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At least 793 records · Page 44
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

The CLAS12 Forward Time-of-Flight system

The Forward Time-of-Flight system for the large-acceptance CLAS12 spectrometer in Hall B at the Thomas Jefferson National Accelerator Facility is described. The system is positioned at distances in the range from 6.2 m to 7.2 m from the beam–target interaction point and spans laboratory polar angles from 5 deg → 45 deg and nearly the full azimuth. The system consists of 540 individual scintillation counters with double-ended readout that range in length from 17 cm to 426 cm of discrete widths of 6 cm, 15 cm, and 22 cm, and of discrete thicknesses of 5 cm and 6 cm. We see the effective counter time resolution for passing charged particles varies from 50 ps for the shortest counters at small angles to 200 ps for the longest counters at large angles. The detectors are part of the forward-angle particle identification system for CLAS12 during offline event reconstruction and are a component of the online data acquisition trigger to select final state event topologies with forward-going charged particles.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

A modular apparatus for use in high-precision measurements of parity violation in polarized eV neutron transmission

We describe a modular apparatus for use in parity-violation measurements in epithermal neutron–nucleus resonances with high instantaneous neutron fluxes at the Manuel Lujan Jr. Neutron Scattering Center at Los Alamos National Laboratory. This apparatus is designed to conduct high-precision measurements of the parity-odd transmission asymmetry of longitudinally polarized neutrons through targets containing nuclei with p-wave neutron–nucleus resonances in the 0.1–10 eV energy regime and to accommodate a future search for time reversal violation in polarized neutron transmission through polarized nuclear targets. The apparatus consists of an adjustable neutron and gamma collimation system, a 3 He- 4 He ion chamber neutron flux monitor, two identical cryostats for target cooling, an adiabatic eV-neutron spin flipper, a near-unit efficiency 6 Li- 7 Li scintillation detector operated in current mode, a flexible CAEN data acquisition system, and a neutron spin filter based on spin-exchange optical pumping of 3 He gas. We describe the features of the apparatus design devoted to the suppression of systematic errors in parity-odd asymmetry measurements. We describe the configuration of the apparatus used to conduct a precision measurement of parity violation at the 0.7 eV p-wave resonance in 139 La which employs two identical 139 La targets, one to polarize the beam on the p-wave resonance using the weak interaction and one to analyze the polarization.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Characterization and pulse-shape discrimination of a multi-stacked structure of ZnS: Ag/PMMA for fast-neutron detection in high-flux environments

The Micro-Layered Fast Neutron Detector (MLFD) is a proton-recoil scintillator that incorporates the basic concept of a Hornyak button detector with an improved design using a layered structure of ZnS:Ag and PMMA (polymethyl methacrylate). The MLFD was predicted to have low sensitivity to gamma rays, hence pulse shape discrimination was performed to determine the gamma-ray contribution. Presented in this paper are the pulse-shape discrimination characteristics of the MLFD. Additionally, the charge integration technique was employed to discriminate between the neutrons and gamma rays using a fast digitzer. The MLFD was found to exhibit excellent neutron/gamma-ray discrimination, with the highest Figure-of-Merit (FoM) being 4.56. With PSD, the neutron signal is distinct from gamma-ray, Ĉerenkov and electronic noise signals. This clear separation was achieved due to the large differences in decay times of the neutron and gamma-ray-induced pulses in the ZnS:Ag phosphor. The MLFD can be employed in high gamma-ray exposure fields, up to at least 1287.7 mR/hr, without appreciable degradation in PSD performance.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

A position and pulse shape discriminant p -terphenyl detector module

We present the development of a neutron detector array module made with para-terphenyl, a bright, fast, n/γ discriminating crystalline organic scintillator. The module is comprised of 2 cm × 2 cm × 2 cm p-terphenyl crystals that have been optically coupled together to create a pseudo-bar module. While only relying on two photo detectors, the module is capable of distinguishing interactions between up to eight crystals. Furthermore, the module retains the p-terphenyl’s pulse shape discrimination (PSD) capability. Together this makes the pseudo-bar module a promising position-sensitive neutron detector. Here we present characteristics of the pseudo-bar module - its timing resolution as well as its pulse shape and position discrimination capabilities, and briefly discuss future plans for utilizing an array of pseudo-bar modules in a useful neutron detector system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

A compact neutron spectrometer system

A portable neutron spectrometer, nSpec, has been developed for passive interrogation of fast neutrons ( 1 MeV) from neutron sources. The design of the system includes four EJ-301 liquid scintillation cells, a custom stand, and tungsten caps for gamma-ray shielding. Data acquisition settings were optimized to provide a dynamic range of up to > 15 MeV neutron energy. Additionally, the detector response matrix was characterized using a time-of-flight method based on gamma-ray tagged neutron emission from 252 Cf. The spectrum unfolding was characterized using measured and simulated spectra of AmBe and 252 Cf with the GRAVEL and MLEM methods. Monte Carlo methods were used to examine the uncertainty propagation and determine sufficient counts for a measurement.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Quantifying spatial resolution in a fast neutron radiography system

