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At least 829 records · Page 46

Dynamics of nonequilibrium magnons in gapped Heisenberg antiferromagnets

Nonequilibrium dynamics in spin systems is a topic currently under intense investigation as it provides fundamental insights into thermalization, universality, and exotic transport phenomena. While most of the studies have been focused on ideal closed quantum many-body systems such as ultracold atomic quantum gases and one-dimensional spin chains, driven-dissipative Bose gases in steady states away from equilibrium in classical systems also lead to intriguing nonequilibrium physics. Here, in this work, we theoretically investigate out-of-equilibrium dynamics of magnons in a gapped Heisenberg quantum antiferromagnet based on Boltzmann transport theory. We show that, by treating scattering terms beyond the relaxation-time approximation in the Boltzmann transport equation, energy and particle number conservation mandate that nonequilibrium magnons cannot relax to equilibrium, but decay to other nonequilibrium stationary states. The only decay channel for these stationary states back to equilibrium is through the nonconserving interactions (i.e., changing particle number and/or energy within the magnon system) such as boundary or magnon-phonon scattering. At low temperatures, these nonconserving interactions are much slower processes than intrinsic magnon-magnon interaction in a gapped spin system. Using magnon-phonon interaction as a quintessential type of nonconserving interaction, we then propose that nonequilibrium steady states of magnons can be maintained and tailored using periodic driving at frequencies faster than relaxation due to phonon interactions. These findings reveal a class of classical material systems that are suitable platforms to study nonequilibrium statistical physics and macroscopic phenomena such as classical Bose-Einstein condensation of quasiparticles and magnon supercurrents that are relevant for spintronic applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Phase control of spin waves in the van der Waals antiferromagnet NiPS 3

Here we demonstrate phase control of magnons in the van der Waals antiferromagnet NiPS3 using optical excitation by polarized light. The sign of the coherent precession of spin amplitude changes upon (i) reversing the helicity of a circularly polarized pump beam, or (ii) rotating the polarization of a linearly polarized pump by π/2. Because these two excitation pathways have comparable generation efficiency, the phase of spin precession can be continuously tuned from 0 to 2π by controlling the polarization state of the pump pulse. The ability to excite magnons with a desired phase has potential applications in the design of a spin-wave phased array and ultrafast spin information processing.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Field-dependent magnons in the honeycomb antiferromagnet CoTiO 3

We report field-dependent high-resolution inelastic neutron scattering (INS) measurements on the honeycomb lattice magnet, CoTiO 3 , to study the evolution of its magnon excitations across a spin reorientation transition driven by an in-plane magnetic field. By carrying out elastic neutron scattering in a magnetic field, we show that the sample transitions from a collinear antiferromagnetic state with multiple magnetic domains at a low field to a monodomain state with a canted magnetic structure at a high field. Concurrent with this transition, we observed significant changes in both the energy and the width of the zone center magnon peak. The observed width change was argued to be consistent with an unusual zero-field state with extended domain walls. On the other hand, the magnon spectra near the K point of the Brillouin zone boundary were found to be largely insensitive to the changes in the ordered moment directions and the domain configuration. We argue that this observation is difficult to explain within the framework of the bond-dependent model proposed in a recent INS study [M. Elliot et al., Nat. Commun. 12, 3936 (2021)]. Our paper therefore calls for alternative explanations for the observed K-point gap in CoTiO 3 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic structure and magnetoelectric effect in the centrosymmetric antiferromagnet Cu 2 ( MoO 4 ) ( SeO 3 )

