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NASA NTRS1993

Atmospheric parameterization schemes for satellite cloud property retrieval during FIRE IFO 2

Satellite cloud retrieval algorithms generally require atmospheric temperature and humidity profiles to determine such cloud properties as pressure and height. For instance, the CO2 slicing technique called the ratio method requires the calculation of theoretical upwelling radiances both at the surface and a prescribed number (40) of atmospheric levels. This technique has been applied to data from, for example, the High Resolution Infrared Radiometer Sounder (HIRS/2, henceforth HIRS) flown aboard the NOAA series of polar orbiting satellites and the High Resolution Interferometer Sounder (HIS). In this particular study, four NOAA-11 HIRS channels in the 15-micron region are used. The ratio method may be applied to various channel combinations to estimate cloud top heights using channels in the 15-mu m region. Presently, the multispectral, multiresolution (MSMR) scheme uses 4 HIRS channel combination estimates for mid- to high-level cloud pressure retrieval and Advanced Very High Resolution Radiometer (AVHRR) data for low-level (is greater than 700 mb) cloud level retrieval. In order to determine theoretical upwelling radiances, atmospheric temperature and water vapor profiles must be provided as well as profiles of other radiatively important gas absorber constituents such as CO2, O3, and CH4. The assumed temperature and humidity profiles have a large effect on transmittance and radiance profiles, which in turn are used with HIRS data to calculate cloud pressure, and thus cloud height and temperature. For large spatial scale satellite data analysis, atmospheric parameterization schemes for cloud retrieval algorithms are usually based on a gridded product such as that provided by the European Center for Medium Range Weather Forecasting (ECMWF) or the National Meteorological Center (NMC). These global, gridded products prescribe temperature and humidity profiles for a limited number of pressure levels (up to 14) in a vertical atmospheric column. The FIRE IFO 2 experiment provides an opportunity to investigate current atmospheric profile parameterization schemes, compare satellite cloud height results using both gridded products (ECMWF) and high vertical resolution sonde data from the National Weather Service (NWS) and Cross Chain Loran Atmospheric Sounding System (CLASS), and suggest modifications in atmospheric parameterization schemes based on these results.

Titlow, James↗
NASA NTRSDate not supplied

Impact of COVID-Global Shutdown on Earth's Radiation Budget

Climate is fueled by how much of the sun’s energy is absorbed by Earth. Changes in aerosol emissions have a direct impact how much solar energy is absorbed under clear-sky conditions, which occurs roughly one-third of the time globally. Aerosol emission changes can also indirectly influence clouds and further alter solar energy absorption. In this presentation, we examine the impact of the COVID-19 global shutdown on Earth’s radiation budget at global and regional scales and compare it with other changes that have had an influence on Earth's radiation budget during the past 20 years—including policy-related emission controls, wildfire events and changes in sea-ice extent in polar regions. We use a novel analysis technique together with data from NASA instruments on the Terra, Aqua and Aura satellites and reanalysis data from MERRA-2. We also compare results with state-of-the-art general circulation models that have been nudged to reanalysis data (winds, air temperature and surface 25 pressure) at all levels. Our preliminary results show that the largest COVID-19 impact occurs regionally over the East Asian Marginal Seas, just off the coast of China. We find a 30% reduction in aerosol optical depth according to the MODIS instrument, and an 8% reduction in reflected solar radiation according to the CERES radiation budget instrument. The climate model simulations show remarkable consistency with the observations and furthermore show no evidence of an indirect effect on cloud properties.

Norman G. Loeb↗
NASA NTRS2002

Mesoscale Convective Systems in SCSMEX: Simulated by a Regional Climate Model and a Cloud Resolving Model

