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At least 811 records · Page 45
All sourcesNASA NTRSDOE OSTI
NASA NTRS1986

Lidar observation of the mesospheric sodium layer in Antarctica

The mesospheric sodium layer has been observed at Syowa Station in Antarctica during the wintering period of the 26th Japanese Antarctic Research Expedition. A lidar observation of the polar middle atmosphere at the station has been performed as a part of the Middle Atmosphere Program since 1983. At first stratospheric aerosols have been observed by the system based on a ruby laser. In 1985 a new transmitting system consisting of a tunable dye laser was added to that system to observe the sodium layer, too. The characteristics of the lidar system are given. The results of the mesospheric sodium layer observed on 42 nights during the period from March to October, 1985 are also given.

Nomura, A.↗
NASA NTRS1986

Laser heterodyne system for obtaining height profiles of minor species in the atmosphere

An infrared laser heterodyne system for obtaining height profiles of minor constituents of the atmosphere was developed and erected. A brief discription of the system is given. The system consists of a tunable CO2 waveguide laser in the 9 to 11 micrometer band, that is used as a local oscillator and a heliostat that follows the sun and brings in solar radiation, that is mixed with the laser beam in a high speed liquid nitrogen cooled mercury cadmium telluride detector. The detected signal is analysed in a RF spectrum analyser that allows tracing absorption line profiles. Absorption lines of a number of minor constituents in the troposphere and stratosphere, such as O3, NH3, H2O, SO2, ClO, N2O, are in the 9 to 11 micrometer band and overlap with that of CO2 laser range. The experimental system has been made operational and trial observations taken. Current measurements are limited to ozone height profiles. Results are presented.

Jain, S. L.↗
NASA NTRS1986

Alexandrite laser source for atmospheric lidar measurements

During the past years, there has been a marked increase in interest in the applications of vibronic solid state lasers to meteorology and atmospheric physics. Two airborne lidar programs are now under development in France. The differential absorption lidar (DIAL) method with vibronic solid state lasers is very attractive for water vapor, temperature and pressure measurements. Alexandrite laser and titanium-sapphire are both suitable for these applications. However, only alexandrite rods are commercially available. The requirements on the laser source for airborne dial applications are two fold: (1) a restriction on laser linewidth and a requirement on stability and tunability with a good spectral purity; and (2) a requirement on the time separation between the two pulses. These constraints are summarized.

Pelon, J.↗
NASA NTRS1985

Estimation of precipitation from GOES IR imagery during FGGE: Application to diagnostic studies

The objectives were to (1) develop a method of estimating open-ocean rainfall and associated latent heat release via GOES IR satellite imagery; (2) to use remote precipitation estimates to investigate the role of diabatic forcing in the maintenance of the South Pacific Convergence Zone (SPCZ) during FGGE SOP-1/; and (3) to assess the significance of non-quasigeostrophic transports of energy in several cyclogenetic events preceding the development of a North Atlantic blocking episode during FGGE SOP-1. The bulk of the early FY-85 work was directed toward development of the single pixel indexing technique (SPI) which assigns a rain rate to GOES IR black-body temperatures, T sub b, via a non-linear statistical relationship developed with raingauge measurements. The method was tested against radar-derived rainfall during GATE raingauge measurements over coastal North Carolina and island stations in the South Pacific Ocean. Skill was found comparable to Arkin's method (1979 MWR) in convective situations. The results suggest that transferring a rain algorithm from one oceanic regime to another may not require substantial modification of coefficients or tunable parameters. Twelve H mean rainfall amounts were produced for the region bounded by 10 deg. N, 50 deg. S, 120 deg W and 170 deg. E during the period January 10 to 16, 1979. These estimates constitute a basic input to diagnostic calculations of diabatic heating over the SPCZ region. ECMWF level III-b data analyses was used to compute several components of the APE balance in the South Pacific during the period January 10 to 18, 1979.

Robertson, F. R.↗
NASA NTRS1986

Fraunhofer filters to reduce solar background for optical communications

A wavelength that lies within a spectral interval of reduced solar emission (a Fraunhofer line) can carry optical communications with reduced interference from direct or reflected background sunlight. Suitable Fraunhofer lines are located within the tuning range of good candidate lasers. The laser should be tunable dynamically to track Doppler shifts in the sunlight incident on any solar system body that may appear in the background as viewed by the receiver. A Fraunhofer filter used with a direct-detection receiver should be tuned to match the Doppler shifts of the source and background. The required tuning calculated here for various situations is also required if, instead, one uses a heterodyne receiver with limited post-detection bandwidth.

