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At least 775 records · Page 43

Nuclear Excitation and Fission Studies with Short Pulsed Laser-Driven High Energy Gamma Rays

We propose the development of a platform to study photon excitation of high Z nuclei utilizing a high energy (70 J) short pulsed (500 fs) laser to drive > 5 MeV γ-radiation. The laser beam will be focused onto a specially prepared foam or corrugated conveying target, where it generates relativistic MeV electrons via ponderomotive and wake-field acceleration mechanisms. γ-emission is produced in the form of bremsstrahlung in the same target or in a separated high-Z γ-production target hit by the accelerated MeV electrons. The high energy γ-rays will be utilized to provide nuclear state excitation in the short time domain. The γ platform will allow to investigate photo fission of high Z target material positioned in an auxiliary target chamber in the γ-ray beam path via the established gas transport scheme. The photo fission yield will provide furthermore diagnostic information on the produced γ-yield. In addition, γ-spectroscopy will be used to identify γ-lines for the diagnostic of the excited state population of high Z target nuclei. This research capability is relevant to the understanding of how nuclear excitation effects fission, in relevance to recent astrophysical observations on element nucleosynthesis. These processes involve neutron-rich fragments and processes such as fission recycling (e. g. in neutron stars outer crusts).

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

233 U(n,$\gamma$) measurements at LANSCE [Slides]

A new measurement at LANSCE combined DANCE and NEUANCE at the end of 2020 and 2021. The 233 U material was provided by Oak Ridge National Laboratory (December 2020).Two samples of 10 mg and 20 mg of 233 U have been prepared at LANL by Evelyn M. Bond (December 2020). The experiment was performed in December 2020 and June/July 2021. Data analysis is ongoing to extract capture data knowing fission. LANL is looking forward to delivering the capture/fission ratio from (1-300) keV by the end of the FY2022.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

LLNL International Working Group on Gamma Spectrometry - Preparation of IDB Dataset

The spectral information and associated metadata, including source information, detector setup, and shielding configuration is described in human readable, comma-separated text files (csv). Five csv files are associated with each material type and include the following information (where [Isotope] is U, Pu, and MOX): [Isotope]_measurement_metadata - Metadata of the measurement configuration, including material composition at time of acquisition (decay corrected from certificate date). Data that is unique to a measurement configuration e.g. detector geometry, source-detector distance, analyzer and other electronics used, attenuating materials are provided in this file. [Isotope]_spectrum_metadata - The information that is unique to the spectrum. This includes detector specifications (e.g. date of acquisition, number of channels, gain (keV/channel), energy range, real and live time, full width half-maximum (FWHM) of the 186 or 208 peak for uranium or plutonium measurements, respectively. [Isotope]_source_metadata - The source material used for the measurement, this includes the ratio and uncertainties of isotopes present and processing information of the material. In addition, the certificate information for the source material is listed. [Isotope]_spectrum_counts_metadata - The counts per channel for each spectrum. This data is linked via the UID.spectrum index to the measurement_metadata file. [Isotope]_spectrum_checksum_metadata The MD5 checksum for the original spectrum file. This data is linked via the UID.spectrum index to the measurement_metadata file. This information is provided to prevent duplication of entries in the database.

42 ENGINEERING↗

NucD-23 Nuclear Diagnostics Development: The future of neutron imaging and gamma reaction history

The Neutron Imaging team has deployed novel, active detection systems along two lines of sight at NIF. Studies aimed to characterize NIS sensitivity to implosion shape will be carried out to further extend reconstruction capabilities. Additionally, an improved camera timing system that will reduce uncertainties stemming from bang time jitter will also be fielded. The NIF GRH data recording system is more then 10 years old needs to be updated. Bandwidth and noise are a key limiting factor for improving data quality. New high bandwidth and low noise components will be tested at OMEGA in advance before fielding the components at NIF.

42 ENGINEERING↗

Evaluation of Gamma Ray Production - Quarterly Report FY22Q2

The LLNL team has performed the first systematic study of the effect of two-body weak currents in β decay rates across the entire mass table. In light and medium-mass nuclei, two-body weak currents from chiral effective field theory account for a significant portion of the phenomenological quenching of Gamow-Teller transition matrix elements. We examined the systematic effects of two-body axial currents on Gamow-Teller strength and β-decay rates in heavy nuclei within energy-density functional theory. We extended the charge-changing finiteamplitude pnFAM code to incorporate the contributions of two-body currents to the usual onebody linear response in the Gamow-Teller channel. We found that the two-body currents, as expected, usually quench both summed Gamow-Teller strength and decay rates, but by an amount that decreases as the neutron excess grows; see Fig. 1. In addition, they can enhance individual low-lying transitions, leading to decay rates that are quite different from those that an energy-independent quenching would produce, particularly in neutron-rich nuclei. This new physics capability is unique and provides the highest-fidelity description of β decay on the market. The underlying computational implementation can be reused to calculate γ-strength functions for finite-range nuclear potentials such as the Gogny force, which will allow us to benchmark some of our future developments against published results. The paper is in print in Phys. Rev. C.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DANCE and NEUANCE measurements of $^{233}U(n, \gamma$) (Q3 Report to NCSP on FY22)

The experiment was performed at the end of the CY20 runcycle and CY21. A total of 20 days were measured using the 20 mg sample, and the 10 mg sample was placed in the beam for a total of 2 days. The rest of the beam time was used to measure radioactive γ sources for energy calibration, background measurements, and tests to define the 233 U windows required during the data taking.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

233 U(n,$\gamma$) measurements at LANSCE [Slides]

A new measurement at LANSCE combined DANCE and NEUANCE at the end of 2020 and 2021. The 233 U material was provided by Oak Ridge National Laboratory (December 2020).Two samples of 10 mg and 20 mg of 233 U have been prepared at LANL by Evelyn M. Bond (December 2020). The experiment was performed in December 2020 and June/July 2021. Data analysis is ongoing to extract capture data knowing fission. LANL is looking forward to delivering the capture/fission ratio from (1-300) keV by the end of the FY2022.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Full Scale Engine Demonstration of Additively Manufactured High Gamma Prime Turbine Blade

Additive manufacturing (AM), also known as 3D printing, is a rapidly developing technology with tremendous potential in both developmental and production applications. Solar Turbines Incorporated is committed to AM technology development for gas turbine applications. The ability to metal 3D print novel designs of turbine blades capable of actual turbine engine operation would effectively reduce design validation cycle time and allow acquisition of key performance data early in a design campaign. In support of Solar’s advanced manufacturing development and ongoing engine efficiency improvement goals, ORNL and Solar conducted a project to 3D print, machine, inspect, and engine test a full set of Mercury TM 50 stage 2 turbine blades. This full-scale, hot-fired engine demonstration has identified both the capabilities and limitations of the current technologies required to produce turbine hot-section AM components.

36 MATERIALS SCIENCE↗

High Intensity Gamma Ray Source Scintillation Attenuation Spectrometer and Filter Stack Monoenergetic Calibration

The Laser-Based X-ray Radiographic Imaging team at Los Alamos National Lab is looking for a monoenergetic MeV X-ray source to both verify our Monte Carlo N-particle simulations of detector performance and calibrate the instruments for future measurements. Funded by the Laboratory Directed Research and Development (LDRD) program, our overall goal is to improve the radiographic quality and reliability of laser-based X-ray sources for deployment at both dynamic and static radiography facilities. Laser-based X-ray sources have demonstrated smaller spot sizes to current electron accelerator based sources. The smaller laser spot size leads to significantly improved resolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