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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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SU-F-T-77: A Novel Test for Coincidence Between Light Fields and Electron Radiation Fields
Purpose: To validate a novel real time quality assurance device, as a means to test coincidence of light fields to electron radiation fields. Method and Materials: Use a Raven™ (LAP of America Laser Applications) detector, both light fields and electron radiation fields of various electron cones and cutouts from two Clinacs (Varian Medical) were sensed by the phosphor screen and registered by a CCD camera of the device. During measurements, the screen surface of Raven was placed at ISO center level facing the radiation field at any setup angle. Subsequently the light field and the electron radiation field (with 100 MU) were captured separately by the device. The measurements were then analyzed using the Raven software with a maximal 25 by 25 cm^2 field size and 0.25 mm resolution. The results were further compared against those using chromic graphic film (EBT3). To ensure consistence only the dimensions through the central axis were recorded. All the films were analyzed with Dose Lab Pro™ v6.70. Coincidence comparisons were done within the tests on one Clinac and between the two Clinacs. Results: The similar difference means of the field coincidence are indicated from the 18 samples by EBT films and 34 by the Raven as 1.33 ± 0.87 mm verses 1.06 ± 0.58 mm (p = 0.74). The mean differences of the field coincidence between the two Clinacs, 1.16 ± 0.68 mm (n=16) and 1.16 ± 0.48 mm (n=18) respectively, also suggest no statistical difference (p= 0.40). Conclusion: The Raven™ is a comparable quality verification device to the chromic graphic film (EBT3) in checking the coincidence between light and electron radiation fields. In this investigation, the Raven device provided highly reproducible results with real time analysis. Further improvements in its resolution and automatic analyzing capability are warranted.
Investigating Laser Preheat and Applied Magnetic Fields Relevant to the MagLIF Fusion Scheme
The MAGnetized Liner Inertial Fusion (MagLIF) scheme has achieved thermonuclear fusion yields on the Z Facility by imploding a cylindrical liner filled with D 2 fuel that is preheated with a multi-kJ laser and pre-magnetized with an axial Bz=10 T magnetic field. Preheating (T e = 100-200 eV) and pre-magnetizing (10-30 T) the fuel serves to reduce the implosion velocity required to achieve multi-keV fusion-relevant temperatures at stagnation with a modest radial convergence. The challenge of fuel preheat in MagLIF is to deposit multiple-kJ of energy into the underdense (n e /n c <0.1) fuel over ~10 mm target length efficiently and without introducing contaminants. Once the fuel is heated the applied axial magnetic field (ω ce τ e ~ 10) needs to suppress electron thermal conduction sufficiently to prevent unacceptable heat losses to the liner walls. In this LDRD we investigated laser energy deposition at two facilities: The OMEGA-EP laser at the Laboratory for Laser Energetics and the Z-beamlet laser at Sandia National Labs utilizing the PECOS chamber. Multiple experiments were carried out investigating laser transmission through LEH foils, laser heating of underdense gasses and the effects of magnetization on laser preheat. The studies find that magneto-hydrodynamic simulations are able to reproduce energy deposition at MagLIF-like conditions but that at the intensities currently used to preheat MagLIF significant laser plasma instabilities (LPI) occur which partly explain the inability of codes to reproduce previous MagLIF preheat studies. The experiments find that reducing the intensity and smoothing the beam dramatically reduces the amount of stimulated Brillouin backscatter and produces deposition profiles more similar to those produced in simulations. The experiments have provided a large and varied dataset that can be compared to simulations. As part of the LDRD new experimental capabilities have also been developed that will be used to design future MagLIF integrated experiments and investigate fuel magnetization.
Ultra-High Operation Temperature SiC-matrix Solar Thermal Air Receiver (HOTSSTAR) enabled by additive manufacturing: Test Facility & Performance Evaluations
Solar Heat for Industrial Processes (SHIP) cavity receivers are capable of generating electricity or industrial process heat by absorbing thermal energy from solar radiation, focused on a small area. The concentration of solar radiation on the small area of the receiver enables the achievement of high temperatures (ranging from 400°C to 1,100°C) of a working fluid, thus making the SHIP technology thermodynamically comparable with conventional power plants. A volumetric receiver consists of a porous structure-generally made of silicon carbide or metal, which absorbs solar radiation and converts it into heat energy. Heat energy from the porous materials is then transferred to the fluid following through them. A volumetric receiver acts as a convective heat exchanger, transferring heat to the fluid through convection. Open-loop volumetric receivers work with air at atmospheric pressure and are suitable for single-cycle or multi-cycle energy plants. A Model Based Systems Engineering (MBSE) approach was used to develop a test bed at Sandia national Laboratories (SNL) capable of demonstrating an open-loop volumetric air receiver developed by General Electric Aerospace (GE Aerospace). This paper presents the development of the various MBSE methods, test bed, and testing operations for the GE air receiver, which was experimentally demonstrated to achieve 1,350°C for over 3 hours of operation and an approximate 70% receiver efficiency. By being able to achieve such high temperatures >1,000°C, this work provides the potential to support many SHIP industrial use cases.
