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At least 811 records · Page 45

Quantum computing using chiral qubits

An apparatus for performing quantum computing includes multiple qubits, each of at least a subset of the qubits comprising a loop formed of a Dirac or Weyl semimetal and having at least two stable quantum states. The apparatus further includes at least one terahertz cavity coupled with the qubits, the terahertz cavity being configured to detect the quantum states of the qubits. Each of at least the subset of qubits is configured to receive a circularly polarized radiation source. The radiation source is adapted to excite a chiral current in each of at least the subset of qubits, the quantum states of the plurality of qubits being a function of the chiral current.

97 MATHEMATICS AND COMPUTING↗

Radiolabeled and fluorescent PARP inhibitors for imaging and radiotherapy

The present disclosure relates to compounds of Formula I and II, wherein R1-R20 and FL are defined herein. Also provided are methods of targeting alpha-radiation to poly(ADP-ribose)polymerase 1 (PARP-1) enzyme expression, reducing proliferation of cancer cells, reducing proliferation of cancer cells, detecting intact and enzymatically active poly(ADP-ribose)polymerase 1 (PARP-1) enzyme expression, detecting PARP-1 enzyme expression in a subjects tissue sample, monitoring cancer treatment in a subject, or detecting a PARP-1 receptive cancer in a subject.

Mach, Robert H.↗

Studies of LAPPD and HRPPD photodetectors for Cherenkov imaging applications

HRPPDs are the baseline single-photon sensors for a classic proximity-focusing RICH (pfRICH) counter, one of the Cherenkov radiation-based PID subsystems of the ePIC detector at the EIC. We report SPE time resolution of 87 ps rms for an LAPPD unit detecting Cherenkov photons in a quartz lens at a CERN PS test beam (2022). We also present the degradation and partial recovery of gain and relative efficiency of an LAPPD unit as a function of the B-field strength (up to 1.5 T) and angular orientation, measured with vertical dipole magnets at CERN (2023–2024). Finally, we report preliminary results of an accelerated ageing study performed on an HRPPD unit in Trieste laboratory (2025).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Detection of Defects in Additively Manufactured Metallic Materials with Machine Learning of Pulsed Thermography Images

Additive manufacturing (AM) is an emerging method for cost-efficient fabrication of nuclear reactor parts. AM of metallic structures for nuclear energy applications is currently based on laser powder bed fusion (LPBF) process, which can introduce internal material flaws, such as pores and anisotropy. Integrity of AM structures needs to be evaluated nondestructively because material flaws could lead to premature failures due to exposure to high temperature, radiation and corrosive environment in a nuclear reactor. Quality control (QC) requires nondestructive evaluation (NDE) of actual AM structures. Pulsed thermography is a potentially promising QC technique because it is scalable to arbitrary structure size. However, detection sensitivity of this method is limited by noises. We investigate separation of signal from noise in thermography images using several machine learning (ML) methods, including new spatio-temporal blind source separation (STBSS) and spatio-temporal sparse dictionary learning (STSDL) methods. Performance of the ML methods is benchmarked using thermography data obtained from imaging stainless steel 316L and Inconel 718 specimens produced LPBF method with imprinted calibrated porosity defects. The ML methods are ranked by F-score and execution runtime. The ML methods with higher accuracy require longer run time. However, this runtime is sufficiently short to perform QC within a realistic time frame.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Examining a hadronic γ-ray scenario for the radiative shell and molecular clouds of the old GeV supernova remnant G298.6−0.0

