Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “Scintillation”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 757 records · Page 42

Measurement of proton light yield of water-based liquid scintillator

Abstract The proton light yield of liquid scintillators is an important property in the context of their use in large-scale neutrino experiments, with direct implications for neutrino-proton scattering measurements and the discrimination of fast neutrons from inverse $$\beta $$ β -decay coincidence signals. This work presents the first measurement of the proton light yield of a water-based liquid scintillator (WbLS) formulated from 5% linear alkyl benzene (LAB), at energies below 20 MeV, as well as a measurement of the proton light yield of a pure LAB + 2 g/L 2,5-diphenyloxazole (PPO) mixture (LABPPO). The measurements were performed using a double time-of-flight method and a pulsed neutron beam from the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. The proton light yields were measured relative to that of a 477 keV electron. The relative proton light yield of WbLS was approximately 3.8% lower than that of LABPPO, itself exhibiting a relative proton light yield 15–20% higher than previous measurements of an analogous anoxic sample. The observed quenching is not compatible with the Birks model for either material, but is well described with the addition of Chou’s bimolecular quenching term.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Saturation of a Ce:Y 3 Al 5 O 12 scintillator response to ultra-short pulses of extreme ultraviolet soft X-ray and X-ray laser radiation

Investigations of radioluminescence saturation in monocrystalline cerium doped yttrium aluminum garnet (Ce:YAG) exposed to intense extreme ultraviolet (XUV), soft X-ray and X-ray radiation delivered from three free-electron lasers are described in this article. The measurements were performed with wavelengths of 98, 25.6, 13.5 and 0.15 nm. We have found that saturation of the photon yield occurs at an excitation level of 2.0 x 10 20 eV/cm 3 resulting in an emission of 1.5 x 10 18 visible photons per cubic centimeter. This number is much smaller than the concentration of Ce3+ in the scintillator that was equal to 2 x 10 20 cm –3 . Because the internal radiance efficiency η does not depend strongly on the irradiating photon energy, i.e., η ≈0.035 ± 0.015 in the range 10 to 100 000 eV, the results presented here could be used to predict saturation effects in scintillator slabs placed in imaging systems of bright XUV, X-ray and particle beams. In conclusion, the saturation of the Ce 3+ emission is explained by mutual quenching of excitons created at high densities, preceding the stage of energy transfer to the Ce 3+ ions.

43 PARTICLE ACCELERATORS↗

Validated Models for Radiation Response and Signal Generation in Scintillators: Final Report

This Final Report presents work carried out at Pacific Northwest National Laboratory (PNNL) under the project entitled “Validated Models for Radiation Response and Signal Generation in Scintillators” (Project number: PL10-Scin-theor-PD2Jf) and led by Drs. Fei Gao and Sebastien N. Kerisit. This project was divided into four tasks: 1) Electronic response functions (ab initio data model) 2) Electron-hole yield, variance, and spatial distribution 3) Ab initio calculations of information carrier properties 4) Transport of electron-hole pairs and scintillation efficiency Detailed information on the results obtained in each of the four tasks is provided in this Final Report. Furthermore, published peer-reviewed articles based on the work carried under this project are included in Appendix. This work was supported by the National Nuclear Security Administration, Office of Nuclear Nonproliferation Research and Development (DNN R&D/NA-22), of the U.S. Department of Energy (DOE).

Environmental Molecular Sciences Laboratory↗

Preliminary study of the inclusion of Water-based Liquid Scintillator in the WATCHMAN Detector

This note summarizes an effort to characterize the effects of adding water-based liquid scintillator to the WATCHMAN detector. A detector model was built in the Geant4 Monte Carlo toolkit, and the position reconstruction of positrons within the detector was compared with and without scintillator. This study highlights the need for further modeling studies and small-scale experimental studies before inclusion into a large-scale detector, as the benefits compared to the associated costs are unclear.