A Regional Land-Atmosphere Climate Simulation (RELACS) System is being developed and implemented at NASA Goddard Space Flight Center. One of the major goals of RELACS is to use a regional scale model with improved physical processes, in particular land-related processes, to understand the role of the land surface and its interaction with convection and radiation as well as the water and energy cycles in Indo-China/ South China Sea (SCS)/China, N. America and S. America. The Penn State/NCAR MM5 atmospheric modeling system, a state of the art atmospheric numerical model designed to simulate regional weather and climate, has been successfully coupled to the Goddard Parameterization for Land-Atmosphere-C loud Exchange (PLACE) land surface model. PLACE allows for the effects of vegetation, and thus important physical processes such as evapotranspiration and interception are included. The PLACE model incorporates vegetation type and has been shown in international comparisons to accurately predict evapotranspiration and runoff over a wide variety of land surfaces. The coupling of MM5 and PLACE creates a numerical modeling system with the potential to more realistically simulate the atmosphere and land surface processes including land-sea interaction, regional circulations such as monsoons, and flash flood events. RELACS has been used to simulate the onset of the South China Sea Monsoon in 1986, 1997 and 1998. Sensitivity tests on various land surface models, cumulus parameterization schemes (CPSs), sea surface temperature (SST) variations and midlatitude influences have been performed. These tests have indicated that the land surface model has a major impact on the circulation over the S. China Sea. CPSs can effect the precipitation pattern while SST variation can effect the precipitation amounts over both land and ocean. RELACS has also been used to understand the soil-precipitation interaction and feedback associated with a flood event that occurred in and around China's Yantz River during 1998. The exact location (region) of the flooding can be effected by the soil-rainfall feedback. Also, the Goddard Cumulus Ensemble (GCE) model which allows for realistic moist processes as well as explicit interactions between cloud and radiation, and cloud and surface processes will be used to simulate convective systems associated with the onset of the South China Sea Monsoon in 1998. The GCE model also includes the same PLACE and radiation scheme used in the RELACS. A detailed comparison between the results from the GCE model and RELACS will be performed.

Tao, W.-K.↗
NASA NTRS1989

Mock gravity and the cosmic structure

The process of generating large-scale cosmic structure from the radiation-pressure or 'mock gravity' instability is studied with particular emphasis on the implications of the Berkeley-Nagoya rocket data for the submillimeter background. The linear theory of perturbations in an absorbing medium embedded in an expanding universe of radiation sources is presented. The instability sets up collapse velocities in linear perturbation theory which far exceed those from gravitational instability, so growth continues even after the instability switches off. Perturbation due to this effect is analyzed and related to the growth of large-scale cosmic structures at recent times; large-scale structure is shown to evolve very little from 1 + z about 5 to the present. Nonlinear small-scale effects of the instability are analyzed; it is shown that radiation pressure would compress gas into small, dense pressure-confined clouds with tau much greater than one.

Hogan, Craig J.↗
NASA NTRS2002

Dynamics and Properties of Global Aerosol using MODIS, AERONET and GOCART Model

Recently produced daily Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol data for the whole year of 2001 are used to show the concentration and dynamics of aerosol over ocean and large parts of the continents. The data were validated against the Aerosol Robotic Network (AERONET) measurements over land and ocean in a special issue in GRL now in press. Monthly averages and a movie based on the daily data are produced and used to demonstrate the spatial and temporal evolution of aerosol. The MODIS wide spectral range is used to distinguish fine smoke and pollution aerosol from coarse dust and salt. The aerosol is observed above ocean and land. The movie produced from the MODIS data provides a new dimension to aerosol observations by showing the dynamics of the system. For example in February smoke and dust emitted from the Sahel and West Africa is shown to travel to the North-East Atlantic. In April heavy dust and pollution from East Asia is shown to travel to North America. In May-June pollution and dust play a dynamical dance in the Arabian Sea and Bay of Bengal. In Aug-September smoke from South Africa and South America is shown to pulsate in tandem and to periodically to be transported to the otherwise pristine Southern part of the Southern Hemisphere. The MODIS data are compared with the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation Transport (GOCART) model to test and adjust source and sink strengths in the model and to study the effect of clouds on the representation of the satellite data.

Kaufman, Yoram↗
NASA NTRS2006

What does reflection from cloud sides tell us about vertical distribution of cloud droplets?

