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At least 757 records · Page 42

Enhancement of edge turbulence concomitant with ELM suppression during boron powder injection in EAST

A reproducible, quasi-stationary edge localized mode (ELM)-suppressed scenario was obtained over a wide range of plasma parameters by continuous injection of boron (B) powder into an upper-single null discharge in the experimental advanced superconducting tokamak [Sun et al., Nucl. Fusion 61, 014002 (2021)]. This powder-induced ELM-absent regime is associated with an edge harmonic mode (EHM) that provides continuous particle exhaust to maintain constant density without confinement degradation and impurity accumulation, the latter of which is often observed in ELM-free regimes. A flow rate threshold of B powder injection, leading to a threshold intensity of the EHM, is necessary for full ELM suppression. The fundamental harmonic of the EHM exhibits a toroidal mode number n = 1. The mode is observable in the entire poloidal cross section with a peak near the upper X-point in an upper-single null configuration. Here, the EHM spans radially across the pedestal and scrape-off layer, peaking inside the separatrix. The EHM appears to be insensitive to q 95 , heating power, plasma toroidal rotation, and pedestal collisionality.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Simulations of ion heating due to ion-acoustic instabilities in presheaths

Particle-in-cell, direct simulation Monte Carlo simulations reveal that ion-acoustic instabilities excited in presheaths can cause significant ion heating. Ion-acoustic instabilities are excited by the ion flow toward a sheath when the neutral gas pressure is small enough and the electron temperature is large enough. A series of 1D simulations were conducted in which neutral plasma (electrons and ions) was uniformly sourced with an ion temperature of 0.026 eV and different electron temperatures (0.1 eV–50 eV). Ion heating was observed when the electron-to-ion temperature ratio exceeded the minimum value predicted by linear response theory to excite ion-acoustic instabilities at the sheath edge (T e /T i ≈ 28). When this threshold was exceeded, the temperature equilibration rate between ions and electrons rapidly increased near the sheath so that the local temperature ratio did not significantly exceed the threshold for instability. This resulted in significant ion heating near the sheath edge, which also extended back into the bulk plasma; presumably due to wave reflection from the sheath. Furthermore, this ion-acoustic wave heating mechanism was found to decrease for higher neutral pressures, where ion-neutral collisions damp the ion-acoustic waves and ion heating is instead dominated by inelastic collisions in the presheath.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Photoionization from the Xe 4d orbitals of XeF 2

Here, we present a comparison of the photoionization dynamics of the 4d shell of XeF 2 from threshold to 250 eV to those of the prototypical 4d shell of atomic Xe. The new experimental data include spin–orbit and ligand-field-resolved partial cross sections, photoelectron angular distributions, branching fractions, and lifetime widths for the 4d-hole states. The spin–orbit branching fractions and angular distributions are remarkably similar to the corresponding distributions from atomic Xe across a broad energy interval that includes both the intense shape resonance in the f continuum and a Cooper minimum in the same channel. The angular distributions and branching fractions are also in reasonably good agreement with our first-principles theoretical calculations on XeF 2 . Data are also presented on the lifetime widths of the substate-resolved 4d-hole states of XeF 2 . While the trends in the widths are similar to those in the earlier experimental and theoretical work, the linewidths are considerably smaller than in the previous measurements, which may require some reinterpretation of the decay mechanism. Finally, we present new data and an analysis of the Auger electron spectra for ionization above the 4d thresholds and resonant Auger spectra for several pre-edge features.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

High temperature characteristics of nitric oxide annealed p-channel 4H-SiC metal oxide semiconductor field effect transistors

In this work, p-channel 4H-SiC MOSFETs were fabricated and analyzed at high temperature. It is demonstrated that nitridation of the gate oxide enables enhancement mode operation in these devices. Nitrogen incorporation at the 4H-SiC/SiO2 interface by nitric oxide annealing reduces the interface trap density energetically located in the lower half of the 4H-SiC bandgap, resulting in viable high temperature p-channel devices. In the 27–300 °C temperature range, the threshold voltage decreases with increasing temperature, consistent with the reduction of occupied interface traps at higher temperatures. The hole channel mobility is weakly temperature dependent under strong inversion conditions. Hall measurements support that above the threshold voltage, the mobility is limited by surface roughness scattering. In weaker inversion, the channel conductivity is limited by interface hole trapping and Coulomb scattering. In addition, high temperature bias stress measurements confirm a temperature activated hole trapping under negative gate bias, which requires further investigations.

