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NASA NTRS1998

Turbulence Measurements on a Flap-Edge Model

Turbulence measurements have been made on a flap-edge and leading-edge slat model using hot-wire anemometry, and, later, particle image velocimetry. The properties of hot-wire anemometry were studied using facilities at NASA Ames Research Center. Hot-film probes were used because of their durability, but cross-films were limited by non-linear end effects. As a warm-up exercise, hot-film probes were used to measure velocities in the farfield wake of a cylinder with an airfoil in the near-field wake. The airfoil reduced the drag coefficient of the system by 10%. A single-wire hot-film probe was used to measure velocity profiles over the top of a NACA 63(sub 2)-215 Mod. B wing with a Fowler flap and leading,-edge slat. Results showed the size of slat wake was dependent upon the slat deflection angle. Velocity increased through the slat gap with increased deflection. The acoustically modified slat decreased the chance of separation. Measurements were taken at the flap edge with a single hot-film. Trends in the data indicate velocity and turbulence levels increase at the flap edge. The acoustically modified flap modifies the mean flow near the flap edge. Correlations were made between the hot-film signal and the unsteady pressure transducers on the wing which were published in a NASA CDTM. The principles of Particle Image Velocimetry (PIV) were studied at Florida State University. Spectral PIV was used to measure the spectra of a subsonic jet. Measured frequencies were close to the predicted frequency of jet shedding. Spectral PIV will be used to measure the spectra of the slat flow in the second 7 x lO-ft. wind tunnel test. PIV has an advantage that it can measure velocity and spectra of the entire flowfield instantaneously. However, problems arise when trying, to store this massive amount of PIV data. Support for this research has continued through a NASA Graduate Student Program Fellowship which will end in June 1999. The thesis should be completed by this time.

Moriarty, Patrick↗
NASA NTRS1998

CART and GSFC raman lidar measurements of atmospheric aerosol backscattering and extinction profiles for EOS validation and ARM radiation studies

The aerosol retrieval algorithms used by the Moderate-Resolution Imaging Spectroradiometer (MODIS) and Multi-Angle Imaging SpectroRadiometer (MISR) sensors on the Earth Observing Satellite (EOS) AM-1 platform operate by comparing measured radiances with tabulated radiances that have been computed for specific aerosol models. These aerosol models are based almost entirely on surface and/or column averaged measurements and so may not accurately represent the ambient aerosol properties. Therefore, to validate these EOS algorithms and to determine the effects of aerosols on the clear-sky radiative flux, we have begun to evaluate the vertical variability of ambient aerosol properties using the aerosol backscattering and extinction profiles measured by the Cloud and Radiation Testbed (CART) and NASA Goddard Space Flight Center (GSFC) Raman Lidars. Using the procedures developed for the GSFC Scanning Raman Lidar (SRL), we have developed and have begun to implement algorithms for the CART Raman Lidar to routinely provide profiles of aerosol extinction and backscattering during both nighttime and ,daytime operations. Aerosol backscattering and extinction profiles are computed for both lidar systems using data acquired during the 1996 and 1997 Water Vapor Intensive Operating Periods (IOPs). By integrating these aerosol extinction profiles, we derive measurements of aerosol optical thickness and compare these with coincident sun photometer measurements. We also use these measurements to measure the aerosol extinction/backscatter ratio S(sub a) (i.e. 'lidar ratio'). Furthermore, we use the simultaneous water vapor measurements acquired by these Raman lidars to investigate the effects of water vapor on aerosol optical properties.

Ferrare, R. A.↗
NASA NTRS1998

Raman Lidar Measurements of Aerosol Extinction and Backscattering: Methods and Comparisons - Report 1

