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All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Characterizing the intracluster light over the redshift range 0.2 < z < 0.8 in the DES-ACT overlap

ABSTRACT We characterize the properties and evolution of bright central galaxies (BCGs) and the surrounding intracluster light (ICL) in galaxy clusters identified in the Dark Energy Survey and Atacama Cosmology Telescope Survey (DES-ACT) overlapping regions, covering the redshift range 0.20 < z < 0.80. Over this redshift range, we measure no change in the ICL’s stellar content (between 50 and 300 kpc) in clusters with log10(M200m,SZ/M⊙) >14.4. We also measure the stellar mass–halo mass (SMHM) relation for the BCG+ICL system and find that the slope, β, which characterizes the dependence of M200m,SZ on the BCG+ICL stellar mass, increases with radius. The outskirts are more strongly correlated with the halo than the core, which supports that the BCG+ICL system follows a two-phase growth, where recent growth (z < 2) occurs beyond the BCG’s core. Additionally, we compare our observed SMHM relation results to the IllustrisTNG300-1 cosmological hydrodynamic simulations and find moderate qualitative agreement in the amount of diffuse light. However, the SMHM relation’s slope is steeper in TNG300-1 and the intrinsic scatter is lower, likely from the absence of projection effects in TNG300-1. Additionally, we find that the ICL exhibits a colour gradient such that the outskirts are bluer than the core. Moreover, for the lower halo mass clusters (log10(M200m,SZ/M⊙) < 14.59), we detect a modest change in the colour gradient’s slope with lookback time, which combined with the absence of stellar mass growth may suggest that lower mass clusters have been involved in growth via tidal stripping more recently than their higher mass counterparts.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Insights into the origin of halo mass profiles from machine learning

ABSTRACT The mass distribution of dark matter haloes is the result of the hierarchical growth of initial density perturbations through mass accretion and mergers. We use an interpretable machine-learning framework to provide physical insights into the origin of the spherically-averaged mass profile of dark matter haloes. We train a gradient-boosted-trees algorithm to predict the final mass profiles of cluster-sized haloes, and measure the importance of the different inputs provided to the algorithm. We find two primary scales in the initial conditions (ICs) that impact the final mass profile: the density at approximately the scale of the haloes’ Lagrangian patch RL ($R\sim 0.7\, R_L$) and that in the large-scale environment (R ∼ 1.7 RL). The model also identifies three primary time-scales in the halo assembly history that affect the final profile: (i) the formation time of the virialized, collapsed material inside the halo, (ii) the dynamical time, which captures the dynamically unrelaxed, infalling component of the halo over its first orbit, (iii) a third, most recent time-scale, which captures the impact on the outer profile of recent massive merger events. While the inner profile retains memory of the ICs, this information alone is insufficient to yield accurate predictions for the outer profile. As we add information about the haloes’ mass accretion history, we find a significant improvement in the predicted profiles at all radii. Our machine-learning framework provides novel insights into the role of the ICs and the mass assembly history in determining the final mass profile of cluster-sized haloes.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1993

Helium-Like Iron Line Temperature Diagnostics in Clusters of Galaxies

The emission complex around 6.7 keV, arising from He-like Fe lines and their dielectronic satellites, has been observed at low resolution in a number of clusters of galaxies. With sufficient spectral resolution as in, e.g., solar flare observations, the ratio, G = (x + y + z)/w, of the intercombination (x and y) and forbidden (z) to the resonance (w) lines arising from the n = 2 level of the He-like ion, is a sensitive temperature diagnostic. We examine this role for G in the context of spatially and spectrally resolved observations of clusters of galaxies. The temperature behavior of this ratio is strongly dependent on the spectral resolution. We introduce an alternative definition for G that includes the contribution of satellite lines and improves the temperature fidelity of this diagnostic. We find that deprojection of the observed value of G along a line of sight through the cluster can yield accurate temperature profiles for temperatures in the range 10(exp 7)-10(exp 8) K that do not suffer from the cluster model uncertainties inherent in deconvolution of broad-band X-ray surface brightness profiles.

