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At least 811 records · Page 45
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Salt-Induced Polymorphs Observed in Colloidal Single Crystals

Polymorphs are solid materials with the same chemical composition but different crystallographic structures. A unique aspect of polymorphs is that they exhibit different physical properties, such as solubility, melting point, density, color, hardness, and bioavailability. Here, we synthesized polymorphs of colloidal crystals engineered with DNA by slow-cooling gold nanoparticle-core programmable atom equivalents (PAEs, particles with DNA sequences that control their bonding characteristics) under salt concentrations ranging from 0.5 to 4 M NaCl. This approach yielded a diverse set of single-crystalline phases with cubic, tetragonal, and hexagonal lattice symmetries. The structural transitions observed here arise solely from the modulation of interparticle repulsion via ionic strength and thermal processing. Notably, in certain cases, we observed diffusionless phase transformations, wherein the superlattices evolve from cubic to lower-symmetry tetragonal lattices. By tuning the thermal stability and salt concentration, we captured intermediate, metastable body-centered tetragonal structures during the slow-cool process, indicating that subtle changes in free energy can direct crystallization to low-symmetry phases. In conclusion, this study demonstrates that thermal and ionic parameters can be tuned to access and stabilize colloidal crystal polymorphs with emergent structures and interesting functional properties.

Colloidal crystallization↗
DOE OSTI2020

Changes to the Appearance of Optical Lightning Flashes Observed From Space According to Thunderstorm Organization and Structure

Optical lightning observations from space reveal a wide range of flash structure. Lightning imagers such as the Geostationary Lightning Mapper and Lightning Imaging Sensor measure flash appearance by recording transient changes in cloud top illumination. The spatial and temporal optical energy distributions reported by these instruments depend on the physical structure of the flash and the distribution of hydrometeors within the thundercloud that scatter and absorb the optical emissions. This study reported herein explores how flash appearance changes according to the scale and organization of the parent thunderstorms with a focus on mesoscale convective systems. Clouds near the storm edge are frequently illuminated by large optical flashes that remain stationary between groups. These flashes appear large because their emissions can reflect off the exposed surfaces of nearby clouds to reach the satellite. Large stationary flashes also occur in small isolated thunderstorms. Optical flashes that propagate horizontally, meanwhile, are most frequently observed in electrified stratiform regions where extensive layered charge structures promote lateral development. Highly radiant “superbolts” occur in two scenarios: embedded within raining stratiform regions or in nonraining boundary/anvil clouds where optical emissions can take a relatively clear path to the satellite.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Evaluation of an Improved Convective Triggering Function: Observational Evidence and SCM Tests

This study provides a strong observational support for a recently developed convective triggering function that uses the large-scale dynamic convective available potential energy (dCAPE) as a constraint combined with an unrestricted air parcel launch level (ULL) to relax the unrealistic strong coupling of convection to surface heating and capture nocturnal elevated convection. Both case study and statistical analysis are conducted using the observations collected from the Department of Energy (DOE)'s Atmospheric Radiation Measurement (ARM) program at its Southern Great Plains (SGP) and Manaus (MAO) sites. They show that dCAPE has a much stronger correlation with precipitation than CAPE and ULL is essential to detect elevated convection above boundary layer under both midlatitude and tropical conditions and for both afternoon and nighttime deep convection regimes. Sensitivity tests with the single-column model (SCM) of DOE's Energy Exascale and Earth System Model (E3SM) indicate that the role of dCAPE in suppressing daytime convection is more effective for tropical convection than midlatitude convection. Even though the dCAPE can suppress the overestimated convection, ULL plays a much bigger role in improving the diurnal cycle of precipitation than dCAPE. It not only helps capture nocturnal elevated convection, but also significantly removes the spurious morning precipitation seen in the default model, due to the release of unstable energy at night. However, the use of ULL has led to an overestimation of light-to-moderate precipitation (1-10 mm/day) due to more convection being triggered above boundary layer.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Simultaneous Observations of Localized and Global Drift Resonance