Neutron imaging is a powerful nondestructive examination modality that has been employed in various applications. Fast neutrons provide advantages over lower energy neutrons, such as examining thicker samples and inducing negligible activation and transmutations. However, fast neutrons interact mostly via elastic scattering with both the neutron detector and the object, causing degradation in spatial resolution. This study explores the quantification of spatial resolution caused by the testing target itself and suggests proper candidate materials for characterizing spatial resolution in terms of modulation transfer function. Knife-edge radiographs of 3 mm, 6 mm, and 5 cm thick Tantalum (Ta) foils, and a 2.54 cm Tungsten (W) cube were acquired using a CCD-based imaging system and a Polyvinyl Toluene (PVT) scintillator at the Ohio State Research Reactor (OSURR)’s fast neutron beam facility. The spatial resolutions calculated were 195 ± 20 μm, 224 ± 22 μm, 248 ± 25 μm, and 435 ± 44 μm for 3 mm, 6 mm, and 5 cm Ta foils, and 2.54 cm W cube, respectively. The results showed a worsening spatial resolution with increasing target thickness. Simulations and calculations estimate that elastic scattering kinematics between neutrons and protons in the PVT medium also limits spatial resolution, and it sets a lower limit of ~44 μm on the spatial resolution for 2 MeV neutrons.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

CLARION2-TRINITY: A Compton-suppressed HPGe and GAGG:Ce-Si-Si array for absolute cross-section measurements with heavy ions

The design and performance of a new Compton-suppressed HPGe and charged-particle array, CLARION2-TRINITY, are described. The TRINITY charged-particle array is comprised of 64 Cerium-doped Gadolinium Aluminum Gallium Garnet (GAGG:Ce) crystals configured into five rings spanning 7–54 degrees, and two annular silicon detectors that can shadow or extend the angular coverage to backward angles with minimal $\gamma$-ray attenuation. GAGG:Ce is a non-hygroscopic, bright, and relatively fast scintillator with a light distribution well matched to SiPMs. Count rates up to 40 kHz per crystal are sustainable. Fundamental characteristics of GAGG:Ce are measured and presented, including light- and heavy-ion particle identification (PID) capability, pulse-height defects, radiation hardness, and emission spectra. The CLARION2 array consists of up to 16 Compton-suppressed HPGe Clover detectors (efficiency at 1 MeV) configured into four rings (eight HPGe crystal rings) using a non-Archimedean geometry that suppresses back-to-back coincident 511-keV gamma rays. The entire array is instrumented with 100- and 500-MHz (14 bit) waveform digitizers which enable triggerless operation, pulse-shape discrimination, fast timing, and pileup correction. Lastly, two examples of experimental data taken during the commissioning of the CLARION2-TRINITY system are given: a PID spectrum from 16 O + 18 O fusion-evaporation, and PID and Doppler-corrected -ray spectra from 48 Ti + 12 C Coulomb excitation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Advancements of the nSpec system

For this study, a new characterization of the detector response for the EJ301 liquid scintillator based nSpec system has been conducted at the Los Alamos Neutron Science Center. The new characterization was accomplished in two orders of magnitude less time and with better statistics than the previous characterization. The new and old characterization methods were compared by conducting both types of characterization on two detectors (one EJ301 and one EJ301D). The two methods show consistent results and compare well to results previously published in the literature; however, the results from the characterization of the original nSpec detector show discrepancies that have been identified as being caused by oxygen being absorbed into the detector due to a leak. The new characterized detector response shows improved spectrum unfolding performance than the previous characterization. The cross talk of the detector system was also characterized as a function of incident neutron energy and found to have a negligible impact on spectrum unfolding results. Alternative materials (EJ301D and stilbene) were also characterized in a first step towards an upgraded system. The different materials show little difference in unfolding performance, but the comparison is ongoing. A SiPM based stilbene detector was used to evaluate the use of SiPMs in a future system upgrade. The SiPM provides adequate performance, but the custom SiPM readout results in a much longer pulse width than PMT based systems. The measured light output of the SiPM based stilbene compares well with the results in literature. Future work will look at additional materials (deuterated stilbene and organic glass) and optimizing the SiPM readout to decrease the pulse width.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Systematic evaluation of fast neutron sensing with Cesium Hafnium Chloride

