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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 811 records · Page 45
All sourcesNASA NTRSDOE OSTI
NASA NTRS2007

Co/Ni Ratio Between Is Approximately 0.35 - 8.0 GeV/nucleon from the TIGER-2001 Flight

The Trans-Iron Galactic Element Recorder (TIGER) was launched in December 2001 and 2003 from McMurdo, Antarctica and was designed to observe elements ranging from 14 < Z < 40 over an extended energy range. Observations of radioactive isotopes produced during explosive nucleosynthesis such as Ni-59 that decay only through electron capture provide important constraints on the delay between nucleosynthesis and the acceleration of galactic cosmic rays (GCRs). The isotopes of Co and Ni at low energies, in particular, the observations of the Ni-59 and Co-59 from the Cosmic Ray Isotope Spectrometer (CRIS) on the Advanced Composition Explorer, indicate a significant time delay (greater than 7.6 x 10^4 yr) between GCR nucleosynthesis and acceleration. While TIGER is not able to resolve isotopes, observations of the elemental abundances of Co and Ni at high energies further constrain models for the acceleration and propagation of GCRs. The 2001 & 2003 flights of TIGER lasted a total of approx. 50 days and collected sufficient statistics to study the Co/Ni elemental ratio over a wide range in energies. We present the elemental ratio of Co/Ni in galactic cosmic rays between approx. 0.8- 5.0 GeV/nucleon and compare these results with previous measurements and models for cosmic-ray propagation.

deNolfo, G. A.↗
DOE OSTI2014

Identification of Leakage Spectra from Neutron Activation in Glass/Cherenkov Detectors - Paper 96

Oak Ridge National Laboratory has developed a new detector system concept that can be deployed in major US cities to identify the leakage spectrum of a nuclear weapon detonation. The detector is based on a small piece of glass that has been doped with an element that has a high activation cross section and creates a radioactive activation product with a reasonable length half-life. The decay of the activation product(s) after exposure creates Cherenkov light which can propagate to a photomultiplier and can be turned into a count-rate signal. The signal from each glass in each detector in a city can be individually analyzed to determine the amount of activation products produced in the initial exposure. Several activation products can be determined in a single glass if the half-lives are not the same. With a known source location and a detailed 3D model of a city, neutron transport simulations can be made by using a library of known sources to predict the activation amounts each source would have made in the glass detectors. A simple comparison of the measured activation amounts and the predicted activation amounts can identify the source spectrum contained in the library that is the best match. Choosing dopants with a large range in the threshold energy for the activation reactions can help to differentiate the spectra in the library. The method of matching the measured activation amounts to the predicted activation amounts to identify the source spectrum is similar to the analysis used for the passive Activation Foil Integrated Detector System (AFIDS), also developed at Oak Ridge National Laboratory. In AFIDS, wires or foils of known mass and isotopic composition are deployed before and then collected after exposure. Counting gammas in a nearby laboratory determines the activation amounts. The glass/Cherenkov system is active - it uses a battery-powered detector to count flashes of Cherenkov light and to communicate its count rates to a remote location for further analysis. Work has been performed in several areas, including glass making, automated detection and communication systems and software tools for analysis of the signal and source spectrum identification. Bell and Boatner have developed phosphate glasses that incorporate elements with high capture cross sections, and Hayward has simulated the response with Geant4 and measured the response with isotopic gamma sources. This paper will focus on the software tools for determining the activation amounts from the Cherenkov count-rate signal and finding the best matching source spectrum. A test problem in an urban environment is used to demonstrate the potential of a spectrum identification system using neutron activation. The analysis methods developed to identify the neutron leakage spectra from Cherenkov light given off by neutron activation in doped glasses work well. The calculation used to unfold the count-rate information into the number of actual activation products uses robust algorithms that can also compute associated uncertainties. These uncertainties and the known uncertainties of the glass tube material compositions are incorporated into the matching analysis to determine which of the source spectra in the library best matches the measured activation data. Any measurement method used to identify a neutron source spectrum relies at some point on a comparison against known sources; no identification method is definitive. Detection systems measure some physical aspect of the source, not its serial number. Many systems measure the physical aspect to determine that the source has some property, and then leave it to experts to determine which potential sources share that property. The analysis system presented here incorporates the comparison into the analysis itself. The statistical tests show which of the known library sources match the measured data the best and whether that match is a good match. If the best match still does not fit the measured data well (a very high χ{sup 2} value), that indicates the true source is not one of the sources in the library. This is still valuable information for decision makers. (authors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Long-lived isomeric states and quasiparticle band structures in neutron-rich 162,164 Gd nuclei from β decay

