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At least 739 records · Page 41
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Hydrodynamical Simulations of Proton Ingestion Flashes in Type I X-Ray Bursts

We perform the first multidimensional fluid simulations of thermonuclear helium ignition underneath a hydrogen-rich shell. This situation is relevant to Type I X-ray bursts on neutron stars that accrete from a hydrogen-rich companion. Using the low-Mach number fluid code MAESTROeX, we investigate the growth of the convection zone due to nuclear burning, and the evolution of the chemical abundances in the atmosphere of the star. We also examine the convective boundary mixing processes that cause the evolution to differ significantly from previous one-dimensional simulations that rely on mixing-length theory. We find that the convection zone grows outward as penetrating fluid elements cool the overlying radiative layer, rather than directly from the increasing entropy of the convection zone itself. Simultaneously, these flows efficiently mix composition, carrying carbon out of and protons into the convection zone even before contact with the hydrogen shell. We discuss the implications of these effects for future modeling of these events and observations.

astrophysical fluid dynamics↗
DOE OSTI2026

Collapse of Nuclear Collectivity along the 𝑁 = 𝑍 Line

The lifetime of the 𝐽 𝜋 = 2 + state in the self-conjugate 88 Ru nucleus has been determined in an experiment performed using rare-isotope beams provided by the new Facility for Rare Isotope Beams. This is the heaviest 𝑁 = 𝑍 nucleus for which such a measurement has been achieved. 88 Ru was populated by both one-neutron knockout and charge-exchange reactions, and the lifetime of 14.3$^{+2.5}_{−3.4}$ ps was determined using the triple-foil plunger technique. The extracted electromagnetic transition strength shows that the quadrupole collectivity has dropped significantly compared with the highly deformed 𝑁 = 𝑍 region around 𝐴 ∼ 80. These results are compared with state-of-the-art large-scale shell-model and discrete nonorthogonal shell-model calculations. The theoretical calculations indicate a moderate triaxial deformation and suggest that low-lying states in this nucleus are no longer dominated by strong many-particle many-hole excitations, unlike the lighter, highly deformed 𝑁 = 𝑍 nuclei nearby.

59 ≤ A ≤ 89↗
NASA NTRS1981

A model for dwarf novae as progenitors of Type I supernovae

It is suggested that a Type I supernova event can be produced as a result of accretion at low rates (less than 10 to the -10th solar mass/year) onto the white dwarf component of a dwarf-nova close binary. At these low rates, diffusion of the CNO nuclei out of the accreted hydrogen envelope can occur on the accretion time scale, and nuclear burning will occur mainly by the proton-proton chain. Studies of this process show that, when the CNO abundance in the envelope is less than 0.0025 of solar, no thermonuclear flash occurs and no mass is lost. The result of the evolution is a gradually increasing layer of helium beneath the hydrogen-burning shell.

Starrfield, S.↗
DOE OSTI2019

Possible evidence of nonstatistical properties in the Cl 35 ( n , p ) S 35 cross section

In this work, the Cl 35 ( n , p ) and Cl 35 ( n , α ) cross sections at incident neutron energies between 2.42 and 2.74 MeV were measured using the Berkeley High Flux Neutron Generator. The cross sections for Cl 35 ( n , p ) were more than a factor of 3 to 5 less than all of the values in the neutron absorption data libraries, while the Cl 35 ( n , α ) cross sections are in reasonable agreement with the data libraries. Furthermore, the measured energy-differential cross section is consistent with a single resonance with a width of 293(46) keV. This finding indicates that, despite the high incident neutron energy, any attempt to model ($n, x$) cross sections in the vicinity of the $N = Z$ = 20 shell gap requires a resolved resonance approach rather than a Hauser-Feshbach approach.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Coupled Calculations in Helical Steam Generator: Validation on Legacy Data