Das, Suman (ORCID:0000000317146287)↗

Hydroscaling indirect-drive implosions on the National Ignition Facility

A goal of the laser-based National Ignition Facility (NIF) is to increase the liberated fusion energy “yield” in inertial confinement fusion experiments well past the ignition threshold and the input laser energy. One method of increasing the yield, hydrodynamic scaling of current experiments, does not rely on improving compression or implosion velocity, but rather increases the scale of the implosion to increase hotspot areal density and confinement time. Indirect-drive (Hohlraum driven) implosions carried out at two target sizes, 12.5% apart, have validated hydroscaling expectations. Moreover, extending comparisons to the best-performing implosions at five different capsule sizes shows that their performance also agrees well with hydroscaling expectations even though not direct hydroscales of one another. In the future, by switching to a reduced loss Hohlraum geometry, simulations indicate that we can drive 20% larger-scale implosions within the current power and energy limitations on the NIF. Finally, at the demonstrated compression and velocity of these smaller-scale implosions, these 1.2× hydroscaled implosions should put us well past the ignition threshold.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Long wavelength interband cascade lasers

InAs-based interband cascade lasers (ICLs) can be more easily adapted toward long wavelength operation than their GaSb counterparts. Devices made from two recent ICL wafers with an advanced waveguide structure are reported, which demonstrate improved device performance in terms of reduced threshold current densities for ICLs near 11 μm or extended operating wavelength beyond 13 μm. Here, the ICLs near 11 μm yielded a significantly reduced continuous wave (cw) lasing threshold of 23 A/cm 2 at 80 K with substantially increased cw output power, compared with previously reported ICLs at similar wavelengths. ICLs made from the second wafer incorporated an innovative quantum well active region, comprised of InAsP layers, and lased in the pulsed-mode up to 120 K at 13.2 μm, which is the longest wavelength achieved for III–V interband lasers.

47 OTHER INSTRUMENTATION↗

Selective amorphization of SiGe in Si/SiGe nanostructures via high energy Si+ implant

Here, the selective amorphization of SiGe in Si/SiGe nanostructures via a 1 MeV Si + implant was investigated, resulting in single-crystal Si nanowires (NWs) and quantum dots (QDs) encapsulated in amorphous SiGe fins and pillars, respectively. The Si NWs and QDs are formed during high-temperature dry oxidation of single-crystal Si/SiGe heterostructure fins and pillars, during which Ge diffuses along the nanostructure sidewalls and encapsulates the Si layers. The fins and pillars were then subjected to a 3 × 10 15 ions/cm 2 1 MeV Si + implant, resulting in the amorphization of SiGe, while leaving the encapsulated Si crystalline for larger, 65-nm wide NWs and QDs. Interestingly, the 26-nm diameter Si QDs amorphize, while the 28-nm wide NWs remain crystalline during the same high energy ion implant. This result suggests that the Si/SiGe pillars have a lower threshold for Si-induced amorphization compared to their Si/SiGe fin counterparts. However, Monte Carlo simulations of ion implantation into the Si/SiGe nanostructures reveal similar predicted levels of displacements per cm 3 . Molecular dynamics simulations suggest that the total stress magnitude in Si QDs encapsulated in crystalline SiGe is higher than the total stress magnitude in Si NWs, which may lead to greater crystalline instability in the QDs during ion implant. The potential lower amorphization threshold of QDs compared to NWs is of special importance to applications that require robust QD devices in a variety of radiation environments.

36 MATERIALS SCIENCE↗

Hybrid simulation of Alfvén wave parametric decay instability in a laboratory relevant plasma

Large-amplitude Alfvén waves are subject to parametric decays, which can have important consequences in space, astrophysical, and fusion plasmas. Although the Alfvén wave parametric decay instability (PDI) was predicted decades ago, observational evidence is limited, stimulating considerable interest in laboratory demonstration of the instability and associated numerical modeling. Here, we report an important step toward direct hybrid simulation of the Alfvén wave PDI in a laboratory plasma, using antenna-like wave injection of a circularly polarized wave and realistic wave-plasma parameters. Considering collisionless damping, we identify the threshold Alfvén wave amplitudes and frequencies required for triggering the instability. These threshold behaviors are corroborated by simple theoretical analysis, considering the balance between PDI growth and ion Landau damping and PDI development in a bounded plasma. Other effects not included in the present model such as finite transverse wave scale and ion–neutral collisions are briefly discussed. These hybrid simulations promise to be a useful tool for investigating laboratory Alfvén wave dynamics and may provide guidance for future laboratory demonstration of the PDI process.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The Vacuum Cherenkov Detector (VCD) for γ-ray measurements in inertial confinement fusion experiments

