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At least 775 records · Page 43
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Atomic-scale visualization of a cascade of magnetic orders in the layered antiferromagnet GdTe3

Abstract GdTe 3 is a layered antiferromagnet which has attracted attention due to its exceptionally high mobility, distinctive unidirectional incommensurate charge density wave (CDW), superconductivity under pressure, and a cascade of magnetic transitions between 7 and 12 K, with as yet unknown order parameters. Here, we use spin-polarized scanning tunneling microscopy to directly image the charge and magnetic orders in GdTe 3 . Below 7 K, we find a striped antiferromagnetic phase with twice the periodicity of the Gd lattice and perpendicular to the CDW. As we heat the sample, we discover a spin density wave with the same periodicity as the CDW between 7 and 12 K; the viability of this phase is supported by our Landau free energy model. Our work reveals the order parameters of the magnetic phases in GdTe 3 and shows how the interplay between charge and spin can generate a cascade of magnetic orders.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Evidence for charge delocalization crossover in the quantum critical superconductor CeRhIn5

Abstract The nature of charge degrees-of-freedom distinguishes scenarios for interpreting the character of a second order magnetic transition at zero temperature, that is, a magnetic quantum critical point (QCP). Heavy-fermion systems are prototypes of this paradigm, and in those, the relevant question is where, relative to a magnetic QCP, does the Kondo effect delocalize their f -electron degrees-of-freedom. Herein, we use pressure-dependent Hall measurements to identify a finite-temperature scale E loc that signals a crossover from f -localized to f -delocalized character. As a function of pressure, E loc ( P ) extrapolates smoothly to zero temperature at the antiferromagnetic QCP of CeRhIn 5 where its Fermi surface reconstructs, hallmarks of Kondo-breakdown criticality that generates critical magnetic and charge fluctuations. In 4.4% Sn-doped CeRhIn 5 , however, E loc ( P ) extrapolates into its magnetically ordered phase and is decoupled from the pressure-induced magnetic QCP, which implies a spin-density-wave (SDW) type of criticality that produces only critical fluctuations of the SDW order parameter. Our results demonstrate the importance of experimentally determining E loc to characterize quantum criticality and the associated consequences for understanding the pairing mechanism of superconductivity that reaches a maximum T c in both materials at their respective magnetic QCP.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Helimagnetic Structure and Heavy-Fermion-Like Behavior in the Vicinity of the Quantum Critical Point in Mn 3 P

Antiferromagnet Mn 3 P with Neel temperature T N =30 K is composed of Mn tetrahedrons and zigzag chains formed by three inequivalent Mn sites. Due to the nearly frustrated lattice with many short Mn-Mn bonds, competition of the exchange interactions is expected. We here investigate the magnetic structure and physical properties including pressure effect in single crystals of this material, and reveal a complex yet well-ordered helimagnetic structure. The itinerant character of this materials is strong, and the ordered state with small magnetic moments is easily suppressed under pressure, exhibiting a quantum critical point at ~1.6 GPa. The remarkable mass renormalization, even in the ordered state, and an incoherent-coherent crossover in the low-temperature region, characterize an unusual electronic state in Mn 3 P, which is most likely effected by the underlying frustration effect.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1993

Magnetohydrodynamic wave propagation in one-dimensional nonhomogeneous, self-gravitating clouds

We study the propagation of magnetohydrodynamic (MHD) waves through nonhomogeneous, selfgravitating, magnetic media representative of molecular cloud environments and focus on the issues of cloud support and line profiles. Since the general treatment of this topic is burdened by a complex mathematical formalism, we consider simplifying geometries which yield analytical solutions in the linear wave limit. In particular, we study both magnetoacoustic and Alfven wave propagation along the density gradient in a one-imensional slab. Of specific relevance to molecular clouds, we find that the back reaction of the Alfven waves can provide a pressure along the direction of the magnetic field lines; this pressure can help support a density enhancement against gravitational collapse. Furthermore, we find that the velocity amplitudes of these waves increase as the density decreases, in rough agreement with observational estimates of line width versus density relations.

