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At least 847 records · Page 47
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Coupled-Channel Analysis of the χ c 1 ( 3872 ) Line Shape with BESIII Data

We perform a study of the χ c 1 ( 3872 ) line shape using the data samples of e + e − → γ χ c 1 ( 3872 ) , χ c 1 ( 3872 ) → D 0 D ¯ 0 π 0 , and π + π − J / ψ collected with the BESIII detector. The effects of the coupled channels and the off-shell D * 0 are included in the parametrization of the line shape. The line shape mass parameter is obtained to be M X = ( 3871.63 ± 0.1 3 − 0.05 + 0.06 ) MeV . Two poles are found on the first and second Riemann sheets corresponding to the D * 0 D ¯ 0 branch cut. The pole location on the first sheet is much closer to the D * 0 D ¯ 0 threshold than the other, and is determined to be 7.04 ± 0.1 5 − 0.08 + 0.07 MeV above the D 0 D ¯ 0 π 0 threshold with an imaginary part − 0.19 ± 0.0 8 − 0.19 + 0.14 MeV . Published by the American Physical Society 2024

Physics↗
DOE OSTI2024

Modification of χ c 1 ( 3872 ) and ψ ( 2 S ) Production in p Pb Collisions at s NN = 8.16 TeV

The LHCb Collaboration measures production of the exotic hadron χ c 1 ( 3872 ) in proton-nucleus collisions for the first time. Comparison with the charmonium state ψ ( 2 S ) suggests that the exotic χ c 1 ( 3872 ) experiences different dynamics in the nuclear medium than conventional hadrons, and comparison with data from proton-proton collisions indicates that the presence of the nucleus may modify χ c 1 ( 3872 ) production rates. This is the first measurement of the nuclear modification factor of an exotic hadron. © 2024 CERN, for the LHCb Collaboration 2024 CERN

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Strong and Weak C P Tests in Sequential Decays of Polarized Σ 0 Hyperons

The J / ψ , ψ ( 3686 ) → Σ 0 Σ ¯ 0 processes and subsequent decays are studied using the world’s largest J / ψ and ψ ( 3686 ) data samples collected with the BESIII detector. The parity-violating decay parameters of the decays Σ 0 → Λ γ and Σ ¯ 0 → Λ ¯ γ , α Σ 0 = − 0.0017 ± 0.0021 ± 0.0018 and α ¯ Σ 0 = 0.0021 ± 0.0020 ± 0.0022 , are measured for the first time. The strong C P symmetry is tested in the decays of the Σ 0 hyperons for the first time by measuring the asymmetry A C P Σ = α Σ 0 + α ¯ Σ 0 = ( 0.4 ± 2.9 ± 1.3 ) × 10 − 3 . The weak C P test is performed in the subsequent decays of their daughter particles Λ and Λ ¯ . Also for the first time, the transverse polarizations of the Σ 0 hyperons in J / ψ and ψ ( 3686 ) decays are observed with opposite directions, and the ratios between the S -wave and D -wave contributions of the J / ψ , ψ ( 3686 ) → Σ 0 Σ ¯ 0 decays are obtained. These results are crucial to understand the decay dynamics of the charmonium states and the production mechanism of the Σ 0 − Σ ¯ 0 pairs. Published by the American Physical Society 2024

Physics↗
DOE OSTI2025

Atomically Dispersed Ni‐N‐C Catalysts for Electrochemical CO 2 Reduction

Abstract The atomic dispersion of nickel in Ni‐N‐C catalysts is key for the selective generation of carbon monoxide through the electrochemical carbon dioxide reduction reaction (CO 2 RR). Herein, the study reports a highly selective, atomically dispersed Ni 1.0% ‐N‐C catalyst with reduced Ni loading compared to previous reports. Extensive materials characterization fails to detect Ni crystalline phases, reveals the highest concentration of atomically dispersed Ni metal, and confirms the presence of the proposed Ni‐N x active site at this reduced loading. The catalyst shows excellent activity and selectivity toward CO generation, with a faradaic efficiency for CO generation (FE CO ) of 97% and partial current density for CO (j co ) of ‐9.0 mA cm −2 at ‐0.9 V in an electrochemical H‐type cell. CO 2 RR activity and selectivity are also studied by rotating disk electrode (RDE) measurements where transport limitations can be suppressed. It is expected that the utility of these Ni‐N‐C catalysts will lie with tandem CO 2 RR reaction schemes to multi‐carbon (C 2+ ) products.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Low-efficiency-droop c -plane InGaN/GaN light-emitting diodes through the use of thick single quantum wells and doped barriers

