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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Neutron generation dynamics inside a MA-class dense plasma focus Z-pinch

Dense plasma focii (DPFs) are appealing as energy efficient sources of short pulses of ions, neutrons, and x rays. The output of these sources is expected to scale with input current (I4), but has been shown to drop at the MA level [S. K. H. Auluck, “On the failure of neutron yield scaling in the dense plasma focus,” Phys. Plasmas 30, 080701 (2023)]. New results on the MegaJOuLe Neutron Imaging Radiography DPF showed neutron yield production in agreement with the input current scaling beyond the previously observed drop. This work provides insight into the pinch formation on a DPF and reports on the two different mechanisms leading to neutron generation inside a DPF using a combination of kinetic simulations and experimental data. A combination of particle-in-cell (PIC) and 1D shock theory results are used to describe the pinch formation and disassembly and the corresponding thermonuclear and beam-target mechanisms. The temporal evolution of the pinch column predicted by the PIC simulations shows qualitative agreement with the experimental data from plasma photon emission as well as temporal neutron pulse shapes. In MJ-class DPFs, both thermonuclear and beam-target mechanisms can occur over the course of the implosion and contribute to the total neutron production. Hence the neutron source size of a DPF will change throughout the implosion. Experimental neutron radiographs show the increase in source size as the pinch breaks apart, in agreement with simulation's prediction.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1986

Effects of high-energy neutrino production and interactions on stars in close X-ray binaries

Limits are discussed that may be placed on binary systems in which a compact partner is a strong source of high-energy particles that produce photons, neutrinos, and other secondary particles in the companion star. The highest energy neutrinos are absorbed deep in the companion and the associated energy deposition may be large enough to affect its structure or lead to its ultimate disruption. This neutrino heating is evaluated, starting with a detailed numerical calculation of the hadronic cascade induced in the atmosphere of the companion star. For some theoretical models, the resulting energy deposition from neutrino absorption may be so great as to disrupt the companion star over a time scale of 10,000-100,000 yr. Even if the energy deposition is smaller, it may still be high enough to alter the system substantially.

Gaisser, T. K.↗
DOE OSTI2023

Completely dark matter from rapid-turn multifield inflation

We study cosmological gravitational particle production as applied to “rapid-turn” models of inflation involving two scalar fields. We are interested in the production of massive spin-0 particles that only interact gravitationally and provide a candidate for the dark matter. Specifically, we study two models of rapid-turn multifield inflation, motivated in part by the de Sitter swampland conjecture, that are distinguished by the curvature of field space and the presence or absence of field space ‘angular momentum’ conservation. We find that one of these models leads to insufficient particle production and cannot explain the observed dark matter relic abundance. The second model is able to explain the origin of spin-0 dark matter via gravitational production, and we identify the relevant region of parameter space that is consistent with measurements of the dark-matter relic abundance, the dark-matter-photon isocurvature perturbations, and the spectrum of curvature perturbations that is probed by cosmological observations. Our work demonstrates the compatibility of the de Sitter swampland conjecture with completely dark matter.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Investigating the Role π -Rich Solvents Play in the Growth of Cesium Lead Bromide Nanocrystals

In this report, the role that a high-boiling-point solvent type plays on the nucleation and growth, morphology, and crystal-phase transformation of cesium lead bromide nanocrystals (CsPbBr 3 ) is studied. The CsPbBr 3 products were compared between a one-pot growth mechanism at room temperature (RT) versus a hot-injection mechanism (HI) control using dibenzyl ether (DBE), diphenyl ether (DPE), dioctyl ether (DOE), or 1- octadecene (ODE). The coordination between these solvents and the PbBr 2 salt precursors resulted in different plumbate [PbSBr n ] 2−n precursors being formed. The S-to-Pb 2+ coordination within [PbSBr n ] 2−n was probed by UV−vis and solvent-phase 207 Pb NMR, both of which showed considerable coordination between [PbSBr n ] 2−n and the π-rich DBE and DPE, whose reactivity affected CsPbBr 3 growth. The effect was more pronounced for CsPbBr 3 prepared via RT, where the morphology was tunable, with π-rich solvents producing thin rod-like CsPbB r3 with a blue emission, compared to the green-emitting thicker platelets formed via HI. While XRD showed crystalline products for both RT and HI, with orthorhombic and cubic forms, respectively, the RT products had considerable surface defects, as was indicated by lower quantum yields, and to understand this the photoluminescent lifetimes were measured by time-correlated single photon counting.

