs must be carefully balanced to ensure sufficient range, resolution and flux of the instrument. An approach to optimize the design of neutron scattering instrumentation via a workflow including ray-tracing simulations, event-based data reduction, heuristic analysis and fitting against realistically simulated spectra is demonstrated here. The case of the DISCOVER beamline concept at the Spallation Neutron Source is used as an example. The results of the calculations are benchmarked through simulation of existing instrumentation and subsequent direct comparison with measured data. Finally, on the basis of the validated models, the ability to explore design characteristics for future beamline concepts or future instrument improvements is demonstrated through the examples of detector tube size and detector layout.

47 OTHER INSTRUMENTATION↗

Response of CR-39 nuclear track detectors to protons with non-normal incidence

This paper presents data from experiments with protons at non-normal incidence to CR-39 nuclear track detectors, analyzing the properties of detection efficiency, proton track diameter, track contrast, and track eccentricity. Understanding the CR-39 response to protons incident at an angle is important for designing charged particle detectors for inertial confinement fusion (ICF) applications. This study considers protons with incident energies less than 3 MeV. In this regime, an incident angle of 10° has no effect on CR-39 detection efficiency, and >85% detection efficiency is preserved up through 25° in the range of 1.0 MeV–2.1 MeV. For ICF applications, incident angles above 30° are deemed impractical for detector design due to significant drops in proton detection at all energies. We observe significant reductions in detection efficiency compared to theoretical predictions, particularly at low energies where proton tracks are etched away. The proton track diameter measured by the scan system is observed to decrease with higher incident angles. The track diameters are analyzed with two fitting models, and it is shown that the diameter–energy relation can be fit with the existing models at angles up to 30° . The optical contrast of the tracks tends to increase with the angle, meaning that the tracks are fainter, and a larger increase is observed for higher energies. Eccentricity, a measure of how elongated proton tracks are, increases with the incident angle and drops after the critical angle. The lowest energy tracks remain nearly circular even at higher angles.

47 OTHER INSTRUMENTATION↗

Measuring the properties of f - mode oscillations of a protoneutron star by third-generation gravitational-wave detectors

Core-collapse supernovae are among the astrophysical sources of gravitational waves that could be detected by third-generation gravitational-wave detectors. Here, we analyze the gravitational-wave strain signals from two- and three-dimensional simulations of core-collapse supernovae generated using the code FORNAX. A subset of the two-dimensional simulations has non-zero core rotation at the core bounce. A dominant source of time changing quadrupole moment is the l = 2 fundamental mode (f- mode) oscillation of the proto-neutron star. From the time-frequency spectrogram of the gravitational-wave strain we see that, starting ~ 400 ms after the core bounce, most of the power lies within a narrow track that represents the frequency evolution of the f-mode oscillations. The f-mode frequencies obtained from linear perturbation analysis of the angle averaged profile of the protoneutron star corroborate what we observe in the spectrograms of the gravitational wave signal. We explore the measurability of the f-mode frequency evolution of protoneutron star for a supernova signal observed in the third-generation gravitational-wave detectors. Measurement of the frequency evolution can reveal information about the masses, radii, and densities of the proto-neutron stars. We find that if the third generation detectors observe a supernova within 10 kpc, we can measure these frequencies to within ~90% accuracy. Here, we can also measure the energy emitted in the fundamental f-mode using the spectrogram data of the strain signal. We find that the energy in the f-mode can be measured to within 20% error for signals observed by Cosmic Explorer using simulations with successful explosion, assuming source distances within 10 kpc.

