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At least 793 records · Page 44

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DOE OSTI2020

High-temperature Majorana fermions in magnet-superconductor hybrid systems

Magnet-superconductor hybrid (MSH) structures represent one of the most promising platforms to realize, control, and manipulate Majorana modes using scanning tunneling methods. By depositing either chains or islands of magnetic atoms on the surface of a conventional, elemental superconductor such as Pb or Re, topological superconducting phases can emerge. They feature either localized Majorana bound states at the chain ends or dispersing chiral Majorana modes at the island's boundary. However, some of these experiments have not reached the spectral resolution to clearly distinguish between topological Majorana and trivial Shiba states due to very small superconducting gap sizes and experiments performed at sub-Kelvin temperatures. Here we consider superconducting substrates with unconventional spin-singlet pairing, including high-temperature d -wave and extended s -wave superconductors. We derive topological phase diagrams and compute edge states for cylinder and island geometries and discuss their properties. Several time-reversal invariant topological superconducting phases of the Zhang-Kane-Mele type are found and discussed. Addiotnally, we review one-dimensional MSH structures and show that parameters to realize topologically nontrivial magnetic chains embedded into a larger, two-dimensional substrate differ from the purely one-dimensional case. Quite generally we find that unconventional superconducting substrates work as well as the conventional s -wave substrates to realize topological phases. In particular, iron-based pnictide and chalcogenide superconductors are the most promising class of substrates for future high-temperature MSH systems.

36 MATERIALS SCIENCE↗

NASA NTRS1994

Coronal mass ejections in the solar wind at high solar latitudes: An overview

Ulysses provided the first direct measurements of coronal mass ejections (CME's) in the solar wind at high heliographic latitudes. An overview of new results from the plasma experiment on Ulysses and magnetic field measurements, during the spacecraft's first excursion to high solar latitudes are summarized. A striking aspect of the high-latitude CME's observed is that they all had high speeds, with the overall average speed being 730 km/sec. A new class of forward-reverse shock pairs, associated with expansion of CME's was discovered at high latitudes. Of six certain CME's observed at high latitudes, three have associated shock pairs of this nature. Combined Ulysses and Yohkoh observations suggest that the flux rope topology characteristic of some CME's results from reconnection within the legs of neighboring magnetic loops embedded within the escaping CME's.

Gosling, Jack T.↗

DOE OSTI2019

A Closer Look at Fe(II) Passivation of Goethite

Our understanding of how Fe(II) reacts with Fe(III) oxides has evolved significantly based on evidence for electron transfer at the oxide-water interface and Fe(II)-catalyzed recrystallization. Recent experiments, as well as computational calculations, further suggest that defects at oxide surfaces can facilitate electron transfer. There is, however, some evidence that these processes cease after continued contact with Fe(II). Here, we explore the sustainability of these processes over longer time frames by measuring whether exposure to Fe(II) inhibits Fe(II)-goethite electron transfer, and whether this inhibition is reversible. To quantify the extent of electron transfer, we used selective isotope labeling with 57Fe Mössbauer spectroscopy. The results revealed that pre-reacting goethite with Fe(II) decreases the extent of electron transfer during subsequent exposures, and that less electron transfer occurs with increasing reaction time. Similarly, X-ray absorption spectroscopy and magnetic circular dichroism suggest that reaction with Fe(II) consumes surface defects and forms a passivation layer, making goethite less susceptible to electron transfer. When Fe(II) is removed by either wet chemical extraction or oxidation, electron transfer is mostly restored, suggesting that inhibition of electron transfer is reversible. Our results show that in environmental systems, which are commonly subjected to transient geochemical fluctuations, electron transfer between Fe(II) and Fe oxides, and processes linked to it, are likely to be relevant beyond just short time scales.