In this study, we present Van Allen Probe observations showing that seed (hundreds of keV) and core ( ≳ 1 MeV) electrons can resonate with ultra-low-frequency (ULF) wave modes with distinctive m values simultaneously. An unusual electron energy spectrogram with double-banded resonant structure was recorded by energetic particle, composition, and thermal plasma (ECT)-magnetic electron ion spectrometer (MagEIS) and, meanwhile, boomerang stripes in pitch angle spectrogram appeared at the lower energy band. A localized drift resonance with m = 10 wave component was responsible for the resonant band peaked at ~200 keV while a global drift resonance with m = 3 component gave rise to the upper band resonance peaked at ~1 MeV. Time-Of-Flight on boomerang stripes suggested that the localized drift resonance with ~200 keV electrons was confined within the plasmaspheric plume. Electron flux modulations were reproduced by numerical simulations in good consistency with the observations, supporting the scenario that localized and global drift resonance could coexist in the outer belt electron dynamics simultaneously.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Observation of High-Energy Electrons Precipitated by NWC Transmitter From PROBA-V Low-Earth Orbit Satellite

The very low-frequency transmitter in the Northwest Cape of Australia (NWC) has previously been observed to pitch-angle scatter electrons with energies from 30–400 keV, creating enhanced fluxes measured by low-Earth orbiting (LEO) satellites. Here we use observations from the Energetic Particle Telescope on PROBA-V. We compare the measured flux, as a function of local magnetic field strength, when the NWC transmitter is “on” versus “off,” and find enhanced fluxes only when NWC is “on” and located on the nightside. The enhanced fluxes occur in the population gradually transitioning from “permanently trapped” to “quasi-trapped.” We show that electrons up to 800 keV, substantially higher energy than previously studied, are scattered by resonant interactions with NWC to produce enhanced fluxes. The enhanced fluxes appear at multiple L-shells for each energy channel, consistent with resonance conditions at distinct wave normal angles, that indicate ducted interactions at L < 1.55 and unducted interactions at L > 1.65.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Sub-Cloud Turbulence Explains Cloud-Base Updrafts for Shallow Cumulus Ensembles: First Observational Evidence

Sub-cloud turbulent kinetic energy has been used to parameterize the cloud-base updraft velocity (w b ) in cumulus parameterizations. The validity of this idea has never been proved in observations. Instead, it was challenged by recent Doppler Lidar observations showing a poor correlation between the two. We argue that the low correlation is likely caused by the difficulty of a fixed-point Lidar to measure ensemble properties of cumulus fields. Taking advantage of the stationarity and ergodicity of early afternoon convection, we developed a Lidar sampling methodology to measure w b of a shallow cumulus (ShCu) ensemble (not a single ShCu). By analyzing 128 ShCu ensembles over the Southern Great Plains, we show that the ensemble properties of sub-cloud turbulence explain nearly half of the variability in ensemble-mean wb, demonstrating the ability of sub-cloud turbulence to dictate w b . Lastly, the derived empirical formulas will be useful for developing cumulus parameterizations and satellite inference of w b .

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

First Simultaneous Observation of STEVE and SAR Arc Combining Data From Citizen Scientists, 630.0 nm All‐Sky Images, and Satellites

Abstract On September 28, 2017 citizen scientist observations at Alberta, Canada (51°N, 113° W) detected aurora and a thin east‐west purplish arc, known as strong thermal emission velocity enhancement (STEVE) that lasted less than 20 min. All‐sky imagers at subauroral latitudes measured stable auroral red (SAR) arcs during the entire night. The imager at Bridger, MT (45.3°N, 108.9°W) also measured a STEVE. The overlapping geometry allowed to determine that the height of STEVE was 225–275 km. STEVE is brighter in the 630.0 nm images in the West and almost merges with the SAR arc in the East. A DMSP satellite pass in the southern hemisphere was at the conjugate location of the Bridger imager during the STEVE observation. When mapped into the northern hemisphere intense subauroral ion drift and subauroral polarization streams were detected associated with the two optical signatures measured in 630.0 nm.