The NEAMS program aims to develop an integrated multi-physics simulation capability “pellet-to-plant” for the design and analysis of future generations of nuclear power plants. In particular, the Reactor Product Line code suite's multi-resolution hierarchy is being designed to ultimately span the full range of length and time scales present in relevant reactor design and safety analyses, as well as scale from desktop to petaflop computing platforms. Flow-induced vibration (FIV) is widespread problem in energy systems because they rely on fluid movement for energy conversion. Vibrating structures may be damaged as fatigue or wear occurs. Given the importance of reliable components in the nuclear industry, flow-induced vibration has long been a major concern in safety and operation of nuclear reactors. In particular, nuclear fuel rods and steam generators have been known to suffer from flow-induced vibration and related failures. Advanced reactors, such as integral Pressurized Water Reactors (PWRs) considered for Small Modular Reactors (SMR), often rely on innovative component designs to meet cost and safety targets. One component that is the subject of advanced designs is the steam generator, some designs of which forego the usual shell-and-tube architecture in order to fit within the primary vessel. In addition to being more cost- and space-efficient, such steam generators need to be more reliable, since failure of the primary vessel represents a potential loss of coolant and a safety concern. A significant amount of data exists on flow-induced vibration in shell-and-tube heat exchangers, and heuristic methods are available to predict their occurrence based on a set of given assumptions. In contrast, advanced designs have far less data available. Advanced modeling and simulation based on coupled structural and fluid simulations have the potential to predict flow-induced vibration in a variety of designs, reducing the need for expensive experimental programs, especially at the design stage. Over the past five years, the Reactor Product Line has developed the integrated multi-physics code suite SHARP. The goal of developing such a tool is to perform multi-physics neutronics, thermal/fluid, and structural mechanics modeling of the components inside the full reactor core or portions of it with a user-specified fidelity. In particular SHARP contains high-fidelity single-physics codes Diablo for structural mechanics and Nek5000 for fluid mechanics calculations. Both codes are state-of-the-art, highly scalable tools that have been extensively validated. These tools form a strong basis on which to build a flow-induced vibration modeling capability. In this report we discuss one-way coupled calculations performed with Nek5000 and Diablo aimed at simulating available FIV experiments in helical steam generators in the turbulent buffeting regime. In this regime one-way coupling is judged sufficient because the pressure loads do not cause substantial displacements. It is also the most common source of vibration in helical steam generators at the low flows expected in integral PWRs. The legacy data is obtained from two datasets developed at Argonne and B&W.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2024

Global properties of nuclei at finite-temperature within the covariant energy density functional theory

In stellar environments nuclei appear at finite temperatures, becoming extremely hot in core-collapse supernovae and neutron-star mergers. However, due to theoretical and computational complexity, most model calculations of nuclear properties are performed at zero temperature, while those existing at finite temperatures are limited only to selected regions of the nuclide chart. In this study we perform the global calculation of nuclear properties for even-even 8 ≤ Z ≤ 104 nuclei at temperatures in range 0 ≤ T ≤ 2 MeV. Calculations are based on the finite-temperature relativistic Hartree-Bogoliubov model supplemented by the Bonche-Levit-Vautherin vapor subtraction procedure. We find that near the neutron-drip line the continuum states have significant contribution already at moderate temperature T ≈ 1 MeV, thus emphasizing the necessity of the vapor subtraction procedure. Results include neutron emission lifetimes, quadrupole deformations, neutron-skin thickness, proton and neutron pairing gaps, entropy and excitation energy. Up to the temperature T ≈ 1 MeV, the nuclear landscape is influenced only moderately by the finite-temperature effects, mainly by reducing the pairing correlations. Here, as the temperature increases further, the effects on nuclear structures become pronounced, reducing both the deformations and the shell effects.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Two-phonon wobbling in 135 Pr

The second-phonon (n ω = 2) wobbling band has been established in the nucleus 135 Pr. Conclusive evidence for its wobbling nature comes from the ΔI = 1, E2 character of the transitions between the new band and the previously identified transverse wobbler band (n ω = 1) in this nucleus. Theoretical calculations in the framework of the quasiparticle triaxial rotor and triaxial projected shell models are found to be in good agreement with the experimental results.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2017