Abstract Based on the 13.7 yr Fermi-LAT data, Yeung, Bamba, and Sano (2023, PASJ, 75, 384) claimed detection of two γ-ray sources (namely Src-NE and Src-NW) associated with the supernova remnant (SNR) G298.6−0.0, and interpreted it as an old GeV SNR interacting with molecular clouds (MCs). In this follow-up study, we refine the flux measurements below 2 GeV with Fermi-LAT event types of better angular reconstruction. Then, we report our γ-ray spectral fittings and cosmic-ray phenomenology in a hadronic scenario, considering both the shell and MC regions of SNR G298.6−0.0. We confirm that the γ-ray spectra of both Src-NE and Src-NW exhibit spectral breaks, at $1.50_{-0.50}^{+0.60}$ and $0.68_{-0.11}^{+0.32}\:$GeV, respectively. Src-NW has a harder broad-band photon index than Src-NE, suggesting an appreciable difference between the physical separations of their respective emission sites from SNR G298.6−0.0. The cosmic-ray spectrum responsible for Src-NE starts with a minimum energy $E_\mathrm{CR,min}=1.38_{-0.16}^{+0.47}\:$GeV, and has a proton index $\Gamma _\mathrm{CR}=2.57_{-0.21}^{+0.18}$ below the exponential cutoff energy $E_\mathrm{CR,max}=240_{-150}^{+240}\:$GeV. Accordingly, we argue that Src-NE is dominated by the SNR shell, while only a minor portion of lower-energy emission is contributed by the MCs interacting with the SNR. The cosmic-ray population for Src-NW starts at a higher energy such that the ECR, min ratio of Src-NW to Src-NE is ≳2. The high ECR, min, as well as the high cosmic-ray energy density required (∼26 eV cm−3), supports the interpretation that Src-NW is predominantly the γ-ray emission from the farther MCs being bombarded by protons that had earlier escaped from SNR G298.6−0.0. By comparing the high-energy features of G298.6−0.0 with those of analogical SNRs, especially SNR W 28 and SNR W 44, we further constrain the age of SNR G298.6−0.0 to be 10–30 kyr, under the assumption of a purely hadronic scenario.

Astronomy & Astrophysics↗

Data trustworthiness signatures for nuclear reactor dynamics simulation

With the increased reliance on digitization in industrial control systems, the need for effective monitoring techniques has risen dramatically. Specifically, there is now a growing concern about the so-called false data injection (FDI) attacks. These attacks aim to alter the raw sensors’ data to cause malicious outcomes. Any serious FDI algorithm is based on an intimate knowledge of the system and its associated physics models, which renders conventional outlier/anomaly detection techniques almost obsolete in the face of such attacks. Thus, a critical need has emerged to develop a new class of defense methods that are capable of detecting FDI attacks under the assumption that the attacker has a strong familiarity with the system and its physics modeling. This class of defense methods are denoted by model-based defenses which are premised on the assumption that the attacker, while having a good understanding of the system, does not have full privileged access to all proprietary data and historical records of operation. However, (s)he is assumed to be capable of learning system behavior using self-learning techniques during an initial lie-in-wait period. To defend against this scenario, we propose a new model-based randomized window algorithm that searches time-series data for signatures that can serve as classifiers between normal and FDI scenarios. The classifiers are based on the correlations between the dominant degrees of freedom (DOFs) and the less-dominant DOFs (expected to be very sensitive to the system details that are unknown to the attacker). For demonstration, RELAP5 models are employed to calculate representative nuclear reactor behavior during a number of transient scenarios. Finally, falsified data are injected into the RELAP5-simulated behavior, and the proposed signature-identification algorithm is employed to detect the injected data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Flow Injection Electrochemical Quartz Crystal Microbalance with ICP-OES Detection: Electroprecipitation and Stripping of Lanthanum and Neodymium in a Flow Cell

We used an improved version of our hyphenated analysis technique, flow injection electrochemical quartz crystal microbalance (EQCM) with inductively coupled optical emission spectroscopy, to investigate the electroprecipitation of lanthanum and neodymium from flowing solutions. The improved version has two independent flow injection circuits, allowing different conditions for electrochemical precipitation (pH=4.3 or 2.6) and quick stripping (2% HNO3) with EQCM mass detection and ICP-OES elemental analysis. Lanthanum or neodymium ions in a 500 uL sample were injected into a carrier stream and deposited onto an EQCM housed in a micro flow cell, owing to a localized high-pH layer. The deposits are subsequently stripped from the electrode using HNO3 and analyzed downstream using an ICP-OES. We found that using acidic solutions without supporting electrolyte leads to an increase of the amount of lanthanum detected by 4-fold. The enhanced deposition can be attributed to enhanced mass transfer by migration. Furthermore, we showed that by applying chronopotentiometry, we can detect a change in the hydrogen evolution reaction mechanism that enables the precipitation of lanthanides on the surface of the electrode. Understanding and enhancing the deposition of lanthanides is relevant for elemental or isotopic detection in nuclear forensics.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Accelerating Surface Radiation Content to Investigate the Impact of Radon Progeny on Superconducting Qubits