This paper examines the aerosol backscattering and extinction profiles measured at night by the NASA Goddard Space Flight Center Scanning Raman Lidar (SRL) during the remote cloud sensing (RCS) intensive operations period (IOP) at the Department of Energy Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) site in April 1994. These lidar data are used to derive aerosol profiles for altitudes between 0.0 1 5 and 5 km. Since this lidar detects Raman scattering from nitrogen and oxygen molecules as well as the elastic scattering from molecules and aerosols, it measures both aerosol backscattering and extinction simultaneously. The aerosol extinction/backscattering ratio varied between approximately 30 sr and 75 sr at 351 nm. Aerosol optical thicknesses derived by integrating the lidar profiles of aerosol extinction measured at night between 0. I and 5 km are found to be about 10-40% lower than those measured by a Sun photometer during the day. This difference is attributed to the contribution by stratospheric aerosols not included in the lidar estimates as well as to diurnal differences in aerosol properties and concentrations. Aerosol profiles close to the surface were acquired by pointing the lidar nearly horizontally. Measurements of aerosol scattering from a tower-mounted nephelometer are found to be 40% lower than lidar measurements of aerosol extinction over a wide range of relative humidities even after accounting for the difference in wavelengths. The reasons for this difference are not clear but may be due to the inability of the nephelometer to accurately measure scattering by large particles.

Ferrare, R. A.↗
NASA NTRS1999

Radiometric Measurement Comparisons Using Transfer Radiometers in Support of the Calibration of NASA's Earth Observing System (EOS) Sensors

EOS satellite instruments operating in the visible through the shortwave infrared wavelength regions (from 0.4 micrometers to 2.5 micrometers) are calibrated prior to flight for radiance response using integrating spheres at a number of instrument builder facilities. The traceability of the radiance produced by these spheres with respect to international standards is the responsibility of the instrument builder, and different calibration techniques are employed by those builders. The National Aeronautics and Space Administration's (NASA's) Earth Observing System (EOS) Project Science Office, realizing the importance of preflight calibration and cross-calibration, has sponsored a number of radiometric measurement comparisons, the main purpose of which is to validate the radiometric scale assigned to the integrating spheres by the instrument builders. This paper describes the radiometric measurement comparisons, the use of stable transfer radiometers to perform the measurements, and the measurement approaches and protocols used to validate integrating sphere radiances. Stable transfer radiometers from the National Institute of Standards and Technology, the University of Arizona Optical Sciences Center Remote Sensing Group, NASA's Goddard Space Flight Center, and the National Research Laboratory of Metrology in Japan, have participated in these comparisons. The approaches used in the comparisons include the measurement of multiple integrating sphere lamp levels, repeat measurements of select lamp levels, the use of the stable radiometers as external sphere monitors, and the rapid reporting of measurement results. Results from several comparisons are presented. The absolute radiometric calibration standard uncertainties required by the EOS satellite instruments are typically in the +/- 3% to +/- 5% range. Preliminary results reported during eleven radiometric measurement comparisons held between February 1995 and May 1998 have shown the radiance of integrating spheres agreed to within +/- 2.5% from the average at blue wavelengths and to within +/- 1.7% from the average at red and near infrared wavelengths. This level of agreement lends confidence in the use of the transfer radiometers in validating the radiance scales assigned by EOS instrument calibration facilities to their integrating sphere sources.

Butler, James J.↗
NASA NTRS1988

Infrared Measurements of Atmospheric Gases Above Mauna Loa, Hawaii, in February 1987

