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Preparing for first launch in 2021, NASA’s Space Launch System (SLS) super heavy-lift launch vehicle will usher in a new era of human spaceflight, returning astronauts to the Moon as part of the Artemis program. Although designed to send crew in the Orion spacecraft and large payloads to the Moon and beyond, SLS also provides CubeSats with rideshare opportunities for missions to deep space. The first launch of SLS and Orion, Artemis I, has 13 6U CubeSats manifested. The payloads have been tested and will soon ship to Kennedy Space Center (KSC) to be integrated into commercial off-the-shelf (COTS) dispensers and integrated into the SLS Block 1 vehicle. Leveraging launches for the Artemis program to deploy rideshare smallsats to deep space provides a low-cost opportunity to perform missions that previously would have required a larger spacecraft and a dedicated launch, and offers additional benefits to both NASA and the smallsat community. CubeSats, including those manifested on the Artemis I flight, have a valuable role to play in the Artemis program, providing data to address NASA’s identified Strategic Knowledge Gaps (SKGs) in its plans to permanently establish humanity in deep space. Payload sponsors and developers for the Artemis I CubeSats hail from a variety of NASA industry partners and mission directorates, as well as international space agencies and universities. Several payloads destined for cislunar space will demonstrate propulsion systems and other technologies useful to future exploration. Science missions manifested on the Artemis I flight include characterizing the effects of deep space radiation on living organisms, searching for hydrogen and other volatiles on the Moon’s South Pole, and studying the lunar radiation environment. Three of the payloads were selected through NASA’s Centennial Challenges Program. Those payloads are competing for prize money while meeting specific technical development goals, such as communication with Earth from millions of miles in space. Student involvement in almost half of the Artemis I payload development allows STEM engagement with SLS and NASA’s Artemis program. As the initial vehicle to fly, the SLS Block 1 vehicle will lay the foundation for a generation of human and robotic deep space exploration missions. The Block 1 core stage is undergoing final testing at Stennis Space Center in 2020 before transportation to KSC for integration and launch in 2021. Following the Block 1 vehicle, the Block 1B and Block 2 vehicles will incorporate propulsion system upgrades and other changes to increase lift capability. In addition to sending the Orion vehicle to TLI, SLS can also be outfitted with large-diameter fairings to send robotic probes to deep space. With unparalleled lift, volume and departure energy, SLS is poised to usher in a new generation of spaceflight. In addition to launching Orion and large-volume missions, CubeSats may also be a part of Artemis missions to deep space.