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At least 793 records · Page 44

Improving climate model coupling through a complete mesh representation: a case study with E3SM (v1) and MOAB (v5.x)

One of the fundamental factors contributing to the spatiotemporal inaccuracy in climate modeling is the mapping of solution field data between different discretizations and numerical grids used in the coupled component models. The typical climate computational workflow involves evaluation and serialization of the remapping weights during the preprocessing step, which is then consumed by the coupled driver infrastructure during simulation to compute field projections. Tools like Earth System Modeling Framework (ESMF) and TempestRemap offer capability to generate conservative remapping weights, while the Model Coupling Toolkit (MCT) that is utilized in many production climate models exposes functionality to make use of the operators to solve the coupled problem. However, such multistep processes present several hurdles in terms of the scientific workflow and impede research productivity. In order to overcome these limitations, we present a fully integrated infrastructure based on the Mesh Oriented datABase (MOAB) library, which allows for a complete description of the numerical grids and solution data used in each submodel. Through a scalable advancing-front intersection algorithm, the supermesh of the source and target grids are computed, which is then used to assemble the high-order, conservative, and monotonicity-preserving remapping weights between discretization specifications. The Fortran-compatible interfaces in MOAB are utilized to directly link the submodels in the Energy Exascale Earth System Model (E3SM) to enable online remapping strategies in order to simplify the coupled workflow process. We demonstrate the superior computational efficiency of the remapping algorithms in comparison with other state-of-the-science tools and present strong scaling results on large-scale machines for computing remapping weights between the spectral element atmosphere and finite volume discretizations on the polygonal ocean grids.

58 GEOSCIENCES↗

Changes in the Regional Water Cycle and Their Impact on Societies

ABSTRACT Changes in “blue water”, which is the total supply of fresh water available for human extraction over land, are quite closely related to changes in runoff or equivalently precipitation minus evaporation, . This article examines how climate change‐driven recent past and future changes in the regional water cycle relate to blue water availability and changes in human blue water demand. Although at the largest scales theoretical and numerical model predictions are in broad agreement with observations, at continental scales and below models predict large ranges of possible future and runoff especially at the scale of individual river catchments and for shorter timescale subseasonal floods and droughts. Nevertheless, it is expected that the occurrence and severity of floods will increase and that of droughts may increase, possibly compounded by human‐driven non‐climatic changes such as changes in land use, dam water impoundment, irrigation and extraction of groundwater. Contemporary assessments predict that increases in 21st century human water extraction in many highly‐populated regions are unlikely to be sustainable given projections of future . To reduce uncertainty in future predictions, there is an urgent need to improve modeling of atmospheric, land surface and human processes and how these components are coupled. This should be supported by maintaining the observing network and expanding it to improve measurements of land surface, oceanic and atmospheric variables. This includes the development of satellite observations stable over multiple decades and suitable for building reanalysis datasets appropriate for model evaluation.

54 ENVIRONMENTAL SCIENCES↗

Insights into the year-round vertical distribution of chlorophyll concentration in high-latitude Arctic Ocean: implications for primary production

Climate-induced rapid changes in the Arctic Ocean, such as decreasing sea ice extent and increasing water temperature, are altering nutrient and light availability, profoundly impacting primary producer growth. However, access to the high-latitude Arctic Ocean is limited, and satellite data are primarily available only during summer, making continuous in-situ data collection challenging. We collected year-round chlorophyll-a (Chl-a) concentration data in high-latitude regions using a mooring system and performed a comparative analysis with reanalysis data. Unlike previous satellite-based studies, which typically rely on surface measurements, we used the annual vertical distribution of Chl-a. These data were applied to the vertically generalized production model to accurately estimate annual primary production. The moored Chl-a concentration data showed that phytoplankton exhibited a typical subsurface chlorophyll maximum (SCM) layer as sea ice retreated in June. Contrary to the gradually deepening SCM distribution predicted by model-based reanalysis data, the SCM layer persisted for approximately 4 months. This indicates that light and nutrient conditions within the SCM layer remained stable, sustaining continuous phytoplankton growth. Annual primary production, reflecting this vertical distribution of Chl-a concentration, was 6.85 gC m −2 yr −1 . This exceeded satellite-based estimates by at least two-fold, highlighting the significant underestimation of primary production by satellite approaches. Estimating primary production while accounting for the vertical distribution of phytoplankton and light is essential for improving ecological models to better understand carbon cycle and food web changes in the Arctic Ocean, with important implications for climate change predictions.