79 ASTRONOMY AND ASTROPHYSICS↗

Online and Offline Analytical Techniques to Quantify Chloride Salts

This report serves as the deliverable for Milestone- M3FT-26AN080502017: Summary of Accomplishments for Online and Offline Analytical Qualification of Chloride Fuel Salts. The qualification of chloride fuel salts is a critical challenge for the development and deployment of molten salt reactors (MSRs), requiring precise control and verification of chemical and isotopic composition to ensure predictable neutronics, manageable radiological behavior, and safe plant operation. Currently, there is no universally accepted standard for fuel salt qualification, particularly for chloride-based systems, which underscores the need for robust, science-based analytical methodologies. This report presents a comprehensive evaluation of both online and offline techniques for quantifying chloride fuel salts, including multielectrode array voltammetry, differential thermal analysis (DTA) probes, inert gas fusion (IGF) analyzers, and gamma spectrometry using the Mirion NAIS-2x2 NaI(Tl) detector. The integration of these methods enables real-time monitoring of actinide concentrations, redox state, and thermophysical properties, as well as high-precision measurement of impurities and isotopic composition. The acquisition of advanced instruments such as the Bruker Leonardo G6 for IGF and the Mirion NaI detector enhances analytical capabilities, supporting the establishment of operational envelopes and impurity thresholds. These approaches provide essential data for neutronic impact evaluation, feedstock documentation, and compliance with nuclear safety standards. The methodologies developed and validated in this report lay the groundwork for future standardized protocols, bridging the gap between laboratory research and commercial reactor operation, and advancing the safe and efficient deployment of chloride-fueled MSRs.

Polke, Amber↗

Exploration of Neutron-Rich Isotopes around N = 50 via the In-Flight Fission of a 345 MeV/Nucleon 238 U Beam

A search for new neutron-rich isotopes beyond $Z=28$ and $N=50$ was performed using a 345 MeV/nucleon $^{238}$U beam at RI Beam Factory in RIKEN Nishina Center. The BigRIPS separator and state-of-the-art radiation detectors were used to efficiently separate and identify the produced nuclei. For the first time, we have observed and determined the production cross sections for eight neutron-rich isotopes $^{72}$Cr, $^{74,75}$Mn, $^{77}$Fe, $^{79,80}$Co, $^{85}$Cu, and $^{90}$Ga. This study broadens our understanding of nuclear existence and paves the way for investigating the properties of neutron-rich medium-mass nuclei.

Shimizu, Yohei [RIKEN, Saitama (Japan); et al.]↗

Fission-product decay studies with the FRIB Decay Station

The Facility for Rare Isotopes Beams (FRIB) will be the flagship facility in low-energy nuclear physics when it comes online in 2022. This U.S. Department of Energy Office of Science user facility will open up a multitude of new opportunities to study exotic nuclei and will lead to new discoveries in nuclear structure, nuclear astrophysics, fundamental symmetries, and isotopes of importance to nuclear applications. The b-decay properties of neutron-rich isotopes will be measured with the FRIB Decay Station, a sophisticated state-of-the-art modular multi-detector system envisioned to perform b, g, n, and charged-particle spectroscopy. In this feasibility study, we use nuclear decay data collected with the FRIB Decay Station precursor, the Beta-Counting Station, currently used at Michigan State University with a radioactive beam produced at the National Superconducting Cyclotron Laboratory to identify the FRIB Decay Station capabilities for future measurements of neutron-rich exotic nuclei at FRIB to help provide a path forward for future measurements of interest to the lab’s mission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A New Era of Nuclear Criticality Experiments: The First 10 Years of Radiation Test Object Operations at NCERC

The work presented in this paper focuses on the first 10 years (2011–2020) of radiation test object (RTO) operations at the National Criticality Experiments Research Center. RTOs are subcritical configurations of special nuclear material that are built by hand. These configurations are utilized for benchmark experiments, detector testing/characterization, and training. An overview of the types of measurements used in RTO operations is given as well as a history of RTO operations at Los Alamos National Laboratory from 1944–2011.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Reconstruction of neutrino events in the Accelerator Neutrino Neutron Interaction Experiment. Part I

The Accelerator Neutrino Neutron Interaction Experiment (ANNIE) was designed to reconstruct neutrino events from the Fermilab Booster Neutrino Beam (BNB) with the parallel goals of measuring neutron production in interactions with oxygen and serving as a testbed for new technology. The ANNIE detector consists of a 26-ton water Cherenkov target tank instrumented with conventional photomultiplier tubes (PMTs), a downstream tracking muon spectrometer, and an upstream double wall of plastic scintillator to serve to veto charged particles incoming from neutrino events that occur upstream of the experimental setup. ANNIE has also deployed multiple Large-Area Picosecond PhotoDetectors (LAPPDs) and a test vessel of water-based liquid scintillator (WbLS). This paper describes the event reconstruction performance of the detector before implementation of these novel technologies, which will serve as a baseline against which their impact can be measured. That said, even the techniques used for event reconstruction using only the conventional PMT array and muon spectrometer are significantly different than those used in other water Cherenkov detectors due to the small size of ANNIE (which makes nanosecond-scale timing not as useful as in a large detector) and the availability of reconstruction information from the tracking muon spectrometer. We demonstrate that combining the information from these two elements into a single fit using only pattern recognition yields a muon vertex uncertainty of 60 cm, a directional uncertainty of 13.2 degrees, and energy reconstruction uncertainty of about 10% for BNB muon neutrino Charged Current Zero Pion (CC0π) events.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Identification of Prompt Proton Emission in $N = Z - 1$ 61 Ga: Isospin Symmetry at the Limit of Nuclear Binding

