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At least 829 records · Page 46

Examination of simulated behavior of ND-LAr and TMS detectors using CAFAna for DUNE analysis framework

Simulations are run using the new DUNE CAFAna framework to generate pseudo-data modeling the interactions of neutrinos in the DUNE near detector at truth-level and detector-level. Truth-level analysis of neutrino kinematics reveals strong agreement with expected behavior, validating the kinematic portion of the simulation. Examination of the detector-level reconstructions of coordinates of interaction vertex appear consistent with an interaction density independent of detector position. Track lengths of particles resultant from neutrino interactions are aligned with varied particle identities, but are misaligned with prediction of uniform position density.

Fein, Jarrett [Fermilab]↗

Integrated Approach to Post-Irradiation Examination of Nuclear Materials at Idaho National Laboratory

Idaho national Laboratory (INL) is the U.S. lead national laboratory for the Department of Energy’s Office of Nuclear Energy (DOE-NE), providing much of the nuclear research, development and demonstration capability needed to move nuclear innovation forward to deployment. INL’s Materials and Fuels Complex hosts a unique combination of personnel, facilities and infrastructure and offers the ability to perform post-irradiation examinations (PIE) of nuclear materials spanning multiple length scales. The ability to combine engineering-scale analysis and sub-microscopic characterization provides valuable insights into fuel and structural material behavior and degradation mechanisms. The holistic approach is used to accelerate these materials demonstration and deployment. Selected studies will be presented, highlighting the impact of these techniques on improving fuel reliability, safety, and efficiency, thereby advancing the development of sustainable and advanced nuclear energy technologies.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Post-irradiation examination of UN-Mo-W fuels for space nuclear propulsion

The National Aeronautics and Space Administration's return to space nuclear propulsion stems from the need for a more efficient method of space travel. Nuclear thermal propulsion systems have been shown to be two times more efficient than chemical propulsion. NASA's Sirius program was created to fabricate and test fuels for space nuclear propulsion, specifically to determine their performance under prototypical startup conditions. The Sirius project featured 4 test capsules, Sirius-1 featured uranium nitride fuel dispersed in a matrix of tungsten and rhenium, while Sirius-2A, -2B, and -3 featured uranium nitride-molybdenum-tungsten fuel (UN-Mo-W). This study discusses the Sirius-2A and -2B irradiation experiments at the Idaho National Laboratory, specifically their performance under irradiation at the Transient Reactor Test Facility. It was found that the fuel samples overall did not exhibit significant cracking, though the Sirius-2A fuel did have one large crack on the surface of the fuel. There was minimal hydrogen absorption in the samples, though it is unknown if the absorption occurred during irradiation or during fabrication. Mechanical testing indicated that the UN fuel demonstrated ceramic behavior as expected, and the Mo/W matrix demonstrated linear elastic behavior to failure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Micro X-ray computed tomography examination of mini plate fuel with hot isostatic pressed aluminum cladding

In order to minimize proliferation risks and improve security of nuclear material, the United States high performance research and test reactors (USHPRR) program is tasked with converting nuclear reactors that are fueled with highly enriched uranium (HEU) fuels to operate with low-enriched uranium (LEU) nuclear fuels. One favorable LEU fuel configuration is plate fuel with a metallic uranium-molybdenum foil clad within an aluminum alloy (AA 6061). In this fuel, the aluminum cladding is bonded with a hot isostatic pressing (HIP) method to seal the cladding around the fuel meat. However, the HIP process parameters influence the cladding performance, as a defective or incomplete bond can cause a pathway for corrosion. Micro X-ray computed tomography (XCT), a nondestructive technique that provides volumetric imaging, can be applied to inspect fuel plate cladding at the engineering scale. In this work, XCT methodology was developed and successfully utilized to not only observe the bond line of unirradiated mini fuel plates, but to also identify subsurface abnormalities in the plates’ cladding. Importantly, in future work, this technique could be applied to fuel plates, pre- and post-irradiation, to quantify irradiation effects on cladding defects and bond line integrity.

