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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Towards Noble-Metal-Free Dyads: Ground and Excited State Tuning by a Cobalt Dimethylglyoxime Motif Connected to an Iron N-Heterocyclic Carbene Photosensitizer: Towards Noble-Metal-Free Dyads: Ground and Excited State Tuning by a Cobalt Dimethylglyoxime Motif Connected to an Iron N-Heterocyclic Carbene Photose
Heteroleptic iron based complexes bearing the 2,6-bis[3-(2,6-diisopropylphenyl)imidazol-2-ylidene]pyridine motif and a polypridine ligand have been synthesized and characterized in their ground and excited state. This series of complexes includes a first example of a hetero-bimetallic complex connecting an iron N-heterocyclic carbene photosensitizer with a cobalt dimethylglyoxime fragment. Focus is set on the influence of the linker and cobalt center as second ligand at the iron center on the photophysics. While electronic absorption spectroscopy and cyclic voltammetry reveal a weak mutual influence of the single ligands in the heteroleptic complexes, an increasing MLCT lifetime with larger pi-accepting abilities was found by time-resolved transient absorption spectroscopy, with maximum lifetime in the case of the hetero-bimetallic dyad. Concurrently the MC lifetimes were observed to decrease. The reported results will allow to develop guidelines for designing bimetallic devices, which may allow electron transfer from the photosensitizer fragment to a catalytically active center.
The potential of ill-nitride laser diodes for solid-state lighting [Advantages of III-Nitride Laser Diodes in Solid-State Lighting]
III-nitride laser diodes (LDs) are an interesting light source for solid-state lighting (SSL). Modelling of LDs is performed to reveal the potential advantages over traditionally used light-emitting diodes (LEDs). The first, and most notable, advantage is LDs have higher efficiency at higher currents when compared to LEDs. This is because Auger recombination that causes efficiency droop can no longer grow after laser threshold. Second, the same phosphor-converted methods used with LEDs can also be used with LDs to produce white light with similar color rendering and color temperature. Third, producing white light from direct emitters is equally challenging for both LEDs and LDs, with neither source having a direct advantage. Lastly, the LD emission is directional and can be more readily captured and focused, leading to the possibility of novel and more compact luminaires. These advantages make LDs a compelling source for future SSL.
Search for the production of single vector-like and excited quarks in the Wt final state in pp collisions at root s=8 TeV with the ATLAS detector
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Search for charged Higgs bosons decaying via H ± → τ ± ν in fully hadronic final states using pp collision data at s $$ \sqrt{s} $$ = 8 TeV with the ATLAS detector
The results of a search for charged Higgs bosons decaying to a τ lepton and a neutrino, H ± → τ ± ν, are presented. The analysis is based on 19.5 fb –1 of proton-proton collision data at √s = 8 TeV collected by the ATLAS experiment at the Large Hadron Collider. Charged Higgs bosons are searched for in events consistent with top-quark pair production or in associated production with a top quark, depending on the considered H ± mass. The final state is characterized by the presence of a hadronic τ decay, missing transverse momentum, b-tagged jets, a hadronically decaying W boson, and the absence of any isolated electrons or muons with high transverse momenta. The data are consistent with the expected background from Standard Model processes. A statistical analysis leads to 95% confidence-level upper limits on the product of branching ratios Β(t → bH ± ) × Β(H ± → τ ± ν), between 0.23% and 1.3% for charged Higgs boson masses in the range 80-160GeV. It also leads to 95% confidence-level upper limits on the production cross section times branching ratio, σ(pp → tH ± + X) × Β(H ± → τ ± ν), between 0.76 pb and 4.5 fb, for charged Higgs boson masses ranging from 180 GeV to 1000 GeV. In the context of different scenarios of the Minimal Supersymmetric Standard Model, these results exclude nearly all values of tan β above one for charged Higgs boson masses between 80 GeV and 160 GeV, and exclude a region of parameter space with high tan β for H ± masses between 200 GeV and 250 GeV.
Search for direct top-squark pair production in final states with two leptons in pp collisions at $ \sqrt{s} $ = 8 TeV with the ATLAS detector
A search is presented for direct top-squark pair production in final states with two leptons (electrons or muons) of opposite charge using 20.3 fb -1 of pp collision data at $ \sqrt{s} $ = 8 TeV, collected by the ATLAS experiment at the Large Hadron Collider in 2012. No excess over the Standard Model expectation is found. The results are interpreted under the separate assumptions (i) that the top squark decays to a b-quark in addition to an on-shell chargino whose decay occurs via a real or virtual W boson, or (ii) that the top squark decays to a t-quark and the lightest neutralino. A top squark with a mass between 150 GeV and 445 GeV decaying to a b-quark and an on-shell chargino is excluded at 95% confidence level for a top squark mass equal to the chargino mass plus 10 GeV, in the case of a 1 GeV lightest neutralino. Top squarks with masses between 215 (90) GeV and 530 (170) GeV decaying to an on-shell (off-shell) t-quark and a neutralino are excluded at 95% confidence level for a 1 GeV neutralino. [Figure not available: see fulltext.]