Magnetic properties of Cu 2 ⁢(MoO 4 )⁢(SeO 3 ), an S = $\frac{1}{2}$ centrosymmetric antiferromagnet (AFM), were investigated using superconducting quantum interference device magnetometry, neutron diffraction, and magnetoelectric (ME) measurements. Here, the magnetic susceptibility measurements indicate a broad peak at ~50 K, followed by a phase transition into AFM order at T N = 23.6⁢(1) K. Above T N , a fit to the Curie-Weiss law gives a Curie-Weiss temperature Θ CW = -68⁢(1) K, suggesting the dominant AFM coupling. Neutron powder diffraction reveals that the C⁢u 2+ spins are aligned AFM along the c axis with weak noncollinearity under the magnetic space group of P2$^{'}_{1}$/c. The ME response indicates that a nondiagonal component of a ME tensor is active, supporting the simultaneous spatial and time reversal symmetry breaking under P2$^{'}_{1}$/c.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Repulsive Tomonaga-Luttinger liquid in the quasi-one-dimensional alternating spin-$\frac{1}{2}$ antiferromagnet NaVOPO 4

Here, we probe the magnetic field-induced Tomonaga-Luttinger liquid (TLL) state in the bond-alternating spin1/2 antiferromagnetic (AFM) chain compound NaVOPO 4 using thermodynamic as well as local μSR and 31 P NMR probes down to mK temperatures in magnetic fields up to 14 T. The μSR and NMR relaxation rates in the gapless TLL regime decay slowly following characteristic power-law behavior, enabling us to directly determine the interaction parameter K as a function of the magnetic field. These estimates are crosschecked using magnetization and specific heat data. The field-dependent K lies in the range of 0.4 < K < 1 and indicates the repulsive nature of interactions between the spinless fermions, in line with the theoretical predictions. This renders NaVOPO 4 the first experimental realization of TLL with repulsive fermionic interactions in hitherto studied S = 1/2 bond-alternating AFM-AFM chain compounds.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Coexistence of ferromagnetism and antiferromagnetic dimers in topological insulators

The addition of magnetic impurities in topological insulators (TIs) can drive ferromagnetic order that leads to quantum anomalous Hall transport well below the Curie temperature. The fragility of the quantized regime has been ascribed to the random nature of the magnetic moment distribution. Here, we refine this hypothesis by using inelastic neutron scattering and density-functional theory calculations to show that two antagonistic components define the magnetism in Mn-substituted SnTe, thereby limiting the effectiveness of dilute magnetic TIs. One component is strongly bound antiferromagnetic dimers that compete with ferromagnetic order. In conclusion, the other component consists of undimerized moments where ferromagnetic order develops via long-range interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Stripe magnetic order and field-induced quantum criticality in the perfect triangular-lattice antiferromagnet CsCeSe 2

The two-dimensional triangular-lattice antiferromagnet (TLAF) is a textbook example of frustrated magnetic systems. Despite its simplicity, the TLAF model exhibits a highly rich and complex magnetic phase diagram, featuring numerous distinct ground states that can be stabilized through frustrated next-nearest-neighbor couplings or anisotropy. In this paper, we report low-temperature magnetic properties of the TLAF material CsCeSe 2 . The inelastic neutron scattering (INS) together with specific heat measurements and density functional theory calculations of crystalline electric field suggest that the ground state of Ce ions is a Kramers doublet with strong easy-plane anisotropy. Elastic neutron scattering measurements demonstrate the presence of stripe-yz magnetic order that develops below T N = 0.35K, with the zero-field ordered moment of m Ce ≈ 0.65μ B . Application of magnetic field first increases the ordering temperature by about 20% at the intermediate field region and eventually suppresses the stripe order in favor of the field-polarized ferromagnetic state via a continuous quantum phase transition (QPT). The field-induced response demonstrates sizable anisotropy for different in-plane directions, B ∥ a and B ⊥ ⁢a, which indicates the presence of bond-dependent coupling in the spin Hamiltonian. As a result, we further show theoretically that the presence of anisotropic bond-dependent interactions can change the universality class of QPT for B ∥ a and B ⊥ ⁢a.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Coupling-dependent antiferromagnetic-ferromagnetic ordering in a pinwheel artificial spin ice