Andrade de Notini, Luiza↗

NASA NTRS2022

The Imprint of Intermittent Interchange Reconnection on the Solar Wind

The solar wind is known to be highly structured in space and time. Observations from Parker Solar Probe have revealed an abundance of so-called magnetic switchbacks within the near-Sun solar wind. In this Letter, we use a high-resolution, adaptive-mesh, magnetohydrodynamics simulation to explore the disturbances launched into the solar wind by intermittent/bursty interchange reconnection and how they may be related to magnetic switchbacks. We find that repeated ejection of plasmoid flux ropes into the solar wind produces a curtain of propagating and interacting torsional Alfvénic waves. We demonstrate that this curtain forms when plasmoid flux ropes dynamically realign with the radial field as they are ejected from the current layer and that this is a robust effect of the 3D geometry of the interchange reconnection region. Simulated flythroughs of this curtain in the low corona reveal an Alfvénic patch that closely resembles observations of switchback patches, but with relatively small magnetic field deflections. Therefore, we suggest that switchbacks could be the solar wind imprint of intermittent interchange reconnection in the corona, provided an in situ process subsequently amplifies the disturbances to generate the large deflections or reversals of radial field that are typically observed. That is to say, our results indicate that a combination of low-coronal and inner-heliospheric mechanisms may be required to explain switchback observations.

corona↗

DOE OSTI2022

Nuclear DFT analysis of electromagnetic moments in odd near doubly magic nuclei

We use the nuclear density functional theory to determine nuclear electric quadrupole and magnetic dipole moments in all one-particle and one-hole neighbours of eight doubly magic nuclei. We align angular momenta along the intrinsic axial-symmetry axis with broken time-reversal symmetry, which allows us to explore fully the self-consistent charge, spin, and current polarisation. Spectroscopic moments are determined for symmetry-restored wave functions and compared with available experimental data. We find that the obtained polarisations do not call for using quadrupole- or dipole-moment operators with effective charges or effective g-factors.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2021

Lower bound for the neutrino magnetic moment from kick velocities induced at the birth of neutron stars

We show that the neutrino chirality flip, which can take place in the core of a neutron star at birth, is an efficient process to allow neutrinos to anisotropically escape, thus providing a to induce the neutron star kick velocities. The process is not subject to the no-go theorem since although the flip from left- to right-handed neutrinos happens at equilibrium, the reverse process does not take place given that right-handed neutrinos do not interact with matter and therefore detailed balance is lost. For simplicity, we model the neutron star core as being made of strange quark matter. We find that the process is efficient when the neutrino magnetic moment is not smaller than [Formula: see text], where [Formula: see text] is the Bohr magneton. When this lower bound is combined with the most stringent upper bound, which uses the luminosity data obtained from the analysis of SN 1987A, our results set a range for the neutrino magnetic moment given by [Formula: see text]. The obtained kick velocities for natal conditions are consistent with the observed ones and span the correct range of radii for typical magnetic field intensities.

Physics↗

DOE OSTI2022

Emergent Magnetic States and Tunable Exchange Bias at 3d Nitride Heterointerfaces

Abstract Interfacial magnetism stimulates the discovery of giant magnetoresistance (MR) and spin–orbital coupling across the heterointerfaces, facilitating the intimate correlation between spin transport and complex magnetic structures. Over decades, functional heterointerfaces composed of nitrides have seldom been explored due to the difficulty in synthesizing high‐quality nitride films with correct compositions. Here, the fabrication of single‐crystalline ferromagnetic Fe 3 N thin films with precisely controlled thicknesses is reported. As film thickness decreases, the magnetization dramatically deteriorates, and the electronic state changes from metallic to insulating. Strikingly, the high‐temperature ferromagnetism is maintained in a Fe 3 N layer with a thickness down to 2 u.c. (≈8 Å). The MR exhibits a strong in‐plane anisotropy; meanwhile, the anomalous Hall resistivity reverses its sign when the Fe 3 N layer thickness exceeds 5 u.c. Furthermore, a sizable exchange bias is observed at the interfaces between a ferromagnetic Fe 3 N and an antiferromagnetic CrN. The exchange bias field and saturation moment strongly depend on the controllable bending curvature using the cylinder diameter engineering technique, implying the tunable magnetic states under lattice deformation. This work provides a guideline for exploring functional nitride films and applying their interfacial phenomena for innovative perspectives toward practical applications.

