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DOE OSTI2020

Grand potential sintering simulations of doped UO 2 accident-tolerant fuel concepts

Chromium-doped UO is a widely-studied near-term deployable accident-tolerant fuel concept because it results in a dense, large-grain structure that increases the fuel resistance to densification, swelling, and fission gas release. A new charged-interstitial mechanism was recently proposed to describe the behavior of dopants like chromium in sintered UO 2 . Based on that mechanism, manganese was suggested as an even stronger dopant than chromium. In the current work we use mesoscale sintering simulations in an effort to validate the new mechanism. We compare the relative behavior of Cr-doped and undoped UO 2 against experimental data in the literature. We also make predictions of the relative behavior of Mn-doped UO 2 . Simulations are done using the phase field-based grand potential sintering model. Dopants have two effects on sintered UO 2 . They marginally increase the densification rate and greatly increase the average grain size. Both of these effects are individually tested in small-scale simulations. Then large 3D sintering simulations are used to test the combined behavior of both effects. The results for the densification rate simulations are consistent with experiments for Cr-doped fuels. However, we note the grain growth rates are lower than what is found in the literature for Cr-doped fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NASA NTRS1999

Particle Detectors and Data Analysis for Cusp Transient Features Campaign

On December 3, 1997, a rocket payload (36.152) was launched from N(sub y) Alesund into the dark cusp at 0906:00 U (1206:00 LT) during an interval of southward B(sub z) and positive B(sub y). Launch occurred during a time interval of northeastward moving auroral forms observed between 0845 and 0945 UT by ground-based meridian scanning photometers. Ground photometric measurements during the flight show that the payload passed over the poleward portion of the most intense 6300 A emissions of the dayside cusp/cleft region. Electrons of energy up to a few hundred eV were detected immediately upon instrument turn-on at an altitude of 205 km and throughout the flight until the payload reached an altitude of -197 km on the downleg. Electron spectra were either quasithermal with peak energies -100 eV or showed evidence of acceleration along the magnetic field line by potentials of 100-200 V. Precipitating ions were observed throughout much of the flight. Their spectra were broadly peaked in energy with the peak energy decreasing from -500 eV to -250 eV as the payload flew approximately westward over the dayside precipitation region. Structure (spatial or temporal intensity variation) was observed between T + 180 s and T + -400 s. At the rocket altitudes (<450 km) the ions were observed to be precipitating. During the flight, the DMSP F-13 satellite passed through the all-sky imager field-of-view just poleward of the brightest dayside emissions enabling the identification of plasma sheet and boundary layer regions along the orbit. We thus conclude that particle fluxes detected by the rocket flight were either cusp plasma or boundary layer/mantle plasma just poleward of the dayside cusp/cleft. A paper describing the fields and plasmas observed during the flight is now being prepared for publication.

Sharber, James R.↗

NASA NTRS1992

Applied-field magnetoplasmadynamic engine developments

There are potential space exploration missions which may significantly benefit from the use of electric propulsion at power levels of hundreds of kilowatts. The applied magnetic field MPD thruster is potentially capable of efficient, high specific impulse operation in this power range. This paper describes current experimental and analytical efforts to further the development of such a thruster and presents the latest results. In particular, efforts to measure, simultaneously, the thrust developed by the archead and by the electromagnet, and to evaluate the effect of a diffuser on vacuum tank back pressure, are presented and discussed. It was found that with ammonia vapor as propellant, the vacuum tank pressure was reduced from 8 to 4.9 Pa at a power level of 80 kW. This pressure decrease is expected to become greater as the power and applied field are increased. Also, the development of a cathode/plasma interaction model for determining the heat loads to the cathode as functions of the various free stream plasma parameters is presented. This model is combined with a cathode thermal model in order to provide a complete and integrated picture of MPD thruster cathode operation. Several computational examples are used to illustrate the combined model.