Martinis, C.↗
DOE OSTI2020

Magnetopause Reconnection as Influenced by the Dipole Tilt Under Southward IMF Conditions: Hybrid Simulation and MMS Observation

Abstract Using a three‐dimensional (3‐D) global‐scale hybrid code, the Magnetospheric Multiscale (MMS) reconnection event around 02:13 UT on 18 November 2015, highlighted in the Geospace Environment Modeling (GEM) Dayside Kinetic Challenge, is simulated, in which the interplanetary magnetic field (IMF) points southward and the geomagnetic field has a −27° dipole tilt angle. Strong southward plasma jets are found near the magnetopause as a result of the dayside reconnection. Our results indicate that the subsolar magnetopause reconnection X line shifts from the subsolar point toward the Northern Hemisphere due to the effect of the tilted geomagnetic dipole angle, consistent with the MMS observation. Subsequently, the reconnection X lines or sites and reconnection flux ropes above the equator propagate northward along the magnetopause. The formation and global distribution of the X lines and the structure of the magnetopause reconnection are investigated in detail with the simulation. Mirror mode waves are also found in the middle of the magnetosheath downstream of the quasi‐perpendicular shock where the plasma properties are consistent with the mirror instability condition. As a special outcome of the GEM challenge event, the spatial and temporal variations in reconnection, the electromagnetic power spectra, and the associated D‐shaped ion velocity distributions in the simulated reconnection event are compared with the MMS observation.

Guo, Zhifang↗
DOE OSTI2021

Investigation of Small-Scale Electron Density Irregularities Observed by the Arase and Van Allen Probes Satellites Inside and Outside the Plasmasphere

In situ electron density profiles obtained from Arase in the night magnetic local time (MLT) sector and from RBSP-B covering all MLTs are used to study the small-scale density irregularities present in the plasmasphere and near the plasmapause. Electron density perturbations with amplitudes >10% from background density and with time-scales less than 30-min are investigated here as the small-scale density irregularities. The statistical survey of the density irregularities is carried out using nearly 2 years of density data obtained from RBSP-B and 4 months of data from Arase satellites. The results show that density irregularities are present globally at all MLT sectors and L-shells both inside and outside the plasmapause, with a higher occurrence at L > 4. The occurrence of density irregularities is found to be higher during disturbed geomagnetic and interplanetary conditions. The case studies presented here revealed: (1) The plasmaspheric density irregularities observed during both quiet and disturbed conditions are found to coexist with the hot plasma sheet population. (2) During quiet periods, the plasma waves in the whistler-mode frequency range are found to be modulated by the small-scale density irregularities, with density depletions coinciding well with the decrease in whistler intensity. Our observations suggest that different source mechanisms are responsible for the generation of density structures at different MLTs and geomagnetic conditions.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Multipoint Observations of Quasiperiodic Emission Intensification and Effects on Energetic Electron Precipitation

The two Van Allen Probes simultaneously recorded a coherently modulated quasiperiodic (QP) emission that persisted for 3 h. The magnetic field pulsation at the locations of the two satellites showed a substantial difference, and their frequencies were close to but did not exactly match the repetition frequency of QP emissions for most of the time, suggesting that those coherent QP emissions probably originated from a common source, which then propagated over a broad area in the magnetosphere. The QP emissions were amplified by local anisotropic electron distributions, and their large-scale amplitudes were modulated by the plasma density. A novel observation of this event is that chorus waves at frequencies above QP emissions exhibit a strong correlation with QP emissions. Those chorus waves intensified when the QP emissions reach their peak frequency. This indicates that embryonic QP emissions may be critical for its own intensification as well as chorus waves under certain circumstances. A Low-Earth-Orbit POES satellite observed enhanced energetic electron precipitation in conjunction with the Van Allen Probes, providing direct evidence that QP emissions precipitate energetic electrons into the atmosphere. Finally, this scenario is quantitatively confirmed by our quasilinear diffusion simulation results.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Electron Dropout Events and Flux Enhancements Associated With Geomagnetic Storms Observed by PROBA-V/Energetic Particle Telescope From 2013 to 2019

