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At least 775 records · Page 43
All sourcesNASA NTRSDOE OSTI
NASA NTRS2011

TPSAS-NF1676L-13040-DND

We examine the feasibility of using airborne lidar data to: 1) infer CRC Convair-580 profiles of submicrometer fraction (SMF) over land (which is the fraction of aerosols with diameters less than 1 micrometer and is closely related to FMF) and 2) provide a proxy for CCN. If these initial Aerosol Extinction Aerosol Effective Radius feasibility studies prove successful, we will then apply these methodologies in subsequent studies to examine the feasibility of using CALIPSO data in a similar manner. We use data acquired by the NASA Langley Research Center airborne High Spectral Resolution Lidar (HSRL) during several recent field missions conducted by NASA, the Department of Energy, and NOAA. The airborne HSRL, which has acquired over 300 hours of data coincident with CALIPSO overpasses, measures aerosol extinction (532 nm), backscatter (532 and 1064 nm), and depolarization (532 and 1064 nm) profiles and thereby provides a dataset directly applicable to the CALIPSO measurements. During several of these field campaigns, airborne in situ measurements were acquired simultaneously within the HSRL “curtains” thereby facilitating direct correlations of the lidar observables to in situ measurements of particle size and composition, including SMF and CCN concentration. Previous studies have used simultaneous in situ measurements of SMF and Angström exponents derived from in situ scattering (Anderson et al., 2005) and remote sensing extinction (Redemann et al. 2009) measurements to build empirical relationships between these parameters. We adopt a similar approach and investigate relationships between the lidar observables, such as backscatter and extinction Angström exponents, with the coincident airborne in situ measurements of SMF and CCN concentration.

Richard Ferrare↗
NASA NTRSDate not supplied

TPSAS-NF1676L-23266-DND

Currently, near-surface air quality information (e.g. PM_2.5) must be inferred from column-integrated quantities (i.e. Aerosol Optical Thickness – AOT) obtained by passive remote sensing from downward-looking satellite instruments. Such retrievals must address the following questions: What do we use for the height of the aerosols? Mixed Layer (ML) height? Can we assume that near-surface aerosol extinction is about the same as the mean aerosol extinction in the ML? How well is near-surface extinction related to surface PM_2.5? How well can column AOT be used to infer near-surface aerosol extinction and PM_2.5?

Richard Ferrare↗
NASA NTRSDate not supplied

Distribution and Sources of Tropospheric Aerosols Over the Western North Atlantic During ACTIVATE (February-March 2020)

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) is a five-year (2019-2023) NASA Earth-Venture Suborbital-3 (EVS-3) mission to robustly characterize aerosol-cloud-meteorology interactions during February-June, with a focus on marine boundary layer clouds. This characterization requires understanding of aerosol composition, distribution, transport pathways, and sources. Here we use the GEOS-Chem chemical transport model driven by the MERRA-2 reanalysis to simulate tropospheric carbon monoxide (CO) and aerosols over the western North Atlantic Ocean (WNAO) during the first field deployment of ACTIVATE (February-March 2020). CO is used as a tracer to diagnose transport pathways for continental pollution outflow to the WNAO. The aerosol simulation represents all major aerosols including sulfate-nitrate-ammonium (SNA), mineral dust, sea salt, black and organic carbon aerosols. Model-simulated mixing ratios of SNA and organic carbon are compared with aircraft observations. We show that intensive aerosol mass measurements in the lower troposphere over the North American outflow region during ACTIVATE provide strong constraints on model aerosol wet scavenging. Comparisons of model aerosol extinctions with the airborne High Spectral Resolution Lidar-2 (HSRL-2) measurements indicate that the model generally captures continental outflow of aerosols and enhanced extinctions associated with sea salt. Simulated aerosol optical depths (AODs) and extinction vertical profiles are also compared with satellite retrievals from MODIS/Aqua and CALIOP/CALIPSO, respectively. CALIOP sometimes observes enhanced aerosol extinction at altitudes between ~1.5km and ~2.0km south of 32°N. The model reproduces this enhancement and attributes it to coarse-mode sea salt associated with high relative humidity. The relative contributions of continental and oceanic sources to the aerosol loading, AOD, and their distributions over the study domain will also be discussed.

