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DOE OSTI2024

Energy dependent nuclear suppression from gluon saturation in exclusive vector meson production

We calculate exclusive J / ψ photoproduction at high energies in the color glass condensate approach. The results are compared to the center-of-mass energy dependent γ + A → J / ψ + A cross sections extracted from measurements in ultraperipheral heavy ion collisions at RHIC and LHC. We predict strong saturation-driven nuclear suppression at high energies, while LHC data prefer even stronger suppression. We explore effects of nucleon shaped fluctuations and show that the most recent measurement of the | t | -differential incoherent J / ψ cross section prefers large event-by-event fluctuations of the nucleon substructure in heavy nuclei, comparable to that found for a free proton. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

Consistent Nuclear Data Evaluations for Criticality Safety

Evaluations of nuclear data are based on statistical analysis of available experimental data and their uncertainties plus model calculations and their uncertainties. As the models are currently rather limited, the evaluations are heavily biassed toward experimental data, with the caveat that a thorough analysis is also required to understand possible discrepancies between data sets. Hence, as new experimental data become available, they are incorporated into the evaluation procedure. Recent measurements of the 233 U capture to fission cross section ratio at the Los Alamos Neutron Science Center have prompted a re-evaluation of the capture cross section in the resonance and fast regions up to 250 keV. We will discuss the challenges of including the new fast neutron experimental data in an evaluation that is consistent with the resonance region. We will also discuss our consistent evaluation procedure based on the Hauser-Feshbach statistical model for nuclear reactions and its application to the evaluations of 239 Pu and 139 La neutron-induced reactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

Validation of the NOνA experiment 2023-tuning on simulated neutrino-matter interactions

NOνA is a long-baseline neutrino oscillation experiment that utilizes a two-detector design to study the oscillations of muon neutrinos into electron neutrinos over a baseline of 810 km. The Near Detector (ND) measures the neutrino beam spectrum and composition before oscillation, which is then compared to the oscillated neutrino energy spectrum observed in the Far Detector (FD). In the ND, the neutrinos are detected through their interactions with the heavy target nuclei within the detector. NOνA employs the GENIE neutrino event generator for simulating these neutrino-nucleus interactions. However, the default GENIE prediction does not adequately reproduce the ND data. To address this, NOνA developed a tune of the neutrino interaction models within GENIE version 3:0:6 to minimize discrepancies between the simulated predictions and the observed data in the ND. This dissertation tests the NOνA’s 2023 tune of the GENIE neutrino cross-section simulations by performing a data/simulations comparison for the ND. The analysis employed datasets comprising $2.55\times10^{21}$ protons-on-target (POT) in neutrino beam mode and $1.14\times10^{21}$ POT in antineutrino beam mode. The NOνA tuning of neutrino-matter interaction simulations matches with ND data within the $1\sigma$ error band, overestimating muon neutrino and antineutrino charged current interactions by approximately 6 % and 9 %, respectively. Discrepancies were observed in the energy region dominated by Quasi-Elastic-like interactions. Systematic uncertainties associated with the modeling of the neutrino cross-section, particularly those pertaining Quasi-Elastic like interactions, contributed considerably to the overall error in the simulations. Furthermore, the reconstruction algorithm used in NOνA for particle classification demonstrated significant misidentifications between charged pions and protons, as well as a tendency to overlook additional pions or protons in multi-particle simulated events.

Cortés Parra, Camilo Andrés↗

DOE OSTI2023

Measurement of the Neutron-Induced Capture-to-Fission Cross Section Ratio in 233 U at LANSCE [Slides]

This presentation finds that new measurement at LANSCE combining DANCE and NEUANCE at the end of 2020 and 2021. Additionally, two samples of 10 mg and 20 mg of 233 U have been prepared at LANL by Evelyn M. Bond (December 2020). Data analysis has been finished and results of the capture-to-fission ratio on 233 U in the neutron energy region from 0.7 eV to 250 keV have been provided. The focus was to provide data from 1-300 keV. We are providing data from 0.7 eV to 1 keV in addition. The result has been normalized to the ENDF/B-VIII.0 broadened capture-to-fission cross section ratio in the neutron energy region recommended by the Luiz Leal and Marco Pigni, between 8.1 and 14.7 eV. This is the first measurement of the capture-to-fission ratio between 2 - 30 keV. The data show some small differences in the RRR with the evaluation though the general trend is consistent. In the URR this data shows a smaller capture-to-fission ratio than the evaluation from 10 to 150 keV