Electron flux variations for E > 500 keV during geomagnetic storms are investigated using the Energetic Particle Telescope (EPT). This detector launched in May 2013 on board the satellite PROBA-V at an altitude of 820 km was designed to provide uncontaminated spectra of electrons, protons, and alpha particles. Electron flux dropout events are observed during the main phase of each storm and even during substorms: a rapid reduction of the electron flux is noted throughout the outer electron radiation belt at all energies above about 0.5 MeV on timescales of a few hours. The electron spectrograms measured by the EPT between 2013 and 2019 show that after each geomagnetic storm, dropout events are followed by a flux enhancement starting first at low L values, and reaching the slot or even the inner belt for the strongest storms. We determine the link between Disturbed Storm Time (Dst) and the minimum value of the L-shell where the dropouts deplete the outer belt, as well as the nonlinear relation between Dst and the minimum L-shell where the flux penetrates in the slot region or even the inner belt during the storms. Dropouts appear at all energies measured by EPT and penetrate down to $\textit{L}$~3.5 for the strongest events. Dropouts are observed at Low Earth Orbit each time Dst has an inverted peak < –40 nT. Flux enhancements appear at lower L only for big storm events with Dst < –50 nT. They penetrate down to an impenetrable barrier with a minimum L-shell related to Dst and to the energy. For E > 1 MeV, this limit is also linked to the plasmapause position.

58 GEOSCIENCES↗
DOE OSTI2021

Observations and Simulations of Dropout Events and Flux Decays in October 2013: Comparing MEO Equatorial With LEO Polar Orbit

We compare ESA PROBA-V observations of electron flux at LEO with those from the NASA Van Allen Probes mostly at MEO for October 2013. Dropouts are visible at all energy during four storms from both satellites. Equatorially trapped electron fluxes are higher than at LEO by 10 2 (<1 MeV) to 10 5 (>2.5 MeV). We observe a quite isotropic structure of the outer belt during quiet times, contrary to the inner belt, and pitch angle dependence of high energy injection. We find a very good overlap of the outer belt at MEO and LEO at ~0.5 MeV. We use test-particle simulations of the energetic electrons trapped in the terrestrial magnetic field to study the outer radiation belt electron flux changes during geomagnetic storms. We show that the Dst (Disturbance storm time) effect during the main phase of a geomagnetic storm results in a betatron mechanism causing outward radial drift and a deceleration of the electrons. This outward drift motion is energy independent, pitch angle-dependent, and represents a significant distance (~1 L-shell at L = 5 for moderate storms). At fixed L-shell, this causes a decay of the LEO precipitating flux (adiabatic outward motion), followed by a return to the normal state (adiabatic inward motion) during main and recovery phases. Dst effect, associated with magnetopause shadowing and radial diffusion can explain the main characteristics of outer radiation belt electron dropouts in October 2013. We also use Fokker-Planck simulations with event-driven diffusion coefficients at high temporal resolution, to distinguish instantaneous loss from the gradual scattering that depopulates the slot region and the outer belt after storms. Simulations reproduce the slot formation and the gradual loss in the outer belt. The typical energy dependence of these losses leads to the absence of scattering for relativistic and ultra-relativistic electrons in the outer belt, oppositely to dropouts.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Intrinsic Elastic Anisotropy of Westerly Granite Observed by Ultrasound Measurements, Microstructural Investigations, and Neutron Diffraction