In order to accurately measure the interaction of clouds with aerosols, we have to resolve the vertical distribution of cloud droplet sizes and determine the temperature of glaciation for clean and polluted clouds. Knowledge of the droplet vertical profile is also essential for understanding precipitation. So far, all existing satellites either measure cloud microphysics only at cloud top (e.g., MODIS) or give a vertical profile of precipitation sized droplets (e.g., Cloudsat). What if one measures cloud microphysical properties in the vertical by retrieving them from the solar and infrared radiation reflected or emitted from cloud sides? This was the idea behind CLAIM-3D (A 3D - cloud aerosol interaction mission) recently proposed by NASA GSFC. This presentation will focus on the interpretation of the radiation reflected from cloud sides. In contrast to plane-parallel approximation, a conventional approach to all current operational retrievals, 3D radiative transfer will be used for interpreting the observed reflectances. As a proof of concept, we will show a few examples of radiation reflected from cloud fields generated by a simple stochastic cloud model with prescribed microphysics. Instead of fixed values of the retrieved effective radii, the probability density functions of droplet size distributions will serve as possible retrievals.

Marshak, A.↗
NASA NTRS2005

The Impact of Surface Albedo on the Retrievals of Low-Level Stratus Cloud Properties: An Updated Parameterization

An updated version of Dong et al. (1998, hereafter D98) parameterization is developed from a total of 40 hours of data with a broad range of surface albedos (0.1-0.8) during the 2000-2002 winter seasons at the DOE ARM SGP site. The updated parameterization includes the impact of surface albedo on the retrievals of stratus cloud microphysical and radiative properties, and has a significant improvement over D98 when surface albedo is high. Comparing the retrievals, the cloud-droplet effective radii (r(sub e)) calculated from the updated parameterization have a higher correlation coefficient (0.733) and lower Root-Mean-Square (RMS) error (1.74 m or 17.4%) than those (0.602, 4.0 m or 40%) from the D98. The cloud albedos also have a much higher correlation coefficient (0.983) and lower RMS (3%) than those 0.465, 26%) from the D98. The upper limit of surface albedo is 0.3 in applying the D98.

Dong, Xiquan↗
NASA NTRS2012

Retrieval of Aerosol Absorption Properties from Satellite Observations

The Angstrom Absorption Exponent (AAE) is a parameter commonly used to characterize the wavelength-dependence of aerosol absorption optical depth (AAOD). It is closely related to aerosol composition. Black carbon (BC) containing aerosols yield AAE values near unity whereas Organic carbon (OC) aerosol particles are associated with values larger than 2. Even larger AAE values have been reported for desert dust aerosol particles. Knowledge of spectral AAOD is necessary for the calculation of direct radiative forcing effect of aerosols and for inferring aerosol composition. We have developed a satellitebased method of determining the spectral AAOD of absorbing aerosols. The technique uses multi-spectral measurements of upwelling radiation from scenes where absorbing aerosols lie above clouds as indicated by the UV Aerosol Index. For those conditions, the satellite measurement can be explained, using an approximations of Beer's Law (BL), as the upwelling reflectance at the cloud top attenuated by the absorption effects of the overlying aerosol layer. The upwelling reflectance at the cloud-top in an aerosol-free atmospheric column is mainly a function of cloud optical depth (COD). In the proposed method of AAE derivation, the first step is determining COD which is retrieved using a previously developed color-ratio based approach. In the second step, corrections for molecular scattering effects are applied to both the observed ad the calculated cloud reflectance terms, and the spectral AAOD is then derived by an inversion of the BL approximation. The proposed technique will be discussed in detail and application results making use of OMI multi-spectral measurements in the UV-Vis. will be presented.

Torres, Omar↗
NASA NTRS1990

On the interannual variation of the earth radiation balance

The interannual variability of the top of the atmosphere net radiation budget as measured from the Nimbus-7 earth radiation budget instruments was calculated for an eight-year period 1979-1986. The largest fluctuations are shown to occur in three tropical areas: the Atlantic off the west coast of Africa, the eastern Pacific near South America, and the western Pacific northeast of Indonesia. The variability in the Atlantic was 20 percent greater than in the eastern Pacific and 35 percent greater than in the Indonesian area. The maximum anomalies in these two Pacific regions occurred during the El Nino year 1982-1983, while the maximum Atlantic anomalies, south of the Gulf of Guinea, were during 1984. An independent data set of derived cloud type and amount from the Temperature Humidity Infrared Radiometer and the Total Ozone Mapping Spectrometer instruments shows interannual changes in multilevel convective cloud systems have a minimal effect of the net balance. However, changes in middle and low clouds drastically affect the balance, and are the most likely cause of the maximum radiation balance variability in the Gulf of Guinea region. This observed interannual variation of the top of the atmosphere net balance denotes the most variable 'cloud radiative forcing' situation observed to date.