Cesium Hafnium Chloride (CHC) is a promising new scintillator for dual mode sensing of both neutrons and gamma-rays. The high chlorine content allows for both 35 Cl(n,p) 35 S and 35 Cl(n,α) 32 P reaction channels leading to reliable detection of fast neutrons. By utilizing pulse shape discrimination (PSD), these neutron interactions may be reliably separated from gamma-ray signals with a high figure-of-merit (FOM) after optimization of the PSD algorithm. Here, in this study, the PSD algorithm settings for CHC were systematically investigated using a bare 252 Cf and a lead shielded plutonium beryllium neutron source. It was found that the PSD algorithm settings affects both the FOM and the neutron detection efficiency, but a FOM as high as 4.5 for alpha particles was observed in one data processing scenario. Further, an intrinsic 5 parts per million alpha emitting contamination was observed in the sample, which we attribute to natural uranium.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Determination of energy-dependent neutron backgrounds using shadow bars

Understanding the neutron background is essential for determining the neutron yield from nuclear reactions. Here, the neutron backgrounds were determined for heavy-ion collision experiment using the shadow-bar method, where beams of 40,48 Ca at 56, 140 MeV/u impinged on targets of 58,64 Ni and 112,124 Sn. In the analysis presented here, brass shadow bars are placed in front of organic liquid scintillator neutron detectors to determine the energy-dependent neutron background fractions. The measurement of neutron spectra with and without shadow bars is important to determine the neutron background more accurately. The neutron background, along with its sources and systematic uncertainties, are explored with a focus on the impact of background models and their dependence on neutron energy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Development of a compact fast-neutron spectrometer for nuclear emergency response applications

We have developed a Compact Fast Neutron Spectrometer (CFNS) for passive assay of special nuclear material (SNM) through the observation of fast neutrons. The CFNS consists of eight organic glass scintillators (OGS) coupled to silicon photomultipliers and a waveform digitizer, which are integrated within a human-portable box. The CFNS determines the neutron energy profile by spectrum unfolding using the Maximum-Likelihood Expectation Maximization method. The detector acquisition system was optimized to have a dynamic range of up to 10 MeV neutron energy. Bulk special nuclear material (SNM) measurements from the National Criticality Experiments Research Center were analyzed for SNM validation/examination. Additionally, the results show that the CFNS can be used to distinguish between fission and (α, n) neutron emitters, regardless of intervening material type (Cu and polyethylene) and thickness, by taking the ratio of neutron counts at different regions in the unfolded energy spectrum. Additionally, by fitting an exponential curve to the unfolded energy spectrum of PuO 2 and Pu neutron emitters, the CFNS showed the ability of distinguishing between pure Pu oxide, pure Pu metal and mixed oxide-metal configurations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Sub-millimeter resolution SiPM-based neutron anger camera

Thermal and cold neutron beamlines require detector systems that have a high neutron efficiency, large active area, and good spatial resolution. One type of detector that has been implemented at beamlines at the Spallation Neutron Source (SNS) is a scintillator-based Anger camera that utilizes photomultiplier tubes (PMTs) as photodetectors. In this work, we present a new Anger camera design that replaces PMTs with silicon photomultipliers (SiPMs). This new design offers better resolution, less distortion, and more compactness than the previous cameras. A camera with active area of ~100 cm 2 was shown to have a spatial resolution better than 0.5 mm. Additionally, the use of SiPMs allows for use in strong magnetic fields, opening the possibility of additional experimental capabilities. In conclusion, prototype has been built that demonstrates vacuum-compatibility, as required for a proposed beamline for the Second Target Station at SNS.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Quantification of the light output anistropy in deuterated stilbene

Deuterated stilbene is an organic scintillator that is a desirable material for fast neutron spectroscopy using spectrum unfolding techniques without requiring time-of-flight information. Due to the crystal structure of the material, some anisotropy of the light output exists, which is dependent on the direction of heavy charged particle recoil relative to the crystal structure. The anisotropy of trans-stilbene (hereafter referred to as stilbene) has been well characterized in previous work, but for deuterated stilbene, the anisotropy has only been partially characterized along the a and b crystal axes, while the artificial c' axis, which shows the largest anisotropy in stilbene, has not been characterized until this publication. Here, in this work, two deuterated stilbene crystals were characterized with neutron energies up to 35 MeV at the Los Alamos Neutron Science Center. For one of the crystals, the response is characterized along the a, b, and c' axes. This characterization shows a distinct anisotropy along the axes in deuterated stilbene, which is very similar to that found in regular stilbene, such that the a axis is the brightest, while the b' and c' axes are approximately 3% and 20%–35% lower relative to the a axis.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Evaluation of the performance of event reconstruction algorithms in the JSNS 2 experiment using a 252 Cf calibration source

