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At least 811 records · Page 45

Multiple satellite observations of leakage of particles from the magnetosphere

The properties of four potential sources for energetic ions and electrons in the magnetosheath are considered: upstream Fermi acceleration and shock drift acceleration of incident solar wind particles at the bow shock, acceleration of magnetosheath ions through merging at the magnetopause, and escape from the magnetosphere. A review of previous observations suggests that the magnetosphere is the dominant source of the magnetosheath energetic particle population. Despite recent work to the contrary, it is questioned whether energetic particle observations alone provide any evidence for merging at the dayside magnetopause.

Sibeck, D. G.↗

A perspective on iron (Fe) in the atmosphere: air quality, climate, and the ocean

As scientists engage in research motivated by climate change and the impacts of pollution on air, water, and human health, we increasingly recognize the need for the scientific community to improve communication and knowledge exchange across disciplines to address pressing and outstanding research questions holistically. Our professional paths have crossed because our research activities focus on the chemical reactivity of Fe-containing minerals in air and water, and at the air-sea interface. (Photo)chemical reactions driven by Fe can take place at the surface of the particles/droplets or within the condensed phase. The extent and rates of these reactions are influenced by water content and biogeochemical activity ubiquitous in these systems. One of these reactions is the production of reactive oxygen species (ROS) that cause damage to respiratory organs. Another is that the reactivity of Fe and organics in aerosol particles alter surficial physicochemical properties that impact aerosol-radiation and aerosol–cloud interactions. Also, upon deposition, aerosol particles influence ocean biogeochemical processes because micronutrients such as Fe or toxic elements such as copper become bioavailable. We provide a perspective on these topics and future research directions on the reactivity of Fe in atmospheric aerosol systems, from sources to short- and long-term impacts at the sinks with emphasis on needs to enhance the predictive power of atmospheric and ocean models.

54 ENVIRONMENTAL SCIENCES↗

Viscoelastic Particle Focusing and Separation in a Spiral Channel

As one type of non-Newtonian fluid, viscoelastic fluids exhibit unique properties that contribute to particle lateral migration in confined microfluidic channels, leading to opportunities for particle manipulation and separation. In this paper, particle focusing in viscoelastic flow is studied in a wide range of polyethylene glycol (PEO) concentrations in aqueous solutions. Polystyrene beads with diameters from 3 to 20 μm are tested, and the variation of particle focusing position is explained by the coeffects of inertial flow, viscoelastic flow, and Dean flow. We showed that particle focusing position can be predicted by analyzing the force balance in the microchannel, and that particle separation resolution can be improved in viscoelastic flows.

42 ENGINEERING↗

Physics of the magnetotail current sheet

The Earth's magnetotail plays an important role in the solar-wind-magnetosphere coupling. At the midplane of the magnetotail is a current sheet where the dominant magnetic field component reverses sign. The charged particle motion in and near the current sheet is collisionless and nonintegrable, exhibiting chaotic scattering. The current understanding of the dynamical properties of the charged particle motion is discussed. In particular, the relationships between particle dynamics and global attributes of the system are elucidated. Geometrical properties of the phase space determine important physical observables on both micro- and macroscales.

Chen, James↗

Characterization of Individual Aerosol Particles Associated with Clouds (CRYSTAL-FACE)

The aim of our research was to obtain data on the chemical and physical properties of individual aerosol particles from near the bottoms and tops of the deep convective systems that lead to the generation of tropical cirrus clouds and to provide insights into the particles that serve as CCN or IN. We used analytical transmission electron microscopy (ATEM), including energy-dispersive X-ray spectrometry (EDS) and electron energy-loss spectroscopy (EELS), and field-emission electron microscopy (FESEM) to compare the compositions, concentrations, size distributions, shapes, surface coatings, and degrees of aggregation of individual particles from cloud bases and the anvils near the tropopause. Aggregates of sea salt and mineral dust, ammonium sulfate, and soot particles are abundant in in-cloud samples. Cirrus samples contain many H2SO4 droplets, but acidic sulfate particles are rare at the cloud bases. H2SO4 probably formed at higher altitudes through oxidation of SO2 in cloud droplets. The relatively high extent of ammoniation in the upper troposphere in-cloud samples appears to have resulted from vertical transport by strong convection. The morphology of H2SO4 droplets indicates that they had been at least yartiy ammoniated at the time of collection. They are internally mixed with organic materials, metal sulfates, and solid particles of various compositions. Ammoniation and internal mixing of result in freezing at higher temperature than in pure H2SO4 aerosols. K- and S-bearing organic particles and Si-Al-rich particles are common throughout. Sea salt and mineral dust were incorporated into the convective systems from the cloud bases and worked as ice nuclei while being vertically transported. The nonsulfate particles originated from the lower troposphere and were transported to the upper troposphere and lower stratosphere.