Swartz, Douglas A.↗
NASA NTRS1993

Textures and clusters

We discuss the properties of galaxy clusters expected in a texture-seeded, CDM-dominated, Omega = 1 universe. Assuming that the textures are spherical, we use the spherical collapse model to compute the cluster velocity dispersion (or temperature) distribution function. For objects of mass 10 exp 11 to 10 exp 15 solar masses, we find v varies as M super gamma with gamma of about 0.25. An unbiased (b = 1) texture model predicts too many high-velocity dispersion clusters. A biased texture model appears to be compatible with cluster properties inferred from optical and X-ray observations. In the texture model, the cluster velocity distribution functio does not evolve rapidly; thus, the model predicts the existence of rich clusters at moderate redshift (about 1-2).

Bartlett, James G.↗
DOE OSTI2023

The Effect of Splashback on Weak Lensing Mass Estimates of Galaxy Clusters and Groups

The splashback radius of a dark matter halo, which corresponds to the first apocenter radius reached by infalling matter and substructures, has been detected around galaxy clusters using a multitude of observational methods, including weak lensing measurements. In this manuscript, we present how the splashback feature in the halo density profile affects galaxy cluster masses derived through weak lensing measurements if it is not accounted for. We find that the splashback radius has an increasingly large effect on group-sized halos towards $M_{200m} \sim 10^{13.5} \mathrm{M_\odot}$. Depending on the model and the radial scale used, the cluster/group masses can be biased low by more than 0.1 dex. This bias, in turn, would result in a slightly lower $\Omega_m$ value if propagated into a cluster cosmology analysis. The splashback effect with group-sized dark matter halos may become important to consider, given the increasingly stringent cosmological constraints coming from optical wide-field surveys.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Bioinformatic and Mechanistic Analysis of the Palmerolide PKS-NRPS Biosynthetic Pathway From the Microbiome of an Antarctic Ascidian

Complex interactions exist between microbiomes and their hosts. Increasingly, defensive metabolites that have been attributed to host biosynthetic capability are now being recognized as products of host-associated microbes. These unique metabolites often have bioactivity targets in human disease and can be purposed as pharmaceuticals. Polyketides are a complex family of natural products that often serve as defensive metabolites for competitive or pro-survival purposes for the producing organism, while demonstrating bioactivity in human diseases as cholesterol lowering agents, anti-infectives, and anti-tumor agents. Marine invertebrates and microbes are a rich source of polyketides. Palmerolide A, a polyketide isolated from the Antarctic ascidian Synoicum adareanum, is a vacuolar-ATPase inhibitor with potent bioactivity against melanoma cell lines. The biosynthetic gene clusters (BGCs) responsible for production of secondary metabolites are encoded in the genomes of the producers as discrete genomic elements. A candidate palmerolide BGC was identified from a S. adareanum microbiome-metagenome based on a high degree of congruence with a chemical structure-based retrobiosynthetic prediction. Protein family homology analysis, conserved domain searches, active site and motif identification were used to identify and propose the function of the ~75 kbp trans-acyltransferase (AT) polyketide synthase-non-ribosomal synthase (PKS-NRPS) domains responsible for the stepwise synthesis of palmerolide A. Though PKS systems often act in a predictable co-linear sequence, this BGC includes multiple trans-acting enzymatic domains, a non-canonical condensation termination domain, a bacterial luciferase-like monooxygenase (LLM), and is found in multiple copies within the metagenome-assembled genome (MAG). Detailed inspection of the five highly similar pal BGC copies suggests the potential for biosynthesis of other members of the palmerolide chemical family. This is the first delineation of a biosynthetic gene cluster from an Antarctic microbial species, recently proposed as Candidatus Synoicihabitans palmerolidicus. These findings have relevance for fundamental knowledge of PKS combinatorial biosynthesis and could enhance drug development efforts of palmerolide A through heterologous gene expression.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Ultra diffuse galaxies in the MATLAS low-to-moderate density fields

