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At least 775 records · Page 43

Gravitation research

Gravitation research - experimental test of Freundlich red-shift hypothesis and measurement of metastable vs ground-state electron exchange cross sections for helium and neon

HELIUM↗

Ground-based measurements of galactic cosmic ray fragmentation in shielding

The mean free path for nuclear interactions of galactic cosmic-rays is comparable to shielding and tissue thicknesses present in human interplanetary exploration, resulting in a significant fraction of nuclear reaction products at depth. In order to characterize the radiation field, the energy spectrum, the angular distribution, and the multiplicity of each type of secondary particles must also be known as a function of depth. Reactions can take place anywhere in a thick absorber; therefore, it is necessary to know these quantities as a function of particle energy for all particles produced. HZE transport methods are used to predict the radiation field; they are dependent on models of the interaction of man-made systems with the space environment to an even greater extent than methods used for other types of radiation. Hence, there is a major need to validate these transport codes by comparison with experimental data. The most cost-effective method of validation is a comparison with ground-based experimental measurements. A research program to provide such validation measurements using neon, iron and other accelerated heavy ion beams will be discussed and illustrated using results from ongoing experiments and their comparison with current transport codes. The extent to which physical measurements yield radiobiological predictions will be discussed.

NASA Discipline Radiation Health↗

A Green's function method for high charge and energy ion transport

A heavy-ion transport code using Green's function methods is developed. The low-order perturbation terms exhibiting the greatest energy variation are used as dominant energy-dependent terms, and the higher order collision terms are evaluated using nonperturbative methods. The recently revised NUCFRG database is used to evaluate the solution for comparison with experimental data for 625A MeV 20Ne and 517A MeV 40Ar ion beams. Improved agreements with the attenuation characteristics for neon ions are found, and reasonable agreement is obtained for the transport of argon ions in water.

Energy Transfer↗

Heavy ion observations by MARIE in cruise phase and Mars orbit

The charged particle spectrum for nuclei from protons to neon, (charge Z=10) was observed during the cruise phase and orbit around Mars by the MARIE charged particle spectrometer on the Odyssey spacecraft. The cruise data were taken between April 23, 2001 and mid-August 2001. The Mars orbit data were taken March 5, 2002 through May 2002 and are scheduled to continue until August 2004. Charge peaks are clearly separated for charges up to Z=10. Especially prominent are the carbon and oxygen peaks, with boron and nitrogen also clearly visible. Although heavy ions are much less abundant than protons in the cosmic ray environment, it is important to determine their abundances because their ionization energy losses (proportional to Z2) are far more dangerous to humans and to instruments. Thus the higher charged nuclei make a significant contribution to dose and dose equivalent received in space. Results of the charged particle spectrum measurements will be reported. c2003 COSPAR. Published by Elsevier Ltd. All rights reserved.

NASA Center JSC↗

IUPAC Periodic Table of Isotopes for the Educational Community

John Dalton first proposed the concept of atomic weights of the elements in the first decade of the nineteenth century. These atomic weights of the chemical elements were thought of as constants of nature, similar to the speed of light. Dmitri Mendeleev arranged the atomic weights of the elements in ascending order of value and used the systematic variation of their chemical properties to produce his Periodic Table of the Elements in 1869. Measurement of atomic weight values became an important chemical activity for a century and a half. Theodore Richards received a Noble Prize for his work in this area. In 1913, Fredrick Soddy found a species of radium, which had an atomic weight value of 228, compared to the familiar radium gas value of 226. Soddy coined the term 'isotope' (Greek for 'in the same place') to account for this second atomic weight value in the radium position of the Periodic Table. Both of these isotopes of radium are radioactive. Radioactive isotopes are energetically unstable and will decay (disintegrate) over time. The time it takes for one half of a sample of a given radioactive isotope to decay is the half-life of that isotope. In addition to having different atomic weight values, radium-226 and radium-228 also have different half-life values. Around the same time as Soddy's work, J.J. Thomson (discoverer of the electron) identified two stable (non-radioactive) isotopes of the same element, neon. Over the next 40 years, the majority of the known chemical elements were found to have two or more stable (or long-lived radioactive isotopes that contribute significantly to the determination of the atomic weights of the elements).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Materials Irradiation Facility (MIF) at the High Flux Isotope Reactor (HFIR)