Neutron-rich nuclei 162,164 Eu were produced by bombarding a proton beam on a 238 U target at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory and mass separating the 162,164 Eu products. New level schemes and new γ-ray transitions of the daughters 162,164 Gd were identified from β-decay spectroscopy studies. Additionally, half-lives of the 162,164 Eu were remeasured to clarify the previous ambiguous results. Two quasiparticle band structures were built and compared with neighboring nuclei. The β and γ bands were extended in 162 Gd and a γ band was extended in 164 Gd. Half-lives of the isomeric states at (6 - ) 1449 keV in 162 Gd and (4 - ) 1096 keV in 164 Gd were measured to be 99(3) μs and 0.56(3) μs, respectively. Projected shell model calculations were performed and found to be in good agreement with all of the experimental data.

150 ≤ A ≤ 189↗
DOE OSTI2026

Radioactivity-in-materials lead for nEXO (Final Scientific Report)

Abstract, introduction, and summary of work completed and products produced by DOE award SC002466. Primary products were six peer-reviewed publications and two PhD theses. This award also supported the operation of an underground HPGe detector and several radioassay measurements: one in a stand alone publication in Phys. Rev. C and the others in an upcoming nEXO radioassay summary paper. The nEXO collaboration aims to demonstrate the Majorana nature of the neutrino by observing the neutrinoless double-beta decay of 136 Xe with a next-generation experiment. The University of Kentucky nEXO group (UKY) operates a world-leading ultra-low-background γ-ray spectrometer as part of the nEXO radioactive background control R&D effort. The nEXO project is a proposed ton-scale neutrinoless double-beta decay experiment. The UKY PI is leading the radioactivity content assessment for all materials required by the nEXO project. As a subset of this task, UKY is also responsible for project-wide management of all low-background γ-ray spectrometry measurements; material assays with these types of instruments, together with ICP-MS, neutron-activation-analysis, and α-spectrometry, are critical to ensuring that the nEXO project can achieve its design sensitivity

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS2007

Iapetus' Geophysics: Rotation Rate, Shape, and Equatorial Ridge

Iapetus has preserved evidence that constrains the modeling of its geophysical history from the time of its accretion until now. The evidence is (a) its present 79.33-day rotation or spin rate, (b) its shape that corresponds to the equilibrium figure for a hydrostatic body rotating with a period of approximately 16 h, and (c) its high, equatorial ridge, which is unique in the Solar System. This paper reports the results of an investigation into the coupling between Iapetus' thermal and orbital evolution for a wide range of conditions including the spatial distributions with time of composition, porosity, short-lived radioactive isotopes (SLRI), and temperature. The thermal model uses conductive heat transfer with temperature-dependent conductivity. Only models with a thick lithosphere and an interior viscosity in the range of about the water ice melting point can explain the observed shape. Short-lived radioactive isotopes provide the heat needed to decrease porosity in Iapetus? early history. This increases thermal conductivity and allows the development of the strong lithosphere that is required to preserve the 16-h rotational shape and the high vertical relief of the topography. Long-lived radioactive isotopes and SLRI raise internal temperatures high enough that significant tidal dissipation can start, and despin Iapetus to synchronous rotation. This occurred several hundred million years after Iapetus formed. The models also constrain the time when Iapetus formed because the successful models are critically dependent upon having just the right amount of heat added by SLRI decay in this early period. The amount of heat available from short-lived radioactivity is not a free parameter but is fixed by the time when Iapetus accreted, by the canonical concentration of Al-26, and, to a lesser extent, by the concentration of Fe-60. The needed amount of heat is available only if Iapetus accreted between 2.5 and 5.0Myr after the formation of the calcium aluminum inclusions as found in meteorites. Models with these features allow us to explain Iapetus? present synchronous rotation, its fossil 16-h shape, and the context within which the equatorial ridge arose.

