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At least 793 records · Page 44

As-Run Physics Analysis for the EPRI Zirconium Growth C Capsule

This engineering calculation and analysis report documents the as-run nuclear-heating term, source-term, and radiation damage (measured in displacements per atom [dpa]) accumulation for the Electric Power Research Institute zirconium growth experiment's C capsule (EPRI-ZG-C). These data have been calculated using MCNP 6.1 and SCALE 6.2.3. These data can be used for: the shipping of the EPRI-ZG-C capsule, the acceptance of the capsule at the Materials and Fuels Complex, and programmatic scientific needs.

36 MATERIALS SCIENCE↗

Compact Bremsstrahlung Diode Development on HERMES-III

Testing of a compact Bremsstrahlung diode at the High Energy Radiation Megavolt Electron Source III (HERMES-III) was performed at Sandia National Laboratories in November, 2023. The compact diode described here is the first prototype diode in a campaign to optimize a Bremsstrahlung diode in terms of size and dose production. The goal was to test the diode at 13MV, and the experiment realized between 10-12MV at the diode. Modeling and simulation of this geometry was performed after the test, shedding insight into several phenomena seen by experimental diagnostics. Modifications to the diode and experiment are proposed for future experiments to help explain the phenomena and approach a better final design.

42 ENGINEERING↗

NCERC 2024 Highlights

The National Nuclear Security Administration (NNSA) is entrusted with ensuring the safety, security, and reliability of the nation’s nuclear weapons stockpile while advancing programs aimed at reducing global nuclear proliferation. These critical mission objectives are achieved through the expertise of a highly skilled team of professionals. The operations at the National Criticality Experiments Research Center (NCERC) play a vital role in developing and enhancing knowledge and expertise in advanced nuclear technologies. NCERC supports a wide range of mission areas, including nuclear criticality safety, nuclear emergency response, and nuclear nonproliferation, safeguards, and arms control. It also provides support to the Department of Homeland Security, advances stockpile stewardship science, and delivers scientific expertise to other government agencies, such as NASA and the Defense Threat Reduction Agency. NCERC conducts experiments utilizing diverse nuclear materials, from small neutron-emitting sources for testing radiation detection equipment to larger quantities of uranium and plutonium for criticality experiments. A cornerstone of NCERC's mission portfolio includes the operation of four critical mass assembly machines—Planet, Comet, Flattop, and Godiva-IV—which are instrumental in advancing nuclear science and ensuring the nation’s nuclear security objectives.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Toward Trustworthy Detectors Detector Characterization for SuperCDMS SNOLAB Commissioning

SuperCDMS SNOLAB is a next generation direct detection experiment searching for low mass dark matter using cryogenic germanium and silicon detectors operated at millikelvin temperatures. As commissioning begins, establishing stable, predictable detector response to energy deposits is a prerequisite for future physics analysis. This work studies detector stability and calibration for four SuperCDMS SNOLAB detectors, det 7 and det 15 (germanium) and det 11 and det 14 (silicon), using Barium-133 calibration data (356 keV gamma ray reference) and low background data (ambient radiation, no external source). The Ba-133 data show no distinct line at the expected energy, and the low background data show a baseline that drifts and oscillates rather than remaining flat, consistently across multiple channels, suggesting a shared, detector wide cause. These observations point to the cryogenic support system as the likely source, since small temperature fluctuations could couple into the temperature sensitive detectors, informing the ongoing commissioning effort.

O'Hanlon, Vika [Skidmore Coll.]↗

Predicting Solar Energetic Particles Using SDO/HMI Vector Magnetic Data Products and a Bidirectional LSTM Network

