SEARCH · Engineering Papers
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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The purpose of this report is to document several use cases of the Ultra-Fast Closure Valve System (UCVS) at the Joint Actinide Shock Physics Experimental Research (JASPER) facility. The goal is to clearly identify the use cases so that an explosive hazard classification may be assigned.
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Today, I will introduce a model-free method to see things that are usually out of sight. By see I mean recover real-space information in the atomic length and timescale of multiple motions, a molecular movie beyond what is traditionally resolved.
The goal of the project has been to theoretically investigate a wide variety of problems related to the use of X-ray spectroscopy in materials science to enhance the impact of the science done at DOE’s user facilities. The focus has generally been on obtaining a deeper understand of new types of X-ray spectroscopy and to provide support for experimentalist working in these fields.
We study charge transfer in dissociating molecules of 2-iodopropane (C 3 H 7 I) in a UV pump – XUV probe regime at the SACLA free-electron laser. Signatures of charge transfer from the recently dissociated iodine atom to the neutral propyl radical are observed in recorded 3D ion momentum distributions. This signature has evaded observation in previous related experiments. Detailed analysis of these signatures allows the identification of a region of internuclear separation where charge transfer occurs.
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The central goal of this proposal was to directly visualize and quantify how electronic correlations, vibronic couplings, and local solute-solvent interactions control intramolecular electron motion on the femtosecond time scale. The proposed research program focused on solvated Ruthenium (Ru) based mixed-valence complexes, a prototypical class of transition-metal complexes, which are of significant interest for their potential applications in photochemical energy conversion. Electron movements following photochemical excitation are closely coupled with atomic/vibrational and solvent motion. To disentangle these various components requires tools designed to directly probe electron correlations and vibronic coupling (coherently coupled motions of electronic and vibrational coordinates) on the timescale of electron motion in the solution phase.
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