Jin, Qiao↗

DOE OSTI2020

Nonreciprocal directional dichroism of a chiral magnet in the visible range

Nonreciprocal directional dichroism is an unusual light–matter interaction that gives rise to diode-like behavior in low-symmetry materials. The chiral varieties are particularly scarce due to the requirements for strong spin–orbit coupling, broken time-reversal symmetry, and a chiral axis. Here we bring together magneto-optical spectroscopy and first-principles calculations to reveal high-energy, broadband nonreciprocal directional dichroism in Ni 3 TeO 6 with special focus on behavior in the metamagnetic phase above 52 T. In addition to demonstrating this effect in the magnetochiral configuration, we explore the transverse magnetochiral orientation in which applied field and light propagation are orthogonal to the chiral axis and, by so doing, uncover an additional configuration with a unique nonreciprocal response in the visible part of the spectrum. In a significant conceptual advance, we use first-principles methods to analyze how the Ni 2+ d-to-d on-site excitations develop magneto-electric character and present a microscopic model that unlocks the door to theory-driven discovery of chiral magnets with nonreciprocal properties.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2020

Twist again: Dynamically and reversibly controllable chirality in liquid crystalline elastomer microposts

Photoresponsive liquid crystalline elastomers (LCEs) constitute ideal actuators for soft robots because their light-induced macroscopic shape changes can be harnessed to perform specific articulated motions. Conventional LCEs, however, do not typically exhibit complex modes of bending and twisting necessary to perform sophisticated maneuvers. Here, we model LCE microposts encompassing side-chain mesogens oriented along a magnetically programmed nematic director, and azobenzene cross-linkers, which determine the deformations of illuminated posts. On altering the nematic director orientation from vertical to horizontal, the post’s bending respectively changes from light-seeking to light-avoiding. Moreover, both modeling and subsequent experiments show that with the director tilted at 45°, the initially achiral post reversibly twists into a right- or left-handed chiral structure, controlled by the angle of incident light. We exploit this photoinduced chirality to design “chimera” posts (encompassing two regions with distinct director orientations) that exhibit simultaneous bending and twisting, mimicking motions exhibited by the human musculoskeletal system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2022

Misalignment of magnetic field in DIII-D assessed by post-mortem analysis of divertor targets

Abstract We assess the toroidal magnetic field B t asymmetry in DIII-D due to a misalignment of the toroidal field coils with respect to the poloidal magnetic field coils and vacuum vessel. The peak-to-peak variation of the divertor strike point (SP) radius is measured to be 1 cm, with an n = 1 toroidal pattern. We use the centre of a narrow carbon deposition band on tungsten-coated divertor tiles just inside the outer strike point (OSP) as a proxy for the divertor SP location. The band occurred in a series of reverse B t discharges with the OSP positioned on the divertor inserts due to strong E × B drift transport of C from the inner to the outer SP through the private flux region. The variation in band radius (and hence the magnetic SP) is a (4.89 ± 0.31) mm shift toward (310 ± 4)° toroidal direction. These measurements agree well with previous measurements of the 3D magnetic field distribution (Luxon 2003 Nucl. Fusion 43 1813), simulations performed by the mafot field line integration code, and recent Langmuir probe measurements in the small-angle-slot (SAS) divertor (Watkins et al 2019 Nucl. Mater. Energy 18 46). Comparison of these measurements in the SAS divertor also indicates that there is the possibility of a tilt (in conjunction with the shift) of the B t coil field of (0.04 ± 0.07)° towards the toroidal angle of (215 ± 25)°. Previous measurements suggested a field misalignment of (4.6 ± 0.3) mm in the 270° toroidal direction, and a tilt of (0.06 ± 0.02)° toward the 114° toroidal direction, which is similar to the results reported here. These studies will be important for better understanding the radial variation of the toroidal strike line in DIII-D, for designing the new generation of SAS divertor, and for developing an understanding of the impact of error fields on tokamaks with tightly baffled slot divertors.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2026

