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At least 739 records · Page 41

UAS Activity Profile Survey

Commercial vendors, trying to tap into the physical protection of critical infrastructure, are offering nuclear facilities the opportunity to borrow detection counter-unmanned aircraft systems (CUAS) equipment to survey the airspace over and around the facility. However, using one vendor or method of detection (e.g., radio frequency [RF], radar, acoustic, visual) will not necessarily provide a complete airspace profile since no single method can detect all UAS threats. Using several detection technologies, the unmanned aircraft systems (UAS) Team, who supports the U.S. National Nuclear Security Administration (NNSA) Office of International Nuclear Security (INS), would like to offer partners a comprehensive airspace profile of the types and frequency of UAS that fly within and around critical infrastructure. Improved UAS awareness will aid in the risk assessment process.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Specification of EBR-II Gamma Scan Data from the Precision Gamma Scanner

The gamma scan data stored in the FIPD was originally measured using the Precision Gamma Scanner (PGS) at the Hot Fuel Examination Facility (HFEF) at Idaho National Laboratory (INL). This system was originally manufactured in 1971 (when the facilities, now at INL, were operated by Argonne National Laboratory) and was upgraded on several occasions. It consists of a germanium gamma ray detector (the exact nature of which changed over time as technology improved), a variable-slit collimator that blocks the view of gamma emissions from all but the selected area of the target, and a computer-controlled system for translating a sample past the slit and logging the data.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Benchmarking Monte Carlo codes for the modelling of low-energy neutron production target reactions

The increasing adoption of accelerator-based neutron sources (ABNS) for applications including neutron capture therapy (NCT) research has highlighted the need for accurate simulation tools. Precise modelling of the neutron production target is crucial to ensure that simulated predictions of neutron beam characteristics used for subsequent beam shaping assembly design are reliable. This work presents a comprehensive benchmarking of four widely-used Monte Carlo codes - Geant4, PHITS, FLUKA (CERN), and MCNP - for modelling low-energy neutron production target reactions. Using their recommended physics models and cross-section libraries, we evaluate each code’s performance in simulating four beam-target reactions: 7 Li(p,n) 7 Be, 9 Be(p,n) 9 B, 9 Be(d,n) 10 B, and C(d,n)N. Predictions of neutron yield, angular distributions, and energy spectra are compared against available thick target experimental data. Results show varying levels of agreement between the codes depending on the reaction type, energy range, and beam characteristics. Geant4, MCNP and PHITS are the overall best performing codes for the simulation of total neutron yield and yield in the forward direction across most reactions. Across energies where experimental benchmarks exist, inter-code discrepancies in total and forward-directed yield are typically 10 to 30%, with larger deviations at near-threshold incident ion energies. PHITS provides the best overall reproduction of experimental spectra, particularly for the 9 Be(p,n) 9 B reaction. Additionally, PHITS demonstrates superior computational performance for most reactions. These findings provide valuable guidance for ABNS design, highlighting the strengths and limitations of each code for the simulation of low-energy neutron production reactions.

43 PARTICLE ACCELERATORS↗

Enhanced Design of Radiation Tolerant High-Temperature Structural Health Monitoring Sensors

Acoustic emission sensors are vital in the nuclear industry for real-time structural health monitoring and early detection of material degradation. By capturing high-frequency stress waves emitted from defects like cracks, corrosion, or fatigue, acoustic emission sensors enable non-invasive monitoring of critical components such as reactor vessels, piping, and containment structures. This technology supports predictive maintenance, enhances safety, and ensures regulatory compliance by providing early warnings of potential failures. It is also instrumental in research, particularly in material testing reactors, where it is used to monitor the behavior of fuels and materials under irradiation, by allowing the detection of cracking or other acoustic signals in real time. This enables the evaluation of performance and accident behavior of advanced fuel concepts.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Boron Nitride Solid-State Neutron Detectors

