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NASA NTRS2015

Multi-Angle Polarimetry: The Once and Future King of Aerosol Remote Sensing

Although aerosols (and their interactions with clouds) are widely known to be one of the most uncertain components of the climate, they remain largely unconstrained in climate simulations. This is because global observations of all the parameters relevant to such simulations - quantity, size, shape, optical properties and chemical composition - are very difficult to simultaneously retrieve from existing remote sensing instruments. The problem can be addressed by maximizing the scene information gathered by a remote sensing instrument, by the use of (passive) multi-spectral, multi-angle and polarimetrically sensitive sensors. These observations, coupled with a radiative transfer model, can be inverted to solve for aerosol parameters. However, the choices to be made when designing an such an observing system and retrieval algorithm are complex, and a variety of approaches have been undertaken by the scientific community. I will review the various multi-spectral, multi-angle, polarimetric observation systems employed for aerosol remote sensing and their corresponding retrieval algorithms. This includes the French Polarization and Directionality of Earth Reflectance (POLDER) instrument, which has been the only such instrument successfully deployed in orbit thus far (most recently from 2004-2013), the NASA Aerosol Polarimetry Sensor (APS) on the ill-fated NASA Glory Mission (launch failure in 2011), potential or planned polarimeters on the NASA Aerosol-Cloud-Ecosystem (ACE) and Pre-Aerosol, Clouds and ocean Ecosystems (PACE) missions, and airborne prototypes from around the world.

Knobelspiesse, Kirk↗

NASA NTRS2021

Surface Melting Over the Greenland Ice Sheet Derived From Enhanced Resolution Passive Microwave Brightness Temperatures (1979–2019)

Surface melting is a major component of the Greenland ice sheet surface mass balance, and it affects sea level rise through direct runoff and the modulation of ice dynamics and hydrological processes, supraglacially, englacially and subglacially. Passive microwave (PMW) brightness temperature observations are of paramount importance in studying the spatial and temporal evolution of surface melting due to their long temporal coverage (1979–present) and high temporal resolution (daily). However, a major limitation of PMW datasets has been the relatively coarse spatial resolution, which has historically been of the order of tens of kilometers. Here, we use a newly released PMW dataset (37 GHz, horizontal polarization) made available through a NASA “Making Earth System Data Records for Use in Research Environments” (MeASUREs) program to study the spatiotemporal evolution of surface melting over the Greenland ice sheet at an enhanced spatial resolution of 3.125 km. We assess the outputs of different detection algorithms using data collected by automatic weather stations (AWSs) and the outputs of the Modèle Atmosphérique Régional (MAR) regional climate model. We found that sporadic melting is well captured using a dynamic algorithm based on the outputs of the Microwave Emission Model of Layered Snowpack (MEMLS), whereas a fixed threshold of 245 K is capable of detecting persistent melt. Our results indicate that, during the reference period from 1979 to 2019 (from 1988 to 2019), surface melting over the ice sheet increased in terms of both duration, up to 4.5 (2.9) d per decade, and extension, up to 6.9 % (3.6 %) of the entire ice sheet surface extent per decade, according to the MEMLS algorithm. Furthermore, the melting season started up to 4.0 (2.5) d earlier and ended 7.0 (3.9) d later per decade. We also explored the information content of the enhanced-resolution dataset with respect to the one at 25 km and MAR outputs using a semi-variogram approach. We found that the enhanced product is more sensitive to local-scale processes, thereby confirming the potential of this new enhanced product for monitoring surface melting over Greenland at a higher spatial resolution than the historical products and for monitoring its impact on sea level rise. This offers the opportunity to improve our understanding of the processes driving melting, to validate modeled melt extent at high resolution and, potentially, to assimilate these data in climate models.