The Material Irradiation Facility (MIF) at the Oak Ridge National Laboratory (ORNIL) High Flux Isotope Reactor (HIFR) controls and monitors instrumented irradiation experiments for materials and fuel research. In 2013 ORNIL founded a Laboratory Directed Research and Development project to reinvigorate the use of instrumented experiments by redesigning MIF to enhance its capabilities. MIF improvements include an updated and more sophisticated experiment monitoring system, a modular design allowing easier addition of simultaneous experiments, and features that allow rapid incorporation of additional instrumentation Interest in materials and fuel irradiation has increased significantly over the last decade. Much of this interest is related to investigating the performance of advanced materials for fusion environments, designing and developing improved fuel and cladding materials, and examining material characteristics and behavior under irradiation conditions. At ORNL, the irradiation engineering team has more than 60 years of experience designing and fabricating various types of irradiation experiments. Rabbit capsule experiments are small scale and relatively inexpensive. These capsules are typically designed to be irradiated in the flux-trap region of the core. Full-length target capsules are larger scale and could be either instrumented or non-instrumented. These more complicated capsules can be irradiated in any of the experiment facilities at HFIR. Instrumented experiment irradiation provides significant advantages for researchers. The unique advantage is that the researcher can monitor and acquire in situ data and change capsule operating conditions in real time during the irradiation. This capability enables tight control of desired experimental conditions so that they match the design specifications throughout the irradiation. Also, the experiment conditions (e.g., temperature and pressure) can be altered during the test, enabling significant flexibility and the ability to collect considerably more data from a single experimental capsule. This capability allows measurement of a variety of material properties (conductivity, fission product composition, etc.) that otherwise would only be available upon post-irradiation examination, where non-equilibrium conditions brought on by irradiation do not exist. The data generated by these experiments contribute significantly to the understanding of material behavior under irradiation. MIF is an experimental platform that can host fully instrumented and monitored experiments in a high neutron flux environment. Its primary functions are to provide clean inert gas (helium, neon, argon) to experiments at controlled pressures and flows, monitor irradiation conditions (typically temperatures and pressures) during irradiation, and monitor effluent gases from experiments. This facility allows monitoring of chemical processes during a fueled irradiation, where this becomes important for detecting fuel failures. This paper reports the efforts towards reestablishing the value of HFIR for instrumented irradiation experiments and the improvements to MIF that ultimately reduce the costs of instrumented irradiation. This project advances ORNL materials capabilities to new levels by providing a state-of-the art, robust and flexible facility that can be expanded as customer requirements change, while supporting the goals of the fusion, advanced fuels, and structural materials programs. (authors)

42 ENGINEERING↗

The thermal equation of state of (Mg, Fe)SiO 3 bridgmanite (perovskite) and implications for lower mantle structures

The high–pressure/high–temperature equation of state (EOS) of synthetic 13% Fe–bearing bridgmanite (Mg silicate perovskite) is measured using powder X–ray diffraction in a laser–heated diamond anvil cell with a quasi–hydrostatic neon pressure medium. We compare these results, which are consistent with previous 300 K sound speed and compression studies, with a reanalysis of Fe–free Mg end–member data from Tange et al. (2012) to determine the effect of iron on bridgmanite's thermoelastic properties. EOS parameters are incorporated into an ideal lattice mixing model to probe the behavior of bridgmanite at deep mantle conditions. With this model, a nearly pure bridgmanite mantle composition is shown to be inconsistent with density and compressibility profiles of the lower mantle. We also explore the buoyant stability of bridgmanite over a range of temperatures and compositions expected for Large Low–Shear Velocity Provinces, concluding that bridgmanite–dominated thermochemical piles are more likely to be passive dense layers externally supported by convection, rather than internally supported metastable domes. Here, the metastable dome scenario is estimated to have a relative likelihood of only 4–7%, given the narrow range of compositions and temperatures consistent with seismic constraints. If buoyantly supported, such structures could not have remained stable with greater thermal contrast early in Earth's history, ruling out formation scenarios involving a large concentration of heat producing elements.

58 GEOSCIENCES↗

Elastic softening in Fe 7 C 3 with implications for Earth's deep carbon reservoirs

Iron carbide Fe 7 C 3 has recently emerged as a potential host of reduced carbon in Earth's mantle and a candidate component of the inner core, but the equation of state of Fe 7 C 3 is still uncertain, partly because the nature of pressure–induced magnetic transitions in Fe 7 C 3 and their elastic effects remain controversial. Here we report the compression curve of hexagonal Fe 7 C 3 in neon medium with dense pressure sampling and in comparison with pure iron in the same loading. Here, the results revealed elastic softening between 7 GPa and 20 GPa, which can be attributed to noncollinear alignment of spin moments in a state between the ferromagnetic and paramagnetic phases, as expected for Invar–type alloys. The volume reduction associated with the softening would enhance the stability of Fe 7 C 3 in the deeper part of the upper mantle and transition zone. As a result of subsequent spin crossover at higher pressures, Fe 7 C 3 at inner core conditions likely occurs as the nonmagnetic phase, which remains a candidate for the major component of the Earth's central sphere.