Westerly granite (WG) has been generally accepted as an isotropic homogeneous rock. Here, we return to WG and observe significant elastic anisotropy using multidirectional ultrasonic sounding on spherical samples at pressures up to 400 MPa. Thermal treatment of WG leads to formation of microcracks that reduce elastic wave velocities and increase its elastic anisotropy. The 3D distribution of P-wave velocities at low pressure is close to orthorhombic symmetry. Application of hydrostatic pressure closes most of thermally induced microcracks and decreases elastic anisotropy of WG, but at high pressure the anisotropy is practically reversed compared to low pressure: maximum P-wave velocity direction at low pressures is near minimum velocity direction at high pressure and vice versa. To understand this effect, microstructures of the rock were investigated by optical and scanning electron microscopy. Preferred orientations of four major rock-forming minerals—quartz, orthoclase, plagioclase, and biotite—were measured by time-of-flight neutron diffraction, which confirms significant crystal alignment. All these data were used to numerically model anisotropic elastic properties of WG. It is shown that WG possesses weak intrinsic elastic anisotropy related mainly to the preferred orientation of feldspars formed during igneous crystallization. Observed microcracks are mostly related to the cleavage planes of feldspars and biotite, and thus also demonstrate preferred orientation. Higher preheating temperatures produce larger quantity of longer microcracks. A numerical model shows that these microcracks act against the weak intrinsic elastic anisotropy of WG, and define the elastic anisotropy at low pressures.

58 GEOSCIENCES↗
DOE OSTI2020

Distinctive Signals in 1-min Observations of Overshooting Tops and Lightning Activity in a Severe Supercell Thunderstorm

This work examines a severe weather event that took place over central Argentina on December 11, 2018. The evolution of the storm from its initiation, rapid organization into a supercell, and eventual decay was analyzed with high-temporal resolution observations. This work provides insight into the spatio-temporal co-evolution of storm kinematics (updraft area and lifespan), cloud-top cooling rates, and lightning production that led to severe weather. The analyzed storm presented two convective periods with associated severe weather. An overall decrease in cloud-top local minima IR brightness temperature (MinIR10.3), increase in overshooting top area, and lightning jump (LJ) preceded both periods. LJs provided the highest lead time to the occurrence of severe weather, with the ground-based lightning networks providing the maximum warning time of around 30 min. Lightning flash counts from the Geostationary Lightning Mapper (GLM) were underestimated when compared to detections from ground-based lightning networks. Among the possible reasons for GLM’s lower detection efficiency were an optically dense medium located above lightning sources and the occurrence of flashes smaller than GLM’s footprint. The minimum MinIR provided the shorter warning time to severe weather occurrence. However, secondary minima in MinIR10.3 that preceded the absolute minima improved this warning time by more than 10 min. Furthermore, trends in MinIR10.3 for time scales shorter than 6 min revealed shorter cycles of fast cooling and warming, which provided information about the lifecycle of updrafts within the storm. The advantages of using observations with high-temporal resolution to analyze the evolution and intensity of convective storms are discussed.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

GLM Observations of the Brightest Lightning in the Americas

Two years of Geostationary Lightning Mapper (GLM) science data are used to document the brightest lighting flashes observed on the Americas continent. The most radiant optical lightning emissions—termed “superbolts”—were first identified by the Vela satellite constellation in the 1970s (Turman, 1977) and are defined in terms of peak optical power. GLM is an integrating sensor that, instead, measures the total optical energy from a lightning pulse. Furthermore, while GLM might not correctly classify short-duration superbolts, its top lightning cases certainly fall in the superbolt category, and the wealth of GLM measurements over its stationary hemispheric field of view provide an unmatched sample of extraordinarily bright lightning. While radiant bolts in excess of 100× the optical energy of typical lightning are ubiquitous across the Americas and result from many types of lightning processes, we find the most radiant cases (>1,000×) are concentrated in the central United States and in the La Plata basin in South America. Coincident Earth Networks Global Lightning Network (ENGLN) observations reveal that these extremely bright emissions usually result from + CG strokes with high peak currents in long horizontal flashes outside of the convective core. Single cases of these megaflashes might produce multiple superbolts over their durations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Clouds and Radiation Processes in Regional Climate Models Evaluated Using Observations Over the Ice‐free Arctic Ocean