The goal of this project is to build upon the work performed under the Texas Tech IDEAS project (DE-AR0000964 monitored by Dr. Isik Kizilyalli) to bring the developed B-10 enriched hexagonal boron nitride (h- 10 BN or 10 BN or BN) semiconductor neutron detector technology to the next level of maturity. In comparison to He-3 ( 3 He) gas detectors, BN neutron detectors possess all the intrinsic advantages of semiconductor devices: light weight, compact size, fast response speed, high spatial resolution, high temperature and low voltage operation capability, ease of mass production via existing semiconductor infrastructures, low cost of operation and maintenance, flexible form factors, and durability. The project will develop a prototype h- 10 BN neutron detector as a potential replacement for the 3 He gas neutron detectors (LND 25185 or equivalent) used in various neutron survey meters currently produced and commercialized by Ludlum Measurements, Inc. (LMI). To increase the overall detection efficiency, it is essential to maximize the collection efficiency of charge carriers (electrons and holes) generated by the nuclear reaction, which demands a further push to achieve 10 BN epilayers with improved material quality. The material growth processes will be guided by characterization of structural, optical, and electrical properties of h-BN. Selective devices will be calibrated at LMI. During ARPA-E supporting period, the key material parameters of h-BN produced by metal organic chemical vapor deposition (MOCVD), including the layer thickness, mobility-lifetime product, surface recombination field and detector size for maintaining a high charge collection efficiency all have been improved by several orders of magnitude. These improvements have enabled the realization of high-performance h 10BN semiconductor thermal neutron detectors. Presently, h- 10 BN thermal neutron detectors developed under ARPA-E’s support hold the record high detection efficiency among all solid-state detectors at 59%. With further development in manufacturing, there is no question that h-BN detectors will replace the traditional He-3 gas detectors in certain application areas by offering obvious advantages of semiconductor technologies over gas detectors and opportunities for users to dedicate the scarce and expensive supply of He-3 gas to other application areas where substitutes of He-3 gas are not possible.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Integration of Control Methods and Digital Twins for Advanced Nuclear Reactors

Advanced nuclear reactors offer a new set of features to energy generation, due to their ability to adapt to variable energy demand, operate autonomously, be deployed in rural locations and monitored remotely, afford compact size and lower power ratings, and rely on novel technologies to achieve safer operations. Thus, a requirement for the success of these reactors is the use of intelligent forms of control to track changing power demands, make autonomous decisions, and reduce the need for human involvement. Regulatory requirements pertaining to control of nuclear reactors could be met via historical means of control; however, these are not expected to enable the level of highly autonomous operations desired in advanced nuclear reactors. Historical control methods rely on both logical and high-performance (HP) control. These two types of control are usually used separately, with a human element being introduced whenever decisions are cascaded from one science to another. AI/ML control, on the other hand, can replace the human element in the current U.S. fleet of nuclear power plants (NPPs) by acting as a supervisory optimizer that understands the plant internal/external variables in order to make control decisions, and can easily handle non-linear and multi-input/multi out (MIMO) decisions—another requirement for advanced nuclear reactors that could be difficult to handle via logical and HP control. Because of the harsh operating environments produced in advanced reactors, resulting in the frequent failure of sensors and other types of equipment, and considering the lack of operating history for advanced nuclear reactors, control of advanced nuclear reactors would necessitate relying on a model that can track and adapt to the actual process (i.e., a digital twin). This digital twin can make approximations when knowledge and data are unavailable and would evolve as more knowledge is gained. The reactor control must also be risk-informed to account for the high-consequence nature of advanced reactors. This report introduces a high-level (i.e., not method- or process-specific) integration of the three different control and digital twinning methods able to meet the requirements for advanced nuclear reactors. These methods could be applied during both the operational and design stages of these reactors. The aim is to demonstrate how each method interfaces with and highlights enabling solutions necessitated by the unique features of advanced nuclear reactors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The Radiation Detection for Nuclear Security Summer School: Fiscal Year 2024 Report