207Pb NMR↗
DOE OSTI2021

Studying Interfacial Dark Reactions of Glyoxal and Hydrogen Peroxide Using Vacuum Ultraviolet Single Photon Ionization Mass Spectrometry

Aqueous secondary organic aerosol (aqSOA) formation from volatile and semivolatile organic compounds at the air–liquid interface is considered as an important source of fine particles in the atmosphere. However, due to the lack of in situ detecting techniques, the detailed interfacial reaction mechanism and dynamics still remain uncertain. In this study, synchrotron-based vacuum ultraviolet single-photon ionization mass spectrometry (VUV SPI-MS) was coupled with the System for Analysis at the Liquid Vacuum Interface (SALVI) to investigate glyoxal dark oxidation products at the aqueous surface. Mass spectral analysis and determination of appearance energies (AEs) suggest that the main products of glyoxal dark interfacial aging are carboxylic acid related oligomers. Furthermore, the VUV SPI-MS results were compared and validated against those of in situ liquid time-of-flight secondary ion mass spectrometry (ToF-SIMS). The reaction mechanisms of the dark glyoxal interfacial oxidation, obtained using two different approaches, indicate that differences in ionization and instrument operation principles could contribute to their abilities to detect different oligomers. Therefore, the mechanistic differences revealed between the VUV SPI-MS and ToF-SIMS indicate that more in situ and real-time techniques are needed to investigate the contribution of the air–liquid interfacial reactions leading to aqSOA formation.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

GRB 221009A: The B.O.A.T. Burst that Shines in Gamma Rays

We present a complete analysis of Fermi Large Area Telescope (LAT) data of GRB 221009A, the brightest gamma-ray burst (GRB) ever detected. The burst emission above 30 MeV detected by the LAT preceded, by 1 s, the low-energy (<10 MeV) pulse that triggered the Fermi Gamma-Ray Burst Monitor (GBM), as has been observed in other GRBs. The prompt phase of GRB 221009A lasted a few hundred seconds. It was so bright that we identify a bad time interval of 64 s caused by the extremely high flux of hard X-rays and soft gamma rays, during which the event reconstruction efficiency was poor and the dead time fraction quite high. The late-time emission decayed as a power law, but the extrapolation of the late-time emission during the first 450 s suggests that the afterglow started during the prompt emission. We also found that high-energy events observed by the LAT are incompatible with synchrotron origin, and, during the prompt emission, are more likely related to an extra component identified as synchrotron self-Compton (SSC). A remarkable 400 GeV photon, detected by the LAT 33 ks after the GBM trigger and directionally consistent with the location of GRB 221009A, is hard to explain as a product of SSC or TeV electromagnetic cascades, and the process responsible for its origin is uncertain. Because of its proximity and energetic nature, GRB 221009A is an extremely rare event.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1994

Predissociation in N2(C'4, 1 Sigma u +) and other N2 states and its importance in the atmospheres of Titan and Triton

The objectives of this program are to further the understanding of the upper atmospheres of Titan, Triton, and the Earth in terms of the observed emissions of the 13-14 eV states of N2. These states are generated at quite high rates, yet very little emission is observed from them. The reasons are complex, involving resonance trapping and predissociation, and it is desired to quantify the effects of predissociation, particularly on the c(sub 4)' 1 Sigma(sub u),(sup +) state of N2. Earlier experiments had indicated that predissociation of the c(sub 4)' state was of little importance, yet over the last two years a growing body of evidence has shown that for levels above v = 2, predissociation is in fact a major process. It is the v = 0 level for which production by electron bombardment and photoexcitation is highest, and so it has been most important to evaluate the effects of predissociation on this particular level. The goal has been to target c(sub 4)' (v = 0) for a thorough analysis, in which both the extent of predissociation as a function of rotational level and the atomic product branching ratio, where the only possible products are N(4S) + N(4S) and N(2D) + N(4S), are determined. For the first year of funding, the intention was to demonstrate two-photon excitation of the intermediate N2(a(sup 1) Pi(sub g)) state, so that the gap to the 13 eV energy region could be bridged, and then use a second laser to reach the c(sub 4)' state itself.