Goodfellow, K. D.↗

NASA NTRS1998

Particle Detectors and Data Analysis for Cusp Transient Features Campaign

On December 3, 1997, a rocket payload (36.152) was launched from Ny Alesund into the dark cusp at 0906:00 U (1206:00 LT) during an interval of southward B(sub Z), and positive B(sub y). Launch occurred during a time interval of northeastward moving auroral forms observed between 0845 and 0945 UT by ground-based meridian scanning photometers. Ground photometric measurements during the flight show that the payload passed over the poleward portion of the most intense 6300 A emissions of the dayside cusp/cleft region. Electrons of energy up to a few hundred eV were detected immediately upon instrument turn-on at an altitude of 205 km and throughout the flight until the payload reached an altitude of approximately 197 km on the downleg. Electron spectra were either quasithermal with peak energies approximately 100 eV or showed evidence of acceleration along the magnetic field line by potentials of 100-200 V. Precipitating ions were observed throughout much of the flight. Their spectra were broadly peaked in energy with the peak energy decreasing from approximately 500 eV to approximately 250 eV as the payload flew approximately westward over the dayside precipitationregion. Structure(spatial or temporal intensity variation) was observed between T + 180 s and T + approximately 400 s. At the rocket altitudes(less than 450km) the ions were observed to be precipitating. During the flight, the DMSPF-13 satellite passed through the all-sky imager field-of-view just poleward of the brightest dayside emissions enabling the identification of plasma sheet and boundary layer regions along the orbit. We thus conclude that particle fluxes detected by the rocket flight were either cusp plasma or boundary layer/mantle plasmajust poleward of the dayside cusp/cleft. Further investigation of the particle characteristics and their relationship to ionospheric convection patterns is continuing.

Sharber, James R.↗

NASA NTRS2011

Demonstrating the Operational Value of Atmospheric Infrared Sounder (AIRS) Retrieved Profiles in the Pre-Convective Environment

The Short-term Prediction Research and Transition Center (SPoRT) is a collaborative partnership between NASA and operational forecasting partners, including a number of National Weather Service offices. SPoRT provides real-time NASA products and capabilities to its partners to address specific operational forecast challenges. One operational forecast challenge is forecasting convective weather in data-void regions such as large bodies of water (e.g. Gulf of Mexico). To address this forecast challenge, SPoRT produces a twice-daily three-dimensional analysis that blends a model first-guess from the Advanced Research Weather Research and Forecasting (WRF-ARW) model with retrieved profiles from the Atmospheric Infrared Sounder (AIRS) -- a hyperspectral sounding instrument aboard NASA's Aqua satellite that provides temperature and moisture profiles of the atmosphere. AIRS profiles are unique in that they give a three dimensional view of the atmosphere that is not available through the current rawinsonde network. AIRS has two overpass swaths across North America each day, one valid in the 0700-0900 UTC timeframe and the other in the 1900-2100 UTC timeframe. This is helpful because the rawinsonde network only has data from 0000 UTC and 1200 UTC at specific land-based locations. Comparing the AIRS analysis product with control analyses that include no AIRS data demonstrates the value of the retrieved profiles to situational awareness for the pre-convective (and convective) environment. In an attempt to verify that the AIRS analysis was a good representation of the vertical structure of the atmosphere, both the AIRS and control analyses are compared to a Rapid Update Cycle (RUC) analysis used by operational forecasters. Using guidance from operational forecasters, convective available potential energy (CAPE) was determined to be a vital variable in making convective forecasts and is used herein to demonstrate the utility of the AIRS profiles in changing the vertical thermodynamic structure of the atmosphere in the pre-convective and convective environment. CAPE is an important metric because of it is a quantitative measure of atmospheric stability, which is necessary information when forecasting for convective weather. Case studies from the summer of 2010 were examined, and most impact from the AIRS retrieved profiles occurred over the data-void Gulf of Mexico with fields of convective potential closer to the RUC than the CNTL. Mixed results were found when AIRS retrieved profiles were used over land, so more cases need to be examined to determine whether AIRS would be an effective tool over land. Additional analyses of problematic convective forecasts over the Gulf Coast will be needed to determine the operational impact of AIRS. SPoRT eventually plans to transition the AIRS product to select Weather Forecast Office (WFO) partners, pending the outcome of these additional analyses.