Surface melting↗

NASA NTRSDate not supplied

Reanalysis Activities at the NASA Global Modeling and Assimilation Office

This talk presents an overview of recent reanalysis activities at the NASA Global Modeling and Assimilation Office (GMAO) as part of a multi-faceted strategy towards an Integrated Earth System retrospective analysis, coupling components of the atmosphere, ocean, chemistry, land, and ice. While elements of the atmosphere-ocean coupled Goddard Earth Observing System (GEOS) model and data assimilation are being actively developed, a suite of reanalysis products is designed to provide further understanding of key aspects of Earth system coupling in a reanalysis context: The baseline atmospheric reanalysis, the GEOS Retrospective analysis for the early 21st Century (GEOS-R21C), features recent advances in the GEOS model and data assimilation, and targets the NASA’s Earth Observing System EOS and post-EOS satellite observations; GEOS-IT, a user-tailored low-resolution atmospheric reanalysis, serves as a second baseline to the NASA Instrument Teams for validation and calibration and drives a one-way coupled ocean reanalysis, GEOSIT-Ocean; PolarMERRA, a high-resolution downscaled product for the polar regions, focuses on improving the representation of polar atmospheric processes with an assessment of current cryospheric biases, and targeted improvements to surface sea ice and glacier conditions; Finally, R21C-Chem, an off-line atmospheric chemistry and composition reanalysis, includes both tropospheric and stratospheric trace gases. The diversity of these reanalysis activities presents unique opportunities for collaborations cross-teams/institutions, with new commercial data partners, and with end-user groups. This talk will discuss these opportunities and explore leveraging the lessons learned along the way on key drivers in Earth system interactions as we converge towards the next generation of the Modern-Era Retrospective analysis for Research and Applications (MERRA) suite.

Amal El Akkraoui↗

DOE OSTI2024

Incident beamline design for a modern cold triple axis spectrometer at the High Flux Isotope Reactor

A modern cold triple axis spectrometer is being planned for the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. Here, we describe the design of an incident beamline that will put a flux of ~ 10 8 $\frac {n}{cm^{2}s}$ on a sample with an area of 2 cm X 2 cm. It takes current physical constraints at HFIR into account and it can accommodate both single and multiplexed analyzer-detector secondary spectrometers and large superconducting magnets. The proposed incident beamline includes a multi-channel guide with horizontal focusing, a neutron velocity selector, components to facilitate an incident beam polarization option, and a double-focusing pyrolytic graphite monochromator. Here, this work describes the process of optimizing the guide system and monochromator and summarizes the expected performance of the incident beamline for non-polarized operation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2023

Hydrodynamic spin-orbit coupling in asynchronous optically driven micro-rotors

Abstract Vortical flows of rotating particles describe interactions ranging from molecular machines to atmospheric dynamics. Yet to date, direct observation of the hydrodynamic coupling between artificial micro-rotors has been restricted by the details of the chosen drive, either through synchronization (using external magnetic fields) or confinement (using optical tweezers). Here we present a new active system that illuminates the interplay of rotation and translation in free rotors. We develop a non-tweezing circularly polarized beam that simultaneously rotates hundreds of silica-coated birefringent colloids. The particles rotate asynchronously in the optical torque field while freely diffusing in the plane. We observe that neighboring particles orbit each other with an angular velocity that depends on their spins. We derive an analytical model in the Stokes limit for pairs of spheres that quantitatively explains the observed dynamics. We then find that the geometrical nature of the low Reynolds fluid flow results in a universal hydrodynamic spin-orbit coupling. Our findings are of significance for the understanding and development of far-from-equilibrium materials.

47 OTHER INSTRUMENTATION↗

NASA NTRS1993

The Marshall Automated Weld System (MAWS)

A fully automated welding system, which can operate totally independent of human intervention, is currently unavailable in the welding industry. Development of the Marshall Automated Weld System (MAWS) has been undertaken to fill this void. The system will enable application of statistical process control practices to assure weld quality prior to post weld nondestructive testing. The Variable Polarity Plasma Arc (VPPA) welding process has been baselined for MAWS because it has eliminated process related defects in the welding of the Space Shuttle External Tank. The few remaining weld defects occurring on the tank can be associated with human error. The system integrates multiple sensors (providing real time information on weld bead geometry, weld joint location, wirefeed entry, and inert gas quality) with a weld model (describing weld geometry in relation to critical parameters) and computer-controlled VPPA weld equipment. This system is designed to provide real-time, closed-loop control of the weld as it is being made.