Abstract The presence of clouds in the Arctic regulates the surface energy budget (SEB) over the sea‐ice surface and the ice‐free ocean. Following several previous field campaigns, the cloud‐radiation relationship, including cloud vertical structure and phase, has been elucidated; however, modeling of this relationship has matured slowly. In recognition of the recent decline in the Arctic sea‐ice extent, representation of the cloud system in numerical models should consider the effects of areas covered by sea ice and ice‐free areas. Using an in situ stationary meteorological observation data set obtained over the ice‐free Arctic Ocean by the Japanese Research Vessel Mirai (September 2014), coordinated evaluation of six regional climate models (RCMs) with nine model runs was performed by focusing on clouds and the SEB. The most remarkable findings were as follows: (1) reduced occurrence of unstable stratification with low‐level cloud water in all models in comparison to the observations, (2) significant differences in cloud water representations between single‐ and double‐moment cloud schemes, (3) extensive differences in partitioning of hydrometeors including solid/liquid precipitation, and (4) pronounced lower‐tropospheric air temperature biases. These issues are considered as the main sources of SEB uncertainty over ice‐free areas of the Arctic Ocean. The results from a coupled RCM imply that the SEB is constrained by both the atmosphere and the ocean (and sea ice) with considerable feedback. Coordinated improvement of both stand‐alone atmospheric and coupled RCMs would promote a more comprehensive and improved understanding of the Arctic air‐ice‐sea coupled system.

Inoue, Jun↗
DOE OSTI2021

Experimental Constraints on Solid Nitride Phases in Rocky Mantles of Reduced Planets and Implications for Observable Atmosphere Compositions

Abstract Astronomical surveys have discovered thousands of transiting exoplanets, revealing that rocky planets are common in the galaxy. A planet's interior chemistry is frequently inferred by average density, described by mass‐radius (M‐R) relationships. However, M‐R relationships give rise to non‐unique interpretations of a planet's interior composition, an issue that limits our ability to characterize far‐away worlds. We present experimental and density functional theoretical results addressing the influence of an ultra‐reducing (oxygen‐poor) interior chemistry on rocky mantle phases and discuss the possible implications for atmospheric observables. We show that silicon carbide (SiC) and molecular nitrogen (N 2 ) react to form solid silicon nitride (γ‐Si 3 N 4 ) at high pressures and high temperatures in a laser‐heated diamond‐anvil cell, consistent with ab initio computations. Si 3 N 4 remains stable under extreme conditions and when quenched to ambient conditions. As SiC is a common compound found under very reducing conditions, these results indicate that nitrogen may form solid phases in an oxygen‐poor rocky planet. If, by sequestering nitrogen in a planet's mantle, the distribution of nitrogen between a planet's interior and atmosphere is altered (i.e., a nitrogen‐rich mantle and nitrogen‐poor atmosphere), these results indicate that there may be atmospheric observables connected to the mantle‐redox state of a rocky planet besides the oxygen‐containing phases ubiquitous in exoplanet literature.

Daviau, Kierstin↗
DOE OSTI2021

Satellite Observations of the Tropical Terrestrial Carbon Balance and Interactions With the Water Cycle During the 21st Century

A constellation of satellites are now in orbit providing information about terrestrial carbon and water storage and fluxes. These combined observations show that the tropical biosphere has changed significantly in the last two decades from the combined effects of climate variability and land use. Large areas of forest have been cleared in both wet and dry forests, increasing the source of carbon to the atmosphere. Concomitantly, tropical fire emissions have declined, at least until 2016, from changes in land-use practices and rainfall, increasing the net carbon sink. Measurements of carbon stocks and fluxes from disturbance and recovery and of vegetation photosynthesis show significant regional variability of net biosphere exchange (NBE) and gross primary productivity (GPP) across the tropics and are tied to seasonal and interannual changes in water fluxes and storage. Comparison of satellite based estimates of evapotranspiration (ET), photosynthesis, and the deuterium content of water vapor with patterns of total water storage and rainfall demonstrate the presence of vegetation-atmosphere interactions and feedback mechanisms across tropical forests. However, these observations of stocks, fluxes and inferred interactions between them do not point unambiguously to either positive or negative feedbacks in carbon and water exchanges. These ambiguities highlight the need for assimilation of these new measurements with Earth System models for a consistent assessment of process interactions, along with focused field campaigns that integrate ground, aircraft and satellite measurements, to quantify the controlling carbon and water processes and their feedback mechanisms.

58 GEOSCIENCES↗