36 MATERIALS SCIENCE↗

Examining transport and integrated modeling predictive capabilities for negative-triangularity scenarios

This paper investigates the predictive capabilities of TGYRO and TGLF models in assessing the performance of negative triangularity (NT) plasmas compared to positive triangularity (PT) plasmas in fusion devices. TGYRO predicts kinetic profiles, while TGLF analyzes turbulent transport. The study reveals that TGYRO reasonably predicts NT profiles similar to PT, although it overpredicts the high-power scenarios where there is increased experimental MHD activity. TGLF analysis finds reduced linear growth rates in NT and altered flux spectra relative to PT. Additionally, the TGLF SAT0 saturation model is observed to predict high-k transport and a reduction of particle transport with the electron temperature gradient. These findings are further corroborated by core-pedestal modeling using the Stability Transport Equilibrium Pedestal workflow, showing stronger confinement improvements in NT, particularly at higher power densities for the SAT0 saturation model. Furthermore, the study underscores the importance of accurately capturing turbulence saturation mechanisms for NT in order to project its performance accurately in fusion reactors.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Evaluation of Manual Ultrasonic Examinations Applied to Detect Flaws in Primary System Dissimilar Metal Welds at North Anna Power Station

During a recent inservice inspection (ISI) of a dissimilar metal weld (DMW) in an inlet (hot leg) steam generator nozzle at North Anna Power Station Unit 1, several axially oriented flaws went undetected by the licensee's manual ultrasonic testing (UT) technique. The flaws were subsequently detected as a result of outside diameter (OD) surface machining in preparation for a full structural weld overlay. The machining operation uncovered the existence of two through-wall flaws, based on the observance of primary water leaking from the DMW. Further ultrasonic tests were then performed, and a total of five axially oriented flaws, classified as primary water stress corrosion cracking (PWSCC), were detected in varied locations around the weld circumference.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Post Irradiation Examination Plan for High-Burnup Demonstration Project Sister Rods

This test plan describes the experimental work to be implemented by the U.S. Department of Energy (DOE) Office of Nuclear Energy (NE) to characterize high burnup (HBU) spent nuclear fuel (SNF) in conjunction with the High Burnup Dry Storage Cask Research and Development Project and serves to coordinate and integrate the multi-year experimental program to collect and develop data regarding the continued storage and eventual transport of HBU (i.e., >45 GWd/MTU) SNF. The work scope involves the development, performance, technical integration, and oversight of measurements and collection of relevant data, guided by analyses and demonstration of need.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nondestructive Examination Guidance for Dry Storage Casks

In this report, an assessment of NDE methods is performed for components of NUHOMS 80 and 102 dry storage system components in an effort to assist NRC staff with review of license renewal applications. The report considers concrete components associated with the horizontal storage modules (HSMs) as well as metal components in the HSMs. In addition, the report considers the dry shielded canister (DSC). Scope is limited to NDE methods that are considered most likely to be proposed by licensees. The document, ACI 349.3R, Evaluation of Existing Nuclear Safety-Related Concrete Structures, is used as the basis for the majority of the NDE methods summarized for inspecting HSM concrete components. Two other documents, ACI 228.2R, Nondestructive Test Methods for Evaluation of Concrete in Structures, and ORNL/TM-2007/191, Inspection of Nuclear Power Plant Structure--Overview of Methods and Related Application, supplement the list with additional technologies that are considered applicable. For the canister, the ASME B&PV Code is used as the basis for NDE methods considered, along with currently funded efforts through industry (Electric Power Research Institute [EPRI]) and the U.S. Department of Energy (DOE) to develop inspection technologies for canisters. The report provides a description of HSM and DSC components with a focus on those aspects of design considered relevant to inspection. This is followed by a brief description of other concrete structural components such as bridge decks, dams, and reactor containment structures in an effort to facilitate comparison between these structures and HSM concrete components and infer which NDE methods may work best for certain HSM concrete components based on experience with these other structures. Brief overviews of the NDE methods are provided with a focus on issues and influencing factors that may impact implementation or performance. An analysis is performed to determine which NDE methods are most applicable to specific components.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Baseline Postirradiation Examination of the AFC-3C, AFC-3D, and AFC-4A Experiments