Buseck, Peter R.↗

Going With the Flow: Using a Particle Dispersion Model to Reveal Links Between Ocean Ecosystems and Marine Aerosols

Marine biogenic particle contributions to atmospheric aerosol concentrations are not well understood though they are important for determining cloud optical and cloud nucleating properties. Here we examine the relationship between marine aerosol measurements with satellite and model fields of ocean biology and meteorological variables during the North Atlantic Aerosols and Marine Ecosystems Study (NAAMES). NAAMES consisted of four field campaigns between November 2015 and April 2018 that aligned with the four major phases of the annual phytoplankton bloom cycle. The FLEXPART Lagrangian particle dispersion model is used to connect these variables spatiotemporally to ship-based aerosol. We find that correlations between some aerosol measurements with satellite measured and modelled variables increase with increasing trajectory length. This indicates biological and meteorological processes over the air mass history are influential to measured particle properties. For example, results show organic aerosol mass is driven by biogenic volatile organic compound (VOC) emissions from photosynthesis by phytoplankton stocks during advection into the region. In contrast, primary marine aerosol (PMA) concentrations showed better correlations to variables weighted with shorter air mass residence times, which reflects their localized origin as primary emissions. Evidence also suggest variability in PMA concentrations likely play an important role in VOC emission removal. The removal of VOCs lessen their impact on particle number and mass concentrations. The sensitivity of marine aerosols to the main ecosystem-atmosphere drivers and its dependence on air mass history are to be further discussed.

Kevin J Sanchez↗

Heat Transfer Characteristics of Particle and Air Flow Through Additively Manufactured Lattice Frame Material Based on Octet-Shape Topology

Particle-to-supercritical carbon dioxide (sCO 2 ) heat exchanger is a critical component in next-generation concentrating solar power (CSP) plants. The inherently low heat transfer between falling particles and sCO 2 imposes a challenge toward economic justification of levelized cost of electricity produced through solar energy. Introduction of integrated porous media with the walls bounding particle flow has the potential to enhance the overall particle-to-sCO 2 heat exchanger performance. Here, this paper presents an experimental study on heat transfer characterization of additively manufactured lattice frame material based on Octet-shaped unit cell with particles and air as working fluids. The lattice structures were additively manufactured in stainless steel (SS) 316L and SS420 (with 40% bronze infiltration) via Binder jetting process, where the lattice porosities were varied between 0.75 and 0.9. The mean particle diameters were varied from 266 μm to 966 μm. The effective thermal conductivity and averaged heat transfer coefficient were determined through steady-state experiments. It was found that the presence of lattice enhances the effective thermal conductivity by 2–4 times when compared to packed bed of particles alone. Furthermore, for gravity-assisted particle flow through lattice panel, significantly high convective heat transfer coefficients ranging from 200 W/m2K to 400 W/m2K were obtained for the range of particle diameters tested. The superior thermal transport properties of Octet-shape-based lattice frame for particle flow makes it a very promising candidate for particle-to-sCO 2 heat exchanger for CSP application.

14 SOLAR ENERGY↗

Atmospheric aerosols: Their Optical Properties and Effects

Measured properties of atmospheric aerosol particles are presented. These include aerosol size frequency distribution and complex retractive index. The optical properties of aerosols are computed based on the presuppositions of thermodynamic equilibrium and of Mie-theory.

Source record↗

Micromechanical Properties of the SiC and Pyrolytic Carbon Layers in Tristructural-Isotropic Coated Particles

Tristructural isotropic (TRISO) coated particle fuel was initially developed for high temperature gas cooled reactors (HTGR) and has been proposed for several other advanced reactor concepts. The design of TRISO particles focuses on preventing the release of fission products in normal and off-normal reactor conditions. The particle design features an actinide bearing fuel kernel that is surrounded by three pyrolytic carbon (PyC) layers and a silicon carbide layer (SiC). The mechanical stability of the particle and fission product retention for both metallic and gaseous fission products depend on the SiC layer. Post irradiation examination (PIE) of TRISO fuel from the first two US DOE Advanced Gas Reactor Fuel Development and Qualification Program irradiation campaigns, AGR-1 and AGR-2, had identified a low rate of particles exhibiting cracking in the SiC layer that did not propagate across the SiC layer. While cracking in the SiC is rare for test conditions and particles associated with the AGR program, understanding the stress state and mechanical properties of the SiC and PyC layers related to particle architecture can aid predicting thermomechanical response of TRISO fuel under the prescribed operation envelope and beyond as well as aiding in the development of similar fuel concepts for other advanced reactors. The presented investigation shows the relationship of the mechanical properties and mechanical response (e.g., understanding crack propagation) of the SiC and PyC layers relative to position within the particle. Testing was conducted on the inner and outer PyC layers of TRISO particles to quantify differences in mechanical behavior.