Arctic Ocean↗

Inline small-angle X-ray scattering-coupled chromatography under extreme hydrostatic pressure

As continuing discoveries highlight the surprising abundance and resilience of deep ocean and subsurface microbial life, the effects of extreme hydrostatic pressure on biological structure and function have attracted renewed interest. Biological small-angle X-ray scattering (BioSAXS) is a widely used method of obtaining structural information from biomolecules in solution under a wide range of solution conditions. Due to its ability to reduce radiation damage, remove aggregates, and separate monodisperse components from complex mixtures, size-exclusion chromatography-coupled SAXS (SEC-SAXS) is now the dominant form of BioSAXS at many synchrotron beamlines. While BioSAXS can currently be performed with some difficulty under pressure with non-flowing samples, it has not been clear how, or even if, continuously flowing SEC-SAXS, with its fragile media-packed columns, might work in an extreme high-pressure environment. Here we show, for the first time, that reproducible chromatographic separations coupled directly to high-pressure BioSAXS can be achieved at pressures up to at least 100 MPa and that pressure-induced changes in folding and oligomeric state and other properties can be observed. Further, the apparatus described here functions at a range of temperatures (0°C–50°C), expanding opportunities for understanding biomolecular rules of life in deep ocean and subsurface environments.

59 BASIC BIOLOGICAL SCIENCES↗

Diurnal cycle of precipitation over global monsoon systems in CMIP6 simulations

Accurate simulation of the diurnal cycle of precipitation over different climate regimes, including global monsoon systems, is an ongoing challenge for current state-of-the-art climate models. Here, in this study, the diurnal cycles of summertime precipitation from 21 CMIP6 historical simulations are evaluated with the NASA IMERG data via the diurnal harmonic amplitude and phase from the Fourier analysis in seven regional monsoon systems: Northern and Southern Africa monsoons, South Asia monsoon, East Asia monsoon, Australia monsoon, and North and South America monsoons. Particularly, we focus on four subregions including ocean, coastal ocean, land, and coastal land considering the different underlying physical processes. It is found that the CMIP6 historical simulations perform fairly well on reproducing the diurnal cycle of precipitation over ocean and coastal ocean, while the simulated diurnal harmonic phase and amplitude over land and coastal land show larger biases and model spread compared to biases over ocean and coastal ocean. The simulation of precipitation diurnal cycle is substantially improved in the multi-model mean of both CMIP6 historical and CMIP6 AMIP simulations compared with that of CMIP5 historical simulations. But the model bias of precipitation diurnal cycle is in general similar between CMIP6 AMIP and CMIP6 historical simulations, which suggests that the impact of the interactive ocean on the simulated diurnal precipitation averaged over a large domain is generally minor. The influence of model resolution on the diurnal cycle is shown in mixed directions across various subregions, and significant improvement from the low- to high-resolution models is only notable over coastal ocean.

54 ENVIRONMENTAL SCIENCES↗

Tropical Cirrus in Global Storm-Resolving Models. Part II: Cirrus Life Cycle and Top-of-Atmosphere Radiative Fluxes

Cirrus clouds of various thicknesses and radiative characteristics extend over much of the tropics, especially around deep convection. They are difficult to observe due to their high altitude and sometimes small optical depths. They are also difficult to simulate in conventional global climate models, which have coarse grid spacings and simplified parameterizations of deep convection and cirrus formation. We investigate the representation of tropical cirrus in global storm-resolving models (GSRMs), which have higher spatial resolution and explicit convection and could more accurately represent cirrus cloud processes. This study uses GSRMs from the DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains (DYAMOND) project. The aggregate life cycle of tropical cirrus is analyzed using joint albedo and outgoing longwave radiation (OLR) histograms to assess the fidelity of models in capturing the observed cirrus cloud populations over representative tropical ocean and land regions. The proportions of optically-thick deep convection, anvils, and cirrus vary across models and are portrayed in the vertical distribution of cloud cover and top-of-atmosphere radiative fluxes. Model differences in cirrus populations, likely driven by subgrid processes such as ice microphysics, dominate over regional differences between convectively-active tropical land and ocean locations.