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2023

Measurement of the Higgs boson inclusive and differential fiducial production cross sections in the diphoton decay channel with pp collisions at $\sqrt{s}$ = 13 TeV

The measurements of the inclusive and differential fiducial cross sections of the Higgs boson decaying to a pair of photons are presented. The analysis is performed using proton-proton collisions data recorded with the CMS detector at the LHC at a centre-of-mass energy of 13 TeV and corresponding to an integrated luminosity of 137 fb -1 . The inclusive fiducial cross section is measured to be σ fid = 73.4$^{+5.4}_{-5.3}$ (stat)$a^{+2.4}_{-2.2 }$(syst) fb, in agreement with the standard model expectation of 75.4 ± 4.1 fb. The measurements are also performed in fiducial regions targeting different production modes and as function of several observables describing the diphoton system, the number of additional jets present in the event, and other kinematic observables. Two double differential measurements are performed. No significant deviations from the standard model expectations are observed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

The cross-section measurement for the 3 H($e, e'K^+)nnΛ$ reaction

The small binding energy of the hypertriton leads to predictions of the non-existence of bound hypernuclei for isotriplet three-body systems such as nnΛ. However, invariant mass spectroscopy at GSI has reported events that may be interpreted as the bound nnΛ state. The nnΛ state was sought by missing-mass spectroscopy via the (e, e'K + ) reaction at Jefferson Lab’s experimental Hall A. The present experiment has higher sensitivity to the nnΛ-state investigation in terms of better precision by a factor of about three. The analysis shown in this article focuses on the derivation of the reaction cross-section for the 3 H(γ*, K + )X reaction. Events that were detected in an acceptance, where a Monte Carlo simulation could reproduce the data well (|δp/p| < 4%), were analyzed to minimize the systematic uncertainty. No significant structures were observed with the acceptance cuts, and the upper limits of the production cross-section of the nnΛ state were obtained to be 21 and $31 nbsr -1 at the 90% confidence level when theoretical predictions of (-B Λ , Γ) = (0.25, 0.8) MeV and (0.55, 4.7) MeV, respectively, were assumed. The cross-section result provides valuable information for examining the existence of nnΛ.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Measurement of the energy-differential 35 Cl( n, p 0 ) 35 S cross section via the ratio with 6 Li( n, α ) 3 H

Knowledge of the neutron-induced 35 Cl ⁢(n, x) cross sections is vital to the design and certification of molten chloride fast reactors (MCFRs) since the 35 Cl (n, p 0 ) 35 S reaction is believed to be a significant reactor poison. However, recently published measurements are inconsistent with each other and with evaluation. Here, the goal of this work is to measure the 35 Cl (n, p 0 ) reaction cross section using a technique that is different from recent measurements. The experiment was conducted at Lawrence Berkeley National Laboratory's (LBNL) 88-Inch Cyclotron using thick target deuteron breakup from a 14 MeV deuteron beam. Energy-differential 35 Cl (n, p 0 ) 35 S cross sections were obtained via ratio with the 6 Li (n, a)⁢ 3 H reaction using an active target experiment with a Cs 2 ⁢LiYCl 6 (CLYC) scintillator. The 35 Cl (n, p 0 ) reaction cross section was measured from 2.02 to 7.46 MeV. The results are consistent with Kuvin et al., confirming a roughly 50% reduction in magnitude relative to the ENDF/B-VIII.0 evaluation. These data provide new insight into the role of natural Cl as an MCFR poison. The reduction of the 35 Cl (n, p 0 ) reaction cross section compared to evaluation suggests that MCFR criticality is less sensitive to Cl enrichment. This may in turn reduce building and operating costs since isotope separation may not be needed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

Machine Learning to Select Experiments Driven by Fundamental Science and Applications for Targeted Nuclear Data Improvement