Montoya, Katherine [ORNL] (ORCID:0000000326955086)↗

EPCAPE-PT-LANL Measurements: Scanning Mobility Particle Sizer

Coastal cities offer a unique environment for studying aerosol-cloud interactions and the effects of urban emissions on cloud properties. As part of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), the Partitioning Thrust by Los Alamos National Laboratory (EPCAPE-PT-LANL) was conducted. Our campaign focused on measuring the optical and chemical properties of aerosols and their interactions within marine stratocumulus clouds in La Jolla, California. EPCAPE-PT-LANL enhances the primary goals of EPCAPE through innovative observations of vapor-phase transitions between aerosols and cloud droplets, the impact of black carbon on aerosol-cloud dynamics, and the effects of cloud processing on aerosol optical properties. Instrument: Scanning Mobility Particle Sizer (TSI), DMA Classifier Model 3082 + CPC Detector Model 3752. Data Notes: The SMPS dataset is limited due to necessary instrument maintenance and subsequent extensive downtime. Data is only available from October 21 to November 8, 2023. Post November 22, 2023, the NanoScan instrument provided coverage for the latter half of the campaign. To ensure consistency, the data was resampled into uniform size bins ranging from 15 nm to 667 nm. This adjustment was required due to changes in size bins and the maximum diameter that occurred after maintenance and repairs. Multiple Charge Correction applied, Nanoparticle Agglomerate Mobility Analysis not applied, and Diffusion Correction applied. Header: - List [15 nm to 667 nm] middle of the size bin in nanometers: Data reports the concentration particles in this size bin per cubic centimeter, dN/dLog(dp). - CVI_Flag[bool]: A boolean flag indicating whether the Counterflow Virtual Impactor (CVI) was active (true) or inactive (false) during the measurement.

54 ENVIRONMENTAL SCIENCES↗

Simulating Fracture Sealing by Granular LCM Particles in Geothermal Drilling

Lost circulation occurs when the returned fluid is less than what is pumped into the well due to loss of fluid to pores or fractures. A lost-circulation event is a common occurrence in a geothermal well. Typical geothermal reservoirs are often under-pressured and have larger fracture apertures. A severe lost-circulation event is costly and may lead to stuck pipe, well instability, and well abandonment. One typical treatment is adding lost-circulation materials (LCMs) to seal fractures. Conventional LCMs fail to properly seal fractures because their mechanical limit is exceeded at elevated temperatures. In this paper, parametric studies in numerical simulations are conducted to better understand different thermal effects on the sealing mechanisms of LCMs. The computational fluid dynamics (CFDs) and the discrete element method (DEM) are coupled to accurately capture the true physics of sealing by granular materials. Due to computational limits, the traditional Eulerian–Eulerian approach treats solid particles as a group of continuum matter. With the advance of modern computational power, particle bridging is achievable with DEM to track individual particles by modeling their interactive forces between each other. Particle–fluid interactions can be modeled by coupling CFD algorithms. Fracture sealing capability is investigated by studying the effect of four individual properties including fluid viscosity, particle size, friction coefficient, and Young’s modulus. It is found that thermally degraded properties lead to inefficient fracture sealing.

15 GEOTHERMAL ENERGY↗

Status of 1eNp0π Charged-Current Electron Neutrino Cross Section on Argon in the NuMI Beam at ICARUS

The Short-Baseline Neutrino (SBN) Program is designed to probe short-baseline neutrino anomalies, including the LSND electron neutrino excess and the MiniBooNE low-energy excess. Essential to interpreting these anomalies and to the success of future experiments like DUNE, is the precise measurement of neutrino-argon interaction cross sections. The program utilizes two liquid argon time projection chamber (LArTPC) detectors: the Short-Baseline Near Detector (SBND) located 110 meters downstream from the Booster Neutrino Beam (BNB) target, and the ICARUS detector positioned 600 meters downstream. Additionally, the ICARUS detector lies off-axis to the NuMI beamline, providing a unique, high-statistics flux of electron neutrinos and sensitivity to energies that overlap with the DUNE spectrum. To analyze the data from these detectors, we have begun employing a machine-learning-based reconstruction algorithm referred to as “Scalable Particle Imaging with Neural Embeddings” (SPINE). SPINE has shown improvement in the ability to reconstruct the properties of final state particles in the detector, like the particle ID and momentum, with the potential to enhance the quality of measurements achievable within the SBN Program e.g., the resolution on kinematics used in differential cross section extraction. This poster presents progress toward measuring the electron neutrino argon interaction cross section in the 1eNp0π topology using the NuMI beam, highlighting the impact of SPINE through the ability to select signal events across a wide kinematic range without sacrificing background rejection power.