Equilibrium spin polarization arising from chirality

Chirality-induced spin selectivity (CISS) describes how chiral molecules and materials generate spin polarization even at thermal equilibrium. This observation has challenged established principles of microscopic reversibility and Onsager reciprocity. We resolve this paradox by formulating a pseudo-Hermitian quantum framework that separates thermodynamic equilibrium from time-reversal symmetry. Within this approach, structural chirality and electron correlations, irrespective of their microscopic origin, are sufficient to produce CISS observables. Chirality enters through a non-local metric η that couples spin and spatial motion, leading to real spectra, unitary evolution, and thermodynamic consistency. The framework predicts a chirality-induced spin magnetic ordering characterized by a spin-displacement order, which reconciles equilibrium spin polarization with detailed balance and explains the persistence of CISS in materials composed of light elements. We derive generalized Onsager-Casimir relations that respect the observed CISS symmetry, i.e., parity $(\mathscr{P})$-odd and time-reversal $(\mathscr{T})$-odd, but exhibiting $\mathscr{PT}$-even symmetry. This approach establishes a coherent foundation for equilibrium CISS and provides a route to link chemical chirality with measurable spin-to-charge conversion effects.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2021

Unconventional chiral charge order in kagome superconductor KV 3 Sb 5

Intertwining quantum order and non-trivial topology is at the frontier of condensed matter physics. A charge-density-wave-like order with orbital currents has been proposed for achieving the quantum anomalous Hall effect in topological materials and for the hidden phase in cuprate high-temperature superconductors. However, the experimental realization of such an order is challenging. Here we use high-resolution scanning tunnelling microscopy to discover an unconventional chiral charge order in a kagome material, KV 3 Sb 5 , with both a topological band structure and a superconducting ground state. Through both topography and spectroscopic imaging, we observe a robust 2 × 2 superlattice. Spectroscopically, an energy gap opens at the Fermi level, across which the 2 × 2 charge modulation exhibits an intensity reversal in real space, signalling charge ordering. At the impurity-pinning-free region, the strength of intrinsic charge modulations further exhibits chiral anisotropy with unusual magnetic field response. Therefore theoretical analysis of our experiments suggests a tantalizing unconventional chiral charge density wave in the frustrated kagome lattice, which can not only lead to a large anomalous Hall effect with orbital magnetism, but also be a precursor of unconventional superconductivity.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Topological edge conduction induced by strong anisotropic exchange interactions

Here, we predict that an interplay between isotropic and anisotropic exchange interactions in a honeycomb lattice structure can lead to topological edge conduction when the anisotropic interaction is at least twice the strength of the isotropic interaction. For materials like Na 2 ⁢IrO 3 , such a strong anisotropic exchange interaction simultaneously induces a zigzag type of antiferromagnetic order that breaks the time-reversal symmetry of the topological edge conductor. We show that the electronic transport in such topological conductors will exhibit a quantized Hall conductance without any external magnetic field when the Fermi energy lies within a particular energy range.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Dispersive nonreciprocity between a qubit and a cavity

The dispersive interaction between a qubit and a cavity is ubiquitous in circuit and cavity quantum electrodynamics. It describes the frequency shift of one quantum mode in response to excitations in the other and, in closed systems, is necessarily bidirectional, i.e., reciprocal. Here, we present an experimental study of a nonreciprocal dispersive-type interaction between a transmon qubit and a superconducting cavity, arising from a common coupling to dissipative intermediary modes with broken time reversal symmetry. We characterize the qubit-cavity dynamics, including asymmetric frequency pulls and photon shot noise dephasing, under varying degrees of nonreciprocity by tuning the magnetic field bias of a ferrite component in situ. We introduce a general master equation model for nonreciprocal interactions in the dispersive regime, providing a compact description of the observed qubit-cavity dynamics agnostic to the intermediary system. Our result provides an example of quantum nonreciprocal phenomena beyond the typical paradigms of non-Hermitian Hamiltonians and cascaded systems.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2021