Kozlowski, Danielle M.↗

DOE OSTI2025

Single-shot measurements of shaped XUV FEL pulses with frequency-resolved optical gating

The ability to control the amplitude and phase of extreme ultraviolet (XUV) and X-ray free-electron laser (FEL) pulses can allow for the extension of optical techniques, such as multidimensional spectroscopy or coherent control, to higher photon energies, for probing and controlling core electronic transitions. However, this requires the ability to make single-shot, and complete, electric field measurements of potentially complex FEL pulses, in order to develop, and verify, pulse shaping strategies. Here, we present direct, single-shot measurements of XUV pulses generated under special operating configurations for producing specific pulse shapes from a laser-seeded XUV FEL. To do this, we built upon our past work using transient grating (TG) cross correlation frequency-resolved optical gating (FROG), where an optical reference pulse is diffracted from an XUV TG produced by a pair of interfering FEL pulses. The resulting nonlinear signal versus frequency and delay, i.e., the FROG trace, contains the electric field of the FEL pulse. The FEL pulse electric field is reconstructed from the FROG trace using a phase retrieval algorithm. Here we confirmed three different pulse shaping strategies for generating chirped, double and multiple FEL pulses by tuning the seed laser and FEL parameters and measuring the resulting shaped FEL pulses with TG XFROG. This work paves the way for generating on-demand pulse shapes with a seeded FEL by improving the characterization of FEL pulses, for transform-limited to more complex shapes.

Elverson, Francesca↗

NASA NTRS1996

Stratospheric Meteorological Conditions for the 3-12 Nov. 1994 ATMOS/ATLAS-3 Measurements

During the ATLAS-3 mission (3-12 Nov 1994), United Kingdom Meteorological Office fields show that the SH vortex was still strong below about 700 K (approximately 16 hPa), with coherent vortex fragments apparent up to about 1300 K (approximately 3 hPa). The SH vortex was shifted off the pole toward 270 deg E throughout ATLAS-3, although its shape varied from day to day. SH temperatures were increasing during ATLAS-3; temperatures below 188 K were last seen 35-45 days before the mission, but were below 195 K as late as 2 Nov 1994. The NH polar vortex had developed at levels above about 550 K (approximately 35 hPa). Simulated high-resolution potential vorticity (PV) fields clearly show low latitude air being drawn up around the polar vortices in both hemispheres. These fields indicate that meteorological analyses underestimate the amount of atmospheric variability, including the strength of local PV gradients, and small-scale structure. Structure such as that in the simulated fields can result in apparent discrepancies between tracer measurements and PV fields.

Manney, G. L.↗

DOE OSTI2021

Small-Signal Stability Analysis of Low-Inertia Power Grids with Inverter-Based Resources and Synchronous Condensers: Preprint

With the potential environmental impacts of conventional fossil fuels and the technology advances of grid interactive power electronics, inverter-based resources (IBRs) are playing a crucial role in modern power grids. However, due to the lack of physical inertia, IBRs are vulnerable to system disturbances. Further, conventional grid-following (GFL) inverters cannot actively establish the frequency and voltage, which could not be a appropriate solution for 100% inverter-based power grids. Grid-forming (GFM) control, as an emerging inverter control function, has drawn great attention in recent years, while it is still under development and pre-mature for large-scale field deployment. A potential solution for gradually transitioning into a 100% inverter-based power grid is to combine both IBRs and synchronous machines into a mixed generation portfolio. More importantly, synchronous machines can be operated as synchronous condensers (SCs) until they are retired. It is also worth mentioning that the stability analysis is of great importance to ensure the smooth transition from existing power grids to 100% inverter-based system, which is the main focus of this work with detailed modeling and modal analysis.

100% renewable↗

NASA NTRS1987

A three-dimensional dual potential procedure with applications to wind tunnel inlets and interacting boundary layers

A dual potential decomposition of the velocity field into a scalar and a vector potential function is extended to three dimensions and used in the finite-difference simulation of steady three-dimensional inviscid rotational flows and viscous flow. The finite-difference procedure was used to simulate the flow through the 80 by 120 ft wind tunnel at NASA Ames Research Center. Rotational flow produced by the stagnation pressure drop across vanes and screens which are located at the entrance of the inlet is modeled using actuator disk theory. Results are presented for two different inlet vane and screen configurations. The numerical predictions are in good agreement with experimental data. The dual potential procedure was also applied to calculate the viscous flow along two and three dimensional troughs. Viscous effects are simulated by injecting vorticity which is computed from a boundary layer algorithm. For attached flow over a three dimensional trough, the present calculations are in good agreement with other numerical predictions. For separated flow, it is shown from a two dimensional analysis that the boundary layer approximation provides an accurate measure of the vorticity in regions close to the wall; whereas further away from the wall, caution has to be exercised in using the boundary-layer equations to supply vorticity to the dual potential formulation.