Solar energetic particles (SEPs) are an essential source of space radiation, and are hazardous for humans in space, spacecraft, and technology in general. In this paper, we propose a deep-learning method, specifically a bidirectional long short-term memory (biLSTM) network, to predict if an active region (AR) would produce an SEP event given that (i) the AR will produce an M- or X-class flare and a coronal mass ejection (CME) associated with the flare, or (ii) the AR will produce an M- or X-class flare regardless of whether or not the flare is associated with a CME. The data samples used in this study are collected from the Geostationary Operational Environmental Satellite's X-ray flare catalogs provided by the National Centers for Environmental Information. We select M- and X-class flares with identified ARs in the catalogs for the period between 2010 and 2021, and find the associations of flares, CMEs, and SEPs in the Space Weather Database of Notifications, Knowledge, Information during the same period. Each data sample contains physical parameters collected from the Helioseismic and Magnetic Imager on board the Solar Dynamics Observatory. Experimental results based on different performance metrics demonstrate that the proposed biLSTM network is better than related machine-learning algorithms for the two SEP prediction tasks studied here. We also discuss extensions of our approach for probabilistic forecasting and calibration with empirical evaluation

79 ASTRONOMY AND ASTROPHYSICS↗

Electron and Proton Energization in 3D Reconnecting Current Sheets in Semirelativistic Plasma with Guide Magnetic Field

Abstract Using 3D particle-in-cell simulation, we characterize energy conversion, as a function of guide magnetic field, in a thin current sheet in semirelativistic plasma, with relativistic electrons and subrelativistic protons. There, magnetic reconnection, the drift-kink instability (DKI), and the flux-rope kink instability all compete and interact in their nonlinear stages to convert magnetic energy to plasma energy. We compare fully 3D simulations with 2D in two different planes to isolate reconnection and DKI effects. In zero guide field, these processes yield distinct energy conversion signatures: ions gain more energy than electrons in 2Dxy(reconnection), while the opposite is true in 2Dyz(DKI), and the 3D result falls in between. The flux-rope instability, which occurs only in 3D, allows more magnetic energy to be released than in 2D, but the rate of energy conversion in 3D tends to be lower. Increasing the guide magnetic field strongly suppresses DKI, and in all cases slows and reduces the overall amount of energy conversion; it also favors electron energization through a process by which energy is first stored in the motional electric field of flux ropes before energizing particles. Understanding the evolution of the energy partition thus provides insight into the role of various plasma processes, and is important for modeling radiation from astrophysical sources such as accreting black holes and their jets.

Astronomy & Astrophysics↗

Distinct responses of Asian summer monsoon to black carbon aerosols and greenhouse gases

Black carbon (BC) aerosols emitted from natural and anthropogenic sources induce positive radiative forcing and global warming, which in turn significantly affect the Asian summer monsoon (ASM). However, many aspects of the BC effect on the ASM remain elusive and largely inconsistent among previous studies, which is strongly dependent on different low-level thermal feedbacks over the Asian continent and the surrounding ocean. This study examines the response of the ASM to BC forcing in comparison with the effect of doubled greenhouse gases (GHGs) by analyzing the Precipitation Driver Response Model Intercomparison Project (PDRMIP) simulations under an extremely high BC level (10 times modern global BC emissions or concentrations, labeled BC×10) from nine global climate models (GCMs). The results show that although BC and GHGs both enhance the ASM precipitation minus evaporation (P–E; a 13.6 % increase for BC forcing and 12.1 % for GHGs from the nine-model ensemble, respectively), there exists a much larger uncertainty in changes in ASM P–E induced by BC than by GHGs. The summer P–E is increased by 7.7 % to 15.3 % due to these two forcings over three subregions, including East Asian, South Asian and western North Pacific monsoon regions. Further analysis of moisture budget reveals distinct mechanisms controlling the increases in ASM P–E induced by BC and GHGs. The change in ASM P–E by BC is dominated by the dynamic effect due to the enhanced large-scale monsoon circulation, whereas the GHG-induced change is dominated by the thermodynamic effect through increasing atmospheric water vapor. Radiative forcing of BC significantly increases the upper-level atmospheric temperature over the Asian region to enhance the upper-level meridional land–sea thermal gradient (MLOTG), resulting in a northward shift of the upper-level subtropical westerly jet and an enhancement of the low-level monsoon circulation, whereas radiative forcing of GHGs significantly increases the tropical upper-level temperature, which reduces the upper-level MLOTG and suppresses the low-level monsoonal circulation. Hence, our results indicate a different mechanism of BC climate effects under the extremely high BC level: that BC forcing significantly enhances the upper-level atmospheric temperature over the Asian region, determining ASM changes, instead of low-level thermal feedbacks as indicated by previous studies.

