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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 757 records · Page 42
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

A Semi-Empirical Density Law for Ternary, Homogeneous PuCl 3 /HCl/H 2 O Solutions

Nuclear material operations pose unique hazards that are not encountered in other chemical, energy, or manufacturing industries. One of these hazards is the potential for a nuclear criticality accident when handling fissile isotopes such as 235 U and 239 Pu. These hazards are particularly high when fissile material is dissolved in solution as the neutron behaviors of the system can change rapidly with the physical and chemical changes accessible in solution. Current estimates of solution density used for criticality safety are outdated and hinder fissile material handling. Developing new estimates for these safety calculations requires experimental characterization and the derivation of empirical density models. We have derived a density law describing PuCl 3 /HCl/H 2 O solutions from experimental data characterizing solution density. Density data was treated using a Pitzer-derived eight-parameter equation, defining density as a function of analyte concentrations, temperature, and interactions between these variables. The model is predictive across the concentration and temperature ranges from which it was derived. The potential effects of varying oxidation states of plutonium, which are easily accessible in aqueous media, on the bulk solution density of the ternary system were also investigated. The resulting Pitzer-derived density law was applied to a nuclear criticality safety model, and the impact of the experimental characterization of solution density relative to previous estimates was demonstrated to be significant and suggest that the current approach to estimating density in nuclear criticality safety calculations may lead to overly conservative controls.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Feasibility study of a compact neutron resonance transmission analysis instrument

Neutron Resonance Transmission Analysis (NRTA) uses resonant absorption of neutrons to infer the absolute isotopic composition of a target object, enabling applications in a broad range of fields such as archaeology, enrichment analysis of nuclear fuel, and arms control treaty verification. In the past, NRTA involved large user facilities and complex detector systems. However, recent advances in the intensity of compact neutron sources have made compact neutron imaging designs increasingly feasible. This work describes the Monte Carlo (MC) based design of a compact epithermal NRTA radiographic instrument which uses a moderated, compact deuterium-tritium (DT) neutron source and an epithermal neutron detector. Such an instrument would have a wide range of applications, and would be especially impactful for such scenarios as nuclear inspection and arms control verification exercises, where system complexity and mobility may be of critical importance. The MC simulations presented in this work demonstrate accurate time-of-flight (TOF) reconstructions for transmitted neutron energies, capable of differentiating isotopic compositions of nuclear material with high levels of accuracy. A new generation of miniaturized and increasingly more intense neutron sources will allow this technique to achieve measurements with greater precision and speed, with significant impact on a variety of engineering and societal problems.

47 OTHER INSTRUMENTATION↗
DOE OSTI2023

Enhancing Monte Carlo Workflows for Nuclear Reactor Analysis with Metamodel-Driven Modeling

Monte Carlo codes are essential components of many reactor physics simulation workflows as high-fidelity continuous-energy neutron transport solvers. Among Monte Carlo radiation transport codes, MCNP is particularly notable due to its diverse simulation capabilities, large user base, and long validation history. Despite being a powerful simulation tool, MCNP provides limited capabilities to allow automated execution, model transformation, or support for user-defined logic and abstractions that limit its compatibility with modern workflows. Here, to better integrate MCNP into a modern scientific workflow, we have developed an intuitive yet full-featured MCNP Application Program Interface (API) in Python, named MCNPy, which provides a specialized set of classes for MCNP input development. Moreover, to guarantee that our reading, writing, and modeling capabilities remain self-consistent (and to render the huge scope of the MCNP API manageable), we have adopted a strategy of model-driven software development in which a generalized model of the MCNP input format has been created. From this generalized model, or “metamodel,” problem-specific implementations such as an engine for input validation or a codebase for programmatic operations may be automatically generated. Since MCNPy primarily acts as a Python front-end to the underlying Java API that directly interfaces with the metamodel, it is intrinsically linked to the metamodel and thus remains maintainable. With MCNPy, users can programmatically read, write, and modify any syntactically valid MCNP input file regardless of its origin. These capabilities allow users to automate complicated tasks like design optimization and model translation for nuclear systems. As examples, this work demonstrates the use of MCNPy to find the critical radius of a plutonium sphere and to translate a 9000+ line MCNP input file into a corresponding OpenMC model.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2026

One-dimensional neutron diffraction from layered graphite: Reciprocal space structure and grating behavior

In this work we report observations of one-dimensional neutron diffraction from highly oriented pyrolytic graphite (HOPG), where the scattering angle varies continuously with incident angle following classical grating-like behavior. The 2D polycrystalline structure of HOPG—with highly aligned layers along the 𝑐 axis but random in-plane rotations—creates planes of scattering intensity in reciprocal space at 𝑄 𝑐 =𝑛⁢(2⁢𝜋/𝑑) where 𝑑=3.35Å is the interlayer spacing. As the Ewald sphere sweeps through reciprocal space during sample rotation, it continuously intersects these planes, producing the observed angular dispersion. We observe both first-order (𝑛=1) and second-order (𝑛=2) diffraction at conventional scattering angles (25°–70°), with peak positions that remain temperature-independent between 10 K and 294 K and follow quantitative agreement with momentum conservation 𝑄 𝑐 =𝑘⁢[sin⁡𝜓−sin⁡𝜓 𝑓 ]=𝑛⁢(2⁢𝜋/𝑑). X-ray diffraction under similar conditions shows no comparable behavior, confirming that sharp nuclear-vacuum contrast is essential. While diffraction intensities are weak (∼10 −6 of Bragg peaks), the observations demonstrate how the interplay of atomic-scale periodicity, nuclear contrast, and structural disorder enables observation of continuous diffraction curves at thermal neutron wavelengths, illustrating how HOPG's unique microstructure determines its scattering properties beyond conventional Bragg diffraction.