Large Volume Airborne Contamination Monitoring To Support Nuclear Processes' Deactivation and Decommissioning
Current D and D operations at Hanford have demonstrated a flaw in the current state of the art capability of defining airborne contamination boundaries - Airborne particulate emissions of Pu-239 from CM2H operations on the Hanford Pu Finishing Plant were detected well beyond areas controlled for airborne Pu, putting numerous workers at risk for radiological assimilations - Current air samplers and CAM systems were surveying insufficient volumes of air to accurately predict where respiratory protection was required - Hanford is located in a high radon environment, making air monitoring for alpha emitting actinides challenging in high alpha radon induced backgrounds. - Inexpensive HEPA based home and industrial air purifiers filter significantly higher volumes of air than commercially available continuous-air monitoring (CAM) systems. - Inexpensive models capable of filtered air volumes exceeding 1000 times that of a CAM. - Detector system can be built to detect x-rays generated from actinide decay. - Branching ratios of x-rays are 4 orders of magnitude more intense from Plutonium decay than its gamma emissions. - Detector system can be a low resolution systems, as x-ray region of interest is not terribly congested. - Detection systems evaluated will be designed based on slabs of NaI or pixelated NaI or CsI panels. - Simple graphical user interface software will be developed to operate the detection system. - Concept is to deploy some of these air-purifying systems in nonradiological areas around SRNL to confirm radon can be rejected with confidence. - Generate some filters contaminated with plutonium via electroplated Pu or lab generated simulated particles. - then deploy units in known airborne radiological environments to establish systems ability to accurately measure actinide based hot particles Lab analyses will follow up the system analyses to ensure hot particles were correctly identified. Analysis by Scintillation: - Application of scintillation media to the surface of the filters is being explored. - Evaluating slabs of ZnS(Ag), application of powdered ZnS(Cu) and spray on Perkin Elmer Enhance. - Scintillation events would then be digitized with a digital camera and quantified. - Comparing against sensitivity of a PMT or SiPD readout. - Currently evaluating a Thorlabs 8 Megapixel Monochrome Scientific CCD Camera, hermetically sealed cooled package with a wide angle lens. - Wide angle lens allows complete view of HEPA filter from 7 inches away. - Images taken of glow in the dark paint, as well as plutonium-induced fluorescence. - Plutonium was flamed mounted on a 1 inch diameter stainless steel planchet, covered with a layer of mylar and a section of scintillating ZnS obtained from Eljon. - Currently working on reducing signal-to-noise levels to boost sensitivity. - Dark box to hold contaminated or electroplated source covered filters under fabrication. Analysis by x-ray Spectroscopy: - Branching ratios for x-ray emissions from Plutonium isotopes are orders of magnitude more intense than gamma-ray emissions. - The nuclear databases are incomplete on the branching ratios of some of the isotopes. - Evaluating some custom built SrI2 x-ray spectrometers vs a conventional windowed NaI detector. - SrI2 detectors are carbon-composite-windowed 51 mm x 51 mm. - MCNP calculations to establish self absorbance of filter media on 17 keV x-ray. Radon Rejection: - Activated charcoal pre-filter acts as a Radon trap. - Adding a time lapse feature to camera to aid in radon rejection. SRS Plutonium Fuel Form D and D Operations: Currently deploying air sampler to D and D operation of Pu-238 facility at SRS to generate some field samples to analyze.