Nanopatterned magnetic thin films offer a platform for exploration of tailored magnetic properties such as emergent long-range order. A prominent example is artificial spin ice (ASI), where an arrangement of nanoscale magnetic elements, acting as macrospins, interact via their dipolar fields. In this study, we discuss the transition from antiferromagnetic (AFM) to ferromagnetic (FM) long-range order in a square lattice ASI as the magnetic elements are gradually rotated through 45⁢° to a “pinwheel” configuration. The AFM-FM transition is observed experimentally using synchrotron radiation x-ray spectromicroscopy and occurs for a certain rotation angle of the nanomagnets, dependent on the dipolar coupling strength determined by the separation of the magnets in the lattice. Large-scale magnetic dipole simulations show that the point-dipole approximation fails to capture the correct AFM-FM transition angle. However, excellent agreement with experimental data is obtained using a dumbbell-dipole model, which better reflects the actual dipolar fields of the magnets. This model also explains the coupling dependence of the transition angle, another feature not captured by the point-dipole model. Our findings resolve a discrepancy between measurement and theory in previous work on “pinwheel” ASIs and establish the coupling dependence of the AFM-FM transition. The revised dipole model, with a more accurate representation of the stray field, offers more precise control of magnetic order in artificial spin systems.

Artificial spin ice↗

Magnetic properties of the double trillium lattice antiferromagnet KBaCr 2 ⁢(PO 4 ) 3

Trillium lattices formed by corner-shared triangular units are the platform for magnetic frustration in three dimensions. Herein, we report structural and magnetic properties of the Cr-based (S = 3/2) double trillium lattice material KBaCr 2 ⁢(PO 4 ) 3 studied by x-ray diffraction, dc and ac magnetization, heat capacity, thermal conductivity, and 31 P nuclear magnetic resonance (NMR) measurements complemented by density-functional band-structure calculations. Magnetization, heat capacity, and 31 P NMR measurements reveal the magnetic transition at T N⁢1 ≃ 12.5 K in zero field followed by another transition (T N⁢2 ) at low temperatures in weak applied fields. The 31 P spin-lattice relaxation rate in the ordered state follows the T 3 behavior indicative of the two-magnon Raman process. Finally, the spin lattice of KBaCr 2 ⁢(PO 4 ) 3 comprises two crystallographically nonequivalent ferromagnetic sublattices that are coupled antiferromagnetically, thus eliminating frustration in this trillium network and leading to weak ferromagnetism in the vicinity of T N⁢1 .

36 MATERIALS SCIENCE↗

Large negative magnetoresistance in antiferromagnetic G⁡d 2 ⁢S⁢e 3

Rare earth chalcogenides provide a great platform to study exotic quantum phenomena such as superconductivity and charge density waves. Among various interesting properties, the coupling between magnetism and electronic transport has attracted significant attention. Here, we report the investigation of such coupling in α-G⁡d 2⁢ S⁢e 3 single crystals through magnetic, calorimetric, and transport property measurements. α-G⁡d 2 ⁢S⁢e 3 is found to display an antiferromagnetic ground state below 11 K with metamagnetic spin-flop transitions. The magnetic fluctuations remain strong above the transition temperature. Transport measurements reveal an overall metallic transport behavior with a large negative magnetoresistance of approximately 65% near the magnetic transition temperature, together with positive magnetoresistance near the field-induced spin-flop transitions, which can be understood in terms of the suppression of spin scattering by the magnetic field.

electrical properties↗

Role of nonmagnetic spacers in the magnetic interactions of antiferromagnetic topological insulators MnBi 4 ⁢Te 7 and MnBi 2 ⁢Te 4

MnBi 4 ⁢Te 7 belongs to a family of antiferromagnetic topological insulators. It forms a natural heterostructure of magnetic (septuple) and nonmagnetic (quintuple) topological blocks. Here, we explore the magnetism and magnetic interactions in this compound using inelastic neutron scattering. We find that the interlayer magnetic coupling is much weaker in MnBi 4 ⁢Te 7 as compared to MnBi 2⁢ Te 4 due to the insertion of nonmagnetic quintuple layers in the former. However, other key magnetic energy scales residing within a single septuple block, the single-ion anisotropy and long-range intralayer exchanges, are essentially the same. In conclusion, this identifies a transferable set of magnetic interactions applicable to the extended family of magnetic topological insulators based on MnBi 2 ⁢Te 4 –Bi 2 ⁢Te 3 heterostructures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Local moments and suppression of antiferromagnetism in correlated Zr4Fe4Si7