Inertial confinement fusion experiments at both the National Ignition Facility (NIF) and the Laboratory for Laser Energetics OMEGA laser facility currently utilize Cherenkov detectors, with fused silica as the Cherenkov medium. At the NIF, the Quartz Cherenkov Detectors improve the precision of neutron time-of-flight measurements; and at OMEGA, the Diagnostic for Areal Density provides measurements of capsule shell areal densities. An inherent property of fused silica is the radiator’s relatively low energy threshold for Cherenkov photon production (E threshold < 1 MeV), making it advantageous over gas-based Cherenkov detectors for experiments requiring low-energy γ detection. The Vacuum Cherenkov Detector (VCD) has been specifically designed for efficient detection of low energy γ’s. Its primary use is in implosion experiments, which will study reactions relevant to stellar and big-bang nucleosynthesis, such as T( 4 He,γ) 7 Li, 4 He( 3 He,γ) 7 Be, and 12 C(p,γ) 13 N. Further, the VCD is compatible with LLE’s standard Ten-Inch Manipulator diagnostic insertion module. This work will outline the design and characterization of the VCD as well as provide results from recent experiments conducted at the OMEGA laser facility.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Linear ion-scale microstability analysis of high and low-collisionality NSTX discharges and NSTX-U projections

Linear gyrokinetic simulations were conducted to investigate ion-gyroradius-scale micro-instability predictions for high-beta NSTX discharges and NSTX-U projections that span over an order of magnitude variation in collisionality. A complex mix of microtearing modes and hybrid trapped electron modes/kinetic ballooning modes (TEM/KBM) is predicted for all experimental or projected conditions. Ion temperature gradient (ITG) instabilities are typically stable in the NSTX discharges investigated, consistent with the observed neoclassical ion thermal transport. ITG thresholds inferred from the simulations are typically much higher than the experimental NSTX gradients, as well as the projected gradients in the NSTX-U scenario, which assumed ion temperatures limited by neoclassical transport only. The analysis suggests ITG instabilities are unlikely to contribute significant anomalous thermal losses in high-beta, lower collisionality NSTX-U scenarios. On the other hand, the NSTX experimental profiles and NSTX-U projections are predicted to be very close to the predicted onset of unstable KBM at most radii investigated. The proximity of the various discharges to the KBM instability threshold implies it may play an important role in setting profile shapes and limiting global energy confinement. Here, it remains to be understood and predicted how KBM contributes to multi-channel transport (thermal and particle transport, for both ions and electrons) in a way that is consistent with experimental inferences.

36 MATERIALS SCIENCE↗

An optoelectronic heterostructure for neuromorphic computing: CdS/V 3 O 5

Nonvolatile resistive switching is one of the key phenomena for emerging applications in optoelectronics and neuromorphic computing. In most of the cases, an electric field is applied to a two terminal dielectric material device and leads to the formation of a low resistance filament due to ion migration. However, the stochastic nature of the ion migration can be an impediment for the device robustness and controllability, with uncontrolled variations of high and low resistance states or threshold voltages. Here, we report an optically induced resistive switching based on a CdS/V 3 O 5 heterostructure which can overcome this issue. V 3 O 5 is known to have a second order insulator to metal transition around T c ≈ 415 K, with an electrically induced threshold switching at room temperature. Upon illumination, the direct transfer of the photoinduced carriers from the CdS into V 3 O 5 produces a nonvolatile resistive switching at room temperature. The initial high resistance can be recovered by reaching the high temperature metallic phase, i.e., temperatures above T c . Interestingly, this resistive switching becomes volatile around the T c . In conclusion, by locally manipulating the volatile and nonvolatile resistive switching using electric field and light, this system is a promising platform for hardware based neuromorphic computing implementations.