Infrared solar absorption spectra recorded at 0.02/ cm resolution from the National Oceanic and Atmospheric Administration (NOAA) Geophysical Monitoring for Climate Change (GMCC) program station at Mauna Loa, Hawaii (latitude 19.5 deg N, longitude 155.6 deg W, elevation 3.40 km), in February 1997 have been analyzed to determine simultaneous total vertical column amounts for 13 atmospheric gases. Average tropospheric concentrations of CO2, N2O, CH4, and CHCIF2 and the daytime diurnal variations or the total columns of NO and NO2 have also been inferred. The retrieved total columns (in molecules /sq cm) of the nondiurnally varying gases are 1.6 +/- 0.2 x 10(exp 15) for HCl, 5.9 +/- 1.2 x 10(exp 15) for HNO3, 2.0 +/- 0.2 x 10(exp 21) for H2O16, 4.4 +/- 0.7 x 10(exp 18) for H2O18, 2.7 +/- 0.1 x 10(exp 17) for HDO, 2.3 +/- 0.2 x 10(exp 19) for CH4, 5.0 +/- 0.5 x 10(exp 21) for CO2, 6.7 +/- 0.8 x 10(exp 18) for O3, 4.3 +/- 0.4 x 10(exp 18) for N2O, 1.0 +/- 0.2 x 10(exp 16) for C2H6, and 9.7 +/- 2.5 x 10(exp 14) for CHClF2. We compare the total column measurements of HCl and HNO3 with previously reported ground-based, aircraft, and satellite measurements. The results for HCl are or particular interest because of the expected temporal increase in the concentration of this gas in the stratosphere. However, systematic differences among stratospheric HCl total column measurements from 1978 to 1980 and the absence of observations of free tropospheric HCl above Mauna Loa make it impossible to obtain a reliable estimate of the trend in the total burden of HCl. The measured HNO3 total column is consistent with aircraft measurements from approx. 12 km altitude. The O3 total column deduced from the IR spectra agrees with correlative Mauna Loa Umkehr measurements within the estimated error limits. The column-averaged D/H ratio of water vapor is (68 +/- 9) x- 10(exp -6), which is 0.44 +/- 0.06 times the reference value of 155.76 x 10(exp -6) for standard mean ocean water (SMOW). This large depletion in the D content of water vapor is similar to published measurements of the upper troposphere and lower stratosphere. Average tropospheric concentrations deduced for CO2, N2O, and CH4 are in good agreement with correlative NOAA GMCC surface data, indicating consistency between the measurement techniques for determining tropospheric volume mixing ratios. Results of the present study indicate that Mauna Loa is a favorable site for infrared monitoring of atmospheric gases. The site is particularly favorable for monitoring the tropospheric volume mixing ratios of long-lived gases, since the high altitude of the tropopause reduces corrections required to account for the decrease in volume mixing ratio in the stratosphere.

Rinsland, C. P.↗
NASA NTRS1995

Laboratory Investigation of Direct Measurement of Ice Water Content, Ice Surface Area, and Effective Radius of Ice Crystals Using a Laser-Diffraction Instrument

The aircraft microphysics probe, PVM-100A, was tested in the Colorado State University dynamic cloud chamber to establish its ability to measure ice water content (IWC), PSA, and Re in ice clouds. Its response was compared to other means of measuring those ice-cloud parameters that included using FSSP-100 and 230-X 1-D optical probes for ice-crystal concentrations, a film-loop microscope for ice-crystal habits and dimensions, and an in-situ microscope for determining ice-crystal orientation. Intercomparisons were made in ice clouds containing ice crystals ranging in size from about 10 microns to 150 microns diameter, and ice crystals with plate, columnar, dendritic, and spherical shapes. It was not possible to determine conclusively that the PVM accurately measures IWC, PSA, and Re of ice crystals, because heat from the PVM evaporated in part the crystals in its vicinity in the chamber thus affecting its measurements. Similarities in the operating principle of the FSSP and PVM, and a comparison between Re measured by both instruments, suggest, however, that the PVM can make those measurements. The resolution limit of the PVM for IWC measurements was found to be on the order of 0.001 g/cubic m. Algorithms for correcting IWC measured by FSSP and PVM were developed.

Gerber, H.↗
NASA NTRS2000

North Atlantic Aerosol Radiative Impacts Based on Satellite Measurements and Aerosol Intensive Properties from TARFOX and ACE-2

We estimate the impact of North Atlantic aerosols on the net short-wave flux at the tropopause by combining satellite-derived aerosol optical depth (AOD) maps with model aerosol properties determined via closure analyses in TARFOX and ACE 2. We exclude African dust, primarily by restricting latitudes to 25-60 N. The analyses use in situ aerosol composition measurements and air- and ship-borne sun-photometer measurements of AOD spectra. The aerosol model yields computed flux sensitivities (dFlux/dAOD) that agree with measurements by airborne flux radiometers in TARFOX. Its midvisible single-scattering albedo is 0.9. which is in the range obtained from in situ measurements of scattering and absorption in both TARFOX and ACE 2. Combining satellite-derived AOD maps with the aerosol model yields maps of 24-hour average net radiative flux changes. For simultaneous AVHRR, radiance measurements exceeded the sunphotometer AODs by about 0.04. However. shipboard sunphotometer and AVHRR AODs agreed Within 0.02 for data acquired during satellite overflights on two other days. We discuss attempts to demonstrate column closure within the MBL by comparing shipboard sunphotometer AODs and values calculated from simultaneous shipboard in-situ aerosol size distribution measurements. These comparisons were mostly unsuccessful, but they illustrate the difficulties inherent in this type of closure analysis. Specifically, AODs derived from near-surface in-situ size distribution measurements are extremely sensitive to the assumed hygroscopic growth model that itself requires an assumption of particle composition as a function of height and size, to the radiosonde-measured relative humidity, and to the vertical profile of particle number. We investigate further the effects of hygroscopic particle growth within the MBL by using shipboard lidar aerosol backscatter profiles together with the sunphotometer AOD.