First-excited state g factor of Te 136 by the recoil in vacuum method

The g factor of the first 2 + state of radioactive 136 Te with two valence protons and two valence neutrons beyond double-magic 132 Sn has been measured by the recoil in vacuum (RIV) method. The lifetime of this state is an order of magnitude longer than the lifetimes of excited states recently measured by the RIV method in Sn and Te isotopes, requiring a new evaluation of the free-ion hyperfine interactions and methodology used to determine the g factor. In this paper, the calibration data are reported and the analysis procedures are described in detail. The resultant g factor has a similar magnitude to the g factors of other nuclei with an equal number of valence protons and neutrons in the major shell. However, an unexpected trend is found in the g factors of the N = 84 isotones, which decrease from 136 Te to 144 Nd. Finally, shell model calculations with interactions derived from the CD Bonn potential show good agreement with the g factors and E2 transition rates of 2 + states around 132 Sn, confirming earlier indications that 132 Sn is a good doubly magic core.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2015

Structure of ²⁰⁷Pb populated in ²⁰⁸Pb + ²⁰⁸Pb deep-inelastic collisions*

The yrast structure of 207 Pb above the 13/2 + isomeric state has been investigated in deep-inelastic collisions of 208 Pb and 208 Pb at ATLAS, Argonne National Laboratory. New and previously observed transitions were measured using the Gammasphere detector array. The level scheme of 207 Pb is presented up to ~ 6 MeV, built using coincidence and γ-ray intensity analyses. In addition, the spin and parity assignments of states were made, based on angular distributions and comparisons to shell model calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Dry Storage Cask Shake Table Experiments - 15733

Recent seismic events have underlined the risks nuclear dry storage casks (DSCs) are exposed. Dominion Virginia Power's North Ann during Virginia 5.8 earthquake, August 2011: - 25 of 27 DSCs moved on their concrete pad; - DSCs shifted from 1.0 to 4 1/2 inches; - Metal components were not damaged; - No radiation was released. The main goals of this study is to evaluate the long-term seismic performance of DSCs using experimental tests. Through use of Scaled DSC Specimens on the UNR six Degree-of-Freedom (DOF) Shaking Table. Scaled model specimen shall satisfy the following: - Model aspect ratio shall cover the range in the available commercial DSCs; - Scaled 1/2.5 specimens shall be presentative for the actual prototype (specially under vertical excitation); - Designed specimen shall sustain handling, sliding and impact during testing. Selected evaluation basis earthquakes: - Near Field Earthquake (M6.0 at 2 km); - Far Field Earthquake (M8.0 at 20 km). The level of spectral acceleration using NUREG 6728 seismic hazard curves. Developed for the following return periods: - 1,000-year return period; - 30,000-year return period. Design: - Design handling system for overpack and MPC; - Check stresses on the outer cylindrical shell of the overpack in case of using anchorage system for the DSCs; - Check resulted stresses due to impact of the scaled specimen on the supporting concrete pad; - Check safety of shell thicknesses; - Design of connections between different parts; - Design of the concrete pads to resist impact during the test. Future Plans: - Evaluate the long-term seismic performance of the existing dry storage casks in U.S. and develop guidelines for re-licensing operating periods of DSCs. - Provide a performance based design guidelines for DSCs to maintain its safety against earthquakes.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2015

Mass Measurement of 56Sc Reveals a Small A=56 Odd-Even Mass Staggering, Implying a Cooler Accreted Neutron Star Crust

We present the mass excesses of 52-57Sc, obtained from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. The masses of 56Sc and 57Sc were determined for the first time with atomic mass excesses of -24.85(59)((+0)(-54)) MeV and -21.0(1.3) MeV, respectively, where the asymmetric uncertainty for 56Sc was included due to possible contamination from a long-lived isomer. The 56Sc mass indicates a small odd-even mass staggering in the A = 56 mass chain towards the neutron drip line, significantly deviating from trends predicted by the global FRDM mass model and favoring trends predicted by the UNEDF0 and UNEDF1 density functional calculations. Together with new shell-model calculations of the electron-capture strength function of 56Sc, our results strongly reduce uncertainties in model calculations of the heating and cooling at the 56Ti electron-capture layer in the outer crust of accreting neutron stars. We find that, in contrast to previous studies, neither strong neutrino cooling nor strong heating occurs in this layer. We conclude that Urca cooling in the outer crusts of accreting neutron stars that exhibit superbursts or high temperature steady-state burning, which are predicted to be rich in A approximate to 56 nuclei, is considerably weaker than predicted. Urca cooling must instead be dominated by electron capture on the small amounts of adjacent odd-A nuclei contained in the superburst and high temperature steady-state burning ashes. This may explain the absence of strong crust Urca cooling inferred from the observed cooling light curve of the transiently accreting x-ray source MAXI J0556-332.