Randel, David L.↗
NASA NTRS1998

Satellite Estimation of Spectral Surface UV Irradiance: Effect of Horizontally Homogeneous Clouds - 2

The local variability of UV irradiance at the Earth's surface is mostly caused by clouds in addition to the seasonal variability. Parametric representations of radiative transfer RT calculations are presented for the convenient solution of the transmission T of ultraviolet radiation through plane parallel clouds over a surface with reflectivity R(sub s). The calculations are intended for use with the Total Ozone Mapping Spectrometer (TOMS) measured radiances to obtain the calculated Lambert equivalent scene reflectivity R for scenes with and without clouds. The purpose is to extend the theoretical analysis of the estimation of UV irradiance from satellite data for a cloudy atmosphere. Results are presented for a range of cloud optical depths and solar zenith angles for the cases of clouds over a low reflectivity surface R(sub s) less than 0.1, over a snow or ice surface R(sub s) greater than 0.3, and for transmission through a non-conservative scattering cloud with single scattering albedo omega(sub 0) = 0.999. The key finding for conservative scattering is that the cloud-transmission function C(sub T), the ratio of cloudy-to clear-sky transmission, is roughly C(sub T) = 1 - R(sub c) with an error of less than 20% for nearly overhead sun and snow-free surfaces. For TOMS estimates of UV irradiance in the presence of both snow and clouds, independent information about snow albedo is needed for conservative cloud scattering. For non-conservative scattering with R(sub s) greater than 0.5 (snow) the satellite measured scene reflectance cannot be used to estimate surface irradiance. The cloud transmission function has been applied to the calculation of UV irradiance at the Earth's surface and compared with ground-based measurements.

Krothov, N.↗
NASA NTRS1990

The intergalactic medium - Initial and boundary conditions for galaxy and primeval star formation

New detailed numerical calculations are presented of the evolution of the intergalactic medium (IGM) in a post recombination Friedmann universe, including a solution of the nonequilibrium rate equations for the ionization and recombination of H and He, the energy equation, and the equation of radiative transfer. The implications of this study for the characteristic mass scale and the epoch of gravitational collapse for the average 'first' star-forming clouds are discussed. The star-formation rate and associated metallicity generation implied if the IGM is fully ionized by starlight by redshift greater than 4 as suggested by recent interpretations of the Gunn-Peterson effect are examined. It is shown that the relative strengths of metal lines from a quasar absorption-line Lyman limit system cloud at z = 3 photoionized by the present intergalactic UV radiation background are compatible with the observations, at least for background sources of either AGN-type or star-forming galaxy spectra.

Giroux, Mark L.↗
NASA NTRS2001

Three Dimensional Atmospheric Radiative Transfer-Applications and Methods Comparison

We review applications of 3D radiative transfer in the atmosphere, emphasizing the wide spectrum of scales important to remote sensing and modeling of cloud fields, and the characteristic scales introduced into observed radiances and fluxes by the distribution of photon pathlengths at conservative and absorbing wavelengths. We define the "plane-parallel bias", which is a measure of the importance of 3D cloud structure in large-scale models, and the "independent pixel errors" that quantify the significance of 3D effects in remote sensing, and emphasize their relative magnitude and scale dependence. A variety of approaches in current use in 3D radiative transfer, and issues of speed, accuracy, and flexibility are summarized. We also describe a recently initiated "International Intercomparison of 3-Dimensional Radiation Codes", or I3RC. I3RC is a 3-phase effort that has as its goals to: (1) understand the errors and limits of 3D methods; (2) provide "baseline" cases for future 3D code development; (3) promote sharing of 3D tools; (4) derive guidelines for 3D tool selection; and (5) improve atmospheric science education in 3D radiative transfer. Selected results from Phases 1 and 2 of I3RC are discussed. These are taken from five cloud fields: a 1D field of bar clouds, a 2D radar-derived field, a 3D Landsat-derived field, a stratiform cloud from the model of C. Moeng, and a convective cloud from the model of B. Stevens. Computations have been carried out for three monochromatic wavelengths (one conservative, one absorptive, and one thermal) and two solar zenith angles (0, 60 degrees).