aerosols↗
NASA NTRSDate not supplied

Effects of Ambient Inert Gas Properties on Cool-Flame Combustion of Normal-Alkane Droplets in Microgravity

Cool-flame-supported quasi-steady droplet combustion was first observed during droplet combustion experiments conducted onboard the International Space Station (ISS) in the Combustion Integrated Rack (CIR) with n-alkane fuels. These cool flames, not visible to the naked eye, result from the existence of the negative-temperature-coefficient (NTC) region during the combustion n-alkane fuels when the chemical-kinetic pathways experience a transition from the low-temperature chemistry to the normal, high-temperature-controlled chemistry. In this study, we present results for the cool-flame-supported droplet burning rates and extinction diameters for n-alkane fuels (n-heptane, n-octane, n-decane, and n-dodecane) in inert-diluent-substituted ambient environments. In these ISS experiments, some of the nitrogen in the ambient gas mixture is replaced by an inert gas, namely, carbon dioxide, helium, or xenon. Different diluents were observed to exert remarkably different influences on the cool-flame combustion of fuel droplets. The results show that the cool-flame extinction diameter is drastically increased with helium dilution compared to N2, CO2 or Xe, and Xe dilution leads to longer burning with a smaller extinction diameter. Unlike hot flames, the cool-flame burning rates are controlled by the cool-flame temperature established in the NTC region by the chemical kinetics, rather than by equilibrium thermodynamics, and the thermo-physical properties of the ambient gases, which control the heat feed back to the liquid droplet. The cool-flame extinction is triggered by the instability that occurs at the low-temperature end of the NTC region, below which cool diffusion flames become statically unstable. A quasi-steady theoretical model, presented earlier, which involves a six-step reduced-chemistry mechanism, valid around the lower end of the NTC region, is shown to explain the observed experimental trends qualitatively.

microgravity↗
NASA NTRS2021

Evidence for the predictability of changes in the stratosphericaerosol size following volcanic eruptions of diverse magnitudesusing space-based instruments

An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption’s main aerosol layer and the wavelength dependence of that perturbation. This relationship spans multiple orders of magnitude in the aerosol extinction coefficient of stratospheric impact of volcanic events. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. We note limitations on this analysis including that the presence of significant amounts of ash in the main sulfuric acid aerosol layer and other factors may significantly modulate these results. Despite these limitations, the findings suggest an avenue for improving aerosol extinction coefficient measurements from single-channel observations such as the Optical Spectrograph and Infrared Imager System as they rely on a prior assumptions about particle size. They may also represent a distinct avenue for the comparison of observations with interactive aerosol models used in global climate models and Earth system models.

Larry W Thomason↗
NASA NTRSDate not supplied

Shortwave Broadband Irradiance Computations Using Cloud Properties Combined from CALIPSO, CloudSat, and MODIS

In this study, cloud properties measured from the CALIPSO, CloudSat, and MODIS (CCM) are used for top-of-atmosphere (TOA) shortwave (SW) broadband (BB) irradiance computations. The CALIPSO and CloudSat active sensors provide detailed cloud vertical profiles, but these occasionally miss parts of the cloud columns due to the full attenuation of sensor signals, surface clutter, or insensitivity to a certain range of cloud particle sizes. As a result, the CCM-merged cloud extinction coefficient profiles can be underestimated. Therefore, we compare the column-integrated visible scaled cloud optical depth (VSCOD) of the CCM-merged cloud extinction coefficient profile with the MODIS-estimated VSCOD and apply a scaling factor to the CCM-merged cloud extinction profile. The VSCOD is defined as a visible cloud optical depth multiplied by (1¬–asymmetry parameter). The SW irradiances are computed using the scaled CCM-merged cloud extinction coefficient and effective radius profiles. It is shown that the multi-sensor-combined cloud profiles significantly reduce positive TOA SW BB biases, compared to those with MODIS-derived cloud properties only. The improvement is more pronounced for optically thick clouds, where MODIS ice particle effective radius is largely underestimated.