A search for top squarks with R-parity-violating decays to all-hadronic final states with the ATLAS detector in $ \sqrt{s}=8 $ TeV proton-proton collisions
A search for the pair production of top squarks, each with R -parity-violating decays into two Standard Model quarks, is performed using 17.4 fb -1 of √s=8 TeV proton-proton collision data recorded by the ATLAS experiment at the LHC. Each top squark is assumed to decay to a b- and an s-quark, leading to four quarks in the final state. Background discrimination is achieved with the use of b-tagging and selections on the mass and substructure of large-radius jets, providing sensitivity to top squark masses as low as 100 GeV. Finally, no evidence of an excess beyond the Standard Model background prediction is observed and top squarks decaying to $\overline{b}$$\overline{s}$ are excluded for top squark masses in the range 100 ≤ m $\overline{t}$ ≤ 315 GeV at 95% confidence level.
Search for microscopic black holes and string balls in final states with leptons and jets with the ATLAS detector at s $ \sqrt{s} $ = 8 TeV
A search for an excess of events with multiple high transverse momentum objects including charged leptons and jets is presented, using 20.3 fb -1 of proton-proton collision data recorded by the ATLAS detector at the Large Hadron Collider in 2012 at a centre-of-mass energy of $ \sqrt{s} $ = 8 TeV. No excess of events beyond Standard Model expectations is observed. Using extra-dimensional models for black hole and string ball production and decay, exclusion contours are determined as a function of the mass threshold for production and the fundamental gravity scale for two, four and six extra dimensions. For six extra dimensions, mass thresholds of 4.8-6.2 TeV are excluded at 95 % confidence level, depending on the fundamental gravity scale and model assumptions. Upper limits on the fiducial cross-sections for non-Standard Model production of these final states are set.
Search for production of vector-like quark pairs and of four top quarks in the lepton-plus-jets final state in pp collisions at √s = 8 TeV with the ATLAS detector
A search for pair production of vector-like quarks, both up-type (T) and down-type (B), as well as for four-top-quark production, is presented. The search is based on pp collisions at \( \sqrt{s}=8 \) TeV recorded in 2012 with the ATLAS detector at the CERN Large Hadron Collider and corresponding to an integrated luminosity of 20.3 fb –1 . Data are analysed in the lepton-plus-jets final state, characterised by an isolated electron or muon with high transverse momentum, large missing transverse momentum and multiple jets. Dedicated analyses are performed targeting three cases: a T quark with significant branching ratio to a W boson and a b-quark \( \left(T\overline{T}\to Wb+\mathrm{X}\right) \), and both a T quark and a B quark with significant branching ratio to a Higgs boson and a third-generation quark (\( T\overline{T}\to Ht+X\;\mathrm{and}\;B\overline{B}\to Hb+\mathrm{X} \) respectively). No significant excess of events above the Standard Model expectation is observed, and 95% CL lower limits are derived on the masses of the vector-like T and B quarks under several branching ratio hypotheses assuming contributions from T → Wb, Zt, Ht and B → Wt, Zb, Hb decays. The 95% CL observed lower limits on the T quark mass range between 715 GeV and 950 GeV for all possible values of the branching ratios into the three decay modes, and are the most stringent constraints to date. In addition, the most restrictive upper bounds on four-top-quark production are set in a number of new physics scenarios.
Search for direct pair production of the top squark in all-hadronic final states in proton-proton collisions at $ \sqrt{s} $ = 8 TeV with the ATLAS detector
The results of a search for direct pair production of the scalar partner to the top quark using an integrated luminosity of 20.1 fb -1 of proton-proton collision data at $ \sqrt{s} $ = 8 TeV recorded with the ATLAS detector at the LHC are reported. The top squark is assumed to decay via $ \bar{t} $ → t $ ^{-0} _ { χ_1 } $ or t → b $ ^{-±} _ { χ_1 } $ → bW(*)$ ^{-0} _ { χ_1 } $, where $ ^{-0} _ { χ_1 } $ ($ ^{-±} _ { χ_1 } $) denotes the lightest neutralino (chargino) in supersymmetric models. The search targets a fully-hadronic final state in events with four or more jets and large missing transverse momentum. No significant excess over the Standard Model background prediction is observed, and exclusion limits are reported in terms of the top squark and neutralino masses and as a function of the branching fraction of $ \bar{t} $ → t $ ^{-0} _ { χ_1 } $. For a branching fraction of 100%, top squark masses in the range 270-645 GeV are excluded for $ ^{-0} _ { χ_1 } $ masses below 30GeV. For a branching fraction of 50% to either $ \bar{t} $ → t $ ^{-0} _ { χ_1 } $ or $ \bar{t} $ → b $ ^{-±} _ { χ_1 } $, and assuming the $ ^{-±} _ { χ_1 } $ mass to be twice the $ ^{-0} _ { χ_1 } $ mass, top squark masses in the range 250-550 GeV are excluded for $ ^{-0} _ { χ_1 } $ masses below 60 GeV.