geophysics↗
DOE OSTI2015

Operating experience in the treatment and storage of LLW in Turkey - 15010

Treatment and storage of low-level radioactive wastes (LLW) are being carried out in Radioactive Waste Management Unit (RWMU) at Cekmece Nuclear Research and Training Center (CNRTC) in Istanbul. The wastes are generated from nuclear research and nuclear applications mainly in medicine, biology, ng to these specifications, LLW are classified as exempt waste, very low level waste (VLLW) etc. Decay storage is applied at a designated area for short lived radionuclide. Long lived spent radioactive sources are immobilized in retrievable packages. Generally liquid radioactive wastes are decontaminated by filtration or chemical precipitation. The radioactive sludge or filtration media from liquid waste processing is solidified using cementation. Solid waste is compacted into drums for size reduction. TENORM wastes and contaminated metal wastes are handled for decontamination and size reduction. Then these types of waste are placed in 20 ton bulk containers for long term storage. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2024

Evaluating Radiation Impact on Transmon Qubits Using a Fast Decay Protocol in Above and Underground Laboratories

Superconducting qubits can be sensitive to sudden energy deposits caused by ambient radioactivity and cosmic rays. Previous studies have focused on understanding possible correlated effects over time and distance due to this radiation. In this study‚ for the first time‚ we directly compare the response of a transmon qubit measured initially at the SQMS above-ground facility (Fermilab‚ Illinois‚ USA) and then at the deep underground Gran Sasso Laboratory (INFN-LNGS‚ Italy). We observe the same average qubit lifetime of roughly 80 microseconds at both facilities. We then apply a fast decay detection protocol and investigate the time structure and relative rates of triggered events due to radiation versus intrinsic noise‚ comparing the above and underground performance of several high-coherence qubits. Using gamma sources of variable intensity we calibrate the response of the qubit to different levels of radiation in an environment with minimal background radiation. Results indicate that qubits respond to a strong gamma source‚ and it is possible to detect particle impacts. However‚ we do not observe a difference in radiation-induced-like events when comparing the above and underground results for niobium-based transmon qubits with sapphire substrates. We conclude that the majority of these events are not radiation-related and are attributed to other noise sources‚ which by far dominate single-qubit errors in modern transmon qubits. [1] Dominicis‚ Roy et al. arXiv:2405.18355

Roy, Tanay↗
DOE OSTI2017

94 {beta}-Decay Half-Lives of Neutron-Rich 55Cs to 67Ho: Experimental Feedback and Evaluation of the r-Process Rare-Earth Peak Formation

The β-decay half-lives of 94 neutron-rich nuclei 144$-$151 Cs, 146$-$154 Ba, 148$-$156 La, 150$-$158 Ce, 153$-$160 Pr, 156$-$162 Nd, 159$-$163 Pm, 160$-$166 Sm, 161$-$168 Eu, 165$-$170 Gd, 166$-$172 Tb, 169$-$173 Dy, 172$-$175 Ho, and two isomeric states 174m Er, 172m Dy were measured at the Radioactive Isotope Beam Factory, providing a new experimental basis to test theoretical models. Strikingly large drops of β-decay half-lives are observed at neutron-number N = 97 for 58 Ce, 59 Pr, 60 Nd, and 62 Sm, and N = 105 for 63 Eu, 64 Gd, 65 Tb, and 66 Dy. Lastly, features in the data mirror the interplay between pairing effects and microscopic structure. r-process network calculations performed for a range of mass models and astrophysical conditions show that the 57 half-lives measured for the first time play an important role in shaping the abundance pattern of rare-earth elements in the solar system

Wu, J.↗
DOE OSTI2014

Status and prospects of investigations into the collinear cluster decay of heavy nuclei