Tidal Turbine Test, Downeast Turbines, July 12, 2021
Downeast Turbines tested a tidal turbine prototype with novel rotor/channel system and lateral effluent discharge apparatus (LEDA), during five days of testing in the flume at Alden Lab. Three days of testing (July 12-14, 2021) focused on turbine power metrics of torque and rpm, which were low, and then two days of follow-up testing (July 27-28, 2021) focused on LEDA performance metrics of pressure differential and rates of volumetric flow, with encouraging results. Next step is to to characterize, and even optimize, configurations of the LEDA, using 3D-CFD as a helpful tool, to refine its shape and explore its limits of performance as a means of effluent discharge that augments performance of an instream turbine. An improved configuration of the LEDA will be re-combined with the rotor/channel system of the turbine prototype, and ultimately, the rotor will be re-sized (enlarged), to better match the LEDA's performance capabilities in drawing through a rate of volumetric flow. This submission is Downeast Turbines' Post Access Report for the test event. It includes the files described here (next below), and several reference links. "Downeast TEAMER-Post-Access-Report...docx" is a document file containing the report. "Appendices A, B, and C" are included in this file, and so are "Figures #1-7." "Appendix D - Test Data Workbooks.zip" is an archive file containing all post access data (raw data tables, calculating tables, and graphs), presented in fourteen Excel workbooks as described in the report. "Appendix E - Post Access Figures.zip" is an archive file containing "Figures #8-52," of the report.
Final Report for Wetlands as a Source of Atmospheric Methane: A Multiscale and Multidisciplinary Approach
Boreal peatlands contain large amounts of old carbon, protected by anaerobic and cold conditions. Climate change could result in favorable conditions for the microbial decomposition and release of this old peat carbon as CO2 or CH4 back into the atmosphere. Our goal was to test the potential for this positive biological feedback to climate change at SPRUCE (Spruce and Peatland Response Under Climatic and Environmental Change), a manipulation experiment funded by DOE and occurring in a forested bog in Minnesota. Taking advantage of LLNL’s capabilities and expertise in chemical and isotopic signatures we found that carbon emissions from peat were dominated by recently fixed photosynthates, even after short-term experimental warming. We also found that subsurface hydrologic transport was surprisingly rapid at SPRUCE, supplying microbes with young dissolved organic carbon (DOC). We also identified which microbes oxidize CH4 to CO2 at SPRUCE and found that the most active of these also fix N2 (which means they can utilize atmospheric N, making it accessible for other microbes and plants). These results reflect important interactions between hydrology, carbon cycling, and nitrogen cycling present at the bog and relevant to interpreting experimental results and modeling the wetland response to experimental treatments. LLNL involvement at SPRUCE continues through collaborations and a small contract with ORNL, the lead lab for the SPRUCE experiment.
Resistively Graded Insulation System for Next-Generation Converter-Fed Motors
The objective of this project was to demonstrate the feasibility of a new insulation material system capable of withstanding 10 kV/μs switching voltage ramp rate (dV/dt) with operating frequencies and temperatures targeted at converter-fed motors. If successful, with additional development, this insulation material can enable 5%-10% electric machine energy savings from advanced silicon carbide (SiC) drive implementation. To accomplish these goals, we propose to eliminate partial discharge as a degradation mechanism in high voltage, taped insulation. This can be accomplished through the use of a two-sided coating on a polymer film system that will envelop any residual defects on all sides, effectively creating a Faraday cage around the defect. This project focused on demonstrating the proof of concept for the coating. It was shown that concept of providing a stress grading coating around voids can prevent partial discharge. Simulation and lab scale experiments showed that the design can be implemented in a practical layered structure without causing overheating of the insulation due to conduction. Short term testing and calculations show there is a reasonable likelihood to improved insulation life. A path to full scale production was demonstrated, with gaps in process optimization identified as needing to be closed for full scale implementation. Longer term testing and integration onto a conductor is required to fully quantify life and show benefits at an application level.
Enabling co-simulation of tokamak plant models and plasma control systems
A system for connecting the Plasma Control System and a model of the tokamak Plant in closed loop co-simulation for plasma control development has been in routine use at DIII-D for more than 20 years and at other fusion labs that use variants of the DIII-D PCS for approximately the last decade. Here, co-simulation refers to the simultaneous execution of two independent codes with the exchange of data - Plant actuator commands and tokamak diagnostic data - between them during execution. Interest in this type of PCS-Plant simulation technology has also been growing recently at other fusion facilities. In fact, use of such closed loop control simulations is assumed to play an even larger role in the development of both the ITER Plasma Control System (PCS) and the experimental operation of the ITER device, where they will be used to support verification/validation of the PCS and also for ITER pulse schedule development and validation. We describe the key use cases that motivate the co-simulation capability and the features that must be provided by the Plasma Control System to support it. These features could be provided by the PCS itself or by a model of the PCS. If the PCS itself is chosen to provide them, there are requirements imposed on its architecture. If a PCS model is chosen, there are requirements imposed on the initial implementation of this simulation as well as long-term consequences for its continued development and maintenance. We describe these issues for each use case and discuss the relative merits of the two choices. Several examples are given illustrating uses of the co-simulation method to address problems of plasma control during the operation of DIII-D and of other devices that use the DIII-D PCS.