Cahalan, Robert F.↗
NASA NTRS1994

Biospheric effects of a large extraterrestrial impact: Case study of the Cretaceous/Tertiary boundary crater

The Chicxulub Crater in Yucatan, Mexico, is the primary candidate for the impact that caused mass extinctions at the Cretaceous/Tertiary boundary. The target rocks at Chicxulub contain 750 to 1500 m of anhydrite (CaSO4), which was vaporized upon impact, creating a large sulfuric acid aerosol cloud. In this study we apply a hydrocode model of asteroid impact to calculate the amount of sulfuric acid produced. We then apply a radiative transfer model to determine the atmospheric effects. Results include 6 to 9 month period of darkness followed by 12 to 26 years of cooling.

Pope, Kevin O.↗
NASA NTRS1994

Effect of stratospheric aerosol layers on the TOMS/SBUV ozone retrieval

An evaluation of the optical effects of stratospheric aerosol layers on total ozone retrieval from space by the TOMS/SBUV type instruments is presented here. Using the Dave radiative transfer model we estimate the magnitude of the errors in the retrieved ozone when polar stratospheric clouds (PSC's) or volcanic aerosol layers interfere with the measurements. The largest errors are produced by optically thick water ice PSC's. Results of simulation experiments on the effect of the Pinatubo aerosol cloud on the Nimbus-7 and Meteor-3 TOMS products are presented.

Torres, O.↗
NASA NTRS2014

Remote Sensing of Cloud Top Height from SEVIRI: Analysis of Eleven Current Retrieval Algorithms

The role of clouds remains the largest uncertainty in climate projections. They influence solar and thermal radiative transfer and the earth's water cycle. Therefore, there is an urgent need for accurate cloud observations to validate climate models and to monitor climate change. Passive satellite imagers measuring radiation at visible to thermal infrared (IR) wavelengths provide a wealth of information on cloud properties. Among others, the cloud top height (CTH) - a crucial parameter to estimate the thermal cloud radiative forcing - can be retrieved. In this paper we investigate the skill of ten current retrieval algorithms to estimate the CTH using observations from the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) onboard Meteosat Second Generation (MSG). In the first part we compare ten SEVIRI cloud top pressure (CTP) data sets with each other. The SEVIRI algorithms catch the latitudinal variation of the CTP in a similar way. The agreement is better in the extratropics than in the tropics. In the tropics multi-layer clouds and thin cirrus layers complicate the CTP retrieval, whereas a good agreement among the algorithms is found for trade wind cumulus, marine stratocumulus and the optically thick cores of the deep convective system. In the second part of the paper the SEVIRI retrievals are compared to CTH observations from the Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) and Cloud Profiling Radar (CPR) instruments. It is important to note that the different measurement techniques cause differences in the retrieved CTH data. SEVIRI measures a radiatively effective CTH, while the CTH of the active instruments is derived from the return time of the emitted radar or lidar signal. Therefore, some systematic differences are expected. On average the CTHs detected by the SEVIRI algorithms are 1.0 to 2.5 kilometers lower than CALIOP observations, and the correlation coefficients between the SEVIRI and the CALIOP data sets range between 0.77 and 0.90. The average CTHs derived by the SEVIRI algorithms are closer to the CPR measurements than to CALIOP measurements. The biases between SEVIRI and CPR retrievals range from −0.8 kilometers to 0.6 kilometers. The correlation coefficients of CPR and SEVIRI observations vary between 0.82 and 0.89. To discuss the origin of the CTH deviation, we investigate three cloud categories: optically thin and thick single layer as well as multi-layer clouds. For optically thick clouds the correlation coefficients between the SEVIRI and the reference data sets are usually above 0.95. For optically thin single layer clouds the correlation coefficients are still above 0.92. For this cloud category the SEVIRI algorithms yield CTHs that are lower than CALIOP and similar to CPR observations. Most challenging are the multi-layer clouds, where the correlation coefficients are for most algorithms between 0.6 and 0.8. Finally, we evaluate the performance of the SEVIRI retrievals for boundary layer clouds. While the CTH retrieval for this cloud type is relatively accurate, there are still considerable differences between the algorithms. These are related to the uncertainties and limited vertical resolution of the assumed temperature profiles in combination with the presence of temperature inversions, which lead to ambiguities in the CTH retrieval. Alternative approaches for the CTH retrieval of low clouds are discussed.