Russell, P. B.↗
NASA NTRS2000

Salinity Measurements During the Gulf Stream Experiment

The salinity of the open ocean is important for understanding ocean circulation, for understanding energy exchange with the atmosphere and for improving models to predict weather and climate. Passive microwave sensors at L-band (1.4 GHz) operating from aircraft have demonstrated that salinity can be measured with sufficient accuracy (1 psu) to be scientifically meaningful in coastal waters. However, measuring salinity in the open ocean presents unresolved issues largely because of the much greater accuracy (approx. 0.1 psu) required to be scientifically viable. In the summer of 1999 a series of measurements called, The Gulf Stream Experiment, were conducted as part of research at the Goddard Space Flight Center to test the potential for passive microwave remote sensing of salinity in the open ocean. The measurements consisted of a compliment of airborne microwave instruments (radiometers and scatterometer) and ships and drifters for surface truth. The study area was a 200 km by 100 km rectangle about 250 km east of Delaware Bay between the continental shelf waters and north wall of the Gulf Stream. The primary passive instruments were the ESTAR radiometer (L-band, H-pol) and the SLFMR radiometer (L-band, V-pol). In addition, the compliment of instruments on the aircraft included a C-band radiometer (ACMR), an ocean wave scatterometer (ROWS) and an infrared radiometer. A GPS backscatter experiment was also part of the package. These instruments were mounted on the NASA P-3 Orion aircraft. Surface salinity measurements were provided by the RN Cape Henlopen and MN Oleander (thermosalinographs) plus salinity and temperature sensors on three surface drifters deployed from the RN Cape Henopen. The primary experiment period was August 26-September 2, 1999. During this period the salinity field within the study area consisted of a gradient on the order of 2-3 psu in the vicinity of the shelf break and a warm core ring with a gradient of 1-2 psu. Detailed maps were made with the airborne sensors on August 28 and 29 and on September 2 flights were made over the surface drifters to look for effects due to a change in surface roughness resulting from the passage of Hurricane Dennis. Preliminary results show a good agreement between the microwave measurements and ship measurements of salinity. The features of the brightness temperature maps correspond well with the features of the salinity field measured by the ship and drifters and a preliminary retrieval of salinity compares well with the ship data.

LeVine, D. M.↗
NASA NTRS2000

Precision of Four Acoustic Bone Measurement Devices

Though many studies have quantified the precision of various acoustic bone measurement devices, it is difficult to directly compare the results among the studies, because they used disparate subject pools, did not specify the estimation methodology, or did not use consistent definitions for various precision characteristics. In this study, we used a repeated measures design protocol to directly determine the precision characteristics of four acoustic bone measurement devices: the Mechanical Response Tissue Analyzer (MRTA), the UBA-575+, the SoundScan 2000 (S2000), and the Sahara Ultrasound Done Analyzer. Ten men and ten women were scanned on all four devices by two different operators at five discrete time points: Week 1, Week 2, Week 3, Month 3 and Month 6. The percent coefficient of variation (%CV) and standardized coefficient of variation were computed for the following precision characteristics: interoperator effect, operator-subject interaction, short-term error variance, and long-term drift, The MRTA had high interoperator errors for its ulnar and tibial stiffness measures and a large long-term drift in its tibial stiffness measurement. The UBA-575+ exhibited large short-term error variances and long-term drift for all three of its measurements. The S2000's tibial speed of sound measurement showed a high short-term error variance and a significant operator-subject interaction but very good values ( < 1%) for the other precision characteristics. The Sahara seemed to have the best overall performance, but was hampered by a large %CV for short-term error variance in its broadband ultrasound attenuation measure.