We report magnetic, transport, and neutron diffraction measurements as well as a doping study of the V-phase compound Zr4Fe4Si7. This compound exhibits collinear antiferromagnetic order below TN = 98 1 K with a staggered moment of 0.57(3) B/Fe as T 0. The magnetic order can be quenched with Co substitution to the Fe site, but even then a 1.5 B/Fe paramagnetic moment remains. The resistivity and heat capacity of Zr4Fe4Si7 are Fermi-liquid-like below 16 and 7 K, respectively, and reveal correlations on the scale of those observed in superconducting Fe pnictides and chalcogenides. Electronic structure calculations overestimate the ordered moment, suggesting the importance of dynamical effects. The existence of magnetic order, electronic correlations, and spin fluctuations make Zr4Fe4Si7 distinct from the majority of Fe-Si compounds, fostering comparison instead with the parent compounds of Fe-based superconductors.

Simonson, Jack↗

Metal-insulator transition in antiferromagnetic Ba 1 - x K x Mn 2 As 2 ( 0 ≤ x ≤ 0.4 ) single crystals studied by 55 Mn and 75 As NMR

The magnetic structure and metal-insulator transition in antiferromagnetic (AFM) BaMn 2 As 2 and Ba 1-x K x Mn 2 As 2 single crystals have been investigated by 55 Mn and 75 As nuclear magnetic resonance (NMR) measurements. In the parent AFM insulator BaMn 2 As 2 with a Néel temperature TN=625 K, we observed a 55 Mn zero-field NMR (ZFNMR) spectrum and confirmed the G-type AFM structure from the field dependence of the 55 Mn spectra and 75 As NMR spectra below TN. In hole-doped crystals with x>0.01, similar 55 Mn ZFNMR spectra were observed and the AFM state was revealed to be robust up to x=0.4 with the ordered moment nearly independent of x. The nuclear spin-lattice relaxation rates (1/T 1 ) for both nuclei in the doped samples follow the Korringa relation T 1 T=const, indicating a metallic state. This confirms the coexistence of AFM ordered localized Mn spins and conduction carriers from a microscopic point of view. From the x dependence of (T 1 T) -1/2 for both nuclei, we conclude that this transition is caused by vanishing of the hole concentration as the transition is approached from the metallic side.

36 MATERIALS SCIENCE↗

Magnetic ordering induced by interladder coupling in the spin-1/2 Heisenberg two-leg ladder antiferromagnet C 9 H 18 N 2 CuBr 4

In this article, we present specific-heat and neutron-scattering results for the S=1/2 quantum antiferromagnet (dimethylammonium)(3,5-dimethylpyridinium)CuBr 4 . The material orders magnetically at T N =1.99(2) K, and magnetic excitations are accompanied by an energy gap of 0.30(2) meV due to spin anisotropy. The system is best described as coupled two-leg spin-1/2 ladders with the leg exchange J leg =0.60(2) meV, rung exchange J rung =0.64(9) meV, interladder exchange J int =0.19(2) meV, and an interaction-anisotropy parameter λ=0.93(2), according to inelastic neutron-scattering measurements. In contrast to most spin ladders reported to date, the material is a rare example in which the interladder coupling is very near the critical value required to drive the system to a Néel-ordered phase without the assistance of a magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Entanglement properties of the antiferromagnetic-singlet transition in the Hubbard model on bilayer square lattices

Here, we calculate the bipartite R enyi entanglement entropy of an L x L x 2 bilayer Hubbard model using a determinantal quantum Monte Carlo method recently proposed by Grover [Phys. Rev. Lett. 111, 130402 (2013)]. Two types of bipartition are studied: (i) One that divides the lattice into two L x L planes, and (ii) One that divides the lattice into two equal-size (L x L=2 x 2) bilayers. Furthermore, we compare our calculations with those for the tight-binding model studied by the correlation matrix method. As expected, the entropy for bipartition (i) scales as L 2 , while the latter scales with L with possible logarithmic corrections. The onset of the antiferromagnet to singlet transition shows up by a saturation of the former to a maximal value and the latter to a small value in the singlet phase. We also comment on the large uncertainties in the numerical results with increasing U, which would have to be overcome before the critical behavior and logarithmic corrections can be quanti ed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic phase diagram and multiferroicity of Ba 3 MnNb 2 O 9 : A spin - 5 2 triangular lattice antiferromagnet with weak easy-axis anisotropy