Rao, K. V.↗

NASA NTRS1987

A three-dimensional dual potential procedure for inlets and indraft wind tunnels

Rao, K. V.↗

NASA NTRS1994

Direct entry of dense flowing plasmas into the distant tail lobes

Electric field, magnetic field, and spacecraft potential measurements on the Geotail satellite have confirmed earlier observations of relatively dense flowing plasmas in the magnetotail lobes. Within these flowing plasmas, density discontinuities of factors of 2 to 4 were observed. At least 15 of the 18 magnetopause crossings that occurred during a 24-hour interval when the spacecraft was at GSM coordinates near X = -140 R(sub e), Y = 0, and Z = 15 R(sub e), were rotational discontinuities across which the magnetosheath plasma had direct entry into the tail lobes. Within the lobes near the rotational discontinuities, the spacecraft typically crossed a second boundary at which the plasma density decreased from its magnetosheath value by a typical factor of 1.5 to 3 while the magnetic field strength and flow speed increased. Equatorward of this density discontinuity, the plasma density and flow remained appreciable. At least 2 of the 18 magnetopause crossings may have been tangential discontinuities across which the density and magnetic field strength both changed. Within the lobes near these tangential discontinuities, significant densities of flowing plasma were observed. Since 11 of the 18 discontinuities were crossed within a time interval of less than 7 seconds, the bondary current layer was well-defined and very thin.

Mozer, F. S.↗

DOE OSTI2020

Constraining axion inflation with gravitational waves from preheating

We study gravitational wave production from gauge preheating in a variety of inflationary models, detailing its dependence on both the energy scale and the shape of the potential. In this work, we show that preheating into Abelian gauge fields generically leads to a large gravitational wave background that contributes significantly to the effective number of relativistic degrees of freedom in the early universe, $N_{\text{eff}}$. We demonstrate that the efficiency of gravitational wave production is correlated with the tensor-to-scalar ratio, $\textit{r}$. In particular, we show that efficient gauge preheating in models whose tensor-to-scalar ratio would be detected by next-generation cosmic microwave background experiments ($\textit{r}$ ≳ 10 –3 ) will be either detected through its contribution to $N_{\text{eff}}$ or ruled out. Furthermore, we show that bounds on $N_{\text{eff}}$ provide the most sensitive probe of the possible axial coupling of the inflaton to gauge fields regardless of the potential.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

Thermal false vacuum decay around black holes

In flat space and at finite temperature, there are two regimes of false vacuum decay in quantum field theory. At low temperature, the decay proceeds through thermally-assisted tunneling described by periodic Euclidean solutions—bounces—with nontrivial time dependence. On the other hand, at high temperatures the bounces are time independent and describe thermal jumps of the field over the potential barrier. Here, we argue that only solutions of the second type are relevant for false vacuum decay catalyzed by a black hole in equilibrium with thermal bath. The argument applies to a wide class of spherical black holes, including d-dimensional anti–de Sitter/de Sitter Schwarzschild black holes and Reissner-Nordström black holes sufficiently far from criticality. It does not rely on the thin-wall approximation and applies to multifield scalar theories.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1991

Sources of field-aligned currents in the auroral plasma

Data from the Dynamics Explorer 1 High Altitude Plasma Instrument (HAPI) and magnetometer are used to investigate the sources of field-aligned currents in the nightside auroral zone. It is found that the formula developed by S. Knight predicts the field-aligned current density fairly accurately in regions where a significant potential drop can be inferred from the HAPI data; there are, however, regions in which the proportionality between potential drop and field-aligned current does not hold. In particular, occurrences of strong upward field-aligned current associated not with inverted-V events but instead with suprathermal bursts are noted. In addition, upward field-aligned currents are often observed to peak near the edges of inverted-V events, rather than in the center as would be predicted by Knight.