Recent advances in deep dedicated imaging surveys over the past decade have uncovered a surprisingly large number of extremely faint low surface brightness galaxies with large physical sizes called ultra diffuse galaxies (UDGs) in clusters and, more recently, in lower density environments. As part of the Mass Assembly of early-Type GaLAxies with their fine Structures (MATLAS) survey, a deep imaging large program at the Canada-France-Hawaii Telescope (CFHT), our team has identified 2210 dwarf galaxies, 59 (~3%) of which qualify as UDGs. Averaging over the survey area, we find ~0.4 UDG per square degree. They are found in a range of low to moderate density environments, although 61% of the sample fall within the virial radii of groups. Based on a detailed analysis of their photometric and structural properties, we find that the MATLAS UDGs do not show significant differences from the traditional dwarfs, except from the predefined size and surface brightness cut. Their median color is as red as the one measured in galaxy clusters, albeit with a narrower color range. The majority of the UDGs are visually classified as dwarf ellipticals with log stellar masses of ~6.5 – 8.7. The fraction of nucleated UDGs (~34%) is roughly the same as the nucleated fraction of the traditional dwarfs. Only five (~8%) UDGs show signs of tidal disruption and only two are tidal dwarf galaxy candidates. A study of globular cluster (GC) candidates selected in the CFHT images finds no evidence of a higher GC specific frequency S N for UDGs than for classical dwarfs, contrary to what is found in most clusters. The UDG halo-to-stellar mass ratio distribution, as estimated from the GC counts, peaks at roughly the same value as for the traditional dwarfs, but spans the smaller range of ~10 – 2000. Finally, we interpret these results to mean that the large majority of the field-to-group UDGs do not have a different formation scenario than traditional dwarfs.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1994

Baryonic dark clusters in galactic halos and their observable consequences

We consider the possibility that approximately 10% of the mass of a typical galaxy halo is in the form of massive (approximately 10(exp 7) solar masses), compact (escape speeds approximately 100 km/s) baryonic clusters made of neutron stars (approximately 10% by mass), black holes (less than or approximately equal to 1%) and brown dwarfs, asteroids, and other low-mass debris (approximately 90%). These general properties are consistent with several different observational and phenomenological constraints on cluster properties subject to the condition that neutron stars comprise approximately 1% of the total halo mass. Such compact, dark clusters could be the sites of a variety of collisional phenomena involving neutron stars. We find that integrated out to the Hubble distance approximately one neutron star-neutron star or neutron star-black hole collision occurs daily. Of order 0.1-1 asteroid-neutron star collisions may also happen daily in the halo of the Milky Way if there is roughly equal cluster mass per logarithmic particle mass interval between asteroids and brown dwarfs. These event rates are comparable to the frequency of gamma-ray burst detections by the Burst and Transient Source Experiment (BATSE) on the Compton Observatory, implying that if dark halo clusters are the sites of most gamma-ray bursts, perhaps approximately 90% of all bursts are extragalactic, but approximately 10% are galactic. It is possible that dark clusters of the kind discussed here could be detected directly by the Infrared Space Observatory (ISO) or Space Infrared Telescope Facility (SIRTF). If the clusters considered in this paper exist, they should produce spatially correlated gravitational microlensing of stars in the Large Magellanic Cloud (LMC). If 10% of the halo is in the form of dark baryonic clusters, and the remaining 90% is in brown dwarfs and other dark objects which are either unclustered or collected into low-mass clusters, then we expect that two events within approximately 1 min of one another are likely to be seen after a total of order 20-30 microlenses have been detected.

Wasserman, Ira↗
DOE OSTI2025

Clustering redshift distribution calibration of weak lensing surveys using the DESI-DR1 spectroscopic dataset