Russell, Carolyn K.↗

NASA NTRS1993

The Marshall Automated Weld System (MAWS)

A fully automated welding system, which can operate totally independent of human intervention, is currently unavailable in the welding industry. Development of the Marshall Automated Weld System (MAWS) has been undertaken to fill this void. The system will enable application of statistical process control practices to assure weld quality prior to post weld nondestructive testing. The Variable Polarity Plasma Arc (VPPA) welding process has been baselined for MAWS because it has eliminated process related defects in the welding of the Space Shuttle External Tank. The few remaining weld defects occurring on the tank can be associated with human error. The system integrates multiple sensors (providing real time information on weld bead geometry, weld joint location, wirefeed entry, and inert gas quality) with a weld model (describing weld geometry in relation to critical parameters) and computer controlled VPPA weld equipment. This system is designed to provide real-time, closed-loop control of the weld as it is being made.

Russell, Carolyn K.↗

NASA NTRS2017

Laser Pulse Bidirectional Reflectance from CALIPSO Mission

In this Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) study, we present a simple way of determining laser pulse bidirectional reflectance over snow/ice surface using the Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) 532 nanometer polarization channels' measurements. The saturated laser pulse returns from snow and ice surfaces are recovered based on surface tail information. The method overview and initial assessment of the method performance will be presented. The retrieved snow surface bidirectional reflectance is compared with reflectance from both CALIOP cloud cover regions and Moderate Resolution Imaging Spectroradiometer (Earth Observing System (EOS)) (MODIS) Bi-directional Reflectance Distribution Function (BRDF) / Albedo model parameters. The comparisons show that the snow surface bidirectional reflectance over Antarctica for saturation region are generally reliable with a mean value of about 0.90 plus or minus 0.10, while the mean surface reflectance from cloud cover region is about 0.84 plus or minus 0.13 and the calculated MODIS reflectance at 555 nanometers from the BRDF / Albedo model with near nadir illumination and viewing angles is about 0.96 plus or minus 0.04. The comparisons here demonstrate that the snow surface reflectance underneath the cloud with cloud optical depth of about 1 is significantly lower than that for a clear sky condition.

Lu, Xiaomei↗

NASA NTRS1992

Theoretical model for frequency locking a diode laser with a Faraday cell

A new method was developed for frequency locking a diode lasers, called 'the Faraday anomalous dispersion optical transmitter (FADOT) laser locking', which is much simpler than other known locking schemes. The FADOT laser locking method uses commercial laser diodes with no antireflection coatings, an atomic Faraday cell with a single polarizer, and an output coupler to form a compound cavity. The FADOT method is vibration insensitive and exhibits minimal thermal expansion effects. The system has a frequency pull in the range of 443.2 GHz (9 A). The method has potential applications in optical communication, remote sensing, and pumping laser excited optical filters.

Wanninger, P.↗

NASA NTRS1991

Sea ice - atmosphere interaction: Application of multispectral satellite data in polar surface energy flux estimates

In the past six months, work has continued on energy flux sensitivity studies, ice surface temperature retrievals, corrections to Advanced Very High Resolution Radiometer (AVHRR) thermal infrared data, modelling of cloud fraction retrievals, and radiation climatologies. We tentatively conclude that the SSM/I may not provide accurate enough estimates of ice concentration and type to improve our shorter term energy flux estimates. SSM/I derived parameters may still be applicable in longer term climatological flux characterizations. We hold promise for a system coupling observation to a ice deformation model. Such a model may provide information on ice distribution which can be used in energy flux calculations. Considerable variation was found in modelled energy flux estimates when bulk transfer coefficients are modulated by lead fetch. It is still unclear what the optimum formulation is and this will be the subject of further work. Data sets for ice surface temperature retrievals were assembled and preliminary data analysis was started. Finally, construction of a conceptual framework for further modelling of the Arctic radiation flux climatology was started.