This work describes a blueprint for a process that accelerates progress in science by quantitatively answering the following question: What is the optimal combination of fundamental-science and application-driven experiments to maximally reduce pertinent data uncertainties? Answering this question entails solving a high-dimensional and complex optimization problem that is best solved with advanced statistic techniques often classified as machine learning. We apply this process within the framework of nuclear data with the aim to select an experiment combination that will reduce uncertainties in 239 Pu nuclear data for neutron energies between 1 and 600 keV. In this field, fundamental-physics driven data, called differential, look at one nuclear physics observable at a time. They are contrasted to application-driven, integral, data where one or few resulting values inform a broad set of nuclear data across several nuclides and energies. The candidates for integral experiments are criticality measurements that were refined by a genetic algorithm to be maximally sensitive to 239 Pu fission cross sections in the desired energy range. Twenty-three candidate differential experiments were investigated and span multiple nuclear physics observables (e.g., total, capture cross sections) for isotopes appearing in the integral experiments. The optimal combination among these candidate experiments was investigated via generalized least squares fitting, augmented with Gaussian processes to ameliorate statistical irregularities in data, and the D-optimality criterion. The latter evaluates for each pair of candidates the joint reduction in uncertainties of all 12200 nuclear data appearing in the integral experiments compared to the knowledge we have from 168 past experiments, theory, and nuclear data. We chose as differential measurements those that investigate 63 Cu and 239 Pu total cross sections, based on D-optimality rank and feasibility constraints. Two integral (criticality) experiments were selected: An experiment with Al 2 ⁢O 3 and graphite interleaved with Pu and a thick Cu reflector explores 1–30 keV, while we target the 30–600 keV range with an experiment that swaps boron in place of graphite with a different geometry.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

Measurement of differential cross sections for the production of a Z boson in association with jets in proton-proton collisions at s = 13 TeV

A measurement is presented of the production of Z bosons that decay into two electrons or muons in association with jets, in proton-proton collisions at a centre-of-mass energy of 13 TeV. The data were recorded by the CMS Collaboration at the LHC with an integrated luminosity of 35.9 fb$^{-1}$. The differential cross sections are measured as a function of the transverse momentum ($p_\mathrm{T}$) of the Z boson and the transverse momentum and rapidities of the five jets with largest $p_\mathrm{T}$. The jet multiplicity distribution is measured for up to eight jets. The hadronic activity in the events is estimated using the scalar sum of the $p_\mathrm{T}$ of all the jets. All measurements are unfolded to the stable particle-level and compared with predictions from various Monte Carlo event generators, as well as with expectations at leading and next-to-leading orders in perturbative quantum chromodynamics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Measurement of ZZ production cross-sections in the four-lepton final state in pp collisions at $\sqrt{s}$ = 13.6 TeV with the ATLAS experiment

This paper reports cross-section measurements of ZZ production in pp collisions at $\sqrt{s}$ = 13.6 TeV at the Large Hadron Collider. The data were collected by the ATLAS detector in 2022, and correspond to an integrated luminosity of 29 fb -1 . Events in the ZZ → 4ℓ(ℓ = e, μ) final states are selected and used to measure the inclusive and differential cross-sections in a fiducial region defined close to the analysis selections. The inclusive cross-section is further extrapolated to the total phase space with a requirement of 66 < m Z < 116 GeV for both Z bosons, yielding 16.8 ± 1.1 pb. The results are well described by the Standard Model predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

Performance improvements of the windowed multipole formalism using a rational fraction approximation of the Faddeeva function

The windowed multipole (WMP) formalism was introduced as a way to calculate Doppler broadened cross sections on the fly during Monte Carlo simulations. While more arithmetic is needed compared to point-wise cross section look-ups, performance remained competitive from the large memory reductions and sequential data access. The single most expensive function call in a depleted fuel assembly problem using WMP comes from the evaluation of the Faddeeva function, which previously relied on a highly accurate, highly-branching algorithm. This paper explores the use of rational fraction approximations tailored to the domain interest of reactor physics applications and the development of lower accuracy approximations sufficient for our application. The rational approximations were implemented and tested in OpenMC on an infinite medium problem to stress the cross section calculation routine and a PWR assembly problem. In both cases, the rational approximation nearly eliminated the ∼ 20% penalty previously observed when comparing to point-wise libraries. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2025