Slanger, Tom G.↗
NASA NTRS2016

Shrink Tape Technique for Heat Forming Aluminum Substrates for Thin Foil X-Ray Mirrors and the Neutron Star Interior Composition Explorer X-Ray Concentrators

Consistent improvements in the design and fabrication of thin-foil, epoxy-replicated x-ray mirrors for astronomical telescopes have yielded increasingly higher quality and more precise astrophysical data. The Neutron Star Interior Composition Explorer (NICER) x-ray timing mission optics continues this tradition and introduces design elements that promise even more accurate measurements and precise astrophysical parameters. The singly reflecting concentrators have a curved axial profile to improve photon concentration and a sturdy full shell structure for enhanced module stability. These design elements introduced the challenge of reliably forming mirror substrates at an acceptable production rate. By developing a technique using heat shrink tape to compress and conform thin aluminum mirror substrates to shaping mandrels, production rate improved with successful fabrication. The technique's efficiency was analyzed by measuring hundreds of substrate profiles postforming, performance testing completely assembled concentrators composed of every size substrate, and comparing the results to simulated fabrication scenarios. On average, the profiles were copied within 4.6 plus or minus 3.7 percent. These measurements and the overall success of NICER's optics, via ground calibration, have shown that the heat-shrink tape method is reliable, repeatable, and could be used in future missions to increase production rate and improve performance.

Balsamo, Erin↗
DOE OSTI2024

Semi-inclusive single-jet production in DIS at next-to-leading order in the Color Glass Condensate

Within the Color Glass Condensate (CGC) effective field theory, we derive the next-to-leading order (NLO) cross-section for the single-jet semi-inclusive cross-section in deep inelastic scattering (DIS) at small x, for both longitudinally and transversely polarized virtual photons. We provide analytic expressions, valid at finite N c and suitable for numerical evaluation, for both the cross-section differential in rapidity and transverse momentum and the cross-section differential in rapidity only. Our NLO formulae demonstrate that the very forward rapidity regime is plagued by large double logarithmic corrections coming from phase space constraints on soft gluons close to the kinematic threshold for jet production. A joint resummation of small-x and threshold logarithms at single logarithmic accuracy is proposed to remedy the instability of the cross-section in this regime. By integrating over the single-jet phase space, we recover known results for the NLO DIS structure functions at small x, previously obtained using the optical theorem.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Gluon dipole factorisation for diffractive dijets

Within the colour dipole picture for deep inelastic scattering at small Bjorken x , we study the production of a pair of relatively hard jets via coherent diffraction. By “relatively hard” we mean that the transverse momenta of the two jets — the quark ($q$) and the antiquark ($\overline{q}$) generated by the decay of the virtual photon — are much larger than the target saturation momentum Q s (Y P ) evaluated at the rapidity gap Y P . We argue that the typical final-state configurations are such that the hard $q$$\overline{q}$ dijets are accompanied by a semi-hard gluon jet, with a transverse momentum of the order of Q s (Y P ). The presence of this third jet ensures that the scattering is strong and thus avoids the strong suppression of exclusive (hard) dijet production due to colour transparency. For such “2+1” jet configurations, we demonstrate that both the emission of the semi-hard gluon and its scattering with the hadronic target can be factorised in terms of an effective gluon-gluon dipole. This effective description, originally proposed in [1–7], builds a bridge between the colour dipole picture and the transverse-momentum dependent (TMD) version of the collinear factorisation: the cross-section for diffractive 2+1 jets can be written as the product between a hard factor describing the $q$$\overline{q}$ dijets and a semi-hard factor expressing the unintegrated gluon distribution of the Pomeron. The latter is controlled by gluon dipole scattering in the black disk limit and hence is strongly sensitive to gluon saturation. By integrating out the kinematics of the 3 jets, we obtain the $q$$\overline{q}$$g$ contribution to the diffractive structure function in collinearly-factorised form.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Search for continuous gravitational wave signals from luminous dark photon superradiance clouds with LVK O3 observations