The Pacific Northwest National Laboratory (PNNL) hosts the Radiation Detection for Nuclear Security (RDNS) Summer School. This unique course provides students with an overview of nuclear security missions, the technical foundation of applied radiation detection technology, and interactive demonstrations and exercises to connect theory to practice in an evolving research and development area. Fiscal year 2024, an off-year year for the school, included reviewing course content, and sharing about the school in a student engagement session at the Institute of Nuclear Materials Management Annual Meeting. Planning is underway for the 10 th RDNS summer school is planned for the summer of 2025.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Fact Sheet - Long-length Scintillating Fibers for Radiation Detection

As the world looks to underground geological repositories for storing nuclear waste, technologies to safeguard the material are needed. An example of a project that developed a new technology is Tripwire. Tripwire proposes a multi-sensor system approach for geological spent nuclear fuel repositories that relies of radiation, vibration, and electromagnetic detection. Tripwire was developed by the Applied Radiation Measurements and Systems (ARMS) group at INL and sponsored by the National Nuclear Security Administration (NNSA). The ARMS group performs research and development, testing and evaluation, operational support, and training focused on applied ionizing radiation detection and measurement. Application areas include nuclear engineering for advanced reactors and fuel cycle operations, nuclear nonproliferation, nuclear counterproliferation, nuclear forensics, and arms control and disarmament.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

UPF and Y-12 Criticality Accident Alarm System (CAAS) Radiation Testing Report

This report documents the experimental conditions and results for the testing of the Mirion Technologies CAAS-3S Criticality Accident Alarm System (CAAS) for the Y-12 National Security Complex (Y-12) and Uranium Processing Facility (UPF). The testing was conducted at the Godiva IV Burst Reactor at the National Criticality Experiments Research Center (NCERC) at the Nevada National Security Site (NNSS) during the week of January 11, 2021. The testing was conducted in accordance with 25774-QL-POA-JR00-00002-VDE-27.0, CAAS-3S Radiation Testing of Cabinet Components Test Plan. The tests subjected the CAAS-3S system to intense and short duration mixed neutron and gamma radiation fields and to high integrated radiation doses. The purpose of the test was to environmentally qualify various CAAS-3S components in a radiation environment. Successful completion of the tests was predicated on the collaborative efforts of several organizations. Sandia National Laboratory (SNL) and Lawrence Livermore National Laboratory (LLNL) provided dosimetry to estimate photon and neutron dose. Los Alamos National Laboratory (LANL) manages the NCERC facility, operated the Godiva IV reactor, and provided field support for CAAS-3S placement and communications interface for data acquisition systems supplied by Mirion Technologies. Throughout the test campaign, Y-12 and UPF personnel provided technical support in determining changes to the test schedule, as needed, interpretation of the results, and comparison between the measured dosimetry data and predicted results. Throughout the test campaign, Mirion personnel provided technical support in the operation of the CAAS-3S system itself.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

WoRDMAp Outbrief: Workshop on Radiation Detection Materials [Slides]

Project Goal: Identify pathway to reliably grow and fabricate high-performance radiation detectors for use in a variety of nonproliferation applications. 1. Create 3 working groups (semiconductors, inorganic and organic scintillators) that bring together international R&D subject-matter experts (national laboratories, industry, and academia), end users, and mission stakeholders 2. Reach expert consensus views regarding current materials related technology gaps and define prioritized R&D directions required to resolve these gaps 3. Envisage the future state of next-generation radiation detection materials and quantify the benefits to nuclear security applications 4. Provide a comprehensive expert report to DNN R&D program office to serve as roadmap with recommendations for future high-impact office investment in radiation-detection materials development

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

M3AS-25IN1002073: Analysis of data from irradiation testing of printed strain gauges in prototypic nuclear environments

Advancement in additively manufactured strain gauges help address critical technology gaps to accurately monitor real-time materials behavior in reactor experiments. This is critical as it provides data to inform predictive models and simulations that enhance the development of reactors and fuel cycle systems. In this report, additively manufactured strain gauges are exposed to a neutron irradiation environment at the Ohio State University Research Reactor. This report goes over a 2-week campaign for neutron irradiating printed resistive strain gauges and capacitive strain gauges. These results complement the prior separate effects (i.e., mechanical strain, temperature, etc.) testing that were performed on these additive manufactured sensors and presented in prior milestone reports. These results also help progress our understanding of their usage in harsh environment applications. The outcome of developing advanced sensing and instrumentation capabilities plays an important role in increasing the safety, reliability, and energy efficiency of both next-generation and existing nuclear reactors.