Kerr, E. L.↗
NASA NTRS1986

Two-photon laser-induced fluorescence detection of OH

The TP-LIF OH sensor is based on the principle that a molecule having multiple energy states, all of which are bonding, can be pumped into the highest state with the resulting fluorescence being blue-shifted relative to all pumping wavelengths. In this way, one can successfully discriminate against virtually all noise sources in the system using long wavelength blocking filters in conjunction with solar-blind photomultiplier tubes. Thus, these systems tend to be signal limited rather than signal-to-noise limited as is true of the SP-LIF technique as well as other conventional analytical methods. The trick to achieving the above sampling scheme, with high efficiency, is in the use of high photon fluxes of short time duration. Obviously, the latter type of light source is fulfilled nicely by available pulsed lasers. From an operational point of view, however, this laser source needs to be tunable. The latter characteristic permits extremely high selectivity for the detection of a diatomic or simple polyatomic molecule by taking advantage of the high-resolution spectroscopic features of these type species.

Davis, D. D.↗
NASA NTRS1986

Ultrasensitive detection of atmospheric trace gases using frequency modulation spectroscopy

Frequency modulation (FM) spectroscopy is a new technique that promises to significantly extend the state-of-the-art in point detection of atmospheric trace gases. FM spectroscopy is essentially a balanced bridge optical heterodyne approach in which a small optical absorption or dispersion from an atomic or molecular species of interest generates an easily detected radio frequency (RF) signal. This signal can be monitored using standard RF signal processing techniques and is, in principle, limited only by the shot noise generated in the photodetector by the laser source employed. The use of very high modulation frequencies which exceed the spectral width of the probed absorption line distinguishes this technique from the well-known derivative spectroscopy which makes use of low (kHz) modulation frequencies. FM spectroscopy was recently extended to the 10 micron infrared (IR) spectral region where numerous polyatomic molecules exhibit characteristic vibrational-rotational bands. In conjunction with tunable semiconductor diode lasers, the quantum-noise-limited sensitivity of the technique should allow for the detection of absorptions as small as .00000001 in the IR spectral region. This sensitivity would allow for the detection of H2O2 at concentrations as low as 1 pptv with an integration time of 10 seconds.

Cooper, David E.↗
NASA NTRS1987

The coupled dynamics of fluids and spacecraft in low gravity and low gravity fluid measurement

The very large mass fraction of liquids stored on broad current and future generation spacecraft has made critical the technologies of describing the fluid-spacecraft dynamics and measuring or gauging the fluid. Combined efforts in these areas are described, and preliminary results are presented. The coupled dynamics of fluids and spacecraft in low gravity study is characterizing the parametric behavior of fluid-spacecraft systems in which interaction between the fluid and spacecraft dynamics is encountered. Particular emphasis is given to the importance of nonlinear fluid free surface phenomena to the coupled dynamics. An experimental apparatus has been developed for demonstrating a coupled fluid-spacecraft system. In these experiments, slosh force signals are fed back to a model tank actuator through a tunable analog second order integration circuit. In this manner, the tank motion is coupled to the resulting slosh force. Results are being obtained in 1-g and in low-g (on the NASA KC-135) using dynamic systems nondimensionally identical except for the Bond numbers.

Hansman, R. John↗
NASA NTRS1987

Experimental Resonance Enhanced Multiphoton Ionization (REMPI) studies of small molecules

Resonance enhanced multiphoton ionization (REMPI) utilizes tunable dye lasers to ionize an atom or molecule by first preparing an excited state by multiphoton absorption and then ionizing that state before it can decay. This process is highly selective with respect to both the initial and resonant intermediate states of the target, and it can be extremely sensitive. In addition, the products of the REMPI process can be detected as needed by analyzing the resulting electrons, ions, fluorescence, or by additional REMPI. This points to a number of exciting opportunities for both basic and applied science. On the applied side, REMPI has great potential as an ultrasensitive, highly selective detector for trace, reactive, or transient species. On the basic side, REMPI affords an unprecedented means of exploring excited state physics and chemistry at the quantum-state-specific level. An overview of current studies of excited molecular states is given to illustrate the principles and prospects of REMPI.

Dehmer, J. L.↗
NASA NTRS1987

Resonant enhanced multiphoton ionization studies of atomic oxygen

In resonant enhanced multiphoton ionization (REMPI), an atom absorbs several photons making a transition to a resonant intermediate state and subsequently ionizing out of it. With currently available tunable narrow-band lasers, the extreme sensitivity of REMPI to the specific arrangement of levels can be used to selectively probe minute amounts of a single species (atom) in a host of background material. Determination of the number density of atoms from the observed REMPI signal requires a knowledge of the multiphoton ionization cross sections. The REMPI of atomic oxygen was investigated through various excitation schemes that are feasible with available light sources. Using quantum defect theory (QDT) to estimate the various atomic parameters, the REMPI dynamics in atomic oxygen were studied incorporating the effects of saturation and a.c. Stark shifts. Results are presented for REMPI probabilities for excitation through various 2p(3) (4S sup o) np(3)P and 2p(3) (4S sup o) nf(3)F levels.

Dixit, S. N.↗
NASA NTRS1987

Free-electron laser simulations on the MPP

Free electron lasers (FELs) are of interest because they provide high power, high efficiency, and broad tunability. FEL simulations can make efficient use of computers of the Massively Parallel Processor (MPP) class because most of the processing consists of applying a simple equation to a set of identical particles. A test version of the KMS Fusion FEL simulation, which resides mainly in the MPPs host computer and only partially in the MPP, has run successfully.