QED with the electron as a very small black-hole-like object

We pursue a simple semi-classical particle-based picture of QED in which the electron is assumed to contain a point massless and chargeless core that interacts with the electromagnetic vacuum in ways that are not dissimilar to the manner in which small black holes may interact with photons. Modifications are made to obtain known properties of the electron including the presence of rest energy, Lamb shift, magnetic moments (both free and bound), charge, Larmor emission, and vacuum polarization. The present study does not provide proofs but is rather an attempt to reverse-engineer the photon-electron and black-hole-electron interaction properties needed to match experimental observations. The ease by which many QED observables can be reproduced suggests further study of the presented framework may be warranted. Future detailed analysis of the exchange of long wavelength Hawking radiation between a pair of small black holes will be of particular interest.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1976

Observations of interaction regions and corotating shocks between one and five AU - Pioneers 10 and 11

Interaction regions between adjacent solar-wind streams have been identified between 1 and 5 AU by Pioneer 10 and 11 magnetic-field and plasma measurements. Beyond 1 AU, a relatively large fraction of the interaction regions have been found to be accompanied by either forward shocks, reverse shocks, or shock pairs. The observations are consistent with previous theoretical proposals that the interaction between adjacent streams leads to the development of corotating interplanetary shocks.

Smith, E. J.↗

NASA NTRS1995

Suprathermal electron loss cone distributions in the solar wind: Ulysses observations

Solar wind suprathermal electron distributions in the solar wind generally carry a field-aligned antisunward heat flux. Within coronal mass ejections and upstream of strong shocks driven by corotating interaction regions (CIRs), counterstreaming electron beams are observed. We present observations by the Ulysses solar wind plasma experiment of a new class of suprathermal electron signatures. At low solar latitudes and heliocentric distances beyond 3.5 AU Ulysses encountered several intervals, ranging in duration from 1 hour to 22 hours, in which the suprathermal distributions included an antisunward field-aligned beam and a return population with a flux dropout typically spanning +/- 60 deg from the sunward field-aligned direction. All events occurred within CIRs, downstream of the forward and reverse shocks or waves bounding the interaction regions. We evaluate the hypothesis that the sunward-moving electrons result from reflection of the antisunward beams at magnetic field compressions downstream from the observations, with wide loss cones caused by the relatively weak compression ratio. This hypothesis requires that field magnitude within the CIRs actually increase with increasing field-aligned distance from the Sun. Details of the electron distributions and ramifications for CIR and shock geometry will be presented.

Phillips, J. L.↗

DOE OSTI2026

Conventional superconductivity in single-crystalline BiPt

Binary Bi-Pd/Pt systems have attracted a lot of interest because of their topologically nontrivial nature along with superconductivity. We report the structural and superconducting properties of high-quality single-crystalline BiPt using a comprehensive range of experimental techniques, including X-ray diffraction, electron microscopy, muon spin rotation/relaxation (𝜇⁢SR), magnetization, resistivity, and heat capacity. Our findings establish that BiPt is a weak type-II superconductor with a transition temperature (𝑇 𝑐 ) of 1.2 K which exhibits pronounced anisotropic superconducting characteristics attributed to its hexagonal crystal structure. Magnetization and electronic transport studies reveal that BiPt lies within the dirty limit, while 𝜇⁢SR and heat capacity data indicate conventional 𝑠-wave superconductivity that maintains time-reversal symmetry. Here, this work provides valuable insights into the pairing symmetry and superconducting mechanism of topologically trivial BiPt, a sound comparison system for other Bi-based topologically nontrivial superconductors.

Demagnetization↗