97 MATHEMATICS AND COMPUTING↗

Effect of outer-cylinder rotation on the radially heated Taylor–Couette flow

A Taylor–Couette setup with radial heating is considered where a Boussinesq fluid is sheared in the annular region between two concentric, independently rotating cylinders maintained at different temperatures. Linear stability analysis is performed to determine the Taylor number for the onset of instability. Two radius ratios corresponding to wide and thin gaps with several rotation rate ratios are considered. The rotation of the outer cylinder is found to have a general stabilizing effect on the stability threshold as compared to pure inner-cylinder rotation, with a few exceptions. The radial heating sets up an axial flow which breaks the reflection symmetry of isothermal Taylor–Couette flow in the axial coordinate. This symmetry breaking separates linear stability thresholds, and we find the fastest growing modes with both positive and negative azimuthal numbers for different parameters. Another important finding of the current study is the discovery of unstable modes in the Rayleigh-stable regime. Furthermore, closed disconnected neutral curves (CDNCs) are observed for both wide and thin gaps which can separate from or merge into open neutral–stability curves. Alternatively, CDNCs can also morph into open neutral stability curves as the rotation rate ratio is changed. CDNCs are observed to be sensitive to changes in control parameters, and their appearance/disappearance is shown to induce discontinuous jumps in the critical Taylor number. Finally, for both wide and thin gaps, the fastest-growing modes found in the pure corotation case are shown to have their origins in the instability islands at smaller values of rotation rate ratios.

97 MATHEMATICS AND COMPUTING↗

Scintillation characteristics of the EJ-299-02H scintillator

Here a study of the dead layer thickness and quenching factor of a plastic scintillator for use in ultracold neutron (UCN) experiments is described. Alpha spectroscopy was used to determine the thickness of a thin surface dead layer to be 630 ± 110 nm. The relative light outputs from the decay of 241 Am and Compton scattering of electrons were used to extract Birks’ law coefficient, yielding a kB value of 0.087 ± 0.003 mm/MeV, consistent with some previous reports for other polystyrene-based scintillators. The results from these measurements are incorporated into the simulation to show that an energy threshold of (∼9 keV) can be achieved for the UCNProBe experiment. This low threshold enables high beta particle detection efficiency and the indirect measurement of UCN. The ability to make the scintillator deuterated, accompanied by its relatively thin dead layer, gives rise to unique applications in a wide range of UCN experiments, where it can be used to trap UCN and detect charged particles in situ.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Observation of bound valence excited electronic states of deprotonated 2-hydroxytriphenylene using photoelectron, photodetachment, and resonant two-photon detachment spectroscopy of cryogenically cooled anions

Polycyclic aromatic hydrocarbons (PAHs) are common atmospheric pollutants, and they are also ubiquitous in the interstellar medium. Here, we report the study of a complex O-containing PAH anion, the deprotonated 2-hydroxytriphenylene (2-OtPh–), using high-resolution photoelectron imaging and photodetachment spectroscopy of cryogenically cooled anions. Vibrationally resolved photoelectron spectra yield the electron affinity of the 2-OtPh radical as 2.629(1) eV and several vibrational frequencies for its ground electronic state. Photodetachment spectroscopy reveals bound valence excited electronic states for the 2-OtPh– anion, with unprecedentedly rich vibronic features. Evidence is presented for a low-lying triplet state (T1) and two singlet states (S1 and S2) below the detachment threshold. Single-color resonant two-photon photoelectron spectroscopy uncovers rich photophysics for the 2-OtPh– anion, including vibrational relaxation in S1, internal conversion to the ground state of 2-OtPh–, intersystem crossing from S2 to T1, and a long-lived autodetaching shape resonance about 1.3 eV above the detachment threshold. The rich electronic structure and photophysics afforded by the current study suggest that 2-OtPh– would be an interesting system for pump–probe experiments to unravel the dynamics of the excited states of this complex PAH anion.

Chemistry↗

Density drop at the divertor target in the prototype material plasma exposure eXperiment (Proto-MPEX)

The steady-state linear device “Material Plasma Exposure eXperiment” (MPEX) is currently under construction at Oak Ridge National Laboratory with the goal of enabling Plasma-Material Interaction studies at future fusion reactor relevant plasma conditions. In this work, a newly in-house developed hybrid Particle-In-Cell code-PICOS++ is applied to understand the experimental results obtained from the prototype of MPEX referred to as the “Proto-MPEX” during its helicon-only and helicon with ion cyclotron resonance heating (ICRH) experiments. This study explains the physics of the experimentally observed plasma density-drop at the divertor target in Proto-MPEX device during ICRH. In contrast to previous work on ICRH in MPEX, this study demonstrates that the mirror force plays a central role in the Proto-MPEX plasma transport during ICRH, which has new features not previously explored. Force balance analyses reveal that the temperature anisotropy produced by ICRH leads to a significant increase in the mirror force downstream of the resonance where the magnetic field is diverging. This force accelerates ions toward the target and leads to a drop in plasma density to ensure conservation of particle flux. Simulations with ICRH where the magnetic field divergence downstream of the resonance has been removed, do not produce plasma acceleration nor density drop at the target despite efficient ion heating at the resonance. Moreover, simulation results demonstrate that for a given ICRH power, lowering the source rate produces ions with increased perpendicular energy which interact with the mirror force to produce higher plasma acceleration which increases the strength of the density-drop at the target. The strength of the density drop appears to reach an asymptotic limit at a certain threshold ICRH power. Simulations show that this threshold power increases with increasing particle source rate.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Characterization of the image plate multi-scan response to mono-energetic x-rays