Marshall, J. A.↗

NASA NTRS2004

Lunar and Planetary Science XXXV: Mars Geophysics

The titles in this section include: 1) Distribution of Large Visible and Buried Impact Basins on Mars: Comparison with Free-Air Gravity, Crustal Thickness, and Magnetization Models; 2) The Early Thermal and Magnetic State of Terra Cimmeria, Southern Highlands of Mars; 3) Compatible Vector Components of the Magnetic Field of the Martian Crust; 4) Vertical Extrapolation of Mars Magnetic Potentials; 5) Rock Magnetic Fields Shield the Surface of Mars from Harmful Radiation; 6) Loading-induced Stresses near the Martian Hemispheric Dichotomy Boundary; 7) Growth of the Hemispheric Dichotomy and the Cessation of Plate Tectonics on Mars; 8) A Look at the Interior of Mars; 9) Uncertainties on Mars Interior Parameters Deduced from Orientation Parameters Using Different Radio-Links: Analytical Simulations; 10) Refinement of Phobos Ephemeris Using Mars Orbiter Laser Altimetry Radiometry.

Source record↗

DOE OSTI2020

Rapid Generation of Hierarchically Porous Metal–Organic Frameworks through Laser Photolysis

Abstract Hierarchically porous metal–organic frameworks (HP‐MOFs) facilitate mass transfer due to mesoporosity while preserving the advantage of microporosity. This unique feature endows HP‐MOFs with remarkable application potential in multiple fields. Recently, new methods such as linker labilization for the construction of HP‐MOFs have emerged. To further enrich the synthetic toolkit of MOFs, we report a controlled photolytic removal of linkers to create mesopores within microporous MOFs at tens of milliseconds. Ultraviolet (UV) laser has been applied to eliminate “photolabile” linkers without affecting the overall crystallinity and integrity of the original framework. Presumably, the creation of mesopores can be attributed to the missing‐cluster defects, which can be tuned through varying the time of laser exposure and ratio of photolabile/robust linkers. Upon laser exposure, MOF crystals shrank while metal oxide nanoparticles formed giving rise to the HP‐MOFs. In addition, photolysis can also be utilized for the fabrication of complicated patterns with high precision, paving the way towards MOF lithography, which has enormous potential in sensing and catalysis.

Wang, Kun‐Yu↗

DOE OSTI2020

Rapid Generation of Hierarchically Porous Metal–Organic Frameworks through Laser Photolysis

Hierarchically porous metal–organic frameworks (HP-MOFs) facilitate mass transfer due to mesoporosity while preserving the advantage of microporosity. This unique feature endows HP-MOFs with remarkable application potential in multiple fields. Recently, new methods such as linker labilization for the construction of HP-MOFs have emerged. To further enrich the synthetic toolkit of MOFs, we report a controlled photolytic removal of linkers to create mesopores within microporous MOFs at tens of milliseconds. Ultraviolet (UV) laser has been applied to eliminate “photolabile” linkers without affecting the overall crystallinity and integrity of the original framework. Presumably, the creation of mesopores can be attributed to the missing-cluster defects, which can be tuned through varying the time of laser exposure and ratio of photolabile/robust linkers. Upon laser exposure, MOF crystals shrank while metal oxide nanoparticles formed giving rise to the HP-MOFs. In addition, photolysis can also be utilized for the fabrication of complicated patterns with high precision, paving the way towards MOF lithography, which has enormous potential in sensing and catalysis.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2022

System and technoeconomic analysis of solar thermochemical hydrogen production

Hydrogen is a promising energy carrier that can be obtained from various feedstocks using renewable energy sources. Direct solar thermochemical hydrogen (STCH) production by water splitting can utilize the full spectrum of solar radiation and has the potential to achieve high solar energy conversion efficiencies. Currently STCH research areas focus on material discovery. This paper evaluates the performance of various STCH materials in the context of a system platform to assess techno-economic benefits and gaps in the path to STCH scale-up. Additionally, to analyze the hydrogen production cost, a concentrating solar thermal (CST) system is introduced as a platform for integrating STCH materials and accommodating generalized thermochemical processes. The thermochemical process is based on a two-step STCH cycle using metal oxide that consists of a high temperature step for metal oxide reduction, followed by an oxidation step for water splitting at a lower temperature. A preferred configuration is to have the high temperature step occurring in a directly irradiated solar receiver reactor. To this end, we conceptualized a receiver design and associated solar field layout and investigated STCH operational boundaries, component costs and sensitivity parameters on the $2/kgH 2 goal of hydrogen production. The study explored system-related variables and factors associated with scaling up. The CST platform allows more comprehensive studies that encompass aspects of STCH materials and systems such as cost, hydrogen productivity and replacement frequency, alongside other system components like heliostat field, tower, and potential receiver costs.

08 HYDROGEN↗