Measurements of the Higgs boson production cross section in the four-lepton final state in proton-proton collisions at $\sqrt{s}$ = 13.6 TeV

The measurements of the Higgs boson (H) production cross sections performed by the CMS Collaboration in the four-lepton (4ℓ, ℓ = e, μ) final state at a center-of-mass energy $\sqrt{s}$ = 13.6 TeV are presented. These measurements are based on data collected with the CMS detector at the CERN LHC in 2022, corresponding to an integrated luminosity of 34.7 fb −1 . Cross sections are measured in a fiducial region closely matching the experimental acceptance, both inclusively and differentially, as a function of the transverse momentum and the absolute value of the rapidity of the four-lepton system. The H → ZZ → 4ℓ inclusive fiducial cross section is measured to be ${2.89}_{-0.49}^{+0.53}{\left({\text{stat}}\right)}_{-0.21}^{+0.29}\left({\text{syst}}\right)$ fb, in agreement with the standard model expectation of ${2.89}_{-0.49}^{+0.53}{\left({\text{stat}}\right)}_{-0.21}^{+0.29}\left({\text{syst}}\right)$ fb.

Higgs physics↗

DOE OSTI2025

Measurements of the Higgs boson production cross section in the four-lepton final state in proton-proton collisions at $\sqrt{s}$ = 13.6 TeV

The measurements of the Higgs boson (H) production cross sections performed by the CMS Collaboration in the four-lepton (4ℓ, ℓ = e, μ) final state at a center-of-mass energy $\sqrt{s}$ = 13.6 TeV are presented. These measurements are based on data collected with the CMS detector at the CERN LHC in 2022, corresponding to an integrated luminosity of 34.7 fb$^{−1}$. Cross sections are measured in a fiducial region closely matching the experimental acceptance, both inclusively and differentially, as a function of the transverse momentum and the absolute value of the rapidity of the four-lepton system. The H → ZZ → 4ℓ inclusive fiducial cross section is measured to be ${2.89}_{-0.49}^{+0.53}{\left({\text{stat}}\right)}_{-0.21}^{+0.29}\left({\text{syst}}\right)$ fb, in agreement with the standard model expectation of ${3.09}_{-0.24}^{+0.27}$ fb.[graphic not available: see fulltext]

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Bayesian Monte Carlo Evaluation Framework for Imperfect Nuclear Data

Bayesian evaluation of resolved resonance region (RRR) nuclear data has historically been carried out using the generalized least squares (GLS) formalism, as implemented in, e.g., SAMMY. We have recently developed a prototype of Bayesian Monte Carlo (BMC) evaluation framework, implemented using a Markov Chain Monte Carlo (MCMC) method with a Metropolis-Hastings (MH) acceptance criterion. This was done in order to remove the approximations underlying the conventional GLS evaluations, namely, the linear approximation, and the approximation that all probability density functions (PDFs) are of the normal kind. Recent works by others have used similar stochastic approaches to quantify cross section uncertainties from ENDF evaluated co-variances, and/or, from integral benchmark data, but those have not been conceived as an evaluation framework like the one presented here.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2023

Observation of large missing-momentum ( e , e ' p ) cross-section scaling and the onset of correlated-pair dominance in nuclei

Herein we report the first measurement of $x_B$-scaling in $(e,e'p)$ cross-section ratios off nuclei relative to deuterium at large missing-momentum of $350 \leq p_{miss} \leq 600$ MeV/c. The observed scaling extends over a kinematic range of $0.7 \leq x_B \leq 1.8$, which is significantly wider than $1.4 \leq x_B \leq 1.8$ previously observed for inclusive $(e,e')$ cross-section ratios. The $x_B$-integrated cross-section ratios become constant (i.e., scale) beginning at $p_{miss}\approx k_F$, the nuclear Fermi momentum. Comparing with theoretical calculations we find good agreement with Generalized Contact Formalism calculations for high missing-momentum ($> 375$ MeV/c), suggesting the observed scaling results from interacting with nucleons in short-range correlated (SRC) pairs. For low missing-momenta, mean-field calculations show good agreement with the data for $p_{miss}\le k_F$, and suggest that contributions to the measured cross-section ratios from scattering off single, un-correlated, nucleons are non-negligible up to $p_{miss}\approx 350$ MeV/c. Therefore, SRCs become dominant in nuclei at $p_{miss}\approx 350$ MeV/c, well above the nuclear Fermi Surface of $k_F \approx 250$ MeV/c.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