We estimate the source redshift distribution of current weak lensing surveys by applying the clustering-based redshift calibration technique, using the galaxy redshift sample provided by the Dark Energy Spectroscopic Instrument Data Release 1 (DESI-DR1). We cross-correlate the Bright Galaxy Survey (BGS), Luminous Red Galaxies (LRGs) and Emission Line Galaxies (ELGs) from DESI, within the redshift range $0.1 < z < 1.6$, with overlapping tomographic source samples from the Dark Energy Survey (DES), Kilo-Degree Survey (KiDS), and Hyper Suprime-Cam (HSC) survey. Using realistic mock catalogues, we test the stability of the clustering-redshift signal to fitting scale, reference-sample choice, and the evolution of source galaxy bias, and we explicitly model and marginalise over magnification contributions, which become non-negligible at $z \gtrsim 1$ due to the depth of the DESI ELG sample. We then compare the resulting bias-weighted redshift distributions to those calibrated using self-organising map (SOM) techniques, finding agreement within uncertainties for all surveys and tomographic bins. Our results demonstrate that clustering redshifts enabled by DESI's unprecedented spectroscopic sample provides a robust, complementary, and independent constraint capable of reducing one of the dominant systematic uncertainties in weak lensing cosmology.

Ruggeri, R. [Queensland U.]↗
NASA NTRS2019

Recently Formed Crater Clusters on Mars

This study maps and measures assorted properties of new dated crater clusters that formed recently when impactors fragmented in the atmosphere of Mars. We report these statistics for 77 clusters: number of craters, size of cluster, dispersion of cluster, direction (azimuth) from which the impactor approached, and an estimate of the angle from vertical of the impact. Clusters range from a few to hundreds of craters, with most containing tens of craters. They are most commonly dispersed over hundreds of meters, with extents ranging from a few meters to a few kilometers. We find that dispersion generally does not correlate with topographic elevation. However, when the highest elevations are disregarded, clusters are more dispersed at lower elevations, as expected. Impact azimuths are randomly distributed and do not express a clear directionality of incoming meteoroids. Results suggest impacts occur closer to horizontal than expected, which could be due to observational effects. The characteristics we report here provide important constraints for future work in understanding atmospheric fragmentation processes; properties of the impactors themselves, such as density and orbital parameters; and the seismic detectability of impacts. These are critical aspects to understand, as approximately half of current impacts are observed to be clusters.

Clusters↗
NASA NTRS2019

Recently Formed Crater Clusters on Mars

This study maps and measures assorted properties of new dated crater clusters that formed recently when impactors fragmented in the atmosphere of Mars. We report these statistics for 77 clusters:number of craters, size of cluster, dispersion of cluster, direction (azimuth) from which the impactor approached, and an estimate of the angle from vertical of the impact. Clusters range from a few to hundreds of craters, with most containing tens of craters. They are most commonly dispersed over hundreds of meters,with extents ranging from a few meters to a few kilometers. We find that dispersion generally does not correlate with topographic elevation. However, when the highest elevations are disregarded, clusters are more dispersed at lower elevations, as expected. Impact azimuths are randomly distributed and do not express a clear directionality of incoming meteoroids. Results suggest impacts occur closer to horizontal than expected, which could be due to observational effects. The characteristics we report here provide important constraints for future work in understanding atmospheric fragmentation processes; properties of the impactors themselves, such as density and orbital parameters; and the seismic detectability of impacts. These are critical aspects to understand, as approximately half of current impacts are observed to be clusters.

I. J. Daubar↗
DOE OSTI2024

Excited state electronic structure of dimethyl disulfide involved in photodissociation at ∼200 nm

Dimethyl disulfide (DMDS), one of the smallest organic molecules with an S–S bond, serves as a model system for understanding photofragmentation in polypeptides and proteins. Prior studies of DMDS photodissociation excited at ∼266 nm and ∼248 nm have elucidated the mechanisms of S–S and C–S bond cleavage, which involve the lowest excited electronic states S 1 and S 2 . Far less is known about the dissociation mechanisms and electronic structure of relevant excited states of DMDS excited at ∼200 nm. Herein we present calculations of the electronic structure and properties of electronic states S 1 –S 6 accessed when DMDS is excited at ∼200 nm. Our analysis includes a comparison of theoretical and experimental UV spectra, as well as theoretically predicted one-dimensional cuts through the singlet and triplet potential energy surfaces along the S–S and C–S bond dissociation coordinates. Finally, we present calculations of spin–orbit coupling constants at the Franck–Condon geometry to assess the likelihood of ultrafast intersystem crossing. We show that choosing an accurate yet computationally efficient electronic structure method for calculating the S 0 –S 6 potential energy surfaces along relevant dissociation coordinates is challenging due to excited states with doubly excited character and/or mixed Rydberg-valence character. Our findings demonstrate that the extended multi-state complete active space second-order perturbation theory (XMS-CASPT2) balances this computational efficiency and accuracy, as it captures both the Rydberg character of states in the Franck–Condon region and multiconfigurational character toward the bond-dissociation limits. In conclusion, we compare the performance of XMS-CASPT2 to a new variant of equation of motion coupled cluster theory with single, double, and perturbative triple corrections, EOM-CCSD(T)(a)*, finding that EOM-CCSD(T)(a)* significantly improves the treatment of doubly excited states compared to EOM-CCSD, but struggles to quantitatively capture asymptotic energies along bond dissociation coordinates for these states.