Hamann, U.↗
NASA NTRS1999

A Study of Direct and Cloud-Mediated Radiative Forcing of Climate Due to Aerosols

The Intergovernmental Panel on Climate Change (IPCC) has reported that in the southeastern US and eastern China, the general greenhouse warming due to anthropogenic gaseous emissions is dominated by the cooling effect of anthropogenic aerosols. To verify this model prediction in eastern China and southeastern US, we analyzed regional patterns of climate changes at 72 stations in eastern China during 1951- 94 (44 years), and at 52 stations in the southeastern US during 1949-94 (46 years) to detect the fingerprint of aerosol radiative forcing. It was found that the mean rates of change of annual mean daily, maximum, minimum temperatures and diurnal temperature range (DTR) in eastern China were 0.8, -0.2, 1.8, and -2.0 C/100 years respectively, while the mean rates of change of annual mean daily, maximum, minimum temperatures and DTR in the southeastern US were -0.2, -0.6, 0.2, and -0.8 C/100 years, respectively. This indicates that the high rate of increase in annual mean minimum temperature in eastern China results in a slightly warming trend of daily temperature, while the high rate of decrease in annual mean maximum temperature and low rate of increase in annual mean minimum temperature lead to the cooling trend of daily temperature in the southeastern US. We found that the warming from the longwave forcing due to both greenhouse gases and aerosols was completely counteracted by the shortwave aerosol forcing in the southeastern US in the past 46 years. A slightly overall warming trend in eastern China is evident; winters have become milder. This finding is explained by hypothesizing that increasing energy usage during the past 44 years has resulted in more coal and biomass burning, thus increasing the emission of absorbing soot and organic aerosols in eastern China. Such emissions, in addition to well-known Asia dust and greenhouse gases, may be responsible for the winter warming trend in eastern China that we have reported here. The sensitivity of aerosol radiative properties to aerosol composition, size distribution, relative humidity (RH) is examined for the following aerosol systems: inorganic and organic ions (Cl-, Br-, NO3 -, SO4 2-, Na+, NH4 +, K+, Ca2+, Mg2+, HCOO-, CH3COO-, CH3CH2COO-, CH3COCOO-, OOCCOO2-, MSA-1); water-insoluble inorganic and organic compounds (elemental carbon, n-alkanes, SiO2, Al2O3, Fe2O3 and other organic compounds). The partial molar refraction method was used to calculate the real part of the refractive index. It was found that the asymmetry factor increased by approximately 48% with the real part varying from 1.40 to 1.65, and the single scattering albedo decreased by 24% with the imaginary part varying from -0.005 to -0.1. The asymmetry factor increased by 5.4 times with the geometric standard deviation varying from 1.2 to 3.0. The radiation transmission is very sensitive to the change in size distribution; other factors are not as significant. To determine the aerosol direct radiative forcing (ADRF), the aerosol optical depth (AOD) values at the three operational wavelengths (415, 500 and 673 nm) were determined at a regionally representative site, namely, Mt. Gibbs (35.78 deg N, 82.29 deg W, elevation 2006 m) in Mt. Mitchell State Park, NC, and a site located in an adjacent valley (Black Mountain, 35.66 deg N, 82.38 deg W, elevation 951 m) in the southeastern US. The two sites are separated horizontally by 10 km and vertically by 1 km. It was found that the representative total AOD values at 500 nm at the valley site for highly polluted (HP), marine (M) and continental (C) air masses were 0.68 +/- 0.33, 0.29 +/- 0.19 and 0.10 +/- 0.04, respectively. A search-graph method was used to retrieve the columnar size distribution (number concentration N, effective radius reff and geometric standard deviation=?g) from the optical depth observations at three operational wavelengths. The ground albedo, single scattering albedo and imaginary part of the refractive index were calculated using a mathematically unique procedure involving