Basic experimental results confirming the existence a new cluster-decay type called collinear cluster tripartition (CCT) are presented. Decays of this type manifest themselves, in particular, as a two-dimensional region of a locally enhanced yield of fragments (bump) that corresponds to specific missing-mass values in the mass-mass distribution of fission fragments. One of the decay modes that contribute to the bump can be treated as a cluster-decay type that is new in relation to the well-known heavy-ion or lead radioactivity. The conclusions drawn from an analysis of correlation mass distributions are confirmed by the results obtained from neutron-gated data, measurements of the nuclear charge for CCT events, and the direct detection of new-decay products.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Experimental study of the β decay of the very neutron-rich nucleus Ge 85

The β -decay properties of the very neutron-rich nucleus 85 Ge, produced in the proton-induced fission of 238 U, were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. The level scheme of 33 85 As 52 populated in 85 Geβ γ decay was reconstructed and compared to shell-model calculations. The investigation of the systematics of low-energy levels in N =52 isotones together with shell-model analysis allowed us to provide an estimate of the low-energy structure of the more exotic N =52 isotone 81 Cu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

The Sporadic History of Rubidium and its Role in Corrosion of Steel Related to Nuclear Material Storage

The influence of rubidium (Rb), both in its metallic and oxidized states, on the corrosion resistance of steels has direct relevance to the storage of radioactive Kr-85 containing nuclear materials. Kr-85 undergoes a ß-decay to generate stable, metallic Rb. The literature to date is sparse, contained primarily in company reports and divisive as to whether Rb metal, or its oxides, can lead to corrosion of steel materials. In both the direct storage of Kr-85 and used nuclear fuel that will contain Kr-85, if Rb is corrosive then continual decay of the Kr-85 will generate an increasingly corrosive environment for the steel canister it is stored in. This review was written to consolidate the known data to date on Rb corrosion of steels to identify consistencies, contradictions and remaining gaps in our understanding of the Rb : steel system.

krypton, corrosion, steel, Rubidium↗
DOE OSTI2019

Segmented YSO scintillation detectors as a new β -implant detection tool for decay spectroscopy in fragmentation facilities

A newly developed segmented YSO scintillator detector was implemented for the first time at the RI-beam Factory at RIKEN Nishina Center as an implantation-decay counter. The results from the experiment demonstrate that the detector is a viable alternative to conventional silicon-strip detectors with its good timing resolution and high detection efficiency for β particles. A Position-Sensitive Photo-Multiplier Tube (PSPMT) is coupled with a 48 × 48 segmented YSO crystal. To demonstrate its capabilities, a known short-lived isomer in 76 Ni and the β decay of 74 Co were measured by implanting those ions into the YSO detector. The half-lives and γ-rays observed in this work are consistent with the known values. The β -ray detection efficiency is more than 80 % for the decay of 74 Co.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Capture cross sections on unstable nuclei

Accurate neutron-capture cross sections on unstable nuclei near the line of beta stability are crucial for understanding the s-process nucleosynthesis. However, neutron-capture cross sections for short-lived radionuclides are difficult to measure due to the fact that the measurements require both highly radioactive samples and intense neutron sources. Essential ingredients for describing the γ decays following neutron capture are the γ-ray strength function and level densities. We will compare different indirect approaches for obtaining the most relevant observables that can constrain Hauser-Feshbach statistical-model calculations of capture cross sections. Specifically, we will consider photon scattering using monoenergetic and 100% linearly polarized photon beams. Here, challenges that exist on the path to obtaining neutron-capture cross sections for reactions on isotopes near and far from stability will be discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

ICP MS selection of radiopure materials for the GERDA experiment

The GERDA (GERmanium Detector Array) experiment, located in the Gran Sasso Underground Laboratory (LNGS, Italy) aims to search for neutrinoless double beta (0νββ) decay of the {sup 76}Ge isotope. Both an ultra-low radioactivity background environment and active techniques to abate the residual background are required to reach the background index (of 10{sup −3} counts/keV kg y) at the Q{sub ββ}. In order to veto and suppress those events that partially deposit energy in Ge detectors, the readout of liquid argon (LAr) scintillation light (SL) has been implemented for the second GERDA experimental Phase. A double veto system has been designed and constructed using highly radiopure materials (scintillating fibers, wavelength shifters, polymeric foils, reflective foils). This work describes the study of lead, thorium and uranium ultra-trace content, performed at the LNGS Chemistry Laboratory by High Resolution Mass Spectrometry (HR ICP MS), for the selection of all materials involved in the construction of the veto system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Determination of the $^8\mathrm{B}$ neutrino energy spectrum using trapped ions