Efficiency droop at high current densities is a problem for InGaN-based light-emitting diodes (LEDs), especially for conventional c-plane devices. The large internal electric fields in c-plane quantum wells (QWs) lead to an increase in the active region carrier density (n), causing the electrical efficiency droop onset to occur at low current densities. Here, we present an approach to reduce the internal electric fields (Eint) in c-plane QWs by placing doped p-type and n-type GaN barriers close to the QW. The reduced Eint also allows a thick QW active region design, which helps to lower n to further reduce the droop. The concept of using doped barriers to control Eint is explained using theory and device simulations. Following that, multiple series of thick single QW (SQW) LEDs were grown and characterized. Key parameters in the epitaxial design such as the doping levels and the relative position of the doped barriers were systematically studied and optimized. In conclusion, by using optimized doped barriers and a thick SQW, c-plane LEDs with a low-efficiency droop of 14% at 300 A/cm2 [with respect to the peak external quantum efficiency (EQE)] and a high peak EQE of 49% were demonstrated.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Anisotropic excitonic magnetism from discrete C 4 symmetry in CeRhIn 5

Anisotropy in strongly correlated materials is a central parameter in determining the electronic ground state and is tuned through the local crystalline electric field. This is notably the case in the CeCo x Rh 1 − x In 5 system where the ground-state wave function can provide the basis for antiferromagnetism and/or unconventional superconductivity. We develop a methodology to understand the local magnetic anisotropy and experimentally investigate with neutron spectroscopy applied to antiferromagnetic ( T N = 3.8 K ) CeRhIn 5 , which is isostructural to d -wave superconducting ( T c = 2.3 K ) CeCoIn 5 . Through diagonalizing the local crystal field Hamiltonian with discrete tetragonal C 4 point group symmetry and coupling these states with the random phase approximation, we find two distinct modes polarized along the crystallographic c and a − b planes, agreeing with experiment. The anisotropy and bandwidth, underlying the energy scale of these modes, are tuneable with a magnetic field which we use experimentally to separate in energy single and multiparticle excitations thereby demonstrating the instability of excitations polarized within the crystallographic a − b plane in CeRhIn 5 . We compare this approach to a S eff = 1 2 parametrizations and argue for the need to extend conventional SU(2) theories of magnetic excitations to utilize the multilevel nature of the underlying crystal-field basis states constrained by the local point-group C 4 symmetry. Published by the American Physical Society 2024

Brener, D. J. (ORCID:0000000333400177)↗
DOE OSTI2024

$K^0_S$ meson production in inelastic p+p interactions at 31, 40 and 80 $\text {Ge}\hspace{-1.00006pt}\text {V}\!/\!c$ beam momentum measured by NA61$/$SHINE at the CERN SPS

The yields of $K^0_S$ mesons have been measured in inelastic p+p interactions at incident projectile momenta of 31, 40 and 80 $\text {Ge}\hspace{-1.00006pt}\text {V}\!/\!c$ ($\sqrt{s_{NN}}=7.7, 8.8$ and 12.3 $\text {Ge}\hspace{-1.00006pt}\text {V}$, respectively). The data were recorded by the NA61$/$SHINE spectrometer at the CERN Super Proton Synchrotron and the $K^0_S$ mesons identified via their decays into $\pi ^{+} \pi ^{-}$ pairs. Double-differential distributions are presented as function of transverse momentum and rapidity. The mean multiplicities of $K^0_S$ mesons were determined to be $(5.95 \pm 0.19 (stat) \pm 0.30 (sys)) \times 10^{-2}$ at 31 $\text {Ge}\hspace{-1.00006pt}\text {V}\!/\!c$, $(7.61 \pm 0.13 (stat) \pm 0.43 (sys)) \times 10^{-2}$ at 40 $\text {Ge}\hspace{-1.00006pt}\text {V}\!/\!c$ and $(11.58 \pm 0.12 (stat) \pm 0.55 (sys)) \times 10^{-2}$ at 80 $\text {Ge}\hspace{-1.00006pt}\text {V}\!/\!c$. The results on $K^{0}_{S}$ production are compared with the production of charged kaons in corresponding reactions and with model calculations (Epos1.99, SMASH 2.0 and PHSD) as well as with published data from other experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Measurement of the ${\Lambda}_c^{+}$ to D 0 production ratio in peripheral PbPb collisions at $\sqrt{s_{\textrm{NN}}}$ = 5.02 TeV