47 OTHER INSTRUMENTATION↗

Low-Afterglow Scintillators for High-Rate Radiation Detection

The present work reports on the development of two types of metal-loaded plastic scintillators that seek to improve the decay kinetics and light-yield properties of existing materials used for high count-rate radiation detection. The strategy followed in this work involves the addition of an organometallic iridium or organometallic tin compound to reduce the extent of deleterious delayed luminescence following exposure to ionizing radiation. Key results include a seven times greater light yield compared to existing high-rate scintillators (i.e. BC422Q plastic, stilbene-doped bizenzyl crystal), while achieving comparable or even faster decay characteristics than these benchmark materials.

36 MATERIALS SCIENCE↗

Final report for the DOE/NA22 project, Physics of Scintillator Nonproportionality

The energy resolution of current scintillators is known to be limited by the adverse impact of light yield nonproportionality. This effort aims to advance the understanding of the physics underlying nonproportionality sufficiently to enable breakthrough performance, by achieving energy resolution beyond the present limit of 2.5% at 662 keV. While we have formulated several mechanistic frameworks that quantitatively describe the basic processes and are able to deduce the impact on resolution (Figure 1), we are in the midst of developing theoretical means of knowing a priori which material properties mediate these intrinsic mechanisms. Addressing the experimental and theoretical challenges of elucidating these mechanisms, we aim to develop and apply a predictive model guiding the improvement of scintillator performance.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Multiple Phase Screen Scintillation Modeling Code

This document describes the underlying theory and use of a computer code written to simulate scintillation effects on propagating electromagnetic (EM) signals. The Multiple Phase Screen (MPS) technique [1, 2, 3, 4] is employed to model the effects of scintillation on EM signals as they travel through the earth’s ionosphere.

97 MATHEMATICS AND COMPUTING↗

Performance of BaFCl:Eu2+ scintillating composites for X-ray imaging screens

A cost-effective solution for improving X-ray imaging detectors is presented through the use of a translucent scintillating composite and pixelated screen structure. A large quantity of BaFCl:Eu 2+ polycrystalline scintillator powder was synthesized via flux growth and its optical properties characterized through photoluminescence (PL) and absolute quantum yield (QY). UV-curable composites containing the BaFCl:Eu 2+ material were fabricated with differing amounts of NOA1665 and NOA170 optical adhesives. It was determined that, when the two resins were combined, the translucency of the resulting composite could be enhanced. The BaFCl:Eu 2+ composite was also cast into a pixelated glass screen containing an array of 160 μm x 160 μm holes by two separate methods: composite paste application and powder-resin application. Based on visual inspection, using a composite paste to fill the apertures proved to be more effective in creating a uniform packing.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Toward A Precision Era Of Neutrino Oscillation Physics: Liquid Argon Scintillation Detector Development for DUNE and Neutrino Oscillation Studies with NOvA

NOvA is an accelerator-based high-energy particle physics experiment that studies oscillations in a beam of mostly muon (anti-)neutrinos, looking for the disappearance of muon (anti-)neutrinos and appearance of electron (anti-)neutrinos. This search is sensitive to several key neutrino oscillation parameters. After the completion of NOvA, DUNE will continue to study neutrino oscillations with a liquid argon time-projection chamber, which provides finer granularity of tracking than NOvA. Furthermore, the beam will be more powerful, the detector fiducial volume is approximately 3 times larger than the full NOvA detector, and the detector will be situated underground. DUNE is therefore expected to usher in a precision era of long-baseline neutrino oscillation physics. While the main signal from a liquid argon time-projection chamber is the ionization signal produced by the passage of charged particles, argon is also a copious source of scintillation. This light is useful for pro viding a precise event time. Scintillation light is potentially especially useful in non-beam studies in DUNE, such as atmospheric neutrinos, supernova neutrinos, and potential nucleon decay. In this dissertation, I will discuss both projects. In addition to a study of the drift in NOvA’s energy calibration, recent oscillation analysis is discussed, which finds a best fit at $\sin^2\theta_{23}=0.56^{+0.04}_{-0.03}$, $\Delta m^{2}_{32}=2.48^{+0.11}_{-0.06}\times10^{-3}\text{eV}^2$, $\delta_{CP}/\pi=0.0^{+1.3}_{-0.4}$, and prefers normal ordering at 1.9$\sigma$. Contributions to NOvA analysis will also be highlighted, especially methods used to perform separation of neutrinos and antineutrinos in the predominantly antineutrino beam for study. This wrong-sign component is initially used to provide further understanding of the beam components. Furthermore, characterization and prototype testing of photon detectors for DUNE is discussed. Finally, a study is performed with wrong-s ign separation techniques applied to the appearance signal i! n both NOvA and DUNE to create two samples: one enriched in signal and the other enriched in the wrong-sign oscillation appearance. Wrong-sign in the oscillation diminishes the sensitivity of the analysis, so this study aimed to determine if such a separation would enhance the sensitivity of the oscillation. Little benefit was found at the ultimate exposure with NOvA with the techniques currently available, but the study showed potential promise when applied to DUNE.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