Fatuzzo, Marco↗
NASA NTRS1977

Lunar electrical conductivity, permeability and temperature from Apollo magnetometer experiments

Magnetometers were deployed at four Apollo sites on the moon to measure remanent and induced lunar magnetic fields. Measurements from this network of instruments were used to calculate the electrical conductivity, temperature, magnetic permeability, and iron abundance of the lunar interior. The measured lunar remanent fields range from 3 gammas minimum at the Apollo 15 site to 327 gammas maximum at the Apollo 16 site. Simultaneous magnetic field and solar plasma pressure measurements show that the remanent fields at the Apollo 12 and 16 sites interact with, and are compressed by, the solar wind. Remanent fields at Apollo 12 and Apollo 16 are increased 16 gammas and 32 gammas, respectively, by a solar plasma bulk pressure increase of 1.5 X 10 to the -7th power dynes/sq cm. Global lunar fields due to eddy currents, induced in the lunar interior by magnetic transients, were analyzed to calculate an electrical conductivity profile for the moon. From nightside magnetometer data in the solar wind it was found that deeper than 170 km into the moon the conductivity rises from .0003 mhos/m to .10 mhos/m at 100 km depth. Recent analysis of data obtained in the geomagnetic tail, in regions free of complicating plasma effects, yields results consistent with nightside values.

Dyal, P.↗
NASA NTRS1999

Measurements of Tc (Q,P): Depression of the Superfluid Transition Temperature by a Heat Current Along the Lambda Line

We report experimental measurements of Tc (Q,P) for heat currents (Q) between I1and 100 micro W/sq cm and pressure (P) between SVP and 15 bar. The measurements were performed in a normal gravity environment, using the low-gravity simulator facility at JPL without the magnet being energized. The sample pressure was controlled to 0.1 micro bar using a hot volume, and a Straty-Adams capacitive pressure gauge. The total volume of helium in the sample cell and the hot volume was held constant using a pneumatic low temperature valve. A melting curve thermometer (MCT) measured the transition temperature (Tc) with a resolution of about 10 nK through a sidewall probe of the thermal conductivity sample cell. We employed the same measurement technique and procedure described by DAS. Preliminary results indicate that Tc (Q,P) depends very little on the pressure in the pressure range between SVP and 15 bar with a variation in the amplitude of Tc(Q,P) of less than about 5% observable in this pressure range. According to the Renormalization-group theory calculation by Haussmann and Dohm, the amplitude of Tc (Q,P) has a leading pressure-dependence term proportional to xi(sub 0) (sup (1/nu)), where xi(sub 0) is the correlation-length amplitude and nu is the correlation-length exponent. Thus, a small pressure dependence of the amplitude of Tc (Q,P) is expected since xi(sub 0) is very weakly dependent on pressure between SVP and 15 bar, consistent with our measurements.

Liu, Yuan-Ming↗
DOE OSTI2020

Experimental evaluation of shear modulus scaling of dynamic strength at extreme pressures

Recent progress in the development of dynamic strength experimental platforms is allowing for unprecedented insight into the assumptions used to construct constitutive models operating in extreme conditions. In this work, we make a quantitative assessment of how tantalum strength scales with its shear modulus to pressures of hundreds of gigapascals through a cross-platform examination of three dynamic strength experiments. Specifically, we make use of Split–Hopkinson pressure bar and Richtmyer–Meshkov instability experiments to assess the low-pressure strain and strain rate dependence. Concurrent examination of magnetically driven ramp-release experiments up to pressures of 350GPa allows us to examine the pressure dependence. In this work, using a modern description of the shear modulus, validated against both ab initio theory and experimental measurements, we then assess how the experimentally measured pressure dependence scales with shear modulus. Furthermore, we find that the common assumption of scaling strength linearly with the shear modulus is too soft at high pressures and offer discussion as to how descriptions of slip mediated plasticity could result in an alternative scaling that is consistent with the data.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Scaling theory of three-dimensional magnetic reconnection spreading

We develop a first-principles scaling theory of the spreading of three-dimensional (3D) magnetic reconnection of finite extent in the out of plane direction. This theory addresses systems with or without an out of plane (guide) magnetic field, and with or without Hall physics. The theory reproduces known spreading speeds and directions with and without guide fields, unifying previous knowledge in a single theory. New results include: (1) Reconnection spreads in a particular direction if an x-line is induced at the interface between reconnecting and non-reconnecting regions, which is controlled by the out of plane gradient of the electric field in the outflow direction. (2) The spreading mechanism for anti-parallel collisionless reconnection is convection, as is known, but for guide field reconnection it is magnetic field bending. We confirm the theory using 3D two-fluid and resistive-magnetohydrodynamics simulations. (3) The theory explains why anti-parallel reconnection in resistive-magnetohydrodynamics does not spread. (4) The simulation domain aspect ratio, associated with the free magnetic energy, influences whether reconnection spreads or convects with a fixed x-line length. (5) We perform a simulation initiating anti-parallel collisionless reconnection with a pressure pulse instead of a magnetic perturbation, finding spreading is unchanged rather than spreading at the magnetosonic speed as previously suggested. The results provide a theoretical framework for understanding spreading beyond systems studied here, and are important for applications including two-ribbon solar flares and reconnection in Earth’s magnetosphere.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