A long term research focus of the US Department of Energy (DOE) Advanced Fuels Campaign (AFC) is to investigate technologies that can allow for increased actinide utilization in nuclear fuel for fast neutron spectrum reactors. This includes both the incorporation of minor actinides into nuclear fuel for transmutation and high utilization of actinides through “ultra high” burnup fuel. This goal is defined as fuel that can reach a burnup of 30-40 percent fission per initial metal atom (%FIMA) which is higher than what has historically been achieved [1],[2]. Historically, Experimental Breeder Reactor II (EBR-II) Mark III/IIIA/IV driver fuel (U 10Zr fuel with stainless steel 316 or ferritic martensitic steel HT-9 cladding) was qualified to 10%FIMA, but many experimental assemblies and fuel pins achieved higher peak burnup up to near 20%FIMA without failure [3]. The motivation of the irradiation tests explored in this work was to screen candidate alloys and forms that could tolerate very high burnup irradiations of up to 30 % FIMA. In these irradiations, termed AFC 3C, AFC-3D and AFC-4A, uranium-based alloys and forms were irradiated in a prototypic fast reactor spectrum to investigate fuel performance. Irradiations were performed in the Idaho National Laboratory (INL) Advanced Test Reactor (ATR). The performance of these fuels is compared to the historic performance of U-10Zr [4]. Metallic fuel for fast reactors has a long history that has been reviewed several time in the literature [3]–[8].

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Examining the Role of Environment in a Comprehensive Sample of Compact Groups

Compact groups, with their high number densities, small velocity dispersions, and an interstellar medium that has not been fully processed, provide a local analog to conditions of galaxy interactions in the earlier universe. The frequent and prolonged gravitational encounters that occur in compact groups affect the evolution of the constituent galaxies in a myriad of ways, for example, gas processing and star formation. Recently, a statistically significant "gap" has been discovered in the mid-infrared (MIR: 3.6-8 μm) IRAC color space of compact group galaxies. This gap is not seen in field samples and is a new example of how the compact group environment may affect the evolution of member galaxies. In order to investigate the origin and nature of this gap, we have compiled a larger sample of 37 compact groups in addition to the original 12 groups studied by Johnson et al. (yielding 174 individual galaxies with reliable MIR photometry). We find that a statistically significant deficit of galaxies in this gap region of IRAC color space is persistent in the full sample, lending support to the hypothesis that the compact group environment inhibits moderate specific star formation rates. Using this expanded sample, we have more fully characterized the distribution of galaxies in this color space and quantified the low-density region more fully with respect to MIR bluer and MIR redder colors. We note a curvature in the color-space distribution, which is fully consistent with increasing dust temperature as the activity in a galaxy increases. This full sample of 49 compact groups allows us to subdivide the data according to physical properties of the groups. An analysis of these subsamples indicates that neither projected physical diameter nor density shows a trend in color space within the values represented by this sample. We hypothesize that the apparent lack of a trend is due to the relatively small range of properties in this sample, whose groups have already been pre-selected to be compact and dense. Thus, the relative influence of stochastic effects (such as the particular distribution and amount of star formation in individual galaxies) becomes dominant. We analyze spectral energy distributions of member galaxies as a function of their location in color space and find that galaxies in different regions of MIR color space contain dust with varying temperatures and/or polycyclic aromatic hydrocarbon emission.

Environment↗

Conjugated Block Copolymers as Model Systems to Examine Mechanisms of Charge Generation in Donor–Acceptor Materials

Abstract Fully conjugated donor–acceptor block copolymers are established as model systems to elucidate fundamental mechanisms of photocurrent generation in organic photovoltaics. Using analysis of steady‐state photoluminescence quenching, exciton dissociation to a charge transfer state within individual block copolymer chains is quantified. By making a small adjustment to the conjugated backbone, the electronic properties are altered enough to disrupt charge transfer almost entirely. Strong intermolecular coupling of the electron donor is introduced by synthesizing block copolymer nanoparticles. Transient absorption spectroscopy is used to monitor charge generation in block copolymer isolated chains and nanoparticles. While efficient charge transfer is observed in isolated chains, there is no indication of complete charge separation. In the nanoparticles, long‐lived polarons are observed as early as ≈15 ns. Thus, aggregation of electron donors can facilitate efficient charge generation.

Aplan, Melissa P.↗