Image plates (IPs), or phosphor storage screens, are a technology employed frequently in inertial confinement fusion (ICF) and high energy density plasma (HEDP) diagnostics because of their sensitivity to many types of radiation, including, x rays, protons, alphas, beta particles, and neutrons. Prior studies characterizing IPs are predicated on the signal level remaining below the scanner saturation threshold. Since the scanning process removes some signal from the IP via photostimulated luminescence, repeatedly scanning an IP can bring the signal level below the scanner saturation threshold. This process, in turn, raises concerns about the signal response of IPs after an arbitrary number of scans and whether such a process yields, for example, a constant ratio of signal between the nth and n + 1st scan. Here, the sensitivity of IPs is investigated when scanned multiple times. It is demonstrated that the ratio of signal decay is not a constant with the number of scans and that the signal decay depends on the x-ray energy. As such, repeatedly scanning an IP with a mixture of signal types (e.g., x ray, neutron, and protons) enables ICF and HEDP diagnostics employing IPs to better isolate a particular signal type.

Instruments & Instrumentation↗

Predissociation-based measurements of bond dissociation energies: US 2 , OUS, and USe

The uranium-containing molecules US 2 , OUS, and USe have been investigated using a pulsed laser ablation supersonic beam molecular source with time-of-flight mass spectrometric detection. Spectra have been recorded using the resonant two-photon ionization method over the spectroscopic range from 277 to 238 nm. These species have a myriad of excited electronic states in this spectroscopic region, leading to spectra that are highly congested and appear quasicontinuous. Sharp predissociation thresholds are observed, allowing precise bond dissociation energies to be measured. In the case of the triatomic molecules, it was necessary to use one laser for excitation and a delayed laser for ionization in order to observe a sharp predissociation threshold that allowed a precise bond dissociation energy to be measured. The resulting thermochemical values are D 0 (SU-S) = 4.910 ± 0.003 eV, D 0 (OU-S) = 5.035 ± 0.004 eV, and D 0 (USe) = 4.609 ± 0.009 eV. These results provide the first measurement of D 0 (USe) and reduce the error limits in the previous values of D 0 (SU-S) and D 0 (OU-S) by a factor of more than 70.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Investigating instabilities in magnetized low-pressure capacitively coupled RF plasma using particle-in-cell (PIC) simulations

The effect of a uniform magnetic field on particle transport in low-pressure radio frequency (RF) capacitively coupled plasma (CCP) has been studied using a particle-in-cell model. Three distinct regimes of plasma behavior can be identified as a function of the magnetic field. In the first regime at low magnetic fields, asymmetric plasma profiles are observed within the CCP chamber due to the effect of $\overrightarrow{E}$ × $\overrightarrow{B}$ drift. As the magnetic field increases, instabilities develop and form self-organized spoke-shaped structures that are distinctly seen within the bulk plasma closer to the sheath. In this second regime, the spoke-shaped coherent structures rotate inside the plasma chamber in the -$\overrightarrow{E}$ × $\overrightarrow{B}$ direction, where $\overrightarrow{E}$ × $\overrightarrow{B}$ are the DC electric and magnetic field vectors, respectively, and the DC electric field exists in the sheath and pre-sheath regions. The spoke rotation frequency is in the megahertz range. As the magnetic field strength increases further, the rotating coherent spokes continue to exist near the sheath. The coherent structures are, however, accompanied by new small-scale incoherent structures originating and moving within the bulk plasma region away from the sheath. This is the third regime of plasma behavior. The threshold values of the magnetic field between these regimes were found not to vary with changing plasma reactor geometry (e.g., area ratio between ground and powered electrodes) or the use of an external capacitor between the RF-powered electrode and the RF source. The threshold values of the magnetic field between these regimes shift toward higher values with increasing gas pressure. Analysis of the results indicates that the rotating structures are due to the lower hybrid instability driven by density gradients and electron-neutral collisions. This paper provides guidance on the upper limit of the magnetic field for instability-free operation in low-pressure CCP-based semiconductor deposition and etch systems that use the external magnetic field for plasma uniformity control.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