54 ENVIRONMENTAL SCIENCES↗

Distinct responses of Asian summer monsoon to black carbon aerosols and greenhouse gases

Black carbon (BC) aerosols emitted from natural and anthropogenic sources induce positive radiative forcing and global warming, which in turn significantly affect the Asian summer monsoon (ASM). However, many aspects of the BC effect on ASM remain elusive and largely inconsistent among previous studies, which is strongly dependent on different low-level thermal feedbacks over the Asian continent and the surrounding ocean. This study examines the response of ASM to BC forcing in comparison with the effect of doubled greenhouse gases (GHGs) by analyzing the Precipitation Driver Response Model Intercomparison Project (PDRMIP) simulations under an extreme high BC level (10 times modern global BC emissions or concentrations, labeled by BC $\times$ 10) from nine global climate models (GCMs). The results show that although BC and GHGs both enhance the ASM precipitation minus evaporation (P–E) (a 13.6 % increase for BC forcing and 12.1 % for GHGs from the nine-model ensemble, respectively), there exists a much larger uncertainty in changes in ASM P–E induced by BC than by GHGs. The summer P–E is increased by 7.7 % to 15.3 % due to these two forcings over three sub-regions including East Asian, South Asian, and western North Pacific monsoon regions. Further analysis of moisture budget reveals distinct mechanisms controlling the increases in ASM P–E induced by BC and GHGs. The change in ASM P–E by BC is dominated by the dynamic effect due to the enhanced large-scale monsoon circulation, whereas the GHG-induced change is dominated by the thermodynamic effect through increasing atmospheric water vapor. Radiative forcing of BC significantly increases the upper-level atmospheric temperature over the Asian region to enhance the upper-level meridional land-sea thermal gradient (MLOTG), resulting in a northward shift of the upper-level subtropical westerly jet and an enhancement of the low-level monsoon circulation; whereas radiative forcing of GHGs significantly increases the tropical upper-level temperature, which reduces the upper-level MLOTG and suppresses the low-level monsoonal circulation. Hence, our results indicate a different mechanism of BC climate effects under the extreme high BC level, that BC forcing significantly enhances the upper-level atmospheric temperature over the Asian region, determining ASM changes, instead of low-level thermal feedbacks as indicated by previous studies.

54 ENVIRONMENTAL SCIENCES↗

OCEANFILMS (Organic Compounds from Ecosystems to Aerosols: Natural Films and Interfaces via Langmuir Molecular Surfactants) sea spray organic aerosol emissions – implementation in a global climate model and impacts on clouds

Sea spray aerosol is one of the major sources of atmospheric particulate matter globally. It has increasingly been recognized that organic matter derived from ocean biological precursors contributes significantly to the composition of submicron sea spray and may modify sea spray aerosol impacts on clouds and climate. This paper describes the implementation of the OCEANFILMS (Organic Compounds from Ecosystems to Aerosols: Natural Films and Interfaces via Langmuir Molecular Surfactants) parameterization for sea spray organic aerosol emissions in a global Earth system model, the Energy Exascale Earth System Model (E3SM). OCEANFILMS is a physically based model that links sea spray chemistry with ocean biogeochemistry using a Langmuir partitioning approach. We describe the implementation details of OCEANFILMS within E3SM, compare simulated aerosol fields with observations, and investigate impacts on simulated clouds and climate. Four sensitivity cases are tested, in which organic emissions either strictly add to or strictly replace sea salt emissions (in mass and number) and are either fully internally or fully externally mixed with sea salt. The simulation with internally mixed, added organics agrees reasonably well with observed seasonal cycles of organic matter in marine aerosol and has been selected as the default configuration of the E3SM. In this configuration, sea spray organic aerosol contributes an additional source of cloud condensation nuclei, adding up to 30 cm -3 to Southern Ocean boundary-layer cloud condensation nuclei concentrations (supersaturation = 0.1 %). The addition of this new aerosol source strengthens shortwave radiative cooling by clouds by -0.36 W m -2 in the global annual mean and contributes more than -3.5 W m -2 to summertime zonal mean cloud forcing in the Southern Ocean, with maximum zonal mean impacts of about -4 W m -2 around 50–60°S. This is consistent with a previous top-down, satellite-based empirical estimate of the radiative forcing by sea spray organic aerosol over the Southern Ocean. Through its mechanistic approach, OCEANFILMS offers a path towards improved understanding of the feedbacks between ocean biology, sea spray organic matter, and climate.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Hybrid phonon-enhanced optical absorbers and emitters

