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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Ballistic Frenkel-exciton gate with a high on-off ratio
Here it is shown that the exciton interactions within organic dye aggregates, as modeled by the Frenkel Hamiltonian, enable the construction of an on/off switchable exciton gate. In this construction, a single exciton residing on a controlling gate molecule may pass or inhibit the ballistic propagation of an exciton in a proximal gate channel consisting of an array of dye molecules. High on-off ratios in excess of 102 can be achieved through the use of static difference dipole-dipole interactions between the gate and the gate channel which effectively creates a switchable Bragg grating. The gate channel and controlling gate molecule exhibit entanglement with the quantum mechanical superposition of the presence and absence of exciton occupation on the gate molecule.
Protecting backaction-evading measurements from parametric instability
Noiseless measurement of a single quadrature in systems of parametrically coupled oscillators is theoretically possible by pumping at the sum and difference frequencies of the two oscillators, realizing a backaction-evading (BAE) scheme. Although this would hold true in the simplest scenario for a system with pure three-wave mixing, implementations of this scheme are hindered by unwanted higher-order parametric processes that destabilize the system and add noise. We show analytically that detuning the two pumps from the sum and difference frequencies can stabilize the system and fully recover the BAE performance, enabling operation at otherwise inaccessible cooperativities. We also show that the acceleration demonstrated in a weak-signal-detection experiment [Jiang , PRX Quantum 4, 020302 (2023)] was only achievable because of this detuning technique.
Insulating moiré homobilayers lack a threefold symmetric second-harmonic generation
Atoms within moiré bilayers relax in plane to minimize elastic energy; such relaxation brings their space group symmetries down to P1. Here, the ab initio second harmonic generation (SHG) of twisted and atomistically optimized hBN bilayers was determined at four twist angles (θ = 38.21°, 60.00°, 73.17°, and 98.21°) and for three displacements τ measured away from the ground state AA' configuration. All moiré bilayers have a P1 space symmetry after structural optimization. This situation is quite different to monolayers with hexagonal lattices, which retain a threefold symmetry. We point out that the actual symmetries of the SHG reported for hBN bilayers on two experimental works do not coincide with the sixfold symmetric theoretical profiles they provide [either sin 2 (3Φ) or cos 2 (3Φ)], and show that the intrinsic low structural symmetry of (atomically optimized) hBN bilayer moirés can in fact be read out from experimental SHG intensity profiles—which are tunable by θ and by the frequency of light ω: The SHG is most definitely not sixfold symmetric because moirés do not retain a threefold symmetry. Furthermore, an extrinsic twofold symmetry of the SHG emission is realized by tilting the pump by an angle α away from the 2D material's normal, regardless of θ and ω. Furthermore, the design of in-plane and ultrathin sources of SHG with low symmetry could be useful for the eventual creation of entanglement sources from 2D materials.
Quantum-enhanced distributed phase sensing with a truncated SU(1,1) interferometer
In recent years, distributed quantum sensing has gained interest for a range of applications requiring networks of sensors, from global-scale clock synchronization to high energy physics. In particular, a network of entangled sensors can improve not only the sensitivity beyond the shot noise limit, but also enable a Heisenberg scaling with the number of sensors. Here, using bright entangled twin beams, we theoretically and experimentally demonstrate the detection of a linear combination of two distributed phases beyond the shot noise limit with a truncated SU(1,1) interferometer. Specifically, we show a quantum noise reduction of 1.7 ± 0.3 dB below what is possible with the corresponding classical configuration. Additionally, we theoretically extend the use of a truncated SU(1,1) interferometer to a multi-phase-distributed sensing scheme that leverages entanglement as a resource to achieve a quantum improvement in the scaling with the number of sensors in the network. Our results pave the way for developing quantum-enhanced sensor networks that can achieve an entanglement-enhanced sensitivity.
Hardware-Efficient, Fault-Tolerant Quantum Computation with Rydberg Atoms
Not Available
Midcircuit Measurements on a Single-Species Neutral Alkali Atom Quantum Processor
Not Available
High-dynamic-range transmission-mode detection of synchrotron radiation using X-ray excited optical luminescence in diamond
Enhancement of X-ray excited optical luminescence in a 100 µm-thick diamond plate by introduction of defect states via electron beam irradiation and subsequent high-temperature annealing is demonstrated. The resulting X-ray transmission-mode scintillator features a linear response to incident photon flux in the range 7.6 × 10 8 to 1.26 × 10 12 photons s -1 mm -2 for hard X-rays (15.9 keV) using exposure times from 0.01 to 5 s. These characteristics enable a real-time transmission-mode imaging of X-ray photon flux density without disruption of X-ray instrument operation.
Mapping the 3D position of battery cathode particles in Bragg coherent diffractive imaging
In Bragg coherent diffractive imaging, the precise location of the measured crystals in the interior of the sample is usually missing. Obtaining this information would help the study of the spatially dependent behavior of particles in the bulk of inhomogeneous samples, such as extra-thick battery cathodes. This work presents an approach to determine the 3D position of particles by precisely aligning them at the instrument axis of rotation. In the test experiment reported here, with a 60 µm-thick LiNi 0.5 Mn 1.5 O 4 battery cathode, the particles were located with a precision of 20 µm in the out-of-plane direction, and the in-plane coordinates were determined with a precision of 1 µm.
In situ X-ray area detector flat-field correction at an operating photon energy without flat illumination
Flat-field calibration of X-ray area detectors is a challenge due to the inability to generate an X-ray flat-field at the selected photon energy the beamline operates at, which has a strong influence on the measurement behavior of the detector. A method is presented in which a simulated flat-field correction is calculated without flat-field measurements. Instead, a series of quick scattering measurements from an amorphous scatterer is used to calculate a flat-field response. The ability to rapidly obtain a flat-field response allows for recalibration of an X-ray detector as needed without significant expenditure of either time or effort. Area detectors on the beamlines used, such as the Pilatus 2M CdTe, PE XRD1621 and Varex XRD 4343CT, were found to have detector responses that drift slightly over timescales of several weeks or after exposure to high photon flux, suggesting the need to more frequently recalibrate with a new flat-field correction map.