36 - MATERIALS SCIENCE↗

Strategic Survey of Antineutrino-based Nonproliferation Technologies

Antineutrinos carry approximately 3% of the total energy released in fission processes. As a consequence, nuclear energy production provides by far the brightest antineutrino sources on Earth. Antineutrino interactions with ordinary matter are weak and these particles cannot be shielded, making them an ideal signature of fissioning systems. However, the same property makes antineutrinos difficult to detect. Antineutrino detection technologies have matured in recent years, and emerging detection approaches warrant further investment. For near-field applications, the major enabling technological advancement, reported in 2018, is the conclusive detection of the antineutrino spectrum in segmented detectors operating at the surface with minimal shielding. For far-field applications, the highlights are the routine detection of reactor antineutrinos at hundreds of kilometer standoff in the kiloton-scale KamLAND and Borexino liquid scintillator detectors, and in particular the observation of the residual South Korean reactor antineutrino flux in KamLAND following the Fukushima disaster that led to shutdown of reactors in Japan

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Thermal Stability of LiNi x Mn y Co z O 2 Cathode Materials

Here, the thermal evolution of LiNi x Mn y Co z O 2 (NMC) lithium-ion battery electrode materials is examined at various states of charge (SOC) or lithium concentrations for a variety of Ni:Mn:Co ratios or electrode compositions. Synchrotron X-ray diffraction (XRD) combined with Rietveld analysis shows the onset decomposition temperatures of phases, decomposition products, lattice parameters, and phase fractions as a function of composition and SOC. SOC impacts the lattice parameters of the NMC phase, where a collapse of the c-axis in the NMC phases is noted due to lithium extraction. Among the compositions examined, the low-Ni NMC111 uncycled sample (NMC111 0% SOC) exhibited the highest thermal stability, with a decomposition temperature approximately 250 °C higher than that of NMC532 0% and NMC811 0%. When the SOC exceeds 50% (i.e., more than 0.4 mol of Li ions extracted), the influence of Ni content on the decomposition temperature becomes negligible, with decomposition occurring around 250−300 °C for all compositions. Ni content also affects the decomposition pathways: NMC111 tends to first form a TM 3 O 4 -type phase, where TM represents transition metals, before transforming into a TMO-type phase, whereas most of the NMC811 samples directly decompose into the TMO phase. The presence of metallic phases was confirmed by both XRD and thermogravimetric-differential scanning calorimetry (TGA-DSC) analysis, as a result of heating under inert conditions. The TGA-DSC results suggest that metallic phase formation is favored at lower SOC in samples with a higher Ni content. This work provides comprehensive insight into the thermal degradation pathways of NMC materials as a function of composition, SOC, and temperature.

Peng, Jian [Univ. of New South Wales, Sydney, NSW ↗

Using cyclotron radiation emission for ultra-high resolution x-ray spectroscopy

Abstract Cyclotron radiation emission spectroscopy (CRES) is an approach to measuring the energy of an electron trapped in an externally applied magnetic field. The bare electron can come from different interactions, including photoelectric absorption, Compton scatters, beta decay, and pair production. CRES relies on measuring the frequency of the electron’s cyclotron motion, and because the measurement times extend over 10 6 –10 7 cycles, the energy resolution is on the order of a single electronvolt. To date, CRES has only been performed on internal beta-emitting radioisotopes, but the technology can be applied to x-ray spectrometery through appropriate selection of a target gas and sufficient intensity of the distinct x-ray source. The applications of this technology range from high-precision measurements of atomic energy levels to calibrations of basic science experiments, to trace element identification. In this work we explore the use of CRES for x-ray spectroscopy within the rubric of measuring the energy levels of argon. Though the energy levels of argon are well established, we adopt this motivation as an example question around which a detector may be designed. The issues we explore include target material, density, electron trapping depth, noise levels, and overall efficiency. We also discuss spectral deconvolution and how the multiple peaks obtained from a single target/source pair can be used to enhance the robustness of the measurement.