JSNS 2 investigates short-baseline neutrino oscillations using a 24-meter baseline and a 17-tonne Gd-loaded liquid scintillator target. Accurate event-reconstruction algorithms are crucial for analyzing experimental data. The algorithms undergo meticulous validation through calibration with a 252 Cf source. This paper outlines the methodology and evaluates the reconstruction performance, focusing on neutrino interactions up to approximately 50 MeV for sterile neutrino searches. Both 252 Cf and Michel electron events are studied to evaluate reconstruction accuracy. The analysis concludes that the uncertainty of the fiducial volume, with an appropriate correction, is much less than the requirement of JSNS 2 requirement (10%). Furthermore, the energy resolution is measured to be 3.3 ± 0.1% for the Michel electron endpoint and 4.3 ± 0.1% for the n-Gd peak in the central region.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Thermal neutron imaging detector with wavelength shifting fiber and digital readout

Here, we developed a large area, digital thermal neutron imaging detector. The detector uses a 6 LiF/ZnS(Ag) neutron-sensitive scintillator combined with wavelength shifting fiber technology. The signals from fiber channels are amplified, integrated, and digitized using individual analog-to-digital converters for each channel. The neutron position is determined from the digitized signal using a least-squares gaussian-fitting algorithm. The detector size was 77 × 38 cm 2 (2926 cm 2 ), it provided 1.3 mm resolution, and its resolution can further be improved. The detector was designed for a powder diffraction neutron scattering beamline and provided substantial improvement of d-space resolution compared with existing detectors. This detector may have broader applications due to its large area and high spatial resolution extended over its large area.

6LiF/ZnS(Ag) scintillator↗
DOE OSTI2025

Multiple Coulomb scattering in acrylic of a 221.3 MeV therapeutic proton beam

Measurements of multiple Coulomb scattering (MCS) distributions for 221.3 MeV therapeutic protons are presented using a novel detector system comprised of a thin scintillator, a pellicle mirror, and a digital camera. The MCS distributions were characterized for three acrylic phantoms of varying lengths and for two biological density-equivalent phantoms simulating bone and muscle. Additionally, beam profiles were measured across an energy range of 80.3–221.3 MeV in 20 MeV increments. The observed energy dependence of the photon yields is consistent with the tabulated stopping power values. Finally, the experimental results are benchmarked against Geant4 simulations, demonstrating consistent agreement and validating the capability of the detector system for radiology measurements.

Digital camera↗
DOE OSTI2025

Evaluating Brightness and Stability of Cathodoluminescence from Colloidal Semiconductor Nanocrystals

Cathodoluminescence offers promise as a technique for correlation of atomic structure with electronic structure at the level of individual nanoparticles or even defects, with the ability to analyze complex nanostructures at length-scales far below those typically available to optical spectroscopy. Unlike other forms of electron microscopy, cathodoluminescence offers direct insights into the electronic structure of the visualized sample. Despite reports more than 10 years ago of individual nanoparticle cathodoluminescence, effective cathodoluminescence collection from colloidal semiconductor materials is relatively rare and remains challenging due to the instability of materials under the conditions of electron beam irradiation. In this work, to clarify the roadblocks for cathodoluminescence analysis of colloidal nanocrystals, we attempt a comprehensive study of the cathodoluminescence properties of semiconductor quantum shells, which have a thin concentric CdSe shell surrounding CdS nanoparticles, then surrounded by a further concentric CdS shell. These same materials were recently demonstrated to show promising scintillation performance in radioluminescence measurements, including high brightness (up to 100 ph/keV) and excellent durability. Comparative quantum yield measurements are designed to assess the brightness of semiconductor nanocrystal films, which show that the quantum shells are much less bright under electron irradiation compared to X-ray photons. Instability of CL emission is assigned to charging effects on the samples—and not thermal effects—through a series of voltage, current, dwell time, and atmospheric pressure experiments.

cathodoluminescence↗
DOE OSTI2025

Effects of Quantum Dot Loading on the Radioluminescence Efficiency in Quantum-Dot-Embedded Composites

Nanoparticle-embedded plastic scintillators are an emerging technology for fast, large-area, high-resolution radiation detection and imaging. Here, this study investigates the properties of such composites, focusing on the effects of the quantum dot (QD) concentration on the radioluminescence (RL) intensity, spectra, and dynamics. Experiments using CdSe/CdS QDs in a polymer reveal a superlinear increase in RL with the QD concentration despite optical losses from inner filtering and interparticle interactions. When corrected for inner filtering, RL shows a quadratic concentration dependence, consistent with simple analytical models of improving the secondary electron capture. Practically, the benefits of high QD concentrations are muted by optical losses, but the findings apply to other systems with insulating hosts. In addition to manipulating emission for large effective Stokes shifts, future improvements may come from hosts with higher stopping power and better charge transport, which enable more effective funneling of excitations but without concomitant optical losses associated with high nanoparticle concentrations.

Auger recombination↗