Carber, Dan [Colorado State U.] (ORCID:00090006451↗

Voyager imaging of Triton's clouds and hazes

Results are presented from a detailed analysis of Voyager images of Triton obtained at the highest solar phase angles; these have been fit to Mie scattering models in order to obtain the mean particle sizes, number densities, and the vertical extent of the two different scattering components of the Triton atmosphere. The 0.001-0.01 optical depths of about 0.17 micron particles are vertically distributed with scale heights of about 10 km throughout Triton. A number of properties of the haze particles in question suggest that they are composed of photochemically produced gases which have condensed in the cold lower atmosphere of Triton.

Rages, Kathy↗

Dam-Break Flow Measurements of Liquid–Granular Mixtures in a Channelized Reservoir

Dam-break flows of granular materials exhibit a complex non-Newtonian rheology, which is strongly influenced by various factors, such as the characteristics of the granular material, the degree of initial compaction, and saturation level of the granular matrix. Specially adapted nonintrusive techniques are required to investigate these flows in the laboratory. This paper investigated the nonintrusive technique of image analysis. The methodologies used in the measurement of bulk flow parameters, such as flow depth, front velocity, and flow rate, and the extraction of detailed flow characteristics such as velocity profiles, were discussed in the context of a series of granular dam-break flow experiments. These experiments were performed under three types of initial conditions: dry, saturated (water filling the pore space), and submerged (a layer of saturated granular material submerged under water) using four types of granular materials—PET pellets, crushed walnut shells, urea, and sand—with grain sizes ranging from 200 μm to 2.9 mm. High-speed cameras were used to capture the evolution and local properties of the flow, such as velocity fields using particle image velocimetry (PIV). Bulk properties of the flow were obtained by tracking the surface profile of the granular matrix and the water table. The extracted profiles were used to measure the evolution of the volume of the granular matrix and the fluid phase separately upstream and downstream of the gate, which allowed measuring the dilatancy (increase in pore space). The study showed that the image analysis techniques are versatile and can be adapted to measure different flow parameters in a variety of granular flows to better understand and analyze their complex behavior. Finally, the advantages and drawbacks of each image analysis technique were discussed and best-practice recommendations were provided.

42 ENGINEERING↗

EPCAPE-PT-LANL Measurements: Soot Particle Aerosol Mass Spectrometer

Coastal cities offer a unique environment for studying aerosol-cloud interactions and the effects of urban emissions on cloud properties. As part of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), the Partitioning Thrust by Los Alamos National Laboratory (EPCAPE-PT-LANL) was conducted. Our campaign focused on measuring the optical and chemical properties of aerosols and their interactions within marine stratocumulus clouds in La Jolla, California. EPCAPE-PT-LANL enhances the primary goals of EPCAPE through innovative observations of vapor-phase transitions between aerosols and cloud droplets, the impact of black carbon on aerosol-cloud dynamics, and the effects of cloud processing on aerosol optical properties. Instrument: Soot particle-Aerosol Mass Spectrometer. (Aerodyne Inc.) Header: - Organic_GCVIoff[ug/m3]: Concentration of organic compounds measured via the Main Inlet (out-of-cloud) in micrograms per cubic meter. - Nitrate_GCVIoff[ug/m3]: Concentration of nitrate measured via the Main Inlet (out-of-cloud) in micrograms per cubic meter. - Sulfate_GCVIoff[ug/m3]: Concentration of sulfate measured via the Main Inlet (out-of-cloud) in micrograms per cubic meter. - Chloride_GCVIoff[ug/m3]: Concentration of chloride measured via the Main Inlet (out-of-cloud) in micrograms per cubic meter. - Ammonium_GCVIoff[ug/m3]: Concentration of ammonium via the Main Inlet (out-of-cloud) in micrograms per cubic meter. - Organic_GCVIon[ug/m3]: Concentration of organic compounds measured in-cloud via CVI in micrograms per cubic meter. - Nitrate_GCVIon[ug/m3]: Concentration of nitrate measured in-cloud via CVI in micrograms per cubic meter. - Sulfate_GCVIon[ug/m3]: Concentration of sulfate measured in-cloud via CVI in micrograms per cubic meter. - Chloride_GCVIon[ug/m3]: Concentration of chloride measured in-cloud via CVI in micrograms per cubic meter. - Ammonium_GCVIon[ug/m3]: Concentration of ammonium measured in-cloud via CVI in micrograms per cubic meter. - CVI_Flag[bool]: A boolean flag indicating whether the CVI was active (true) or inactive (false) during the measurement.

54 ENVIRONMENTAL SCIENCES↗