Maia Mapper: high definition XRF imaging in the lab
Here, Maia Mapper is a laboratory μXRF mapping system for efficient elemental imaging of drill core sections serving minerals research and industrial applications. It targets intermediate spatial scales, with imaging of up to ~80 M pixels over a 500×150 mm 2 sample area. It brings together (i) the Maia detector and imaging system, with its large solid-angle, event-mode operation, millisecond pixel transit times in fly-scan mode and real-time spectral deconvolution and imaging, (ii) the high brightness MetalJet D2 liquid metal micro-focus X-ray source from Excillum, and (iii) an efficient XOS polycapillary lens with a flux gain ~15,900 at 21 keV into a ~32 μm focus, and (iv) a sample scanning stage engineered for standard drill-core sections. Count-rates up to ~3 M/s are observed on drill core samples with low dead-time up to ~1.5%. Automated scans are executed in sequence with display of deconvoluted element component images accumulated in real-time in the Maia detector. Application images on drill core and polished rock slabs illustrate Maia Mapper capabilities as part of the analytical workflow of the Advanced Resource Characterisation Facility, which spans spatial dimensions from ore deposit to atomic scales.
Numerical Simulation of Vibrational Sum Frequency Generation Intensity for Non-Centrosymmetric Domains Interspersed in an Amorphous Matrix: A Case Study for Cellulose in Plant Cell Wall
Vibrational sum frequency generation (SFG) spectroscopy can specifically probe molecular species non-centrosymmetrically arranged in a centrosymmetric or isotropic medium. This capability has been extensively utilized to detect and study molecular species present at the two-dimensional (2D) interface at which the centrosymmetry or isotropy of bulk phases is naturally broken. The same principle has been demonstrated to be very effective for the selective detection of non-centrosymmetric crystalline nanodomains interspersed in three-dimensional (3D) amorphous phases. However, the full spectral interpretation of SFG features has been difficult due to the complexity associated with the theoretical calculation of SFG responses of such 3D systems. This paper describes a numerical method to predict the relative SFG intensities of non-centrosymmetric nanodomains in 3D systems as functions of their size and concentration as well as their assembly patterns, i.e., the distributions of tilt, azimuth, and rotation angles with respect to the lab coordinate. We applied the developed method to predict changes in the CH and OH stretch modes characteristic to crystalline cellulose microfibrils distributed with various orders, which are relevant to plant cell wall structures. As a result, the same algorithm can also be applied to any SFG-active nanodomains interspersed in 3D amorphous matrices.
Redox-homogeneous, gel electrolyte-embedded high-mass-loading cathodes for high-energy lithium metal batteries
Lithium metal batteries have higher theoretical energy than their Li-ion counterparts, where graphite is used at the anode. However, one of the main stumbling blocks in developing practical Li metal batteries is the lack of cathodes with high-mass-loading capable of delivering highly reversible redox reactions. To overcome this issue, here we report an electrode structure that incorporates a UV-cured non-aqueous gel electrolyte and a cathode where the LiNi 0.8 Co 0.1 Mn 0.1 O 2 active material is contained in an electron-conductive matrix produced via simultaneous electrospinning and electrospraying. This peculiar structure prevents the solvent-drying-triggered non-uniform distribution of electrode components and shortens the time for cell aging while improving the overall redox homogeneity. Moreover, the electron-conductive matrix eliminates the use of the metal current collector. When a cathode with a mass loading of 60 mg cm -2 is coupled with a 100 µm thick Li metal electrode using additional non-aqueous fluorinated electrolyte solution in lab-scale pouch cell configuration, a specific energy and energy density of 321 Wh kg -1 and 772 Wh L -1 (based on the total mass of the cell), respectively, can be delivered in the initial cycle at 0.1 C (i.e., 1.2 mA cm -2 ) and 25 °C.