Superradiance clouds of kinetically mixed dark photons around spinning black holes can produce observable multimessenger electromagnetic and gravitational wave signals. The cloud generates electric fields of up to a teravolt-per-meter, which leads to a cascade production of charged particles, yielding a turbulent quasiequilibrium plasma around the black hole, and resulting in electromagnetic fluxes ranging from supernova to pulsar-like luminosities. For stellar mass black holes, such systems resemble millisecond pulsars and are expected to emit pulsating radio waves and continuous gravitational waves (CWs) within the LIGO-Virgo-KAGRA (LVK) sensitivity band. We select 44 sources with approximately coincident frequencies or positive frequency drifts from existing pulsar catalogs as potential candidates of long-lasting superradiance clouds around old Galactic black holes. For a subset of 34 sources that are well measured and have not been previously targeted, we perform the first search for CW emission in LVK data from the third observing run. We find no evidence of a CW signal and place 95% confidence level upper limits on the emitted strain amplitude. We interpret these results, together with limits from previous searches, in terms of the underlying dark photon theory by performing an analysis of the expected signals from superradiance clouds from Galactic black holes. Finally, we find that, even for moderately spinning black holes, the absence of an observed CW signal disfavors a discrete set of dark photon masses between about 10 −13 and 10 −12 eV/c 2 and kinetic mixing couplings in the range of 10 −9 –10 −7 , subject to assumptions about the properties of the black hole population and the cloud’s electromagnetic emission.

astronomical black holes↗
DOE OSTI2023

Characterization of a platform for the gas transport, collection, and identification of fission products in the high-intensity laser environment

Recent progress in the production of laser accelerated high flux proton beams opens new possibilities for the study of fission in unique environments. To this end, we are currently pursuing the development of a platform for the swift gas transport, collection, and identification of fission products. Fission is induced in targets fixed inside a sealed chamber through which a carrier gas flows, transporting fission products to a carbon filter for collection and online spectroscopy. This has been recently demonstrated using target normal sheath accelerated protons at the PHELIX laser facility. There were large discrepancies between measured rates and those expected based on established fission yields and measured beam parameters. These discrepancies prompted a large number of tests at the Idaho Accelerator Center (IAC), where fission in uranium is induced by bremsstrahlung photons generated by 21 MeV electrons from a linear electron accelerator. Here, the results are compared to a series of models that account for the slowing of energetic fission fragments in the carrier gas and the fluid dynamics of the gas flow that transports fission products to the collection filter. Characterization of the apparatus reveals a few mechanisms that together account for a portion of the previously observed discrepancies at the PHELIX laser facility. However, additional research is necessary before high-accuracy experiments can be performed with the apparatus. Work performed under the auspices of the U.S. Department of Energy by LLNL under contract DE-AC52-07NA27344.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Measurement of the cross-sections of the electroweak and total production of a Zγ pair in association with two jets in pp collisions at s = 13 TeV with the ATLAS detector

This Letter presents the measurement of the fiducial and differential cross-sections of the electroweak production of a Zγ pair in association with two jets. The analysis uses 140 fb –1 of LHC proton–proton collision data taken at $\sqrt{s}$ = 13 TeV recorded by the ATLAS detector during the years 2015–2018. Events with a Z boson candidate decaying into either an e + e – or μ + μ – pair, a photon and two jets are selected. The electroweak component is extracted by requiring a large dijet invariant mass and by using the information about the centrality of the system and is measured with an observed and expected significance well above five standard deviations. The fiducial pp→Zγjj cross-section for the electroweak production is measured to be 3.6 ± 0.5 fb. The total fiducial cross-section that also includes contributions where the jets arise from strong interactions is measured to be $16.8_{–1.8}^{+2.0}$ fb. The results are consistent with the Standard Model predictions. Differential cross-sections are also measured using the same events and are compared with parton-shower Monte Carlo simulations. Good agreement is observed between data and predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Revisiting supernova constraints on a light CP-even scalar

A light CP-even Standard Model (SM) gauge-singlet scalar S can be produced abundantly in the supernova core, via the nucleon bremsstrahlung process NN → NNS, due to its mixing with the SM Higgs boson. Including the effective S coupling to both nucleons and the pion mediators, we evaluate the production amplitude for the S particle and point out a key difference with the well-known light CP-odd scalar (axion) and vector boson (dark photon) cases. Taking the subsequent decay and re-absorption of S into account, we present a complete calculation of the energy loss rate for the S particle. We then use the SN1987A luminosity constraints to derive updated supernova limits on the mixing of the scalar S with the SM Higgs boson. We find that the mixing angle sin θ with the SM Higgs is excluded only in the narrow range of 3.9 × 10 -7 to 7.0 × 10 -6 , depending on the scalar mass up to about 147 MeV, beyond which the supernova limit disappears.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1984