2-dimensional systems↗
DOE OSTI2024

Extraction of the neutron F 2 structure function from inclusive proton and deuteron deep-inelastic scattering data

The available world deep-inelastic scattering (DIS) data on proton and deuteron structure functions F 2 p , F 2 d , and their ratios are leveraged to extract the free neutron F 2 n structure function, the F 2 n / F 2 p ratio, and associated uncertainties using the latest nuclear effect calculations in the deuteron. Special attention is devoted to the normalization of the proton and deuteron experimental datasets and to the treatment of correlated systematic errors, as well as the quantification of procedural and theoretical uncertainties. The extracted F 2 n dataset is utilized to evaluate the Q 2 dependence of the Gottfried sum rule and the nonsinglet F 2 p − F 2 n moments. To facilitate replication of our study, as well as for general applications, we provide a comprehensive DIS database including all recent Jefferson Lab 6 GeV measurements, the extracted F n 2 , a modified CTEQ-JLab global parton distribution function fit named CJ15nlo_mod, and grids with calculated proton, neutron, and deuteron DIS structure functions. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

High-burnup isotopics bias and uncertainty estimations for LANCR02

Calculated nuclide concentrations are compared against destructive radiochemical assays of modern, high-burnup BWR fuel to validate the LANCR02 lattice physics code. Good agreement is observed between different lattice physics methodologies - including the LANCR02 implementation of Method of Characteristics neutron and gamma transport solver and the TGBLA06 methodology - and against measurements. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

Producing ENDF/B-quality Evaluations of 239 Pu(n,f) and 235 U(n,f) Average Prompt Neutron Multiplicities using the CGMF Model

This report documents evaluations of the neutron-induced 239 Pu and 235 U average prompt neutron multiplicities, $\overline{v}_p$, using the CGMF model developed at LANL. These evaluations are not updates of existing ENDF/B-VIII.0 nuclear data, but were both re-done from "scratch". That is, all experimental data were extracted from EXFOR, re-normalized to the newest nuclear data representing monitor observables, and detailed uncertainties were estimated from information in EXFOR as well as from templates of expected measurement uncertainties. We also included experimental data that were not yet available for ENDF/B-VIII.0, for instance, the data of Marini et al. for 239 Pu(n,f) $\overline{v}_p$ or the data of Khoklov et al. for 235 U(n,f) $\overline{v}_p$. Finally, we include the CGMF model; it computes $\overline{v}_p$ based on model parameters that at the same time calculate fission fragments as a function of mass, Y (A), the average total kinetic energy as a function of incident-neutron energy, $\langle TKE \rangle$(E inc ), etc. Such a detailed fission model that ties together many fission quantities has not been used to date for any $\overline{v}_p$ evaluation in ENDF/B. Here, we show that we can get evaluated 235 U(n,f) and 239 Pu $\overline{v}_p$ that not only correspond well to experimental $\overline{v}_p$, but that the associated evaluated model parameters also yield parameterizations of Y (A), $\langle TKE \rangle$(E inc ), etc., that correspond well to their respective experimental data. The new evaluated 239 Pu(n,f) $\overline{v}_p$ was also combined into a 239 Pu test file with the newest nuclear data for the 239 Pu prompt-fission neutron spectrum and fission cross sections. This new 239 Pu file performed reasonably well in predicting PU-MET-FAST assemblies, reaction rates in Jezebel and Flattop and three LLNL pulsed spheres. Due to that, the new 239 Pu(n,f) $\overline{v}_p$ evaluation presented here is being considered for ENDF/B-VIII.1. Hence, we can show here that CGMF is able to produce ENDF/B quality $\overline{v}_p$ nuclear data.

239Pu, 235U, Average Prompt-fission Neutron Multip↗
DOE OSTI2024

Scintillating Bubble Chambers for Direct Dark Matter Detection, and an Update on SBC-LAr10

The Scintillating Bubble Chamber (SBC) Collaboration aims to use the liquid-noble bubble chamber technology as a low-threshold detector for dark matter particles of 1-10 GeV/c2. The detector combines the remarkable electron recoil (ER) discrimination of the bubble chamber with the event-by-event energy resolution provided by liquid argon (LAr) scintillation, with the crucial added benefit that ER discrimination in liquid-noble bubble chambers extends to much lower thresholds than in past freon-filled bubble chambers, with the potential for quasi-background-free operation at thresholds of 100 eV in nuclear recoil (NR) energy. SBC has developed two functionally identical 10 kg detectors: SBC-LAr10 at Fermilab will calibrate low-threshold performance, while the radio-pure SBC-SNOLAB chamber will execute SBC s first deep-underground dark matter search. SBC-LAr10 at Fermilab was recently installed in the MINOS tunnel 100 meters underground, and the first bubbles are expected this fall. I will present the current status of SBC-LAr10 and describe the suite of gamma and neutron calibrations we will execute. The calibrations will confirm the physics reach of this new technology, motivating not just the SBC-SNOLAB chamber now being assembled but also future searches into the solar neutrino fog at 1 GeV/c2.