Excited states in the proton drip line nucleus 61 Ga were populated via the fusion-evaporation reaction 24 Mg ⁢( 40 Ca, 𝑝⁢2⁢𝑛)⁢ 61 Ga. The experimental setup at Argonne National Laboratory comprised a novel combination of the Gammasphere array with two CD-shaped double-sided Si-strip detectors inside the Microball CsI(Tl) charged-particle detection array, as well as the Neutron-Shell liquid scintillators and the Fragment Mass Analyzer. Owing to the setup’s unprecedented in-beam proton spectroscopy and tracking capabilities, a coincidence between a 957.6(5)-keV 𝛾 ray and a 1.876(24)-MeV proton line was observed, which identifies the quasibound proton 𝜋⁢𝑔 9/2 single-particle state in 61 Ga at 𝐸 𝑥 = 2150⁢(34) keV. This probes isospin symmetry at the limit of nuclear binding by providing a unique challenge for the shell-model interpretation of mirror nuclei beyond doubly magic 56 Ni .

Hrabar, Yuliia [Lund Univ. (Sweden)] (ORCID:000000↗

Measurement of the 75 As ⁢(𝑛, 2⁢𝑛) cross section at 14.1 MeV at the National Ignition Facility

Here, a new measurement of the 75 As (𝑛, 2⁢𝑛) measurement was performed using the 14.1 MeV neutron pulse produced by fusion experiments at the National Ignition Facility (NIF). The target material consisted of GaAs foils encapsulated in aluminum irradiation containers, along with Au monitor foils, and positioned in the NIF chamber during high neutron yield shots. After irradiation, the GaAs and Au foils were counted with high purity germanium detectors to assess the production of (𝑛, 2⁢𝑛) activation products to determine the flux and the cross section of interest. The measured cross section was 966 ± 71 mb at 14.1 ± 0.37 MeV. This work provides a proof of concept for a platform for performing “ride-along” cross section measurements at NIF to contribute to existing nuclear data as well as measure new cross sections in the future.

and nuclear chemistry↗

Spin-phonon coupling in AFM transition-metal mono-oxide

Time-of-flight INS measurements were performed on single crystal NiO with the Wide Angular Range Chopper Spectrometer (ARCS) at the Spallation Neutron Source. Experiments were performed on NiO single crystal mounted in an aluminum can and cooled using a closed-cycle helium refrigerator. Measurements were conducted at T = 100 K and 650 K, with the [HHL] scattering plane aligned horizontally. A Fermi chopper with slit spacing of 1.52mm, spinning at 300 Hz, was used to select an incident neutron energy of 100 meV. All datasets were normalized to a vanadium standard to correct for detector efficiency and solid angle coverage. The data sets include the .nxs files, the generated .hdf5 files (for use with Phonon Explorer), and Python scripts used to create them.

36 MATERIALS SCIENCE↗

24.1.3.1 - Verification of Spent Fuel Inside Dry Storage Casks by Fast/Epi-thermal Neutron Mapping

Development of a spent-fuel verification method based upon positional measurement of fast neutrons emitted from the top surface of the dry storage casks. A proof-of-principle field test on a partially loaded spent-fuel cask will be conducted by measuring the fast neutron flux on the top of the cask as a function of position using a single detector. If a useful verification signature is demonstrated, a multi-detector scanning array will be built and tested in FY2021 to demonstrate a practical rapid verification system in FY2022.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Verification of Spent Fuel Inside Dry Storage Casks Using Neutron Mapping (2022 Midyear Report)

Development of a spent-fuel verification method based upon positional measurement of fast neutrons emitted from the top surface of the dry storage casks. A proof-of-principle field test on a partially loaded spent-fuel cask will be conducted by measuring the fast neutron flux on the top of the cask as a function of position using a single detector. If a useful verification signature is demonstrated, a multi-detector scanning array will be built and tested to demonstrate a practical rapid verification system.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