54 ENVIRONMENTAL SCIENCES↗

Multiscale Temporal Variability of the Global Air‐Sea CO 2 Flux Anomaly

Abstract The global air‐sea CO 2 flux (F) impacts and is impacted by a plethora of climate‐related processes operating at multiple time scales. In bulk mass transfer formulations, F is driven by physico‐ and bio‐chemical factors such as the air‐sea partial pressure difference (∆pCO 2 ), gas transfer velocity, sea surface temperature, and salinity–all varying at multiple time scales. To de‐convolve the impact of these factors on variability in F at different time scales, time‐resolved estimates of F were computed using a global data set assembled between 1988 and 2015. The F anomalies were defined as temporal deviations from the 28‐year time‐averaged value. Spectral analysis revealed four dominant timescales of variability in F–subseasonal, seasonal, interannual, and decadal with relative amplitude differences varying across regions. A second‐order Taylor series expansion was then conducted along these four timescales to separate drivers across differing regions. The analysis showed that on subseasonal timescales, wind speed variability explains some 66% of the global F anomaly and is the dominant driver. On seasonal, interannual, and decadal timescales, the ∆pCO 2 effect controlled by the ∆pCO 2 anomaly, explained much of the F anomaly. On decadal timescales, the F anomaly was almost entirely governed by the ∆pCO 2 effect with large contributions from high latitudes. The main drivers across timescales also dominate the regional F anomaly, particularly in the mid‐high latitude regions. Finally, the driver of the ∆pCO 2 effect was closely connected with the relative strength of atmospheric pCO 2 and the nonthermal component of oceanic pCO 2 anomaly associated with dissolved inorganic carbon and alkalinity.

Environmental Sciences & Ecology↗

The Influence of Air‐Sea CO 2 Disequilibrium on Carbon Sequestration by the Ocean's Biological Pump

Abstract The ocean's biological carbon pump (BCP) affects the Earth's climate by sequestering CO 2 away from the atmosphere for decades to millennia. One primary control on the amount of carbon sequestered by the biological pump is air‐sea CO 2 disequilibrium, which is controlled by the rate of air‐sea CO 2 exchange and the residence time of CO 2 in surface waters. Here, we use a data‐assimilated model of the soft tissue BCP to quantify carbon sequestration inventories and time scales from remineralization in the water column to equilibration with the atmosphere. We find that air‐sea CO 2 disequilibrium enhances the global biogenic carbon inventory by ∼35% and its sequestration time by ∼70 years compared to identical calculations made assuming instantaneous air‐sea CO 2 exchange. Locally, the greatest enhancement occurs in the subpolar Southern Ocean, where air‐sea disequilibrium increases sequestration times by up to 600 years and the biogenic dissolved inorganic carbon inventory by >100% in the upper ocean. Contrastingly, in deep‐water formation regions of the North Atlantic and Antarctic margins, where biological production creates undersaturated surface waters which are subducted before fully equilibrating with the atmosphere, air‐sea CO 2 disequilibrium decreases the depth‐integrated sequestration inventory by up to ∼150%. The global enhancement of carbon sequestration by air‐sea disequilibrium is particularly important for carbon respired in deep waters that upwell in the Southern Ocean. These results highlight the importance of accounting for air‐sea CO 2 disequilibrium when evaluating carbon sequestration by the biological pump and for assessing the efficacy of ocean‐based CO 2 removal methods.