Sheng, Zhiheng↗
DOE OSTI2022

Effect of the Nuclear Equation of State on Relativistic Turbulence-induced Core-collapse Supernovae

Abstract The nuclear equation of state (EOS) is an important component in the evolution of core-collapse supernovae. In this paper we make a survey of various EOSs in the literature and analyze their effect on spherical core-collapse models in which the effects of three-dimensional turbulence is modeled by a general relativistic formulation of Supernova Turbulence In Reduced-dimensionality (STIR). We show that the viability of the explosion is quite EOS dependent and that it best correlates with the early-time interior entropy density of the proto–neutron star. We check that this result is not progenitor dependent, although the lowest-mass progenitors show different explosion properties, due to the different pre-collapse nuclear composition. Larger central entropies also induce more vigorous proto–neutron star convection in our one-dimensional turbulence model, as well as a wider convective layer.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Could a Kilonova Kill: A Threat Assessment

Abstract Binary neutron star mergers produce high-energy emissions from several physically different sources, including a gamma-ray burst (GRB) and its afterglow, a kilonova (KN), and, at late times, a remnant many parsecs in size. Ionizing radiation from these sources can be dangerous for life on Earth-like planets when located too close. Work to date has explored the substantial danger posed by the GRB to on-axis observers; here we focus instead on the potential threats posed to nearby off-axis observers. Our analysis is based largely on observations of the GW170817/GRB 170817A multi-messenger event, as well as theoretical predictions. For baseline KN parameters, we find that the X-ray emission from the afterglow may be lethal out to ∼1 pc and the off-axis gamma-ray emission may threaten a range out to ∼4 pc, whereas the greatest threat comes years after the explosion, from the cosmic rays accelerated by the KN blast, which can be lethal out to distances up to ∼11 pc. The distances quoted here are typical, but the values have significant uncertainties and depend on the viewing angle, ejected mass, and explosion energy in ways we quantify. Assessing the overall threat to Earth-like planets, KNe have a similar kill distance to supernovae, but are far less common. However, our results rely on the scant available KN data, and multi-messenger observations will clarify the danger posed by such events.

Astronomy & Astrophysics↗
DOE OSTI2025

Impact of Magnetic-field-driven Anisotropies on the Equation of State Probed in Neutron Star Mergers

Binary neutron star mergers can produce extreme magnetic fields, some of which can lead to strong magnetar-like remnants. While strong magnetic fields have been shown to affect the dynamics of outflows and angular momentum transport in the remnant, they can also crucially alter the properties of nuclear matter probed in the merger. In this work, we provide a first assessment of the latter, determining the strength of the pressure anisotropy caused by Landau-level quantization and the anomalous magnetic moment. To this end, we perform the first numerical relativity simulation with a magnetic polarization tensor and a magnetic-field-dependent equation of state using a new algorithm we present here, which also incorporates a mean-field dynamo model to control the magnetic field strength present in the merger remnant. Our results show that—in the most optimistic case—corrections to the anisotropy can be in excess of 10% and are potentially largest in the outer layers of the remnant. This work paves the way for a systematic investigation of these effects.

General relativity↗
DOE OSTI2021

Safeguards Material Control And Accountancy Considerations For Molten Salt Reactors

Molten salt reactors are a class of nuclear reactor designs with features and operational characteristics that vary significantly. Variations in design features include the physical, chemical, and isotopic composition of fresh and irradiated fuel, neutron energy spectrums, breeding ratios, and the design’s plans for chemical processing. Specific designs within these variations affect the material control and accountancy approaches implemented by both domestic and international nuclear safeguards. This paper identifies safeguards-relevant design features for molten salt reactors and describes how each feature might influence both domestic and international nuclear safeguards implementation. Additionally, this paper describes two potential general categories of material control and accountancy approaches that may be appropriate for molten salt reactors: a black box material-balance approach with measurements on the feed and waste streams combined with robust containment and surveillance on the nuclear material within the reactor or an approach that aims to quantify the nuclear material throughout the reactor (i.e., a process monitoring approach). This paper describes the benefits and challenges of these approaches to meet technical safeguards objectives and identifies gaps in current technologies.

Hogue, Karen↗
DOE OSTI2022

Neutrinoless Double Beta Decay

This White Paper, prepared for the Fundamental Symmetries, Neutrons, and Neutrinos Town Meeting related to the 2023 Nuclear Physics Long Range Plan, makes the case for double beta decay as a critical component of the future nuclear physics program. The major experimental collaborations and many theorists have endorsed this white paper.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