A semiconductor optical device is comprised of a phonon donating material structurally connected to an indirect bandgap material to improve absorption and emission of light in the indirect bandgap material. An excitation energy source provides excitation radiation to the semiconductor optical device to excite electrons in the semiconductor optical device. Phonons from the phonon donating material present in the indirect bandgap material provide a mechanism for increased rates of electron-hole generation and recombination, and electrical leads provide an electrical connection to the semiconductor optical device.

Husko, Chad↗

Representing Anthropogenic Dust From Agricultural Sources in E3SMv1: Implementation, Evaluation, and Assessment of the Radiative Forcing

Dust emissions related to anthropogenic activities (i.e., anthropogenic dust) is not represented in most global climate models and its radiative impact remains unassessed. In this study, we develop a new and physically based method to parameterize anthropogenic dust emission from agricultural sources (i.e., agricultural dust, or AD) based on the DOE's Energy Exascale Earth System Model version 1 (E3SMv1). This method relates AD emission to the crop land use fraction in the E3SMv1 land component. Major AD sources simulated by our parameterization include those over Central America, the Sahel, North India, and North China. The annual averaged AD emission with diameter less than 10 μm is 567 Tg yr −1 in present-day (year 2000), which contributes to 13.3% of total dust emission. Model evaluation against satellite and ground-based observations shows that the new parameterization can represent AD emissions and global dust cycle reasonably well. We find that the total dust emission increases by 13.1% (495 Tg yr −1 ) from 1850 to 2000 due to the cropland land use fraction changes without considering the impact from climate changes. This induces a net dust direct effective radiative forcing of −0.041 W m −2 at top of the atmosphere. This dust-induced cooling exceeds 10% of the total anthropogenic aerosol direct effective radiative forcing from 1750 to 2014 estimated by the Intergovernmental Panel on Climate Change Sixth Assessment Report. Our findings indicate an important role of anthropogenic dust in global climate change, which should be included in future climate change assessments.

agricultural dust↗

Radiological Impact of 2020 Operations at the Savannah River Site

This report presents environmental dose assessment methods and the estimated potential doses to the public from 2020 Savannah River Site (SRS) atmospheric and liquid radioactive releases. It also documents potential doses from special-case exposure scenarios, such as the consumption of wildlife and/or goat milk. Unless noted, the generic term “dose,” as used in this report, includes both the committed effective dose (50-year committed dose) from internal deposition of radionuclides and the effective dose attributable to sources external to the body. Using the effective dose allows doses from different types of radiation and to different parts of the body to be expressed on the same basis. Humans, plants, and animals potentially receive radiation doses from natural and man-made occurrences. The average annual “background” dose for all people living in the United States is 625 mrem. This includes an average background dose of 311 mrem from naturally occurring radionuclides (found in our bodies and in the earth) and from cosmic radiation. Man-made sources include medical procedures (300 mrem), consumer products (13 mrem), and industrial and occupational exposures (less than 1 mrem).