High-pressure neutron diffraction at ultra-low temperature

Neutron diffraction is a powerful tool in the study of quantum materials and associated emergent phenomena as it allows for direct detection of magnetic structure even at ultra-low temperatures. As pressure can drive systems across quantum critical points and tune emergent behaviors at the quantum scale, coupling neutron diffraction with extreme conditions of high pressure at (ultra-)low temperatures has been a key research target over decades. This has proven challenging as magnetic neutron diffraction typically requires large sample volumes due to flux limitations, whereas high-pressure studies require small sample volumes due to pressure limitations. Combining these two contradictory requirements poses many difficulties, but also brings opportunities in research and development. Here, we address these shortcomings through the use of a diamond anvil cell equipped with polycrystalline anvils with relatively large sample volumes coupled with the high neutron flux made available by the high-pressure diffractometer of the Spallation Neutron Source. This particular diamond anvil cell configuration has previously proven useful for single-crystal samples and is here coupled with the ultra-low temperatures of a dilution refrigerator for the first time. Our study on a single crystal of Yb 2 ⁢O 3 successfully collected magnetic neutron diffraction data at 5.3 GPa below 200 mK inside a dilution refrigerator. We have performed a detailed analysis of the magnetic diffraction data to investigate the magnetic structure under pressure and observed a subtle shift in the transition temperature. This development will open the door for future studies on magnetic materials with these much-desired coupled extremes of high pressure and ultra-low temperatures.

Wu, Yan [Oak Ridge National Laboratory (ORNL), Oak↗
NASA NTRS1974

Magnetic pinch compression of silica glass

SiO2 glass has been irreversibly densified by pressures up to 250 kbar produced in a magnetic pinch apparatus. The threshold for significant densification was about 60 kbar. The recovered densities agree better with published shock wave results than with static results.

Bless, S. J.↗
NASA NTRS1978

Interplanetary magnetic holes: Theory

Magnetic holes in the interplanetary medium are explained as stationary, non-propagating, equilibrium structures in which there are field-aligned enhancements of the plasma density and/or temperature. Magnetic anti-holes are considered to be associated with depressions in the plasma pressure. In this model, the observed changes in the magnetic field intensity and direction are due to diamagnetic currents that are carried by ions which drift in a sheath as the result of gradients in the magnetic field and in the plasma pressure within the sheath. The thickness of the sheaths considered is approximately a few ion Larmor radii. An electric field is normal to the magnetic field in the sheath. Solutions of Vlasov's equation and Maxwell's equations are presented which account for several types of magnetic holes, including null-sheets, that were observed.

Burlaga, L. F.↗
NASA NTRS1989

Electronically Variable Pressure Regulator (EVPR)

A new programmable electronically variable pressure regulator (EVPR) concept accurately controls the local outlet or remote system pressure. It uses an integral pulse width modulated rare earth permanent magnet motor operating in response to redundant pressure transducer feedback signals. The EVPR is a simple single stage device that does not use dynamic seals or pilot valving. Conversion of partial revolution motor torque to poppet lifting force is accomplished by pure flexure action to avoid using bearings. The flexure drive (called the ROTAX) has a variable lead to minimize motor weight and power consumption. Breadboard tests were completed successfully on two critical design elements of the EVPR: the ROTAX and the motor. The ROTAX cable system was tested for 250,000 cycles without failure. The breadboard motor met the basic design requirements including the design torque and power consumption. Prototype parts were fabricated, and testing of the prototype EVPR has started. It is PC computer controlled to facilitate programming, data acquisition and analysis. A lightweight dedicated microprocessor is planned for the flightweight EVPR.

Reinicke, R. H.↗
NASA NTRS1964

Magnetic fields and solar wind

Solar corpuscular radiation interaction with geomagnetic field - solar wind, interplanetary magnetic fields, magnetosphere boundary, and solar wind heating and sudden pressure changes

INTERPLANETARY MAGNETIC FIELD↗
NASA NTRS1992

Formation of the stable auroral arc that intensifies at substorm onset

Observational evidence that the auroral arc that intensifies at substorm onset is formed on magnetic field lines that map to within about 1 to 2 Re of synchronous orbit, where plasma pressures are about 1 to 10 nPa during the substorm growth phase, is discussed. It is proposed that the arc is formed by a perpendicular magnetospheric-current divergence that results from a strong dawn-to-dusk directed pressure gradient in the vicinity of magnetic midnight. It is estimated that the current divergence is sufficiently strong that a greater than 1 kV field-aligned potential drop is required to maintain ionospheric-current continuity. It is suggested that the azimuthal pressure gradient results from proton drifts in the vicinity of synchronous orbit that are directed nearly parallel to the cross-tail electric field.