Steffen, Konrad↗

DOE OSTI2024

Colossal Strain Tuning of Ferroelectric Transitions in KNbO 3 Thin Films

Strong coupling between polarization ( P ) and strain (ɛ) in ferroelectric complex oxides offers unique opportunities to dramatically tune their properties. Here colossal strain tuning of ferroelectricity in epitaxial KNbO 3 thin films grown by sub‐oxide molecular beam epitaxy is demonstrated. While bulk KNbO 3 exhibits three ferroelectric transitions and a Curie temperature ( T c ) of ≈676 K, phase‐field modeling predicts that a biaxial strain of as little as −0.6% pushes its T c > 975 K, its decomposition temperature in air, and for −1.4% strain, to T c > 1325 K, its melting point. Furthermore, a strain of −1.5% can stabilize a single phase throughout the entire temperature range of its stability. A combination of temperature‐dependent second harmonic generation measurements, synchrotron‐based X‐ray reciprocal space mapping, ferroelectric measurements, and transmission electron microscopy reveal a single tetragonal phase from 10 K to 975 K, an enhancement of ≈46% in the tetragonal phase remanent polarization ( P r ), and a ≈200% enhancement in its optical second harmonic generation coefficients over bulk values. These properties in a lead‐free system, but with properties comparable or superior to lead‐based systems, make it an attractive candidate for applications ranging from high‐temperature ferroelectric memory to cryogenic temperature quantum computing.

36 MATERIALS SCIENCE↗

NASA NTRS1995

Short-range precipitation forecasts using assimilation of simulated satellite water vapor profiles and column cloud liquid water amounts

These observing system simulation experiments investigate the assimilation of satellite-observed water vapor and cloud liquid water data in the initialization of a limited-area primitive equations model with the goal of improving short-range precipitation forecasts. The assimilation procedure presented includes two aspects: specification of an initial cloud liquid water vertical distribution and diabatic initialization. The satellite data is simulated for the next generation of polar-orbiting satellite instruments, the Advanced Microwave Sounding Unit (AMSU) and the High-Resolution Infrared Sounder (HIRS), which are scheduled to be launched on the NOAA-K satellite in the mid-1990s. Based on cloud-top height and total column cloud liquid water amounts simulated for satellite data a diagnostic method is used to specify an initial cloud water vertical distribution and to modify the initial moisture distribution in cloudy areas. Using a diabatic initialization procedure, the associated latent heating profiles are directly assimilated into the numerical model. The initial heating is estimated by time averaging the latent heat release from convective and large-scale condensation during the early forecast stage after insertion of satellite-observed temperature, water vapor, and cloud water formation. The assimilation of satellite-observed moisture and cloud water, together withy three-mode diabatic initialization, significantly alleviates the model precipitation spinup problem, especially in the first 3 h of the forecast. Experimental forecasts indicate that the impact of satellite-observed temperature and water vapor profiles and cloud water alone in the initialization procedure shortens the spinup time for precipitation rates by 1-2 h and for regeneration of the areal coverage by 3 h. The diabatic initialization further reduces the precipitation spinup time (compared to adiabatic initialization) by 1 h.