Ionizing radiation in the form of $α$, $β$, $γ$, and additional high-energy particles can induce decoherence via phonon and quasiparticle poisoning in superconducting qubits. Recent studies have explored this effect using cosmic rays or controlled radioactive sources held in the proximity of a qubit package, and have concluded that reductions in such ``external'' environmental radiation may benefit stable operation of qubit devices. However, the effect of long-lived, unstable daughters of $^{222}$Rn that ``plate out'' directly on device and packaging surfaces has not been as extensively explored. This plate-out process, well-known to the dark matter direct detection field, occurs throughout the fabrication and testing lifecycle of a device and (separately) its packaging, and produces a local source of $α$-decays which can remain active for decades. As this scales with chip area, understanding and managing this source of ionizing radiation is relevant for successfully scaling quantum computing architectures to larger numbers of qubits in a radiation-robust way. We present a setup capable of accelerating and enhancing radon daughter plateout by a factor of $7\times10^4$ over ambient, in order to study, \textit{in situ}, the impact of these events on superconducting qubits. We also provide outlook on the potential impact of this source of ionizing radiation on current and future qubit arrays.

Poudel, Sagar S. [South Dakota Sch. Mines Tech.]↗

A semi-supervised machine learning detector for physics events in tokamak discharges

Databases of physics events have been used in various fusion research applications, including the development of scaling laws and disruption avoidance algorithms, yet they can be time-consuming and tedious to construct. This paper presents a novel application of the label spreading semi-supervised learning algorithm to accelerate this process by detecting distinct events in a large dataset of discharges, given few manually labeled examples. A high detection accuracy (>85%) for H-L back transitions and initially rotating locked modes is demonstrated on a dataset of hundreds of discharges from DIII-D with manually identified events for which only 3 discharges are initially labeled by the user. Lower yet reasonable performance (~75%) is also demonstrated for the core radiative collapse, an event with a much lower prevalence in the dataset. Additionally, analysis of the performance sensitivity indicates that the same set of algorithmic parameters is optimal for each event. This suggests that the method can be applied to detect a variety of other events not included in this paper, given that the event is well described by a set of 0D signals robustly available on many discharges. Procedures for analysis of new events are demonstrated, showing automatic event detection with increasing fidelity as the user strategically adds manually labeled examples. Detections on Alcator C-Mod and EAST are also shown, demonstrating the potential for this to be used on a multi-tokamak dataset.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Deforestation reshapes land-surface energy-flux partitioning

Land-use and land-cover change significantly modify local land-surface characteristics and water/energy exchanges, which can lead to atmospheric circulation and regional climate changes. In particular, deforestation accounts for a large portion of global land-use changes, which transforms forests into other land cover types, such as croplands and grazing lands. Many previous efforts have focused on observing and modeling land–atmosphere–water/energy fluxes to investigate land–atmosphere coupling induced by deforestation. However, interpreting land–atmosphere–water/energy-flux responses to deforestation is often complicated by the concurrent impacts from shifts in land-surface properties versus background atmospheric forcings. In this study, we used 29 paired FLUXNET sites, to improve understanding of how deforested land surfaces drive changes in surface-energy-flux partitioning. Each paired sites included an intact forested and non-forested site that had similar background climate. We employed transfer entropy, a method based on information theory, to diagnose directional controls between coupling variables, and identify nonlinear cause–effect relationships. Transfer entropy is a powerful tool to detective causal relationships in nonlinear and asynchronous systems. The paired eddy covariance flux measurements showed consistent and strong information flows from vegetation activity (gross primary productivity (GPP)) and physical climate (e.g. shortwave radiation, air temperature) to evaporative fraction (EF) over both non-forested and forested land surfaces. More importantly, the information transfers from radiation, precipitation, and GPP to EF were significantly reduced at non-forested sites, compared to forested sites. We then applied these observationally constrained metrics as benchmarks to evaluate the Energy Exascale Earth System Model (E3SM) land model (ELM). ELM predicted vegetation controls on EF relatively well, but underpredicted climate factors on EF, indicating model deficiencies in describing the relationships between atmospheric state and surface fluxes. Moreover, changes in controls on surface energy flux partitioning due to deforestation were not detected in the model. We highlight the need for benchmarking model simulated surface-energy fluxes and the corresponding causal relationships against those of observations, to improve our understanding of model predictability on how deforestation reshapes land surface energy fluxes.