Vonlaven, Scott A.↗
NASA NTRS1987

Mathematical modeling of a Ti:sapphire solid-state laser

The project initiated a study of a mathematical model of a tunable Ti:sapphire solid-state laser. A general mathematical model was developed for the purpose of identifying design parameters which will optimize the system, and serve as a useful predictor of the system's behavior.

Swetits, John J.↗
NASA NTRS1987

Titanium-doped sapphire laser research and design study

Three main topics were considered in this study: the fundamental laser parameters of titanium-doped sapphire, characterization of commercially grown material, and design of a tunable, narrow-linewidth laser. Fundamental parameters investigated included the gain cross section, upper-state lifetime as a function of temperature and the surface-damage threshold. Commercial material was found to vary widely in the level of absorption of the laser wavelength with the highest absorption in Czochralski-grown crystals. Several Yi:sapphire lasers were constructed, including a multimode laser with greater than 50mJ of output energy and a single-transverse-mode ring laser, whose spectral and temporal characteristics were completely characterized. A design for a narrow-linewidth (single-frequency) Ti:sapphire laser was developed, based on the results of the experimental work. The design involves the use of a single-frequency, quasi-cw master oscillator, employed as an injection source for a pulsed ring laser.

Moulton, Peter F.↗
NASA NTRS1986

Solid-state radio frequency oscillator for optogalvanic spectroscopy - Detection of nitric oxide using the 2-0 overtone transition

A compact, solid-state radio-frequency oscillator of low-power consumption is described, which allows quantitative measurement of the optogalvanic effect in low-pressure gas discharges. The oscillator has been used to record a portion of the 2-0 overtone band of nitric oxide at a pressure of about 1 Torr using a tunable color-center laser operating at 2.65 microns.

May, R. D.↗
NASA NTRS1986

Pulsed injection control of a titanium-doped sapphire laser

Injection control of a tunable Ti:sapphire laser using a narrow-bandwidth pulsed dye laser operating at a wavelength removed from the peak of the Ti:sapphire-laser gain curve is reported. The free-running Ti:sapphire laser had broadband laser emission from 750 to 790 nm. Injection at 727 nm resulted in essentially complete energy extraction at that wavelength in a 2.5-pm bandwidth matching the injection source.

Brockman, Philip↗
NASA NTRS1986

Picosecond coherent anti-Stokes Raman scattering (CARS) study of vibrational dephasing of carbon disulfide and benzene in solution

The vibrational dephasing of the 656/cm mode (nu1, a1g) of CS2 and the 991/cm mode (nu2, a1g) of benzene have been studied as a function of concentration in mixtures with a number of solvents using a ps time-resolved CARS technique. This technique employs two tunable synchronously-pumped mode-locked dye lasers in a stimulated Raman pump, coherent anti-Stokes Raman probe time-resolved experiment. Results are obtained for CS2 in carbon tetrachloride, benzene, nitrobenzene, and ethanol and for benzene nu2 in CS2. The dephasing rates of CS2 nu1 increase on dilution with the polar solvents and decrease or remain constant on dilution with the nonpolar solvents. The CS2/benzene solutions show a contrasting behavior, with the CS2 nu1 dephasing rate being nearly independent of concentration whereas the benzene nu2 dephasing rate decreases on dilution. These results are compared to theoretical models for vibrational dephasing of polyatomic molecules in solution.

Perry, Joseph W.↗
NASA NTRS1986

Transient gain-versus-absorption laser probing of spin-orbit states, kinetics and dynamics

The spin-orbit populations of excited (2P1/2) and ground (2P3/2) state Br atoms at 2714 nm and I atoms at 1315 nm are examined using a tunable F-center laser and a diode laser. The transient laser gain-versus-absorption measurements are utilized to estimate quantum yields of the spin-orbit states in the photodissociation of Br- and I-containing compounds; the continuum yields for Br2 are investigated in terms of temperature. The collisional release, Doppler velocity effects, and differing reactivity of the spin-orbit excited and ground state atoms are studied. It is noted that the transient gain versus absorption technique is applicable to the analysis of kinetic phenomena due to its high sensitivity and excellent time resolution.

Smedley, John E.↗
NASA NTRS1986

A Fabry-Perot interferometer for accurate measurement of temporal changes in stellar Doppler shift

The scrambling of incident light by an optical filter, and the stability obtainable through wavelength calibration by means of a tilt-tunable Fabry-Perot etalon, allow the accurate observation of Doppler shift changes in stellar absorption lines. Distinct, widely spaced monochromatic images of the entrance aperture are formed in the focal plane of the camera through a sampling of about 350 points on the profile of the stellar spectrum by successive orders of interferometric transmission through the etalon. Changes in Doppler shift modify the relative intensities of these images, in proportion to the slope of the spectral profile at each point sampled.

Mcmillan, R. S.↗