Environmental Sciences & Ecology↗

Trends in Warm Season Mesoscale Convective Systems Over Asia in 2001–2020

Mesoscale convective systems (MCSs) frequently occur over Asia during the warm season, often producing intense precipitation with associated socioeconomic impacts. Here we reveal significant trends in MCS occurrence frequency and related precipitation in Asia during the warm season (March–September) in 2001–2020, using a tracking method that combines cloud and precipitation criteria with high-resolution satellite data from the Global Precipitation Measurement mission. To examine whether there are differences between MCSs of different scales, both meso-α scales (MαCSs) and meso-β scales (MβCSs), with horizontal scales of 200–2,000 km and 20–200 km, are tracked. The distribution pattern of frequency and related precipitation of both MαCSs and MβCSs are quite similar and manifest positive trends over East Asia (EA) and Northeast Asia, and negative trend over Southeast Asia (SEA). The MCS precipitation trend contributes significantly to total precipitation trend, with MαCSs contributing the most. Our analysis indicates the trend in lower-tropospheric water vapor flux convergence has a similar spatial pattern to the MCS frequency and related precipitation trend. Based on an atmospheric moisture flux decomposition analysis, the water vapor flux convergence trend can largely be explained by the change in horizontal wind convergence, while the specific humidity trend driven largely by temperature change plays a minor role. In conclusion, the trend in wind convergence in EA and SEA is possibly related to the evident trend in the lower-tropospheric anticyclone over the western North Pacific and SEA, which might be due to the relatively stronger warming in the Indian Ocean during the past two decades.

54 ENVIRONMENTAL SCIENCES↗

Delayed coastal inundations caused by ocean dynamics post-Hurricane Matthew

Post Hurricane Abnormal Water Level (PHAWL) poses a persistent inundation threat to coastal communities, yet unresolved knowledge gaps exist regarding its spatiotemporal impacts and causal mechanisms. Using a high-resolution coastal model with a set of observations, we find that the PHAWLs are up to 50 cm higher than the normal water levels for several weeks and cause delayed inundations around residential areas of the U.S. Southeast Coast (USSC). Numerical experiments reveal that while atmospheric forcing modulates the coastal PHAWLs, ocean dynamics primarily driven by the Gulf Stream control the mean component and duration of the shelf-scale PHAWLs. Because of the large spatial impact of the post-hurricane oceanic forcing, the coastal hazards are not limited to a direct hit from a hurricane but can be detected throughout the USSC where the oceanic processes reach.

54 ENVIRONMENTAL SCIENCES↗

Heterotrophic Thaumarchaea with Small Genomes Are Widespread in the Dark Ocean

The Thaumarchaeota is a diverse archaeal phylum comprising numerous lineages that play key roles in global biogeochemical cycling, particularly in the ocean. To date, all genomically characterized marine thaumarchaea are reported to be chemolithoautotrophic ammonia oxidizers. In this study, we report a group of putatively heterotrophic marine thaumarchaea (HMT) with small genome sizes that is globally abundant in the mesopelagic, apparently lacking the ability to oxidize ammonia. We assembled five HMT genomes from metagenomic data and show that they form a deeply branching sister lineage to the ammonia-oxidizing archaea (AOA). We identify this group in metagenomes from mesopelagic waters in all major ocean basins, with abundances reaching up to 6% of that of AOA. Surprisingly, we predict the HMT have small genomes of ~1 Mbp, and our ancestral state reconstruction indicates this lineage has undergone substantial genome reduction compared to other related archaea. The genomic repertoire of HMT indicates a versatile metabolism for aerobic chemoorganoheterotrophy that includes a divergent form III-a RuBisCO, a 2M respiratory complex I that has been hypothesized to increase energetic efficiency, and a three-subunit heme-copper oxidase complex IV that is absent from AOA. We also identify 21 pyrroloquinoline quinone (PQQ)-dependent dehydrogenases that are predicted to supply reducing equivalents to the electron transport chain and are among the most highly expressed HMT genes, suggesting these enzymes play an important role in the physiology of this group. Our results suggest that heterotrophic members of the Thaumarchaeota are widespread in the ocean and potentially play key roles in global chemical transformations.