First Observation of Large Missing-Momentum (e,e'p) Cross-Section Scaling and the onset of Correlated-Pair Dominance in Nuclei

We report the first measurement of $x_B$-scaling in $(e,e'p)$ cross-section ratios off nuclei relative to deuterium at large missing-momentum of $350 \leq p_{miss} \leq 600$ MeV/c. The observed scaling extends over a kinematic range of $0.7 \leq x_B \leq 1.8$, which is significantly wider than $1.4 \leq x_B \leq 1.8$ previously observed for inclusive $(e,e')$ cross-section ratios. The $x_B$-integrated cross-section ratios become constant (i.e., scale) beginning at $p_{miss}\approx k_F$, the nuclear Fermi momentum. Comparing with theoretical calculations we find good agreement with Generalized Contact Formalism calculations for high missing-momentum ($> 375$ MeV/c), suggesting the observed scaling results from interacting with nucleons in short-range correlated (SRC) pairs. For low missing-momenta, mean-field calculations show good agreement with the data for $p_{miss}\le k_F$, and suggest that contributions to the measured cross-section ratios from scattering off single, un-correlated, nucleons are non-negligible up to $p_{miss}\approx 350$ MeV/c. Therefore, SRCs become dominant in nuclei at $p_{miss}\approx 350$ MeV/c, well above the nuclear Fermi Surface of $k_F \approx 250$ MeV/c.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Measurement of B$_\mathrm{c}$(2S)$^+$ and B$_\mathrm{c}^*$(2S)$^+$ cross section ratios in proton-proton collisions at $\sqrt{s} =$ 13 TeV

The ratios of the Bc(2S)+ to Bc+, Bc*(2S)+ to Bc+, and Bc*(2S)+ to Bc(2S)+ production cross sections are measured in proton-proton collisions at s=13 TeV, using a data sample collected by the CMS experiment at the LHC, corresponding to an integrated luminosity of 143 fb-1. The three measurements are made in the Bc+ meson phase space region defined by the transverse momentum pT>15 GeV and absolute rapidity |y|<2.4, with the excited Bc(*)(2S)+ states reconstructed through the Bc(*)+π+π−, followed by the Bc+→J/ψπ+ and J/ψ→μ+μ− decays. The Bc(2S)+ to Bc+, Bc*(2S)+ to Bc+, and Bc*(2S)+ to Bc(2S)+ cross section ratios, including the unknown Bc(*)(2S)+→Bc(*)+π+π− branching fractions, are (3.47±0.63(stat)±0.33(syst))%, (4.69±0.71(stat)±0.56(syst))%, and 1.35±0.32(stat)±0.09(syst), respectively. None of these ratios shows a significant dependence on the pT or |y| of the Bc+ meson. The normalized dipion invariant mass distributions from the decays Bc(*)(2S)+→Bc(*)+π+π− are also reported.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

New H2O–H2O collisional rate coefficients for cometary applications

ABSTRACT We re-introduce a semiclassical methodology based on theories developed for the determination of broadening coefficients. We show that this simple and extremely fast methodology provides results that are in good agreement with results obtained using the more sophisticate MQCT approach. This semiclassical methodology could be an alternative approach which allows to provide large sets of collisional data for very complex molecular systems. It saves time both on the determination of potential energy surfaces and on the collisional dynamical calculations. In addition, this paper provides more complete sets of rotational de-excitation cross-sections and rate coefficients of H2O perturbed by a thermal average of water molecules. Those data can be used in the radiative transfer modelling of cometary atmospheres.

Boursier, C.↗