Cloud↗
NASA NTRSDate not supplied

Evaluation of GEOS Aerosols Using CAMP2Ex Observations

Biomass burning aerosol impacts aspects of the atmosphere and Earth system through direct and semi-direct effects, as well as influencing air quality. Despite its importance, the representation of biomass burning aerosol is not always accurate in numerical weather prediction and climate models or reanalysis products. Using observations collected as part of the Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) in August through October of 2019, aerosol concentration and optical properties are evaluated within the Goddard Earth Observing System (GEOS) and its underlying aerosol module, GOCART. In the operational configuration, GEOS assimilates aerosol optical depth observations at 550 nm from AERONET and MODIS to constrain aerosol fields. Particularly for biomass burning aerosol, without the assimilation of aerosol optical depth, aerosol extinction is underestimated compared to observations collected in the Philippines region during the CAMP2Ex campaign. The assimilation process adds excessive amounts of carbon to account for the underestimated extinction, resulting in positive biases in the mass of black and organic carbon, especially within the boundary layer, relative to in situ observations from the Langley Aerosol Research Group Experiment. Counteracting this, GEOS is deficient in sulfate and nitrate aerosol just above the boundary layer. Aerosol extinction within GEOS is a function of the mass of different aerosol species, the ambient relative humidity, the assumed spectral optical properties, and particle size distribution per species. The relationship between dry and ambient extinction in GEOS reveals that hygroscopic growth is too high within the model for biomass burning aerosol. An additional concern lies in the assumed particle size distribution for GEOS, which has a single mode radius that is too small for organic carbon. Variability in the observed particle size distribution for biomass burning aerosol within a single flight also illuminates the fact that a single assumed particle size distribution is not sufficient and that for a proper representation, a more advanced aerosol module within GEOS may be necessary.

Allison Collow↗
NASA NTRS2024

CREST: a Climate Data Record of Stratospheric Aerosols

Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived using data from six limb and occultation satellite instruments: SAGE (Stratospheric Aerosol and Gas Experiment) II on ERBS (Earth Radiation Budget Satellite), GOMOS (Global Ozone Monitoring by Occultation of Stars) and SCIAMACHY (Scanning Imaging Spectrometer for Atmospheric Chartography) on Envisat, OSIRIS (Optical Spectrograph and InfraRed Imaging System) on Odin, OMPS (Ozone Monitor Profiling Suite Limb Profiler) on Suomi NPP, and SAGE III on the ISS (International Space Station). The merging of aerosol profiles is performed via the transformation of the aerosol datasets from individual satellite instruments to the same wavelength (750 nm) and their de-biasing and homogenization by adjusting the seasonal cycles. After such homogenization, the data from individual satellite instruments are in good agreement. The merged aerosol extinction coefficient is computed as the median of the adjusted data from the individual instruments. The merged time series of vertically resolved monthly mean aerosol extinction coefficients at 750 nm is provided in 10° latitudinal bins from 90° S to 90° N, in the altitude range from 8.5 to 39.5 km. The time series of the stratospheric aerosol optical depth (SAOD) is created via the integration of aerosol extinction profiles from the tropopause to 39.5 km; it is also provided as monthly mean data in 10° latitudinal bins. The created aerosol climate record covers the period from October 1984 until December 2023, and it is intended to be extended in the future. The merged CREST aerosol dataset (v2) is available at https://doi.org/10.57707/fmib2share.dfe14351fd8548bcaca3c2956b17f665 (Sofieva et al., 2024a). It can be used in various climate-related studies.

Viktoria F Sofieva↗
NASA NTRS1971

Absorbing ice model of interstellar grains.