We report on a measurement of the ${\Lambda}_c^{+}$ to D 0 production ratio in peripheral PbPb collisions at $\sqrt{s_{\textrm{NN}}}$ = 5.02 TeV with the LHCb detector in the forward rapidity region 2 < y < 4.5. The ${\Lambda}_c^{+}$ (D 0 ) hadrons are reconstructed via the decay channel ${\Lambda}_c^{+}$ → pK – π + (D 0 → K – π + ) for 2 < p T < 8 GeV/c and in the centrality range of about 65–90%. The results show no significant dependence on p T , y or the mean number of participating nucleons. They are also consistent with similar measurements obtained by the LHCb collaboration in pPb and Pbp collisions at $\sqrt{s_{\textrm{NN}}}$ = 5.02 TeV. The data agree well with predictions from PYTHIA in pp collisions at $\sqrt{s}$ = 5 TeV but are in tension with predictions of the Statistical Hadronization model.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

${\Lambda}_c^{+}$ polarimetry using the dominant hadronic mode

The polarimeter vector field for multibody decays of a spin-half baryon is intro duced as a generalisation of the baryon asymmetry parameters. Using a recent amplitude analysis of the ${\Lambda}_c^{+}$ → $pK^-π^+$ decay performed at the LHCb experiment, we compute the distribution of the kinematic-dependent polarimeter vector for this process in the space of Mandelstam variables to express the polarised decay rate in a model-agnostic form. The obtained representation can facilitate polarisation measurements of the ${\Lambda}_c^{+}$ baryon and eases inclusion of the ${\Lambda}_c^{+}$ → $pK^-π^+$ decay mode in hadronic amplitude analyses.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Enhanced plasma performance in C-2W advanced beam-driven field-reversed configuration experiments

TAE Technologies’ fifth-generation fusion device, C-2W (also called ‘Norman’), is the world’s largest compact-toroid device and has made significant progress in field-reversed configuration (FRC) plasma performance. C-2W produces record breaking, macroscopically stable, high-temperature advanced beam-driven FRC plasmas, dominated by injected fast particles and sustained in steady state, which is primarily limited by neutral-beam (NB) pulse duration. The NB power supply system has recently been upgraded to extend the pulse length from 30 ms to 40 ms, which allows for a longer plasma lifetime and thus better characterization and further enhancement of FRC performance. An active plasma control system is routinely used in C-2W to produce consistent FRC performance as well as for reliable machine operations using magnet coils, edge-biasing electrodes, gas injection and tunable-energy NBs. Google’s machine learning framework for experimental optimization has also been routinely used to enhance plasma performance. D

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Extraction of the non-spin- and spin-transfer isovector responses via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B reaction

The isovector response in 12 B was investigated via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B* reaction at 100⁢𝐴MeV. By utilizing the 𝛾-decay properties of the 1.74 MeV 0 + and 0.718 MeV 1 + states in 10 B, the separate extraction of the non-spin-transfer (Δ⁢𝑆 = 0) and spin-transfer (Δ⁢𝑆 = 1) isovector responses up to an excitation energy of 50 MeV in 12 B in a single measurement is demonstrated. The experimental setup employed the S800 spectrometer to detect and analyze the 10 B ejectiles and the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA) for obtaining the Doppler-reconstructed spectrum for 𝛾 rays emitted in flight by 10 B. A 12 C foil was placed at the pivot point of the spectrograph. Here, the 12 B reaction product was not detected. Contributions from transitions associated with the transfer of different units of angular momentum in the non-spin- and spin-transfer responses were analyzed using a multipole decomposition analysis. The extracted non-spin-dipole (Δ⁢𝑆 = 0, Δ⁢𝐿 = 1) and spin-dipole (Δ⁢𝑆 = 1, Δ⁢𝐿 = 1) responses were found to be consistent with available data from other charge-exchange probes, validating the non-spin- and spin-transfer filters used. While statistical uncertainties and experimental resolutions were relatively large due to the modest intensity of the 10 Be secondary beam, the results show that, with the much higher intensities that will be available at new rare-isotope beam facilities, the ( 10 Be, 10 B + 𝛾) reaction and its Δ⁢𝑇 𝑧 = −1 partner, the ( 10 C, 10 B + 𝛾) reaction, are powerful tools for elucidating the isovector non-spin- and spin-transfer responses in nuclei.