Miller, Christopher↗
NASA NTRS2000

Precision of Four Acoustic Bone Measurement Devices

Though many studies have quantified the precision of various acoustic bone measurement devices, it is difficult to directly compare the results among the studies, because they used disparate subject pools, did not specify the estimation methodology, or did not use consistent definitions for various precision characteristics. In this study, we used a repeated measures design protocol to directly determine the precision characteristics of four acoustic bone measurement devices: the Mechanical Response Tissue Analyzer (MRTA), the UBA-575+, the SoundScan 2000 (S2000), and the Sahara Ultrasound Bone Analyzer. Ten men and ten women were scanned on all four devices by two different operators at five discrete time points: Week 1, Week 2, Week 3, Month 3 and Month 6. The percent coefficient of variation (%CV) and standardized coefficient of variation were computed for the following precision characteristics: interoperator effect, operator-subject interaction, short-term error variance, and long-term drift. The MRTA had high interoperator errors for its ulnar and tibial stiffness measures and a large long-term drift in its tibial stiffness measurement. The UBA-575+ exhibited large short-term error variances and long-term drift for all three of its measurements. The S2000's tibial speed of sound measurement showed a high short-term error variance and a significant operator-subject interaction but very good values (less than 1%) for the other precision characteristics. The Sahara seemed to have the best overall performance, but was hampered by a large %CV for short-term error variance in its broadband ultrasound attenuation measure.

Miller, Christopher↗
NASA NTRS1999

Sea Surface Slope Statistics for Intermediate and Shore Scale Ocean Waves Measured Using a Low-Altitude Aircraft

Ocean surface remote sensing techniques often rely on scattering or emission linked to shorter- scale gravity-capillary ocean wavelets. However, it is increasingly apparent that slightly longer wavelengths of O(10 to 500 cm) are vital components in the robust sea surface description needed to link varied global remote sensing data sets. This paper describes a sensor suite developed to examine sea surface slope variations in the field using an aircraft flying at very low altitude (below 30 m) and will also provide preliminary measurements detailing changes in slope characteristics versus sea state and friction velocity. Two-dimensional surface slope is measured using simultaneous range measurements from three compact short-range laser altimeters mounted in an equilateral triangle arrangement with spacing of about 1 m. In addition, all three lasers provide independent wave elevation profiles after GPS-aided correction for aircraft altitude. Laser range precision is 1 cm rms while vertical motion correction is 15 cm rms. The measurements are made along-track at approximately 1 m intervals setting the spatial scale of the measurement to cover waves of intermediate to long scale. Products available for this array then include surface elevation, two-dimensional slope distribution, and the cross- and along-track 1-D slope distributions. To complement the laser, a down-looking mm-wave radar scatterometer is centered within the laser array to measure radar backscatter simultaneously with the laser slope. The radar's footprint is nominally 1 m in diameter. Near-vertical radar backscatter is inversely proportional to the small-scale surface slope variance and to the tilt of the underlying (laser-measured) surface facet. Together the laser and radar data provide information on wave roughness from the longest scales down to about 1 cm. These measurements are complemented by aircraft turbulence probe data that provides robust surface flux information.

Vandemack, Douglas↗
NASA NTRS2000

Quantitative Measurements of Nitric Oxide Concentration in High-Pressure, Swirl-Stabilized Spray Flames

Lean direct-injection (LDI) spray flames offer the possibility of reducing NO(sub x) emissions from gas turbines by rapid mixing of the liquid fuel and air so as to drive the flame structure toward partially-premixed conditions. We consider the technical approaches required to utilize laser-induced fluorescence methods for quantitatively measuring NO concentrations in high-pressure LDI spray flames. In the progression from atmospheric to high-pressure measurements, the LIF method requires a shift from the saturated to the linear regime of fluorescence measurements. As such, we discuss quantitative, spatially resolved laser-saturated fluorescence (LSF), linear laser-induced fluorescence (LIF), and planar laser-induced fluorescence (PLIF) measurements of NO concentration in LDI spray flames. Spatially-resolved LIF measurements of NO concentration (ppm) are reported for preheated, LDI spray flames at pressures of two to five atmospheres. The spray is produced by a hollow-cone, pressure-atomized nozzle supplied with liquid heptane. NO is excited via the Q(sub 2)(26.5) transition of the gamma(0,0) band. Detection is performed in a two nanometer region centered on the gamma(0,1) band. A complete scheme is developed by which quantitative NO concentrations in high-pressure LDI spray flames can be measured by applying linear LIF. NO is doped into the reactants and convected through the flame with no apparent destruction, thus allowing a NO fluorescence calibration to be taken inside the flame environment. The in-situ calibration scheme is validated by comparisons to a reference flame. Quantitative NO profiles are presented and analyzed so as to better understand the operation of lean-direct injectors for gas turbine combustors. Moreover, parametric studies are provided for variations in pressure, air-preheat temperature, and equivalence ratio. Similar parametric studies are performed for lean, premixed-prevaporized flames to permit comparisons to those for LDI flames. Finally, PLIF is expanded to high pressure in an effort to quantify the detected fluorescence image for LDI flames. Success is achieved by correcting the PLIF calibration via a single-point LIF measurement. This procedure removes the influence of any preferential background that occurs in the PLIF detection window. In general, both the LIF and PLIF measurements verify that the LDI strategy could be used to reduce NO(sub x) emissions in future gas turbine combustors.