Extinction curves have been calculated for Mie scattering by grains with a refractive index m equals to n - ik, where n was between 1.3 and 2.0 and k varied from 0 to 0.5. A good fit for the observed interstellar extinction in the wavelength region of 0.1 to 2.0 microns was obtained for particles with a radius of 0.1 micron and m equal to 1.3 - 0.2i. Inclusion of the changes in the refractive index in the vacuum ultraviolet region due to the strong absorptions of methane, ammonia and water does not appreciably alter these results. Theoretical extinction curves for the composite medium of H2O, NH3, CH4, and graphite show a general agreement with the observed interstellar reddening curve over the whole spectral range, in addition to producing kinks in the far-ultraviolet region.

Swamy, K. S. K.↗
NASA NTRS1974

Dust in the galactic center

The strength of the 9.7 microns absorption band in the radiation from the galactic center is used to deduce a range of measures of the visual extinction from 20 to 400 magnitudes. A possible way of arriving at a unique value of the visual extinction consistent with variations in the wavelength dependence of extinction as a function of grain characteristics is indicated. The mass of silicates deduced from the 9.7 microns band appears to imply a gradient of metallicity towards the galactic center.

Greenberg, J. M.↗
NASA NTRS1975

The rocket ultraviolet spectrum of the planetary nebula NGC 7027

An ultraviolet spectrum of NGC 7027 was obtained with a rocket-borne telescope. The observed fluxes are given on an absolute basis and upper limits are given for the strongest predicted lines which were not observed. The extinction correction was made on the basis of the observed and calculated line ratios for the hydrogenic recombination line of He 2 at 1640A to H beta. The extinction is in agreement with ground based determinations. When corrected for extinction the C 4 resonance line at 1549A is in good agreement with the intensity calculated from models, but the C 3 intercombination line at 1909A is a factor of ten too bright. The addition of dielectronic recombination to the models sufficiently changes the C 3 concentration to reduce the discrepancy to a factor of four. The abundance of carbon is assumed to be 2 x 0.0001 that of hydrogen. Using carbon abundances for the sun, this discrepancy disappears and there must be attenuation in the C 4 line. Since the optical depth is approximately 10,000 at the line center, no appreciable number of absorbing grains can exist in the C 4 producing region of the nebula.

Bohlin, R. C.↗
NASA NTRS1974

Respirable particulate monitoring with remote sensors. (Public health ecology: Air pollution)

The feasibility of monitoring atmospheric aerosols in the respirable range from air or space platforms was studied. Secondary reflectance targets were located in the industrial area and near Galveston Bay. Multichannel remote sensor data were utilized to calculate the aerosol extinction coefficient and thus determine the aerosol size distribution. Houston Texas air sampling network high volume data were utilized to generate computer isopleth maps of suspended particulates and to establish the mass loading of the atmosphere. In addition, a five channel nephelometer and a multistage particulate air sampler were used to collect data. The extinction coefficient determined from remote sensor data proved more representative of wide areal phenomena than that calculated from on site measurements. It was also demonstrated that a significant reduction in the standard deviation of the extinction coefficient could be achieved by reducing the bandwidths used in remote sensor.

Severs, R. K.↗
NASA NTRS1977

Seismotectonic, structural, volcanologic, and geomorphic study of New Zealand; indigenous forest assessment in New Zealand; mapping, land use, and environmental studies in New Zealand, volume 1

The author has identified the following significant results. Results of the atmospheric extinction measurements show clearly the greater opacity of the atmosphere in MSS band 4 which is due to Rayleigh scattering. Atmospheric water vapor absorbs strongly in a wide region between 900 nm and 1000 nm, and this results in a consistently higher extinction coefficient than would otherwise be expected in MSS band 7. The short term fluctuations tend to be greater in band 7 than in the other bands, and this effect is probably due to variations of water vapor concentration in the instrument line of sight. These high extinction coefficients and short term fluctuations in band 7 were observed at Menindee which is in a semi-desert region in western New South Wales.