The nitrogen cycle: Atmosphere interactions

Atmospheric interactions involving the nitrogen species are varied and complex. These interactions include photochemical reactions, initiated by the absorption of solar photons and chemical kinetic reactions, which involve both homogeneous (gas-to-gas reactions) and heterogeneous (gas-to-particle) reactions. Another important atmospheric interaction is the production of nitrogen oxides by atmospheric lightning. The nitrogen cycle strongly couples the biosphere and atmosphere. Many nitrogen species are produced by biogenic processes. Once in the atmosphere nitrogen oxides are photochemically and chemically transformed to nitrates, which are returned to the biosphere via precipitation, dry deposition and aerosols to close the biosphere-atmosphere nitrogen cycle. The sources, sinks and photochemistry/chemistry of the nitrogen species; atmospheric nitrogen species; souces and sinks of nitrous oxide; sources; sinks and photochemistry/chemistry of ammonia; seasonal variation of the vertical distribution of ammonia in the troposphere; surface and atmospheric sources of the nitrogen species, and seasonal variation of ground level ammonia are summarized.

Levine, J. S.↗
NASA NTRSDate not supplied

AMEGO: Exploring the Extreme Multimessenger Universe

The All-sky Medium Energy Gamma-ray Observatory (AMEGO) is a Probe-class mission concept that will provide essential contributions to multimessenger astrophysics in the next decade. AMEGO operates both as a Compton and pair telescope to achieve unprecedented sensitivity between 200 keV and>5 GeV. The instrument consists of four subsystems. A double-sided strip silicon Tracker gives a precise measure of the first Compton scatter interaction and tracks of pair-conversion products. A novel CdZnTe Low Energy Calorimeter with excellent position and energy resolution surrounds the bottom and sides of the Tracker to detect the Compton-scattered photons which enhances the polarization and narrow-line sensitivity. A thick CsI High Energy Calorimeter contains the high-energy Compton and pair events. The instrument is surrounded by aplastic anti-coincidence detector to veto the cosmic-ray background. We have performed detailed simulations to predict the telescope performance and are currently building a prototype instrument. The AMEGO prototype, known as ComPair, will be tested at the High Intensity Gamma-Ray Source in 2021, followed by a balloon flight in Fall of 2022. In this presentation we will give an overview of the science motivation, a description of the observatory, and an update of the prototype instrument development.

Carolyn Ann Kierans↗
DOE OSTI2021

The importance of kinematic twists and genuine saturation effects in dijet production at the Electron-Ion Collider

We compute the differential yield for quark anti-quark dijet production in high-energy electron-proton and electron-nucleus collisions at small x as a function of the relative momentum P ⊥ and momentum imbalance k ⊥ of the dijet system for different photon virtualities Q 2 , and study the elliptic and quadrangular anisotropies in the relative angle between P ⊥ and k ⊥ . We review and extend the analysis in [1], which compared the results of the Color Glass Condensate (CGC) with those obtained using the transverse momentum dependent (TMD) framework. In particular, we include in our comparison the improved TMD (ITMD) framework, which resums kinematic power corrections of the ratio k ⊥ over the hard scale Q ⊥ . By comparing ITMD and CGC results we are able to isolate genuine higher saturation contributions in the ratio Q s /Q ⊥ which are resummed only in the CGC. These saturation contributions are in addition to those in the Weizsäcker-Williams gluon TMD that appear in powers of Q s /k ⊥ . We provide numerical estimates of these contributions for inclusive dijet production at the future Electron-Ion Collider, and identify kinematic windows where they can become relevant in the measurement of dijet and dihadron azimuthal correlations. We argue that such measurements will allow the detailed experimental study of both kinematic power corrections and genuine gluon saturation effects.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Photon-In/Photon-Out X-ray Free-Electron Laser Studies of Radiolysis

Understanding the origin of reactive species following ionization in aqueous systems is an important aspect of radiation–matter interactions as the initial reactive species lead to production of radicals and subsequent long-term radiation damage. Tunable ultrafast X-ray free-electron pulses provide a new window to probe events occurring on the sub-picosecond timescale, supplementing other methodologies, such as pulse radiolysis, scavenger studies, and stop flow that capture longer timescale chemical phenomena. We review initial work capturing the fastest chemical processes in liquid water radiolysis using optical pump/X-ray probe spectroscopy in the water window and discuss how ultrafast X-ray pump/X-ray probe spectroscopies can examine ionization-induced processes more generally and with better time resolution. Ultimately, these methods will be applied to understanding radiation effects in complex aqueous solutions present in high-level nuclear waste.

47 OTHER INSTRUMENTATION↗