Cooper, Clayton S.↗
NASA NTRS2000

Continuing Measurements of CO2 Crystals with a Hand-Held 35 GHz Radiometer

In order to increase our knowledge of the Martian polar caps, an improved understanding of the behavior of both frozen H2O and CO2 in different parts of the electromagnetic spectrum is needed. The thermal microwave part of the spectrum has received relatively little attention compared to the visible and infrared wavelengths. A simple experiment to measure the brightness temperature of frozen CO2 was first performed in the winter of 1998 using a 35 GHz radiometer. in experiments performed during the winter of 1999 and 2000, passive microwave radiation emanating from within layers of manufactured CO2 (dry ice) crystals was again measured with a 35 GHz handheld radiometer. Both large (0.8 cm) and small (0.3 cm) cylindrical-shaped dry ice pellets, at a temperature of 197 K (-76 C), were measured. A 1 sq m plate of aluminum sheet metal was positioned beneath the dry ice so that microwave emissions from the underlying soil layers would be minimized. Non-absorbing foam was positioned around the sides of the plate in order to keep the dry ice in place and to assure that the incremental deposits were level. Thirty-five GHz measurements of this plate were made through the dry ice deposits in the following way. Layers of dry ice were built up and measurements were repeated for the increasing CO2 pack. First, 7 cm of large CO2 pellets were poured onto the sheet metal plate, then an additional 7 cm were added, and finally, 12 cm were added on top of the 14 cm base. Hand-held 35 GHz measurements were made each time the thickness of the deposit was increased. The same process was repeated for the smaller grain pellets. Furthermore, during the past winter, 35 GHz measurements were taken of a 25 kg (27 cm x 27 cm x 27 cm) solid cube Of CO2, which was cut in half and then re-measured. Additional information is contained in the original extended abstract.

Foster, J.↗
NASA NTRS2000

Ground Based, Millimeter Wave Measurement of Ozone in the Middle Atmosphere

There is a need for highly reliable measurements of stratospheric ozone. Policy makers worldwide concerned with public health rely oil a clear consensus from the scientific community as a basis for ozone-related environmental policy that has a significant impact oil national economies. Tile latest Such consensus was presented in WMO, and used in a 1999 meeting of the parties considering amendments to the Montreal Protocol oil Substances that Deplete the Ozone Layer. Tile scientific community, in turn, needs highly precise and accurate measurements of ozone levels, and small time derivatives of these levels, both in continued - development of its understanding of the physical and chemical processes involved and as clear evidence that these processes are occurring as stated. Over most of the world, changes in ozone levels are small. For example, over the heavily populated northern midlatitudes, the linearized rate of ozone decline is between 0.2% per year and 0.7% per year, depending on altitude. These values are small enough to make measurement requirements technically challenging. Data quality may suffer from imperfections in individual instruments. In one instance, early results from a satellite-borne ozone sensor were later found to be invalid because of calibration drift. Even in the absence of drift, tile absolute calibration of a new sensor may differ slightly from that of its predecessor in service. Most ozone remote sensing instruments operate at ultraviolet or infrared wavelengths where scattering from dust and aerosols must be taken into account; results from these systems may be or are affected following a major volcanic eruption, such as tile one at Mt. Pinatubo in 1991. Given these difficulties, a consensus of measurements from several independent systems is required to insure a reliable understanding of stratospheric ozone levels. Because of the above-described need for highly precise and accurate ozone measurements using several independent techniques, there was interest in developing several techniques which were known but not highly developed in the 1980's into systems capable of being used in ail operational manner to make measurements with the level of quality needed to-detect small trends in ozone levels. A ground-based microwave instrument capable of remotely sensing stratospheric ozone had been designed by tile Principal Investigator of the present project. This instrument was built at tile Millitech Corporation in South Deerfield, Massachusetts before tile present work began. (Funding for design and construction of the instrument came from sources other than the present grant.) Tile instrument measured the spectrum of one of the many emission lines produced by purely rotational transitions of ozone, one at a frequency of 110.8 GHz. The altitude distribution of ozone can. in principle, be retrieved from the details of the pressure-broadened spectrum of the ozone transition. However, the level of contamination of the spectral measurement by instrumentally induced artifacts must be very low in order to retrieve a ozone profile of useful quality from it. The Millitech instrument demonstrated spectral purity at ail adequate level, and there were promising ideas for instrumental improvements and for further development of the technique. The initial objectives of the present project, then, were to develop techniques for calibrating the Millitech instrument, to minimize artifacts in tile spectra it produces, to optimally retrieve ozone profiles from tile spectra, to test tile quality of the microwave profiles by comparing them with profiles obtained using several other, independent techniques over both short and periods of time, and to perform research using the ozone data gathered with the instrument.