a Mie code and a radiative transfer code in conjunction with the retrieved aerosol size distribution, AOD, and diffuse-direct irradiance ratio. It was found that N, r(eff) and sigma(g) were in the ranges of 10 to 1.7 x 10(exp 4)/cubic cm, 0.09 to 0.68 micrometers and 1.12 to 2.95, respectively. The asymmetry factor and single scattering albedo were in the ranges of 0.63 to 0.75 and 0.74 to 0.97 respectively. The ground albedo for the forested terrain and imaginary part of refractive index were found to be in the ranges of 0.06 to 0.29 and 0.005 to 0.051 respectively. On the basis of these aerosol radiative properties obtained at the research sites and computations using the Column Radiation Model (CRM) of National Center of Atmospheric Research (NCAR) Community Climate Model (CCM3), it was found that the average cloud-free 24-hour ADRF values were -13 +/- 8, -8 +/- 3, -33 +/- 16 W/square m for marine, continental, and polluted air masses, respectively. On the assumption that the fractional coverage of clouds is 0.61, it was estimated that the annual mean ADRF was 7 +/- 2 W/square m in the southeastern US. The review with respect to the current knowledge of organic acids shows that aerosol formate and acetate concentrations range from 0.02 to 5.3 nmol/cubic m and from 0.03 to 12.4 nmol/cubic m respectively, and that between 34% to 77% of formate and between 21% to 66% of acetate are present in the fine fraction of aerosols. It was found that although most (98-99%) of these volatile organic acids were present in the gas phase, their concentrations in the aerosol particles were sufficient to make them a good candidate for cloud condensation nuclei (CCN). It is hypothesized that organic acids are at least one of the primary sources of CCN in the atmosphere due to their ubiquitous presence in the troposphere, especially over the continental forested areas. The results of our measurements at Palmer Station, Antarctica show that the daily average CCN concentrations at 0.3% and 1% supersaturations ranged from 0.3 to 160/cubic cm and from 4 to 168/cubic cm, respectively, during the period from 17 January to 26 February, 1994. New evidence for substantial and definitive CCN enhancement near and within cloud has been observed at Mt. Mitchell, North Carolina. The results show that the average monthly CCN concentrations were 460 +/- 217, 386 +/- 286, 429 +/- 228 and 238 +/- 134/cubic cm for in-cloud, overcast, clear and rainy conditions, respectively. The typical CCN spectra show that there were a lot of small CCN produced and the ion concentrations (especially H+ and SO4 2-) were very high during the CCN enhancement period. The significantly positive correlation between black carbon (BC) and CCN at 1% supersaturation indicates that a percentage of the BC measured at the site may be in the form of an internal mixture and participated in the formation of CCN.

Yu, Shao-Cai↗
NASA NTRS1980

A time variable model of Earth's albedo

A time variable model of Earth's albedo was prepared for use in climate studies and as an aid to the interpretation of satellite Earth radiation budget data. The features of the model include: a 10 deg latitude 10 deg longitude grid for numerical integration, surface albedo specified at 1 month intervals, calculation of zenith angle effect for surface albedo and of the additional effect of the atmosphere on the albedo. Percent cloud cover is specified for 29 different climatological cloud type regions at 8 times of the day for 12 months of the year. Cloud albedos were specified for each of the cloud climatological types. Diurnal and monthly variations of this model are described and results are compared with a model which is based on satellite measurements. A computer program was also written for use in studying the sampling effects in satellite radiation budget measurements. An example of the results of calculations with this program are compared with a previous study of the sampling effects. This program for satellite orbit characteristics is to be combined with the time-variable albedo model for further study of the sampling problem.

Bartman, F. L.↗