(U) Endpoint Energy and Scintillator Geometry Effects on the Swank Factor, Quantum Efficiency, and DQE(0) for High-Energy Radiography

High-energy radiography is used to image imploding materials to better understand weapon design and performance. The Enhanced Capabilities for Subcritical Experiments (ECSE) is a new facility proposal that aims to collect radiographic images of nuclear material. As part of the facility design, we aim to optimize data quality and radiographic performance by investigating different detector designs. We addressed design decisions by simulating different scintillator designs using M CNP6 and calculated the quantum efficiency, Swank factor, and detective quantum efficiency at zero-frequency (DQE(O)). First, we investigated the effects of the x-ray endpoint energy on the detector response. We generated three x-ray spectra with endpoint energies of 20 MeV, 22 MeV, and 24 MeV. The three raw spectra were filtered using the Dual-Axis Radiographic Hydrodynamic Test facility (DARHT) line-of-sight materials along with 1) flat field filtration using 7 cm tungsten alloy in the bullnose and 2) an FTO with 4 plates. The scatter-to-direct radiation ratio was much larger for FTO with 4 plates (50-60%) compared to the flat field with 7 cm of bullnose material (8%). We used these filtered spectra to calculate the detector response for the original DARHT segmented scintillator design. We found that the endpoint energy and filtration had a negligible effect on the detector response. The quantum efficiency was 0.63, the Swank factor was 0.84, and the DQE(O) was 0.53 for all six spectra.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Linearity for Ca 2+ -Doped CeBr 3 Scintillating Materials [Slides]

This project seeks to develop low-cost, high-resolution gamma scintillators based on new fracture-resistant alloys of cerium bromide. These alloys will eliminate limitations imposed by self-activity and fracture of currently available lanthanum-based scintillators.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

External Release of Organic Scintillator DRiFT Software - Technology Evaluation and Demonstration Project Accomplishments [Slides]

Overview and Objectives: DRiFT post processes radiation transport output from MCNP, and generates realistic nuclear instrumentation response; Organic scintillator response has been developed, tested, and validated with measurements, these instruments are widely used in nuclear safeguards. At the beginning of this project, DRiFT was only available to LANL employees with access to yellow High Performance Computing clusters. Additionally, there are many complicated external software dependencies. Our TED project request proposed using funds to: Comment and clean up code, friendly testing, generating test suites and examples; Expansion of scintillator types natively supported by DRiFT; External release of DRiFT accompanied by documentation. We accomplished all objectives (and many others), they are highlighted in these slides.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Summer 2021 Co-op Report: X-Ray Scintillation Detector (A Co-op Work Experience Report)

The M-3 team was in need of a detector that could be used properly characterize their X-Ray machines. It can also be used to diagnose the X-ray in the case that problems arise before or during an experiment. They put me in charge of designing, ordering, and constructing said detector. After doing research, I found that scintillation-based detectors would be the best diagnostic tool for this purpose. It will allow the team to collect a full photon count of the X-ray pulse as well as provide spectroscopy functions with which we can view photon counts at different energy levels. This will also allow them to calculate an accurate dose given from the machine. Due to lead times, the crystals are still in manufacturing, thus the detector could not be completed. Although the designs and calculations needed to construct and operate the scintillator have been completed which is what I will be presenting in this document. Compared to the detectors being used before, my design offers a cheaper and far more efficient alternative.