54 ENVIRONMENTAL SCIENCES↗

Laser Ablation Plasmas and Spectroscopy for Nuclear Applications

The development of measurement methodologies to detect and monitor nuclear-relevant materials remains a consistent and significant interest across the nuclear energy, nonproliferation, safeguards, and forensics communities. Optical spectroscopy of laser-produced plasmas is becoming an increasingly popular diagnostic technique to measure radiological and nuclear materials in the field without sample preparation, where current capabilities encompass the standoff, isotopically resolved and phase-identifiable (e.g., UO and UO[Formula: see text]) detection of elements across the periodic table. These methods rely on the process of laser ablation (LA), where a high-powered pulsed laser is used to excite a sample (solid, liquid, or gas) into a luminous microplasma that rapidly undergoes de-excitation through the emission of electromagnetic radiation, which serves as a spectroscopic fingerprint for that sample. This review focuses on LA plasmas and spectroscopy for nuclear applications, covering topics from the wide-area environmental sampling and atmospheric sensing of radionuclides to recent implementations of multivariate machine learning methods that work to enable the real-time analysis of spectrochemical measurements with an emphasis on fundamental research and development activities over the past two decades. Background on the physical breakdown mechanisms and interactions of matter with nanosecond and ultrafast laser pulses that lead to the generation of laser-produced microplasmas is provided, followed by a description of the transient spatiotemporal plasma conditions that control the behavior of spectroscopic signatures recorded by analytical methods in atomic and molecular spectroscopy. High-temperature chemical and thermodynamic processes governing reactive LA plasmas are also examined alongside investigations into the condensation pathways of the plasma, which are believed to serve as chemical surrogates for fallout particles formed in nuclear fireballs. Laser-supported absorption waves and laser-induced shockwaves that accompany LA plasmas are also discussed, which could provide insights into atmospheric ionization phenomena from strong shocks following nuclear detonations. Furthermore, the standoff detection of trace radioactive aerosols and fission gases is reviewed in the context of monitoring atmospheric radiation plumes and off-gas streams of molten salt reactors. Finally, concluding remarks will present future outlooks on the role of LA plasma spectroscopy in the nuclear community.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Ultra-compact x-ray spectrometer for high-repetition-rate laser–plasma experiments

Here, we present in this work the development of an ultra-compact, multi-channel x-ray spectrometer (UCXS). This diagnostic has been specially built and adapted to perform at high-repetition-rate (>1 Hz) for high-intensity, short-pulse laser plasma experiments. X-ray filters of varying materials and thicknesses are chosen to provide spectral resolution up to ΔE ≈ 1 keV over the x-ray energy range of 1–30 keV. These filters are distributed over a total of 25 channels, where each x-ray filter is coupled to a single scintillator. The UCXS is designed to detect and resolve a large variety of laser-driven x-ray sources such as low energy bremsstrahlung emission, fluorescence, and betatron radiation (up to 30 keV). Preliminary results from commissioning experiments at the ABL laser facility at Colorado State University are provided.

47 OTHER INSTRUMENTATION↗

Plasmonics-enhanced photoconductive terahertz detector pumped by Ytterbium-doped fiber laser

We present a photoconductive terahertz detector operating at the 1 µm wavelength range at which high-power and compact Ytterbium-doped femtosecond fiber lasers are available. The detector utilizes an array of plasmonic nanoantennas to provide sub-picosecond transit time for the majority of photo-generated carriers to enable high-sensitivity terahertz detection without using a short-carrier-lifetime substrate. By using a high-mobility semiconductor substrate and preventing photocarrier recombination, the presented detector offers significantly higher sensitivity levels compared with previously demonstrated broadband photoconductive terahertz detectors operating at the 1 µm wavelength range. We demonstrate pulsed terahertz detection over a 4 THz bandwidth with a record-high signal-to-noise ratio of 95 dB at an average terahertz radiation power of 6.8 µW, when using an optical pump power of 30 mW.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Modernizing Accelerator Responsiveness and Controls in Operations

Accelerators increasingly use artificial intelligence (AI) and machine learning (ML) software and workflows for a variety of tasks, from optimization to fault detection and recovery. Efficient and sustainable application of these technologies necessitates specialized and facility-specific infrastructure commitments. Accelerator facilities also introduce unique radiation and security hazards, placing additional demands on operational infrastructure. These needs further escalate the prioritization of effective collaboration models and associated funding mechanisms and legal frameworks.