Search for squarks and gluinos with the ATLAS detector in final states with jets and missing transverse momentum using $\sqrt{s}=8 $ TeV proton-proton collision data
A search for squarks and gluinos in final states containing high-p T jets, missing transverse momentum and no electrons or muons is presented. The data were recorded in 2012 by the ATLAS experiment in $ \sqrt{s} $ = 8 TeV proton-proton collisions at the Large Hadron Collider, with a total integrated luminosity of 20.3 fb -1 . Results are interpreted in a variety of simplified and specific supersymmetry-breaking models assuming that R-parity is conserved and that the lightest neutralino is the lightest supersymmetric particle. An exclusion limit at the 95% confidence level on the mass of the gluino is set at 1330 GeV for a simplified model incorporating only a gluino and the lightest neutralino. For a simplified model involving the strong production of first- and second-generation squarks, squark masses below 850 GeV (440 GeV) are excluded for a massless lightest neutralino, assuming mass degenerate (single light-flavour) squarks. In mSUGRA/CMSSM models with tan β = 30, A 0 = -2m 0 and μ > 0, squarks and gluinos of equal mass are excluded for masses below 1700 GeV. Additional limits are set for non-universal Higgs mass models with gaugino mediation and for simplified models involving the pair production of gluinos, each decaying to a top squark and a top quark, with the top squark decaying to a charm quark and a neutralino. These limits extend the region of supersymmetric parameter space excluded by previous searches with the ATLAS detector.
Search for charged Higgs bosons decaying via H ± → τ ± ν τ in the τ+jets and τ+lepton final states with 36 fb -1 of $pp$ collision data recorded at $ \sqrt{s}=13 $ TeV with the ATLAS experiment
Charged Higgs bosons produced either in top-quark decays or in association with a top-quark, subsequently decaying via H ± → τ ± ν τ , are searched for in 36.1 fb -1 of proton-proton collision data at $ \sqrt{s}=13 $ TeV recorded with the ATLAS detector. Depending on whether the top-quark produced together with H ± decays hadronically or leptonically, the search targets τ+jets and τ+lepton final states, in both cases with a hadronically decaying τ-lepton. No evidence of a charged Higgs boson is found. For the mass range of mH ± = 90–2000 GeV, upper limits at the 95% confidence level are set on the production cross-section of the charged Higgs boson times the branching fraction β(H ± → τ ± ν τ ) in the range 4.2–0.0025 pb. In the mass range 90–160 GeV, assuming the Standard Model cross-section for $ t\bar{t} $ production, this corresponds to upper limits between 0.25% and 0.031% for the branching fraction β(t→bH ± )×β(H ± →τ ± ν τ ).
Search for direct third-generation squark pair production in final states with missing transverse momentum and two b-jets in root s=8 TeV pp collisions with the ATLAS detector
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Search for the direct production of charginos, neutralinos and staus in final states with at least two hadronically decaying taus and missing transverse momentum in pp collisions at $ \sqrt{s}=8 $ TeV with the ATLAS detector
We present results of a search for the electroweak associated production of charginos and next-to-lightest neutralinos, pairs of charginos or pairs of tau sleptons. These processes are characterised by final states with at least two hadronically decaying tau leptons, missing transverse momentum and low jet activity. The analysis is based on an integrated luminosity of 20.3 fb ₋1 of proton-proton collisions at √s = 8TeV recorded with the ATLAS experiment at the Large Hadron Collider. We observed no significant excess with respect to the predictions from Standard Model processes. Limits are set at 95% confidence level on the masses of the lighter chargino and next-to-lightest neutralino for various hypotheses for the lightest neutralino mass in simplified models. In the scenario of direct production of chargino pairs, with each chargino decaying into the lightest neutralino via an intermediate tau slepton, chargino masses up to 345 GeV are excluded for a massless lightest neutralino. For associated production of mass-degenerate charginos and next-tolightest neutralinos, both decaying into the lightest neutralino via an intermediate tau slepton, masses up to 410 GeV are excluded for a massless lightest neutralino.
Measurement of ZZ production in the ll nu nu final state with the ATLAS detector in pp collisions at root s=13 TeV
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