Charge-exchange reactions↗
DOE OSTI2025

The SHMS 11 GeV/c spectrometer in Hall C at Jefferson Lab

The Super High Momentum Spectrometer (SHMS) has been built for Hall C at the Thomas Jefferson National Accelerator Facility (Jefferson Lab). With a momentum capability reaching 11 GeV/ c , the SHMS provides measurements of charged particles produced in electron-scattering experiments using the maximum available beam energy from the upgraded Jefferson Lab accelerator. The SHMS is an ion-optics magnetic spectrometer comprised of a series of new superconducting magnets which transport charged particles through an array of triggering, tracking, and particle-identification detectors that measure momentum, energy, angle and position in order to allow kinematic reconstruction of the events back to their origin at the scattering target. The detector system is protected from background radiation by a sophisticated shielding enclosure. The entire spectrometer is mounted on a rotating support structure which permits measurements to be taken with a large acceptance over laboratory scattering angles from 5.5° to 40°, thus allowing a wide range of low cross-section experiments to be conducted. Finally, these experiments complement and extend the previous Hall C research program to higher energies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Reexamination of isoscalar giant resonances in 12 C and 93 Nb through 6 Li scattering

Inelastic Li 6 scattering at 100 MeV/u on C 12 and Nb 93 has been measured with the high-resolution magnetic spectrometer Grand Raiden. The magnetic-rigidity settings of the spectrometer covered excitation energies from 10 to 40 MeV and scattering angles in the range 0 ° < θ lab. < 2 ° . The isoscalar giant monopole resonance was selectively excited in the present data. Measurements free of instrumental background and the very favorable resonance-to-continuum ratio of Li 6 scattering allowed for precise determination of the E 0 strengths in C 12 and Nb 93 . Additionally, it was found that the monopole strength in C 12 exhausts 52 ± 3 (stat.) ± 8 (sys.) % of the energy-weighted sum rule (EWSR), which is considerably higher than results from previous α -scattering experiments. The monopole strength in Nb 93 exhausts 92 ± 4 (stat.) ± 10 (sys.) % of the EWSR, and it is consistent with measurements of nuclei with mass number of A ≈ 90 . Such comparison indicates that the isoscalar giant monopole resonance distributions in these nuclei are very similar, and no influence due to nuclear structure was observed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Search for Time-Dependent C P Violation in D 0 → π + π − π 0 Decays

A measurement of time-dependent C P violation in D 0 → π + π − π 0 decays using a p p collision data sample collected by the LHCb experiment in 2012 and from 2015 to 2018, corresponding to an integrated luminosity of 7.7 fb − 1 , is presented. The initial flavor of each D 0 candidate is determined from the charge of the pion produced in the D * ( 2010 ) + → D 0 π + decay. The decay D 0 → K − π + π 0 is used as a control channel to validate the measurement procedure. The gradient of the time-dependent C P asymmetry Δ Y in D 0 → π + π − π 0 decays is measured to be Δ Y = ( − 1.3 ± 6.3 ± 2.4 ) × 10 − 4 , where the first uncertainty is statistical and the second is systematic, which is compatible with C P conservation. © 2024 CERN, for the LHCb Collaboration 2024 CERN

Aaij, R. (ORCID:0000000305331952)↗
DOE OSTI2020

Measurement of the absolute branching fraction of the inclusive decay $\Lambda _c^+ \rightarrow K_S^0X$: (BESIII Collaboration)