Wu, Xiaohua↗

NASA NTRS2002

Application of LES (Large Eddy Simulation) to Understanding and Parameterizing the Arctic Cloudy Boundary Layer

The GEWEX (Global Energy and Water Cycle Experiment) Cloud Systems Studies Working Group 5 Polar Clouds was formed largely to exploit the enormous potential of the FIRE.ACE (FIRE Arctic Cloud Experiment) and SHEBA (Surface Heat Budget of the Arctic Ocean) data sets to improve parameterizations of clouds, radiation, and atmospheric boundary layer processes in the polar regions. The web page for this project is a clearinghouse of information for polar clouds in general and specifically for FIRE.ACE and SHEBA modelling activities. Note that the GCSS Working Group and Polar Clouds leverages heavily the FIRE.ACE investment, since it involves a large group of international scientists and has adopted the modelling goals and other issues related to cloud and radiation processes that are articulated by the FIRE.ACE Science Plan. The supplemental funds in this proposal are targeted at providing the continued coordination for the GCSS Working Group on Polar Clouds, which will insure that final FIRE.ACE project objectives regarding modelling and cloud and radiative processes are achieved.

Curry, Judith↗

NASA NTRS2007

Testing Special Relativity at High Energies with Astrophysical Sources

Since the group of Lorentz boosts is unbounded, there is a question as to whether Lorentz invariance (LI) holds to infinitely short distances. However, special and general relativity may break down at the Planck scale. Various quantum gravity scenarios such as loop quantum gravity, as well as some forms of string theory and extra dimension models may imply Lorentz violation (LV) at ultrahigh energies. The Gamma-Ray Large Area Space Telescope (GLAST), to be launched in mid-December, will measure the spectra of distant extragalactic sources of high energy gamma-rays, particularly active galactic nuclei and gamma-ray bursts. GLAST can look for energy-dependent gamma-ray propagation effects from such sources as a signal of Lorentz invariance violation. These sources may also exhibit the high energy cutoffs predicted to be the result of intergalactic annihilation interactions with low energy photons having a flux level as determined by various astronomical observations. With LV the threshold for such interactions can be significantly raised, changing the predicted absorption turnover in the observed spectrum of the sources. Stecker and Glashow have shown that the existence such absorption features in the spectra of extragalactic sources puts constraints on LV. Such constraints have important implications for some quantum gravity and large extra dimension models. Future spaceborne detectors dedicated to measuring gamma-ray polarization can look for birefringence effects as a possible signal of loop quantum gravity. A very small LV may also result in the modification or elimination of the GZK effect, thus modifying the spectrum of ultrahigh energy cosmic rays. This possibility can be explored with ground-based arrays such as Auger or with a space based detector system such as the proposed OWL satellite mission.

Stecker, F. W.↗

NASA NTRS2012

Linking Plasma Conditions in the Magnetosphere with Ionospheric Signatures

Modeling of the full magnetosphere, ring current and ionosphere system has become an indispensable tool in analyzing the series of events that occur during geomagnetic storms. The CCMC has a full model suite available for the magnetosphere, together with visualization tools that allow a user to perform a large variety of analyses. The January, 21, 2005 storm was a moderate-size storm that has been found to feature a large penetration electric field and unusually large polar caps (low-latitude precipitation patterns) that are otherwise found in super storms. Based on simulations runs at CCMC we can outline the likely causes of this behavior. Using visualization tools available to the online user we compare results from different magnetosphere models and present connections found between features in the magnetosphere and the ionosphere that are connected magnetically. The range of magnetic mappings found with different models can be compared with statistical models (Tsyganenko) and the model's fidelity can be verified with observations from low earth orbiting satellites such as DMSP and TIMED.

Rastaetter, Lutz↗

NASA NTRS2018

Snow in the Changing Sea-Ice Systems

Snow is the most reflective, and also the most insulative, natural material on Earth. Consequently, it is an integral part of the sea-ice and climate systems. However, the spatial and temporal heterogeneities of snow pose challenges for observing, understanding and modelling those systems under anthropogenic warming. Here, we survey the snow-ice system, then provide recommendations for overcoming present challenges. These include: collecting process-oriented observations for model diagnostics and understanding snow-ice feedbacks, and improving our remote sensing capabilities of snow for monitoring large-scale changes in snow on sea ice. These efforts could be achieved through stronger coordination between the observational, remote sensing and modelling communities, and would pay dividends through distinct improvements in predictions of polar environments.