We report the β + decay of 8 B provides the dominant source of solar neutrinos above 2 MeV. Consequently, experiments that detect neutrinos from the sun require an accurate determination of the 8 B neutrino energy spectrum. In this work, the β -decay Paul trap surrounded by double-sided silicon strip detectors was utilized to precisely measure the decay products of trapped 8 B ions. The results were used to determine the 8 Be final-state distribution and to reconstruct the neutrino energy spectrum. This measurement using trapped ions is the first of its kind and puts the neutrino energy spectrum on much firmer footing by discriminating between recently reported values for the maximum of the final-state distribution.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Toward complete spectroscopy using β decay: The example of Cl 32 ( β γ ) S 32

$^{32}\textbf{Cl}$ is a neutron-deficient isotope with a $β$-decay half-life of 298 ms and a spin and parity of $J^π=1^+$. Previous measurements of $^{32}\textbf{Cl}$ $β$-delayed $γ$ rays have yielded a $β$-decay scheme with twelve $β$-decay transitions, contributing to studies of nuclear structure and fundamental symmetries. Those experiments have been limited to the observation of $^{32}\textbf{S}$ states with $J^π = 0^+,1^+, 2^+$. Our goal is to search for new $β$-delayed $γ$ rays and $β$-decay transitions of $^{32}\textbf{Cl}$ to $^{32}\textbf{S}$. A measurement of $^{32}\textbf{Cl}$ $β$-delayed $γ$ decay has been performed using the Clovershare array of high-purity germanium detectors at the National Superconducting Cyclotron Laboratory. By acquiring the highest-statistics $^{32}\textbf{Cl}$ $β$-delayed $γ$-ray spectrum to date and exploiting a new sensitivity to $γ-γ$ coincidences, this experiment has enabled the observation of nine previously unobserved $β$-delayed $γ$-ray transitions, leading to the inference of five $β$-decay transitions never before observed in $^{32}\textbf{Cl}$ $β$-delayed $γ$ decay. The set of observed states includes negative-parity states for the first time. By combining the new information with data from previous work, the lifetimes and partial widths of the 8861- and 9650-keV states of $^{32}\textbf{S}$ have been determined. In addition, the $^{31}\textbf{P}$($p,α$)$^{28}\textbf{Si}$ resonance strength of the 9650-keV state has been limited to $ωγ<9.8$ meV, which is an improvement over direct measurements. An enhanced decay scheme has been constructed. Most of the excited bound $^{32}\textbf{S}$ states that would correspond to allowed and first-forbidden $β$-decay transitions have been observed, demonstrating the potential of $β$-decay experiments to approach complete spectroscopy measurements at the next generation of radioactive beam facilities. The observed positive-parity levels are well matched by $sd$ shell-model calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Improved Tensor Current Limit from 8 B 𝛽 Decay Including New Recoil-Order Calculations

A precision measurement of the 𝛽 + decay of 8 B was performed using the Beta-decay Paul Trap to determine the 𝛽−𝜈 angular correlation coefficient 𝑎 𝛽⁢𝜈 . The experimental results were combined with new ab initio symmetry-adapted no-core shell-model calculations to yield the second-most precise measurement from Gamow-Teller decays, 𝑎 𝛽⁢𝜈 = −0.3345 ± 0.001⁢9 stat ± 0.002⁢1 syst . This value agrees with the standard model value of −1/3 and improves uncertainties in 8 B by nearly a factor of 2. By combining results from 8 B and 8 Li , a tight limit on tensor current coupling to right-handed neutrinos was obtained. A recent global evaluation of all other precision 𝛽 decay studies suggested a nonzero value for right-handed neutrino coupling in contradiction with the standard model at just above 3⁢𝜎. Finally, the present results are of comparable sensitivity and do not support this finding.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