We report the first measurement of the absolute branching fraction of the inclusive decay Λ c + → K S 0 X . The analysis is performed using an e + e - collision data sample corresponding to an integrated luminosity of 567 pb - 1 taken at s = 4.6 GeV with the BESIII detector. Using eleven Cabibbo-favored Λ ¯ c - decay modes and the double-tag technique, this absolute branching fraction is measured to be B ( Λ c + → K S 0 X ) = ( 9.9 ± 0.6 ± 0.4 ) % , where the first uncertainty is statistical and the second systematic. The relative deviation between the branching fractions for the inclusive decay and the observed exclusive decays is ( 18.7 ± 8.3 ) % , which indicates that there may be some unobserved decay modes with a neutron or excited baryons in the final state.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Triggering C-N Coupling on Metal Oxide Nanocomposite for the Electrochemical Reduction of CO 2 and NO x ⁻ to Formamide

The co-electroreduction of CO 2 and NO x ⁻ (NO 3 ⁻ /NO 2 ⁻ ) to generate formamide (HCONH 2 ) offers an opportunity for downstream chemical and polymer manufacturing decarbonization; however, significant challenges lie in the C-N coupling and the associated low product selectivity. Herein, p-block metal oxides are incorporated in copper oxides to provide more accessible active sites for reactant adsorption and activation, tuning the reaction selectivity toward the formamide production. Through in situ Raman and synchrotron-based infrared spectroscopy measurements, C-N bond formation is demonstrated in real-time with the CuO x /BiO x catalyst, where the C-N bond is detected via a *CHO and *NH 2 intermediates formation, in agreement with the density functional theory calculations. When tested in a flow electrolyzer, a formamide yield rate of 134 ± 11 mmol h -1 g cat -1 is reported, the first report of co-electroreduction of CO 2 and NO x ⁻ to formamide beyond conventional H-cell measurements. These new insights on the C-N coupling mechanisms and scale-up capability provide directions for further development of electrocatalysts for the formamide production.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Chapter One - Selectivity in the activation of C–H bonds by rhodium and iridium complexes

Trispyrazolylborate complexes of rhodium and iridium have been extensively investigated over the past 3 decades with special attention to their ability to activate C–H bonds. The rhodium complexes of tris-(3,5-dimethylpyrazolyl)borate have been the subject of numerous thermodynamic investigations that provide information about rhodium-metal carbon bond strengths. This insight arises as a result of the reversibility of C–H activation with rhodium. In the case of iridium, C–H bond activation reactions are also widespread, and some of these also show reversibility. Access to some key trispyrazolylborate iridium(I) and iridium(III) starting materials has given way to a multitude of studies of reactions with small molecules in which C–H bonds are made and broken reversibly. The stability of Fischer carbenes plays a role in the observed products. Here, the reactivity of trispyrazolylborate complexes of rhodium and iridium compounds over the past decade (since 2010) are summarized here. Related reactions of X–H bonds with these trispyrazolylborate compounds are also included for completeness (X = O, N, S, B, Si).

02 PETROLEUM↗
DOE OSTI2021

Position-specific isotope effects during alkaline hydrolysis of 2,4-dinitroanisole resolved by compound-specific isotope analysis, 13 C NMR, and density-functional theory

Compound-specific isotope analysis (CSIA), position-specific isotope analysis (PSIA), and computational modeling (e.g., quantum mechanical models; reactive-transport models) are increasingly being used to monitor and predict biotic and abiotic transformations of organic contaminants in the field. However, identifying the isotope effect(s) associated with a specific transformation remains challenging in many cases. We describe and interpret the position-specific isotope effects of C and N associated with a SN 2 Ar reaction mechanism by a combination of CSIA and PSIA using quantitative 13 C nuclear magnetic resonance spectrometry, and density-functional theory, using 2,4-dinitroanisole (DNAN) as a model compound. The position-specific 13 C enrichment factor of O–C 1 bond at the methoxy group attachment site (ε C1 ) was found to be approximately -41‰, a diagnostic value for transformation of DNAN to its reaction products 2,4-dinitrophenol and methanol. Theoretical kinetic isotope effects calculated for DNAN isotopologues agreed well with the position-specific isotope effects measured by CSIA and PSIA. This combination of measurements and theoretical predictions demonstrates a useful tool for evaluating degradation efficiencies and/or mechanisms of organic contaminants and may promote new and improved applications of isotope analysis in laboratory and field investigations.

13C NMR↗