Direct measurement of thermal Knudsen forces in rarefied gas environments
At micro- and nanoscales, momentum transfer between surfaces is influenced by various physical mechanisms, including quantum fluctuations, electromagnetic interactions, electric charges, and the dynamics of (rarefied) gases. Under non-isothermal conditions, rarefied gases give rise to thermal Knudsen forces whose magnitudes strongly depend on the gas species and surface characteristics. Knudsen forces are particularly relevant in nanotechnology, optical manipulation, and aerospace systems, where gas rarefaction occurs due to highly confined geometries, sub-micrometer length scales, and reduced particle densities. Despite their significance, predictive modeling of Knudsen forces is limited by a lack of comprehensive experimental data across diverse materials and surface morphologies. Here, in this work, we present a highly sensitive and adaptable measurement platform capable of directly quantifying Knudsen forces using a suspended, interchangeable micro-cantilever within controlled rarefied helium and nitrogen environments. The system integrates optical fiber interferometry to precisely capture out-of-plane displacements at sub-micrometer resolution, driven by Knudsen forces. From the empirical data, we derive a robust correlation linking the magnitudes of Knudsen forces to energy accommodation coefficients, offering deeper insights into the underlying gas–surface interaction mechanisms.
A combined experimental and machine learning exploration of Ti 2-x Zr x MnCrFeNi high entropy Laves hydrides
A series of high entropy AB 2 -type Ti 2-x Zr x MnCrFeNi alloys (x = 0.6, 0.7, 0.8, 0.9, 1.0, 1.1 and 1.2) were synthesized to investigate their potential for hydrogen storage and chemical compression. The influence of the Ti/Zr ratio was explored in terms of structural, microstructural and thermodynamic properties. The storage capacity together with the reaction enthalpy and entropy changes of the synthesized high entropy alloys were compared to predictions from Machine Learning (ML) to investigate changes in these properties across the explored composition space. The results revealed that a decreasing Zr content consistently lowered the hydride formation enthalpy and increased the plateau pressure from 8 to >90 bar H 2 at 25 °C, in good agreement with ML predictions. Selected compositions (x = 1.0 and 1.2) demonstrated reversible hydrogen storage capability over 150 cycles, with capacities of 1.34–1.40 wt % H 2 and remarkable reaction kinetics (<4 min) at ambient temperature. These experimental and computational findings highlight the potential of this Laves-HEA system as tuneable, stable, and cost-effective materials suitable for long-term operations in stationary hydrogen storage and compression applications.
Adaptive Sparse Grid Discretization (ASGarD)
This code solves the Vlasov-Poisson equations in 6-dimensions without approximation. It uses sparse grid discretization to solve the high-dimensional PDEs. The code functions as a discontinuous Galerkin finite element solver. Advantages/benefits include no approximations, supports high-dimensionality, leadership-scale capability, and implicit time advance.
TMDs and GPDs at a future Electron-Ion Collider
With two options studied at Brookhaven National Lab and Jefferson Laboratory the U.S., an Electron-Ion Collider (EIC) of energy √s=20-100 GeV was under design. Furthermore, the recent 2015 US Nuclear Science Long-Range Planning effort included a future EIC as a recommendation for future construction. The EIC will be unique in colliding polarised electrons off polarised protons and light nuclei, providing the spin degrees of freedom essential to pursue its physics program driven by spin structure, multi-dimensional tomographic images of protons and nuclei, and discovery of the role of collective effects of gluons in nuclei. The foreseen luminosity of the EIC, coupled with its energy variability and reach, will allow unprecedented three-dimensional imaging of the gluon and sea quark distributions, via both TMDs and GPDs, and to explore correlations amongst them. Its hermetic detection capability of correlated fragments promises to similar allow for precise tomographic images of the quark-gluon landscape in nuclei, transcending from light few-body nuclei to the heaviest nuclei, and could uncover how the TMD and GPD landscape changes when gluons display an anticipated collective behavior at the higher energies.
Power Flow in Pulsed-Power Systems: The Influence of Hall Physics and Modeling of the Plasma–Vacuum Interface
Abstract not provided.
Assessing the Implementation of an SDM at Sandia and LLNL
This report assesses the proposed implementation of a Scientific Data Management system that could be co-developed by LLNL and SNL and installed at each lab. In the current view, the systems would not be connected to each other. This report examines the different collaboration possibilities and status of planning and implementation of the teams at LLNL and SNL. The report uses identified requirements from previous work that has been done and documented in [1]. In that work, a set of simulation data management requirements was developed during a series of meetings, starting from requirements developed by Sandia Laboratory. These requirements are expected to evolve, and it is recommended that these requirements be revisited and updated for the following reasons: 1- Advancement in the computing hardware and software which leads to more processing power and better data movement speeds. 2- Advancement in computer algorithms which creates opportunities for better data management and analysis. 3- The need to expand and add to the capabilities of the SDM tools due to advancement in the applications software and due to new requirements by the scientific community. This report builds upon the experience from the work that has been done by some of the team members and the current SDM development efforts at LLNL and Sandia.