43 PARTICLE ACCELERATORS↗

Evaluation of WRF-Solar Cloud Forecast Using the NSRDB: Preprint

Cloud forecast is a crucial component in predicting solar irradiance from numerical weather prediction (NWP) models. Assessing cloud properties from the NWP models requires significant work due to the need for high-quality data, spatial analysis covering model extent, and detailed analysis of model performance for different types of clouds. This study presents an evaluation of the WRF-Solar cloud forecast using the National Solar Radiation Database (NSRDB). We propose an evaluation framework applied to a single model prediction as well as ensemble-based forecasts. Various cloud detection metrics are calculated when comparing with the satellite-derived dataset. The mismatched clouds from the WRF-Solar model are quantified using nine cloud types classified by cloud top height and cloud optical depth. The results based on the WRF-Solar forecasts covering the entire U.S. for the full year of 2018 shows mismatched cloud frequency in the range of 8% - 46% for thick and high-level (deep convective) to thin and low-level (cumulus) clouds.

cloud mask forecast↗

A semi-supervised machine learning detector for physics events in tokamak discharges

Databases of physics events have been used in various fusion research applications, including the development of scaling laws and disruption avoidance algorithms, yet they can be time-consuming and tedious to construct. This paper presents a novel application of the label spreading semi-supervised learning algorithm to accelerate this process by detecting distinct events in a large dataset of discharges, given few manually labeled examples. A high detection accuracy (> 85%) for H-L back transitions and initially rotating locked modes is demonstrated on a dataset of hundreds of discharges from DIII-D with manually identified events for which only 3 discharges are initially labeled by the user. Lower yet reasonable performance (~75%) is also demonstrated for the core radiative collapse, an event with a much lower prevalence in the dataset. Additionally, analysis of the performance sensitivity indicates that the same set of algorithmic parameters is optimal for each event. Furthermore, this suggests that the method can be applied to detect a variety of other events not included in this paper, given that the event is well described by a set of 0D signals robustly available on many discharges. Procedures for analysis of new events are demonstrated, showing automatic event detection with increasing fidelity as the user strategically adds manually labeled examples. Detections on Alcator C-Mod and EAST are also shown, demonstrating the potential for this to be used on a multi-tokamak dataset.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Modeling Global Vegetation Gross Primary Productivity, Transpiration and Hyperspectral Canopy Radiative Transfer Simultaneously Using a Next Generation Land Surface Model—CliMA Land

Recent progress in satellite observations has provided unprecedented opportunities to monitor vegetation activity at global scale. However, a major challenge in fully utilizing remotely sensed data to constrain land surface models (LSMs) lies in inconsistencies between simulated and observed quantities. For example, gross primary productivity (GPP) and transpiration (T) that traditional LSMs simulate are not directly measurable from space, although they can be inferred from spaceborne observations using assumptions that are inconsistent with those LSMs. In comparison, canopy reflectance and fluorescence spectra that satellites can detect are not modeled by traditional LSMs. To bridge these quantities, we presented an overview of the next generation land model developed within the Climate Modeling Alliance (CliMA), and simulated global GPP, T, and hyperspectral canopy radiative transfer (RT; 400–2,500 nm for reflectance, 640–850 nm for fluorescence) at hourly time step and 1° spatial resolution using CliMA Land. CliMA Land predicts vegetation indices and outgoing radiances, including solar-induced chlorophyll fluorescence (SIF), normalized difference vegetation index (NDVI), enhanced vegetation index (EVI), and near infrared reflectance of vegetation (NIRv) for any given sun-sensor geometry. The spatial patterns of modeled GPP, T, SIF, NDVI, EVI, and NIRv correlate significantly with existing data-driven products (mean R 2 = 0.777 for 9 products). CliMA Land would be also useful in high temporal resolution simulations, for example, providing insights into when GPP, SIF, and NIRv diverge.

54 ENVIRONMENTAL SCIENCES↗

Exclusion and Verification of Remote Nuclear Reactors with a 1-kiloton Gd -Doped Water Detector

To date, antineutrino experiments built for the purpose of demonstrating a nonproliferation capability have typically employed organic scintillators situated as close to the core as possible (typically at a distance of a few meters to tens of meters) and have not exceeded a few tons in size. One problem with this approach is that proximity to the reactor core requires accommodation by the host facility. Water Cherenkov detectors located offsite, at distances of a few kilometers or greater, may facilitate nonintrusive monitoring and verification of reactor activities over a large area. As the standoff distance increases, the detector target mass must scale accordingly. This paper quantifies the degree to which a kiloton-scale gadolinium-doped water Cherenkov detector can exclude the existence of undeclared reactors within a specified distance, and remotely detect the presence of a hidden reactor in the presence of declared reactors, by verifying the operational power and standoff distance using a Feldman-Cousins-based likelihood analysis. A 1-kton scale (fiducial) water Cherenkov detector can exclude gigawatt-scale nuclear reactors up to tens of kilometers within a year. In conclusion, when attempting to identify the specific range and power of a reactor, the detector energy resolution is not sufficient to delineate between the two.

42 ENGINEERING↗