58 GEOSCIENCES↗

Electronic environments of ferrous iron in rhyolitic and basaltic glasses at high pressure: Silicate Glasses at High Pressure

The physical properties of silicate melts within Earth's mantle affect the chemical and thermal evolution of its interior. Chemistry and coordination environments affect such properties. We have measured the hyperfine parameters of iron-bearing rhyolitic and basaltic glasses up to ~120 GPa and ~100 GPa, respectively, in a neon pressure medium using time domain synchrotron Mössbauer spectroscopy. The spectra for rhyolitic and basaltic glasses are well explained by three high-spin Fe 2+ -like sites with distinct quadrupole splittings. Absence of detectable ferric iron was confirmed with optical absorption spectroscopy. The sites with relatively high and intermediate quadrupole splittings are likely a result of fivefold and sixfold coordination environments of ferrous iron that transition to higher coordination with increasing pressure. The ferrous site with a relatively low quadrupole splitting and isomer shift at low pressures may be related to a fourfold or a second fivefold ferrous iron site, which transitions to higher coordination in basaltic glass, but likely remains in low coordination in rhyolitic glass. These results indicate that iron experiences changes in its coordination environment with increasing pressure without undergoing a high-spin to low-spin transition. We compare our results to the hyperfine parameters of silicate glasses of different compositions. With the assumption that coordination environments in silicate glasses may serve as a good indicator for those in a melt, this study suggests that ferrous iron in chemically complex silicate melts likely exists in a high-spin state throughout most of Earth's mantle.

58 GEOSCIENCES↗

New Directions in Focused Ion Beam Induced Deposition for the Nanoprinting of Functional 3D Heterostructures

The focused ion beam (FIB) microscope is well established as a high-resolution machining instrument capable of site-selectively removing material down to the nanoscale. Beyond subtractive processing, however, the FIB can also add material via a technique known as focused ion beam induced deposition (FIBID). Using FIBID, the FIB can thus be employed for the direct-write of complex nanostructures. This work explores new directions in three-dimensional FIBID nanoprinting, harnessing unique features of helium and neon FIBs. In particular, the superior spatial resolution of these novel FIBs is leveraged to fabricate precise multimaterial architectures, an isotope effect is used to create satellite deposits, and dose-controlled implantation of the gaseous ions is used to engineer internal voids. In the context of voids, the fabrication of hollow nanopillars by helium-FIBID due to concurrent milling (as shown previously by others) is revisited. Insight into the chemical and structural composition of the nanostructures is obtained using advanced electron microscopy, accurately revealing buried interfaces, crystallite distributions, chemical compositions, and material transformations. Next-generation devices and technologies that could be enabled by the novel heterostructures demonstrated here are discussed, setting the stage for the potential evolution of FIBID into a versatile platform for functional nanomaterials design and fabrication.

FIBID↗

UEDGE modelling of detached divertor operation for long-leg divertor geometries in ARC

In this work, simulations of the ARC scrape-off layer and divertor configuration are carried out using UEDGE to perform the first power-handling assessment for the divertor design. A convective–diffusive anomalous transport model is implemented in the code to reproduce the radial plasma profiles anticipated for the device at the outer mid-plane. Levels of exhaust power from the core are varied, and a 0.5% fixed fraction neon impurity seeding is included in investigations to find steady-state detached solutions. Initial studies employing a super-X divertor configuration have shown that a stable detached divertor-operational window exists for reactor exhaust powers in the range of 72–92 MW, which is close to projected levels of exhaust power of 105 MW across the separatrix anticipated for ARC. Under these conditions, the divertor heat flux is fully dissipated by radiation and radial losses to the sidewalls of the divertor channel, leading to acceptable levels of power flux density on plasma-facing components. Simulations are being extended to study the performance of the X-point target geometry and to explore the sensitivity to the physics model and input parameters.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

UEDGE modeling of plasma detachment of CFETR with ITER ‐like divertor geometry by external impurity seeding

Abstract Efficient handling of high heat flux on the plasma‐facing components, particularly the divertor targets, poses a significant challenge for the Chinese Fusion Engineering Testing Reactor (CFETR) with fusion power of Gigawatt. This work investigates the divertor plasma detachment of CFETR with a standard ITER‐like divertor geometry by neon (Ne) or argon (Ar) impurity seeding using UEDGE code. The cross‐field drifts terms are switched off, and fluid neutral models and a “fixed‐fraction” impurity model are applied to enable efficient simulations for the study of CFETR detachment. In order to reduce the heat load on the divertor targets below the acceptable level (<10 MW/m 2 ), the impurity fraction ( f ), pumping speed ( S ), and upstream density are varied to identify the suitable operations window during Ne seeding. The effects of Ne and Ar impurities on the plasma detachment are compared. It is found that with the power across the core‐edge interface P SOL = 200 MW and separatrix density of 2.8 10 19 , Ne impurity fraction ≥1.7%, and Ar impurity fraction ≥0.24% can achieve the partial detachment. Achieving similar total radiation power (˜148 MW), the Ne fraction is 2.3% and the Ar fraction is 0.24%. Moreover, the simulation results indicate that Ar exhibits better power radiation efficiency and core compatibility compared with Ne.

Zhang, M. Z.↗