54 ENVIRONMENTAL SCIENCES↗

Optimized Viewing Techniques to Minimize Radiation Damage From X-ray Imaging Systems

X-ray inspection of ball grid arrays (BGAs) is typically performed at one or more viewing angles to examine adhesion sites for errors such as voids, joint cracking, or head-in-pillow. During this inspection process, the cir cuit board assembly is subject to ionizing radiation exposure, which can cause trapped charge within oxide layers of semiconductor devices. Some x-ray machines allow for programmable inspection routines, which could be used to optimize radiation exposure to semiconductor components. Using Monte Carlo methods, x-ray inspection of a BGA was simulated to determine a range of acceptable viewing angles. Dose rates to circuit board components were estimated at each inspection angle to determine the view resulting in optimized radiation exposure. Results showed that for each BGA, the maximum unobstructed viewing times without exceeding a 5 Gy dose limit to a single part ranged from 82 to 94 minutes. Using a radiation cost function method, optimized viewing across all components was found. Here, it was observed that for a consistent dose limit applied to silicon-based components, performing inspection with BGAs facing the x-ray source was optimal. A third method was applied, assigning individual dose limits based on empirical data from the NASA Goddard Space Flight Center radiation database. This method showed that optimized viewing maximizes the distance between the radiation source and highly sensitive components. It was also observed that cumulative effects from viewing two BGAs will influence viewing angles, causing the optimal view of one BGA to exist nearly 180° from the other.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Efficient smoothed particle radiation hydrodynamics I: Thermal radiative transfer

This work presents efficient solution techniques for radiative transfer in the smoothed particle hydrodynamics discretization. Two choices that impact efficiency are how the material and radiation energy are coupled, which determines the number of iterations needed to converge the emission source, and how the radiation diffusion equation is solved, which must be done in each iteration. The coupled material and radiation energy equations are solved using an inexact Newton iteration scheme based on nonlinear elimination, which reduces the number of Newton iterations needed to converge within each time step. During each Newton iteration, the radiation diffusion equation is solved using Krylov iterative methods with a multigrid preconditioner, which abstracts and optimizes much of the communication when running in parallel. The code is verified for an infinite medium problem, a one-dimensional Marshak wave, and a two and three-dimensional manufactured problem, and exhibits first-order convergence in time and second-order convergence in space. For these problems, the number of iterations needed to converge the inexact Newton scheme and the diffusion equation is independent of the number of spatial points and the number of processors.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TORONE: Total Characterisation by Remote Observation of Nuclear Environments - 20591

This paper describes the autonomous robotic systems developed in the TORONE project (Total Characterisation by Remote Observation of Nuclear Environments) for combined characterisation by remote techniques in nuclear environments. There are four main components to the system. Firstly, robot operation which uses a Robot Operating System (ROS) allowing ease of communication between hardware and software alongside robot vision systems such as Lidar and/or photogrammetry. Secondly, radiation detection instrumentation for gamma and neutron sources which is also collimated for spatial resolution. Thirdly, photonic characterisation instrumentation for remote material identification by means of Raman spectroscopy and Laser induced breakdown spectroscopy (LIBS). Finally, a data management system is described which contains the TORONE characterisation data with the ability to overlay material characterisation information onto 3D maps of the nuclear environment. Preliminary results are described alongside discussion of some of the synergies of the combined approach. There are many applications of such an autonomous system in nuclear decommissioning, waste management and asset management. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Space radiation measurements during the Artemis I lunar mission

Space radiation is a notable hazard for long-duration human spaceflight. Associated risks include cancer, cataracts, degenerative diseases and tissue reactions from large, acute exposures. Space radiation originates from diverse sources, including galactic cosmic rays, trapped-particle (Van Allen) belts5 and solar-particle events. Previous radiation data are from the International Space Station and the Space Shuttle in low-Earth orbit protected by heavy shielding and Earth’s magnetic field and lightly shielded interplanetary robotic probes such as Mars Science Laboratory and Lunar Reconnaissance Orbiter. Limited data from the Apollo missions and ground measurements with substantial caveats are also available. Here we report radiation measurements from the heavily shielded Orion spacecraft on the uncrewed Artemis I lunar mission. At differing shielding locations inside the vehicle, a fourfold difference in dose rates was observed during proton-belt passes that are similar to large, reference solar-particle events. Interplanetary cosmic-ray dose equivalent rates in Orion were as much as 60% lower than previous observations. Furthermore, a change in orientation of the spacecraft during the proton-belt transit resulted in a reduction of radiation dose rates of around 50%. These measurements validate the Orion for future crewed exploration and inform future human spaceflight mission design.

79 ASTRONOMY AND ASTROPHYSICS↗