59 BASIC BIOLOGICAL SCIENCES↗

The Cryosphere/Ocean Distributed Acoustic Sensing (CODAS) Experiment

Distributed acoustic sensing (DAS) has a demonstrated potential for wide-scale and continuous in situ monitoring of near-surface environmental and anthropogenic processes. DAS is attractive for development as a multi-geophysical observatory due to the prevalence of existing fiber infrastructure in regions with environmental, cultural, or strategic significance. To evaluate the efficacy of this technology for monitoring of polar environmental processes, we collected DAS data from a 37-km long section of seafloor telecommunications fiber located on the continental shelf of the Beaufort Sea, Alaska. This experiment spanned eight, one-week, seasonally-distributed periods across two years. This was the first ever deployment of seafloor DAS beneath sea ice, and the first deployment in any marine environment to span multiple seasons. We recorded a variety of environmental and anthropogenic signals with demonstrable utility for the study of sea ice dynamics and tracking of ocean vessels and ice-traversing vehicles.

54 ENVIRONMENTAL SCIENCES↗

Information Entropy as Quantifier of Potential Predictability in the Tropical Indo-Pacific Basin

Global warming is posed to modify the modes of variability that control much of the climate predictability at seasonal to interannual scales. The quantification of changes in climate predictability over any given amount of time, however, remains challenging. Here we build upon recent advances in non-linear dynamical systems theory and introduce the climate community to an information entropy quantifier based on recurrence. The entropy, or complexity of a system is associated with microstates that recur over time in the time-series that define the system, and therefore to its predictability potential. A computationally fast method to evaluate the entropy is applied to the investigation of the information entropy of sea surface temperature in the tropical Pacific and Indian Oceans, focusing on boreal fall. In this season the predictability of the basins is controlled by two regularly varying non-linear oscillations, the El Niño-Southern Oscillation and the Indian Ocean Dipole. We compute and compare the entropy in simulations from the CMIP5 catalog from the historical period and RCP8.5 scenario, and in reanalysis datasets. Discrepancies are found between the models and the reanalysis, and no robust changes in predictability can be identified in future projections. The Indian Ocean and the equatorial Pacific emerge as troublesome areas where the modeled entropy differs the most from that of the reanalysis in many models. A brief investigation of the source of the bias points to a poor representation of the ocean mean state and basins' connectivity at the Indonesian Throughflow.

54 ENVIRONMENTAL SCIENCES↗

Global Precipitation Experiment—A New World Climate Research Programme Lighthouse Activity

The future state of the global water cycle and the prediction of freshwater availability for humans around the world remain among the challenges of climate research and are relevant to several United Nations Sustainable Development Goals. The Global Precipitation Experiment (GPEX) takes on the challenge of improving the prediction of precipitation quantity, phase, timing, and intensity, characteristics that are products of a complex integrated system. It will achieve this by leveraging existing World Climate Research Programme (WCRP) activities and community capabilities in satellite, surface-based, and airborne observations, modeling, and experimental research and by conducting new and focused activities. It was launched in October 2023 as a WCRP Lighthouse Activity. Here, we present an overview of the GPEX Science Plan that articulates the primary science questions related to precipitation measurements, process understanding, model performance and improvements, and plans for capacity development. The central phase of GPEX is the WCRP Years of Precipitation for 2–3 years with coordinated global field campaigns focusing on different storm types (atmospheric rivers, mesoscale convective systems, monsoons, and tropical cyclones, among others) over different regions and seasons. Activities are planned over the three phases (before, during, and after the Years of Precipitation) spanning a decade. These include gridded data evaluation and development, advanced modeling, enhanced understanding of processes critical to precipitation, multiscale prediction of precipitation events across scales, and capacity development. These activities will be further developed as part of the GPEX Implementation Plan.