Parrish, Alan↗
NASA NTRS2000

Desert Dust Layers Over Polluted Marine Boundary Layers: ACE-2 Measurements and ACE-Asia Plans

Aerosols in ACE-Asia are expected to have some commonalties with those in ACE-2, along with important differences. Among the commonalities are occurrences of desert dust layers over polluted marine boundary layers. Differences include the nature of the dust (yellowish in the East Asia desert outflow, vs. reddish-brown in the Sahara Outflow measured in ACE-2) and the composition of boundary-layer aerosols (e.g., more absorbing, soot and organic aerosol in-the Asian plume, caused by coal and biomass burning, with limited controls). In this paper we present ACE-2 measurements and analyses as a guide to our plans for ACE-2 Asia. The measurements include: (1) Vertical profiles of aerosol optical depth and extinction (380-1558 nm), and of water vapor column and concentration, from the surface through the elevated desert dust, measured by the 14-channel Ames Airborne Tracking Sunphotometer (AATS-14); (2) Comparisons of airborne and shipborne sunphotometer optical depths to satellite-retrieved values, with and without desert dust; (3) Comparisons between airborne Sunphotometer optical depth and extinction spectra and those derived from coincident airborne in situ measurements of aerosol size distribution, scattering and absorption; (4) Comparisons between size distributions measured in situ and retrieved from sunphotometer optical depth spectra; (5) Comparisons between aerosol single scattering albedo values obtained by several techniques, using various combinations of measurements of backscatter, extinction, size distribution, scattering, absorption, and radiative flux. We show how analyses of these data can be used to address questions important to ACE-Asia, such as: (1) How do dust and other absorbing aerosols affect the accuracy of satellite optical depth retrievals? How important are asphericity effects? (2) How important are supermicron dust and seasalt aerosols to overall aerosol optical depth and radiative forcing? How well are these aerosols sampled by aircraft inlets and instruments? (3) How consistent are suborbital in situ and remote measurements of aerosols, among themselves and with satellite retrievals? What are the main reasons for observed inconsistencies?

Russell, Philip B.↗
NASA NTRS2001

Information Retrieval from SAGE II and MFRSR Multi-Spectral Extinction Measurements

Direct beam spectral extinction measurements of solar radiation contain important information on atmospheric composition in a form that is essentially free from multiple scattering contributions that otherwise tend to complicate the data analysis and information retrieval. Such direct beam extinction measurements are available from the solar occultation satellite-based measurements made by the Stratospheric and Aerosol Gas Experiment (SAGE II) instrument and by ground-based Multi-Filter Shadowband Radiometers (MFRSRs). The SAGE II data provide cross-sectional slices of the atmosphere twice per orbit at seven wavelengths between 385 and 1020 nm with approximately 1 km vertical resolution, while the MFRSR data provide atmospheric column measurements at six wavelengths between 415 and 940 nm but at one minute time intervals. We apply the same retrieval technique of simultaneous least-squares fit to the observed spectral extinctions to retrieve aerosol optical depth, effective radius and variance, and ozone, nitrogen dioxide, and water vapor amounts from the SAGE II and MFRSR measurements. The retrieval technique utilizes a physical model approach based on laboratory measurements of ozone and nitrogen dioxide extinction, line-by-line and numerical k-distribution calculations for water vapor absorption, and Mie scattering constraints on aerosol spectral extinction properties. The SAGE II measurements have the advantage of being self-calibrating in that deep space provides an effective zero point for the relative spectral extinctions. The MFRSR measurements require periodic clear-day Langley regression calibration events to maintain accurate knowledge of instrument calibration.