Lyons, L. R.↗
DOE OSTI2023

Recent progress in MnBi2 n Te3 n +1 intrinsic magnetic topological insulators: crystal growth, magnetism and chemical disorder

ABSTRACT The search for magnetic topological materials has been at the forefront of condensed matter research for their potential to host exotic states such as axion insulators, magnetic Weyl semimetals, Chern insulators, etc. To date, the MnBi2nTe3n+1 family is the only group of materials showcasing van der Waals-layered structures, intrinsic magnetism and non-trivial band topology without trivial bands at the Fermi level. The interplay between magnetism and band topology in this family has led to the proposal of various topological phenomena, including the quantum anomalous Hall effect, quantum spin Hall effect and quantum magnetoelectric effect. Among these, the quantum anomalous Hall effect has been experimentally observed at record-high temperatures, highlighting the unprecedented potential of this family of materials in fundamental science and technological innovation. In this paper, we provide a comprehensive review of the research progress in this intrinsic magnetic topological insulator family, with a focus on single-crystal growth, characterization of chemical disorder, manipulation of magnetism through chemical substitution and external pressure, and important questions that remain to be conclusively answered.

36 MATERIALS SCIENCE↗
NASA NTRS2010

Suprathermal Ion Pressure in the Local Interstellar Medium

The first published results from IBEX and Cassini, and the earlier termination shock crossings by the Voyagers, are strongly suggestive of geometric relation of the local interstellar magnetic field to the outer boundary region of the heliosphere. The inferred pressure of the magnetic field is not, however, high enough to balance the heliosheath particle pressure computed from the IBEX and Cassini measurements. Since the interstellar ram pressure is also relatively low, and higher energy Ge V cosmic ray ions are not trapped on the local interstellar field lines, the pressure balance at the heliopause is more likely dominated by suprathermal keV-MeV particles on both sides. This should not be surprising in view of the long history of early work by Parker and others on cosmic ray particle pressure in interstellar space but with the new insight that the dominant contribution may be at suprathermal keV-MeV energies. Supporting pressure calculations are reviewed for a model interstellar proton spectrum from earlier work of Cooper et al. (2003, 2006, 2008).

Cooper, John F.↗
NASA NTRS1994

Loop heating by D.C. electric current and electromagnetic wave emissions simulated by 3-D EM particle zone

We have shown that a current-carrying plasma loop can be heated by magnetic pinch driven by the pressure imbalance between inside and outside the loop, using a 3-dimensional electromagnetic (EM) particle code. Both electrons and ions in the loop can be heated in the direction perpendicular to the ambient magnetic field, therefore the perpendicular temperature can be increased about 10 times compared with the parallel temperature. This temperature anisotropy produced by the magnetic pinch heating can induce a plasma instability, by which high-frequency electromagnetic waves can be excited. The plasma current which is enhanced by the magnetic pinch can also excite a kinetic kink instability, which can heat ions perpendicular to the magnetic field. The heating mechanism of ions as well as the electromagnetic emission could be important for an understanding of the coronal loop heating and the electromagnetic wave emissions from active coronal regions.

Sakai, J. I.↗
DOE OSTI2023

Incommensurate Spiral Spin Order in CaMn 2 Bi 2 Observed via High-Pressure Neutron Diffraction

Here, high-pressure neutron diffraction is employed to investigate the magnetic behavior of CaMn 2 Bi 2 in extreme conditions. In contrast to antiferromagnetic ordering on Mn atoms reported at ambient pressure, our results reveal that at high pressure, incommensurate spiral spin order emerges due to the interplay between magnetism on the Mn atoms and strong spin–orbit coupling on the Bi atoms: sinusoidal spin order is observed at pressures as high as 7.4 GPa. First-principles calculations with a noncollinear spin orientation demonstrate band crossing behavior near the Fermi level as a result of strong hybridization between the d orbitals of Mn and the p orbitals of Bi atoms. Competing antiferromagnetic order is observed at different temperatures in the partially frustrated lattice. Theoretical models have been developed to investigate spin dynamics. This research provides a unique toolbox for conducting experimental and theoretical magnetic and spin dynamics studies of magnetic quantum materials via high-pressure neutron diffraction.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