Climate change↗

2020 State of the Science Report, Chapter 7: Changes in Oceanographic Systems Associated with Marine Renewable Energy Devices

Oceanographic processes define the marine environment: the flow of water determines the concentrations of dissolved gases and nutrients, transports sediments, and maintains the habitats and water quality that support marine organisms and healthy ecosystems. Important physical processes in the ocean include, but are not limited to, tidal circulation and basin flushing, wave action, local and basin-scale ocean currents, temperature and salinity gradients, sediment transport forming and shaping coastlines, and the exchange of heat and dissolved gases at the air-water interface. Harnessing energy with marine renewable energy (MRE) devices has the potential to affect these processes in both the nearfield (within a few device lengths) and the farfield (farther from the device, from the scale of multiple devices to the scale of an enclosed basin) by removing energy from the system, changing natural flow patterns around devices, and/or decreasing wave heights. https://tethys.pnnl.gov/publications/state-of-the-science-2020-chapter-7-oceanographic-systems

54 ENVIRONMENTAL SCIENCES↗

Impacts of projected changes in sea surface temperature on ozone pollution in China toward carbon neutrality

The global sea surface temperatures (SSTs) are expected to change diversely in the future under different climate scenarios, which will affect the near-surface ozone (O 3 ) distribution and concentration by influencing meteorological states and large-scale atmospheric circulation. Many countries have planned to reach carbon neutrality by the mid-21st century. Here in this study, the impacts of global and regional SST changes on near-surface O 3 concentrations in China in the middle of the 21st century under the carbon-neutral scenario (Shared Socioeconomic Pathway 1-1.9), compared with the high-emission scenario (Shared Socioeconomic Pathway 5-8.5), and possible physical and chemical mechanisms are investigated using the Community Earth System Model version 1 (CESM1). Under future climate change, the changes in SSTs in the carbon-neutral scenario relative to the high-emission scenario lead to a dipole change in near-surface O 3 concentrations in eastern and western China, with a significant decrease of 0.79 ppbv in the eastern China and a significant increase of 1.05 ppbv in the western China. The cooling of North Pacific Ocean under the carbon-neutral scenario causes a decrease in near-surface O 3 concentrations by 0.48 ppbv in eastern China due to the weakened chemical production and an increase by 0.74 ppbv in western China attributed to the enhanced O 3 transport from Eurasia. Cooling of Southern Hemisphere oceans leads to anomalous upward air motions over eastern China, which weaken the vertical transport of high-altitude O 3 to the surface. Our results suggest that future changes in SSTs in the carbon-neutral scenario will positively benefit O 3 air quality improvement in the polluted eastern China, with the North Pacific and Southern Hemisphere oceans playing important roles.

54 ENVIRONMENTAL SCIENCES↗

A Mineralogy–Based Anthropogenic Combustion–Iron Emission Inventory

Atmospheric supply of iron can modulate ocean biogeochemistry, due to its key role in global nitrogen and carbon cycles. Current estimates predict up to 20% of global ocean net primary productivity depends on an atmospheric iron source. Using a technology–based methodology, we revise total and soluble anthropogenic iron emissions and resolve iron into its mineral components, which allows modeling mineral–specific atmospheric reactions. We compare different methodologies for representing anthropogenic iron solubility: measured in mild and strong leaches and estimated using a mineralogy basis and identify the emissions that are most affected by such assumptions. The inclusion of metal smelting as an iron source increases iron emissions by up to 10 times higher in the fine aerosol fraction (smaller than 1 μm) than most previous inventories. Different solubility assumptions alter anthropogenic soluble iron emissions and deposition by a factor of 20 and 10, respectively. Using solubilities measured in mild leaches and calculated by mineralogy give 20–30 Gg/yr anthropogenic emissions and 40–50 Gg/yr deposition, while those measured in strong leaches give 80–440 Gg/yr emissions and 200–450 Gg/yr deposition. Here, this range of anthropogenic soluble iron deposition leads to global soluble iron deposition of 1,900–2,300 Gg/yr when dust, wildfires, and atmospheric processing are included, indicating such assumptions can affect global soluble iron supply by about 30%. In regions where marine primary productivity is iron limited, anthropogenic combustion–iron contributes up to half of the atmospheric soluble iron flux to the North Pacific Ocean but supplies less than 5% to the Southern Ocean.

54 ENVIRONMENTAL SCIENCES↗