Snow↗

DOE OSTI2020

Predicting molecular dipole moments by combining atomic partial charges and atomic dipoles

The molecular dipole moment ( μ ) is a central quantity in chemistry. It is essential in predicting infrared and sum-frequency generation spectra as well as induction and long-range electrostatic interactions. Furthermore, it can be extracted directly—via the ground state electron density—from high-level quantum mechanical calculations, making it an ideal target for machine learning (ML). Here, we choose to represent this quantity with a physically inspired ML model that captures two distinct physical effects: local atomic polarization is captured within the symmetry-adapted Gaussian process regression framework which assigns a (vector) dipole moment to each atom, while the movement of charge across the entire molecule is captured by assigning a partial (scalar) charge to each atom. The resulting “MuML” models are fitted together to reproduce molecular μ computed using high-level coupled-cluster theory and density functional theory (DFT) on the QM7b dataset, achieving more accurate results due to the physics-based combination of these complementary terms. The combined model shows excellent transferability when applied to a showcase dataset of larger and more complex molecules, approaching the accuracy of DFT at a small fraction of the computational cost. We also demonstrate that the uncertainty in the predictions can be estimated reliably using a calibrated committee model. The ultimate performance of the models—and the optimal weighting of their combination—depends, however, on the details of the system at hand, with the scalar model being clearly superior when describing large molecules whose dipole is almost entirely generated by charge separation. These observations point to the importance of simultaneously accounting for the local and non-local effects that contribute to μ ; furthermore, they define a challenging task to benchmark future models, particularly those aimed at the description of condensed phases.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS2006

Increasing Efficiency at the NTF by Optimizing Model AoA Positioning

The National Transonic Facility (NTF) at NASA Langley Research Center (LaRC) is a national resource for aeronautical research and development. The government, military and private industries rely on the capability of this facility for realistic flight data. Reducing the operation costs and keeping the NTF affordable is essential for aeronautics research. The NTF is undertaking an effort to reduce the time between data points during a pitch polar. This reduction is being driven by the operating costs of a cryogenic facility. If the time per data point can be reduced, a substantial cost savings can be realized from a reduction in liquid nitrogen (LN2) consumption. It is known that angle-of-attack (AoA) positioning is the longest lead-time item between points. In January 2005 a test was conducted at the NTF to determine the cause of the long lead-time so that an effort could be made to improve efficiency. The AoA signal at the NTF originates from onboard instrumentation then travels through a number of different systems including the signal conditioner, digital voltmeter, and the data system where the AoA angle is calculated. It is then fed into a closed loop control system that sets the model position. Each process along this path adds to the time per data point affecting the efficiency of the data taking process. Due to the nature of the closed loop feed back AoA control and the signal path, it takes approximately 18 seconds to take one pitch pause point with a typical AoA increment. Options are being investigated to reduce the time delay between points by modifying the signal path. These options include: reduced signal filtering, using analog channels instead of a digital volt meter (DVM), re-routing the signal directly to the AoA control computer and implementing new control algorithms. Each of these has potential to reduce the positioning time and together the savings could be significant. These timesaving efforts are essential but must be weighed against possible loss of data quality. For example, a reduction in filtering can introduce noise into the signal and using analog channels could result in some loss of accuracy. Data quality assessments need to be performed concurrently with timesaving techniques since data quality parameters are essential in maintaining facility integrity. This paper will highlight time saving efforts being undertaken or studied at the NTF. It will outline the instrumentation and computer systems involved in setting of the model pitch attitude then suggest changes to the process and discuss how these system changes would effect the time between data points. It also discusses the issue of data quality and how the potential efficiency changes in the system could affect it. Lastly, it will discuss the possibility of using an open loop control system and give some pros and cons of this method.

Crawford, Bradley L.↗