07 ISOTOPE AND RADIATION SOURCES↗

A Measurement of the Total Hadronic $\pi^-$ on Argon Cross Section in the Kinetic Energy Range from 0.2-1 Giga-Electron Volts in a Liquid Argon Time Projection Chamber

The liquid argon time projection chamber (LArTPC) technology offers fine-grained tracking along with excellent calorimetric and particle identification capabilities, making it a powerful tool for experimental neutrino physics. Thus, the LArTPC has become the technology of choice for studying neutrino oscillations over short ( 1000 km) baselines by experiments such as MicroBooNE, SBND, ICARUS, and DUNE. The LArIAT (Liquid Argon in a Test-beam) experiment exposes a LArTPC to a controlled beam of charged particles at the Fermilab Test Beam Facility to perform calibration studies and measurements of charged hadron-argon cross sections, with the goal of helping to reduce systematic uncertainties in LArTPC-based neutrino experiments. This work presents a measurement of the total hadronic π⁻-Ar cross section in the kinetic energy range from 0.2 GeV to 1 GeV, using data from the LArIAT experiment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Steady-State Irradiation of Characterized Instruments for Nuclear Thermal Rockets Using In-Pile Experiment Apparatus

The development of nuclear rocket technology is critical for further exploration of extra-terrestrial bodies. Nuclear rockets can provide various advantages over current chemical rockets. However, the harsh environment provides several challenges regarding instrument performance. Temperature extremes, radiation (reactor and space), and the inability to conduct traditional maintenance activities can lead to severe degradation in instrument performance. To better understand the effects of radiation on instrumentation, an irradiation campaign has been designed to test a set of instruments provided by a collaborator in the aerospace industry. Details concerning instrument performance before and after irradiation are provided to allow for an analysis of the tested instruments. Additionally, the design of the irradiation test is described in detail.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Digital risk analysis in nuclear engineering projects: Designing for safety, performance, reliability, and security

Cyber-informed engineering and security-by-design frameworks are important in promoting the need to identify cybersecurity concerns early in the systems engineering lifecycle so risks from adversarial cyber-attacks can be eliminated or reduced through engineering design practices. In addition to adversarial risk, risk in operational technology systems also includes non-adversarial and unintentional risk from other factors such as human performance errors, environmental conditions, design flaws, and device degradation or failure. This paper introduces a new concept for characterizing digital risk, both adversarial and non-adversarial, and provides the basis for initial research into a novel digital risk analysis approach focused on incorporating attack difficulty into a multi-attribute analysis technique using robust decision-making. This digital risk characterization is also used to frame a discussion on the challenges of competing objectives and competing stakeholder requirements in an integrated energy system project that incorporates a small modular reactor and industrial facility.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Workshop on Radiographic Imaging and Applications Research and Development Recommendations for Field Radiography

The Workshop on Radiographic Imaging and Applications (WORIA) brought together subject matter experts from industry, academia, US and UK government agencies, and the national laboratories to provide a forum to liaise and share information between technology developers in government and industry, end users, and mission stakeholder to produce an “expert consensus view” regarding future research directions toward a comprehensive radiography/penetrating imaging portfolio in the Defense Nuclear Nonproliferation Research and Development Near Field Detection Portfolio. The inaugural WORIA was held at the Spallation Neutron Source at Oak Ridge National Laboratory on February 7–9, 2023. The inaugural WORIA meeting focused on field radiography applications, or situations in which a portable imaging system must be brought to an item of interest (rather than the item brought to an imaging facility). This report documents consensus views derived from the meeting and provides research and development recommendations for federal program managers.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