Meisel, Z.↗
DOE OSTI2018

Theory of Carbon Dioxide Absorption by Hanford Waste - 18208

Hanford nuclear waste has a very high pH, and Hanford tanks are ventilated with air. Air has CO{sub 2(g)} in it, which is an acid, so it has some affinity for the waste. The absorption of CO{sub 2} by the waste is important because CO{sub 2} absorption consumes hydroxide at the liquid-air interface, and the hydroxide is important for inhibiting tank corrosion. NaOH is periodically added to some tanks in order to mitigate the surface acidification. The NaOH added then becomes part of the waste and must be treated as waste, increasing the cost of the mission. The Hobbs Equation, developed at the Savannah River site, is used at Hanford to predict CO{sub 2} absorption from the tank ventilation system. In this study, the Hobbs Equation functional form is theoretically evaluated from thermodynamic calculations of CO{sub 2} absorption, and diffusion rates in the waste surface. This study theoretically justifies the empirical equation reported by Hobbs. Thermodynamic calculations performed using the Environmental Simulation Program (ESP) software on a typical double-shell tank waste composition indicate that essentially 100 % of CO{sub 2} that contacts the waste will react with the waste whenever the pH is above 10. In the 1990's, a substantial amount of data was collected on the concentration of CO{sub 2} in the off-gas of ventilated double-shell tanks at Hanford. This historic data was mined in order to determine the quantity of CO{sub 2} absorbed by the waste. The results of this data mining activity determined that tanks below approximately pH 10 (i.e., tank 241-AN-107) will show limited CO{sub 2} absorption, consistent with both the Hobbs model and the theory developed here. Two other tank with higher pH showed contrasting CO{sub 2} absorption. One showed substantial CO{sub 2} absorption, and the other showed minimal CO{sub 2} absorption despite the high waste pH in one tank, presumably because there was minimal contact between the waste surface and most of the air flow. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2024

Analog-antianalog isospin mixing in 47 K 𝛽−decay

Here, we have measured the isospin mixing of the 𝐼 𝜋 =1/2 + , 𝐸 𝑥 = 2.599 MeV state in nearly doubly magic 47 Ca with the isobaric analog 1/2 + state of 47 K . Using the TRIUMF atom trap for 𝛽 decay, we have measured a nonzero asymmetry of the progeny 47 Ca with respect to the initial 47 K spin polarization, which together with the 𝛽 asymmetry implies a nonzero ratio of Fermi to Gamow-Teller matrix elements 𝑦 = 0.098 ± 0.037 for the 1/2 + → 1/2 + transition. Interpreting 𝑦 as mixing between this state and the isobaric analog state implies a Coulomb matrix element magnitude 101 ± 37 keV. This relatively large matrix element supports a model from the literature of analog-antianalog isospin mixing, which predicts large matrix elements in cases involving excess neutrons over protons occupying more than one major shell. The result supports pursuing a search for time-reversal odd, parity-even, isovector interactions using a correlation in 47 K 𝛽 decay.

beta decay↗
DOE OSTI2017

Unexpected distribution of ν 1 f 7 / 2 strength in Ca 49

Here, the calcium isotopes have emerged as a critical testing ground for new microscopically derived shell-model interactions, and a great deal of experimental and theoretical focus has been directed toward this region. We investigate the relative spectroscopic strengths associated with 1f 7/2 neutron hole states in 47,49 Ca following one-neutron knockout reactions from 48,50 Ca. The observed reduction of strength populating the 7/2 – 1 state in 49 Ca, as compared to 47 Ca, is inconsistent with shell-model calculations using both phenomenological interactions such as GXPF1, and interactions derived from microscopically based two- and three-nucleon forces. The result suggests a fragmentation of the l = 3 strength to higher-lying states as suggested by the microscopic calculations, but the observed magnitude of the reduction is not reproduced in any shell-model description.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Impact of areal-density asymmetries on the loss of confinement and ignition threshold in inertial confinement fusion capsules