Lacis, Andrew A.↗
NASA NTRS2000

Satellite and Skin Layer Effects on the Accuracy of Sea Surface Temperature Measurements from the GOES Satellites

The latest Geostationary Operational Environmental Satellites (GOES) have facilitated significant improvements in our ability to measure sea surface temperature (SST) from geostationary satellites. Nonetheless, difficulties associated with sensor calibration and oceanic near-surface temperature gradients affect the accuracy of the measurements and our ability to estimate and interpret the diurnal cycle of the bulk SST. Overall, measurements of SST from the GOES Imagers on the GOES 8-10 satellites are shown to have very small bias (less than 0.02 K) and rms differences of between 0.6 and 0.9 K relative to buoy observations. Separate consideration of individual measurement times, however, demonstrates systematic bias variations of over 0.6 K with measurement hour. These bias variations significantly affect both the amplitude and shape of estimates of the diurnal SST cycle. Modeled estimates of the temperature difference across the oceanic cool skin and diurnal thermocline show that bias variations up to 0.3 K can result from variability in the near-surface layer. Oceanic near-surface layer and known "satellite midnight" calibration effects, however, explain only a portion of the observed bias variations, suggesting other possible calibration concerns. Methods of explicitly incorporating skin layer and diurnal thermocline effects in satellite bulk SST measurements were explored in an effort to further improve the measurement accuracy. While the approaches contain more complete physics, they do not yet significantly improve the accuracy of bulk SST measurements due to remaining uncertainties in the temperature difference across the near-surface layer.

Wick, Gary A.↗
NASA NTRS1995

A Unified Picture of Pinatubo Aerosol Global-to Micro-Scale Evolution, From Space, Air, and Ground Measurements

We combine a variety of measurements to develop a composite picture of the post-Pinatubo aerosol and assess the consistency and uncertainties of the measurement and retrieval techniques. Satellite infrared spectroscopy, particle morphology, and evaporation temperature measurements are in accord with theoretical calculations in showing a dominant particle composition of H2SO4-H2O mixture, with H2SO4 weight fraction of 65-80% for most stratospheric temperatures and humidities. Important exceptions are: (1) the presence of volcanic ash at all altitudes initially and in a layer just above the tropopause until at least March 1992, and (2) much smaller H2SO4 weight fractions at the low temperatures attained in high latitude winters and at the tropical tropopause, Laboratory spectroscopy and theoretical calculations yield wavelength- and temperature-dependent refractive indices for the dominant H2SO4-H2O droplets. These in turn permit derivation of particle size spectra from measured optical depth spectra, for comparison to direct measurements by impactors and optical counters. All three techniques paint a generally consistent picture of the evolution of R(sub eff), the effective, or area-weighted, particle radius. In the first month after the eruption, although particle numbers increased by orders of magnitude, R(sub eff) was similar to the preemption value of 0.1 to 0.2 microns, because both small (r less than 0.2 microns) and large (r greater than 0.6 micron particles increased in number. Over the next 3-6 months, R(sub eff) increased to about 0.5 microns reflecting particle growth through condensation and coagulation. In general, R(sub eff) continued to increase for about a year after the eruption. Extinction spectra computed from in situ size distribution measurements are consistent with optical depth measurements, which show spectra with maxima initially at wavelengths of 0.42 microns or less, and thereafter progressively increasing to between 0.78 and 1 micron. Not until 1993 do optical depth spectra begin to show a clear return to the preemption signature of maximizing at the shortest visible wavelengths or in the near UV. This coupled evolution in particle size distribution and optical depth spectra helps explain the relationship between the global maps of 0.5- 1.0- micron optical depth derived from the AVHRR and SAGE satellite measurements.

Russell, Philip B.↗