Here we have performed magnetic, electric, thermal and neutron powder diffraction (NPD) experiments as well as density functional theory (DFT) calculations on Ba 3 MnNb 2 O 9 . All results suggest that Ba 3 MnNb 2 O 9 is a spin-5/2 triangular lattice antiferromagnet (TLAF) with weak easy-axis anisotropy. At zero field, we observed a narrow two-step transition at T N1 = 3.4 K and T N2 = 3.0 K. The neutron diffraction measurement and the DFT calculation indicate a 120 spin structure in ab plane with out-of-plane canting at low temperatures. With increasing magnetic field, the 120 spin structure evolves into up-up-down (uud) and oblique phases showing successive magnetic phase transitions, which fits well to the theoretical prediction for the 2D Heisenberg TLAF with classical spins. Ultimately, multiferroicity is observed when the spins are not collinear but suppressed in the uud and oblique phases.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Unified molecular field theory for collinear and noncollinear Heisenberg antiferromagnets

In this study, a unified molecular field theory (MFT) is presented that applies to both collinear and planar noncollinear Heisenberg antiferromagnets (AFs) on the same footing. The spins in the system are assumed to be identical and crystallographically equivalent. This formulation allows calculations of the anisotropic magnetic susceptibility χ versus temperature T below the AF ordering temperature T N to be carried out for arbitrary Heisenberg exchange interactions J ij between arbitrary neighbors j of a given spin i without recourse to magnetic sublattices. The Weiss temperature θ p in the Curie-Weiss law is written in terms of the J ij values and T N in terms of the J ij values and an assumed AF structure. Other magnetic and thermal properties are then expressed in terms of quantities easily accessible from experiment as laws of corresponding states for a given spin S. For collinear ordering these properties are the reduced temperature t=T/T N , the ratio f = θ p /T N , and S. For planar noncollinear helical or cycloidal ordering, an additional parameter is the wave vector of the helix or cycloid. The MFT is also applicable to AFs with other AF structures. The MFT predicts that χ(T ≤ T N ) of noncollinear 120° spin structures on triangular lattices is isotropic and independent of S and T and thus clarifies the origin of this universally observed behavior. The high-field magnetization and heat capacity for fields applied perpendicular to the ordering axis (collinear AFs) and ordering plane (planar noncollinear AFs) are also calculated and expressed for both types of AF structures as laws of corresponding states for a given S, and the reduced perpendicular field versus reduced temperature phase diagram is constructed.

36 MATERIALS SCIENCE↗

CaMn 2 Sb 2 : Spin waves on a frustrated antiferromagnetic honeycomb lattice

We present inelastic neutron scattering measurements of the antiferromagnetic insulator CaMn 2 Sb 2 :, which consists of corrugated honeycomb layers of Mn. The dispersion of magnetic excitations has been measured along the H and L directions in reciprocal space, with a maximum excitation energy of ≈ 24 meV. These excitations are well described by spin waves in a Heisenberg model, including first and second neighbor exchange interactions, J 1 and J 2 , in the Mn plane and also an exchange interaction between planes. The determined ratio J 2 /J 1 ≈ 1/6 suggests that CaMn 2 Sb 2 : is the first example of a compound that lies very close to the mean field tricritical point, known for the classical Heisenberg model on the honeycomb lattice, where the N´eel phase and two different spiral phases coexist. The magnitude of the determined exchange interactions reveal a mean field ordering temperature ≈ 4 times larger than the reported N´eel temperature T N = 85 K, suggesting significant frustration arising from proximity to the tricritical point.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