Probine, M. C.↗
NASA NTRS1977

The spectral energy distribution of Zeta Puppis and HD 50896

The ultraviolet spectral energy distribution of the O5f star Zeta Pup and the WN5 star HD 50896 are derived from OAO-2 observations with the calibration of Bless, Code, and Fairchild (1976). An estimate of the interstellar reddening (0.12 magnitude) of the Wolf-Rayet star is determined from the size of the characteristic interstellar extinction bump at 4.6 inverse microns. After correction for extinction, both stars show a flat energy distribution in the ultraviolet. The distribution of HD 50896 from 1100 A to 2 microns is in good agreement with results of extended model atmospheres, but some uncertainty remains because of the interstellar-extinction correction. The absolute energy distribution of Zeta Pup is fitted by a 42,000-K plane-parallel model if the model's flux is adjusted for the effects of electron scattering in the stellar wind and for UV line blanketing that was determined empirically from high-resolution Copernicus satellite observations. To achieve this fit, it is necessary to push both the spectroscopically determined temperature and the ultraviolet calibration to the limits of their probable errors.

Holm, A. V.↗
NASA NTRS1976

Monitoring stratospheric ozone and aerosols using orbiting photoelectric detectors

Application of slightly modified off-the-shelf automatic celestial navigation systems ('star trackers') is considered for the purposes of monitoring variations in the optical depth of the stratospheric aerosol and ozone layers. The basic principle of the technique is to observe stars from an orbiting station as they are occulted by the stratospheric aerosol layer. Since molecular and refraction extinction are directly calculable, total extinction measurements using a dual-sensor (S4 and S20) approach allows us to directly solve for ozone and aerosol extinction and look for correlations between these two parameters. The technique appears promising for remotely monitoring aerosol and ozone optical depth in the 15-25 km region over selected locations and is independently accurate if aerosol composition and relative size distribution are invariant.

Matloff, G. L.↗
NASA NTRS1979

Stellar occultation studies of the solar system

The paper covers the principles, observational procedures, and results relating to occultations of stars by solar system bodies other than the moon. Physical processes involved in occultations are presented including (1) extinction by ring material, (2) differential refraction by a planetary atmosphere, (3) extinction by a planetary atmosphere, and (4) Fresnel diffraction by sharp edges. It is noted that from a sufficient number of immersion and emersion timings of a stellar occultation, the radius and ellipticity of the occulting body can be accurately determined. From an occultation by a planet having an atmosphere, temperature, pressure, and number density profiles can be obtained along with information about the composition of the atmosphere and the extinction.

Elliot, J. L.↗
NASA NTRS1979

Ultraviolet observations of interstellar molecules and grains from Spacelab

The paper presents observational results obtained on interstellar grains and molecules and suggests promising areas for Spacelab research. Regarding grains, useful data can be expected on the shape of the ultraviolet extinction curve for new interstellar regions, on the nature of UV extinction at short wavelengths, the presence of structure in the UV extinction curve comparable to the visible-wavelength diffuse bands, and the polarization properties of grains in UV wavelengths. The advances in observations of molecules will include the ability to prove more heavily-obscured regions, coverage of wavelength regions inadequately studied with previous instruments, and the capability of observing in optical absorption species detected in the same line of sight in radio emission.

Snow, T. P., Jr.↗
NASA NTRS1981

H I and dust in Kutner's cloud

A map in the 1.420 GHz line of H I, with an angular resolution of 9.1 arcmin, is made toward Kutner's Cloud and the region between Kutner's Cloud and Heiles' Cloud. It is assumed that the cold H I in the clouds is located only in front of, and absorbs the H I background; the column density of cold H I, N(H I), is obtained from this absorption. The visual extinction for this region is determined from star counts on red and blue POSS prints. It is noted that most of the gas in the cloud is in the form of H2. The column density of H2 is obtained from the visual extinction and the extinction-to-gas ratio given by Bohlin et al. (1978).

Batrla, W.↗