In inertial confinement fusion implosion experiments, variations in the shell areal density reduce the shell’s inertia to confine the core pressure. Distorted capsules with large areal-density modulations decompress faster than uniform capsules in the disassembly phase. A simple 3-D analytic hot-spot model is derived to include the effects of low-mode areal-density modulations in the ignition criterion. The generalized 3-D ignition criterion for low modes is shown to depend on both the harmonic mean and the arithmetic mean of the areal density. Here, the “thin spots” in the shell are shown to dominate the loss of confinement as reflected by the harmonic mean definition of areal densities.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Correlations of neutron multiplicity and γ -ray multiplicity with fragment mass and total kinetic energy in spontaneous fission of Cf 252

The dependence of correlations of neutron multiplicity ν and γ-ray multiplicity M γ in spontaneous fission of 252 Cf on fragment mass A* and total kinetic energy (TKE) have been investigated by employing the ratio of M γ /ν and the form of M γ (ν). We show for the first time that M γ and ν have a complex correlation for heavy fragment masses, while there is a positive dependence of Mγ for light fragment masses and for near-symmetric mass splits. The ratio M γ /ν exhibits strong shell effects for neutron magic number N=50 and near doubly magic number shell closure at Z=50 and N=82. The γ-ray multiplicity Mγ has a maximum for TKE=165-170 MeV. Above 170 MeV M γ (TKE) is approximately linear, while it deviates significantly from a linear dependence at lower TKE. The correlation between the average neutron and γ-ray multiplicities can be partly reproduced by model calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Generator-coordinate reference states for spectra and 0 ν β β decay in the in-medium similarity renormalization group

We use a reference state based on symmetry-restored states from deformed mean-field or generator-coordinate-method (GCM) calculations in conjunction with the in-medium similarity- renormalization group (IMSRG) to compute spectra and matrix elements for neutrinoless double- beta (0$v$ββ) decay. Because the decay involves ground states from two nuclei, we use evolved operators from the IMSRG in one nucleus in a subsequent GCM calculation in the other. We benchmark the resulting IMSRG+GCM method against complete shell-model diagonalization for both the energies of low-lying states in 48 Ca and 48 Ti and the 0$v$ββ matrix element for the decay of 48 Ca, all in a single valence shell. Our approach produces better spectra than either the IMSRG with a spherical-mean-field reference or GCM calculations with unevolved operators. For the 0$v$ββ matrix element the improvement is slight.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

Phase transitions in core-collapse supernova matter at sub-saturation densities

Phase transitions in hot, dense matter in the collapsing cores of massive stars have an important impact on the core-collapse supernova mechanism as they absorb heat, disrupt homology, and so weaken the developing shock. We perform a three-dimensional, finite temperature Skyrme-Hartree-Fock (SHF) study of inhomogeneous nuclear matter to determine the critical density and temperature for the phase transition between the pasta phase and homogeneous matter and its properties. We employ four different parametrizations of the Skyrme nuclear energy-density functional, SkM*, SLy4, NRAPR, and SQMC700, which span a range of saturation-density symmetry energy behaviors constrained by a variety of nuclear experimental probes. For each of these interactions we calculate free energy, pressure, entropy, and chemical potentials in the range of particle number densities where the nuclear pasta phases are expected to exist, 0.02–0. 12 fm -3 , temperatures 2–8 MeV, and a proton fraction of 0.3. We find unambiguous evidence for a first-order phase transition to uniform matter, unsoftened by the presence of the pasta phases. No conclusive signs of a first-order phase transition between the pasta phases is observed, and it is argued that the thermodynamic quantities vary continuously right up to the first-order phase transition to uniform matter. We compare our results with thermodynamic spinodals calculated using the same Skyrme parametrizations, finding that the effect of short-range Coulomb correlations and quantum shell effects included in our model leads to the pasta phases existing at densities up to 0. 01 fm -3 above the spinodal boundaries, thus increasing the transition density to uniform matter by the same amount. The transition density is otherwise shown to be insensitive to the symmetry energy at saturation density within the range constrained by the concordance of a variety of experimental constraints, and can be taken to be a well determined quantity.

79 ASTRONOMY AND ASTROPHYSICS↗