42 ENGINEERING↗

Assessment of the Imaging Properties of Plastic Scintillators at FP60R for Neutron Imaging Applications [Slides]

4mm thick Stilbene gives the brightest signal but at the cost of resolution. 1 and 2 cm BC412 gave the highest resolution images. The HI-LY scintillator is better suited for DD neutrons. Future work includes: measurements this summer using an event-mode imaging camera which promises sub-pixel resolution through center-of-mass techniques, opportunities for DD neutron tests during laser-driven z-pinch experiments at UNR, and assess scatter within scintillator.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Comparison of Supervised and Un-Supervised Machine Learning Algorithms for Threat Detection and Scintillator Performance for Radiation Portal Monitoring

Following the events of September 11, 2001, international border crossing have been equipped with radiation portal monitors (RPMs) to identify illicit radioactive material. Polyvinyl toluene (PVT) scintillators are commonly used due to their low cost and reasonable maintainability, however they offer low spectral resolution. Despite the fact that over twenty years has transpired since this event, radioisotopes are still typically identified by hand-crafted classification algorithms, e.g., total counts or energy windowing, and exhibit relatively poor performance in detecting threats at the low false alarm rates required to support the stream of commerce. While some improvement to performance has been realized via the use of supervised machine learning, these classification algorithms typically utilize simulations in lieu of real data due to the sparsity of data for one or more classes. Accordingly, the performance of these algorithms is somewhat less than optimal when examining experiments or simulations with model mismatch. Consequently, in this work, we examine the application of a number of unsupervised machine learning, anomaly detection based algorithms, to circumvent the inverse crime when analyzing spectroscopy data for RPMs. We also compare anomaly detection results with those obtained via the use of supervised classification detection ML algorithms when model mismatch is introduced between the simulated threat items utilized for training/testing. Finally, we compared the performance of the PVT scintillators to those obtained with higher resolution detectors using both anomaly detection and supervised classification algorithms.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Scintillating Bubble Chambers for Direct Dark Matter Detection, and an Update on SBC-LAr10

The Scintillating Bubble Chamber (SBC) Collaboration aims to use the liquid-noble bubble chamber technology as a low-threshold detector for dark matter particles of 1-10 GeV/c2. The detector combines the remarkable electron recoil (ER) discrimination of the bubble chamber with the event-by-event energy resolution provided by liquid argon (LAr) scintillation, with the crucial added benefit that ER discrimination in liquid-noble bubble chambers extends to much lower thresholds than in past freon-filled bubble chambers, with the potential for quasi-background-free operation at thresholds of 100 eV in nuclear recoil (NR) energy. SBC has developed two functionally identical 10 kg detectors: SBC-LAr10 at Fermilab will calibrate low-threshold performance, while the radio-pure SBC-SNOLAB chamber will execute SBC s first deep-underground dark matter search. SBC-LAr10 at Fermilab was recently installed in the MINOS tunnel 100 meters underground, and the first bubbles are expected this fall. I will present the current status of SBC-LAr10 and describe the suite of gamma and neutron calibrations we will execute. The calibrations will confirm the physics reach of this new technology, motivating not just the SBC-SNOLAB chamber now being assembled but also future searches into the solar neutrino fog at 1 GeV/c2.

Sheng, Zhiheng↗

Systematic study of radioluminescence and light propagation effects in scintillating nanoguide materials

Nanoguide optical waveguides are thermally processed materials based on polymers that have different refractive indices. Scintillating versions of these materials have been under development since 2019 and feature PMMA as the low refractive index constituent and Organic Glass Scintillator-polymer blends as the high index component. Characterization efforts to date have focused on the functional characteristics of nanoguide pertaining to its envisioned use in high-resolution transmission radiography applications.

36 MATERIALS SCIENCE↗

Optimization of scintillated imaging detectors for MeV X-ray radiography

Radiographic imaging at X-ray energies in the MeV range poses a complex problem. Detection of high energy X-rays depends heavily on the ability of the detection material, in this work the scintillator, to attenuate and ultimately stop the X-ray. Attenuation is more readily achieved by increasing material thickness, however thick scintillators are plagued with relatively high internal scattering, leading to an overall decrease in spatial resolution and image quality.

42 ENGINEERING↗