Rishi, Varun↗
DOE OSTI2024

Leveraging Hydropower Multi-Sensor Data for Inference and Age-Informed Modeling

Increased demand of operational flexibility such as faster ramp up/down in generation, and more frequent start/stops are putting hydropower plants and their associated components in unprecedented stress. Consequently, these plants are at the high risk of extended and more frequent outage to accommodate unscheduled, and unexpected maintenance. Therefore, hydropower plants are in critical need of data driven and age-informed analysis for their regular and unscheduled operation. Yet not all hydropower plants are exhaustively equipped with sensors and/or measurement streams for their respective components – demanding solutions on how to detect, identify, and locate the cause of any event from the unobservable. Idaho National Laboratory (INL) analyzed the anonymized measurements and event records from the Hydropower Research Institute (HRI) to address this issue, as part of the Water Power Technologies Office (WPTO) funded one year multi-lab project. First, we investigated how time series of multiple sensor measurements can be leveraged to identify an event “root cause” as well as to develop an inference (i.e., estimate the unobservable) problem. INL also investigated how individual hydropower components’ reaction or response times vary across the pre-event, during event, and post-event conditions – enabling the hydropower dynamic models to be age-informed. Finally, the impact of clustering multi-sensor time series on short-term vibration prediction is analyzed. INL will present key findings from these analyses and recommend next steps for stakeholder adoption.

13 HYDRO ENERGY↗
DOE OSTI2022

Surface warming in global cities is substantially more rapid than in rural background areas

Warming trends in cities are influenced both by large-scale climate processes and by local-scale urbanization. However, little is known about how surface warming trends of global cities differ from those characterized by weather observations in the rural background. Here, through statistical analyses of satellite land surface temperatures (2002 to 2021), we find that the mean surface warming trend is 0.50 ± 0.20 K·decade –1 (mean ± one S.D.) in the urban core of 2000-plus city clusters worldwide, and is 29% greater than the trend for the rural background. On average, background climate change is the largest contributor explaining 0.30 ± 0.11 K·decade –1 of the urban surface warming. In city clusters in China and India, however, more than 0.23 K·decade –1 of the mean trend is attributed to urban expansion. We also find evidence of urban greening in European cities, which offsets 0.13 ± 0.034 K·decade –1 of background surface warming.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Characterization of DESI fiber assignment incompleteness effect on 2-point clustering and mitigation methods for DR1 analysis

We present an in-depth analysis of the fiber assignment incompleteness in the Dark Energy Spectroscopic Instrument (DESI) Data Release 1 (DR1). This incompleteness is caused by the restricted mobility of the robotic fiber positioner in the DESI focal plane, which limits the number of galaxies that can be observed at the same time, especially at small angular separations. As a result, the observed clustering amplitude is suppressed in a scale-dependent manner, which, if not addressed, can severely impact the inference of cosmological parameters. We discuss the methods adopted for simulating fiber assignment on mocks and data. In particular, we introduce the fast fiber assignment (FFA) emulator, which was employed to obtain the power spectrum covariance adopted for the DR1 full-shape analysis. We present the mitigation techniques, organised in two classes: measurement stage and model stage. We then use high fidelity mocks as a reference to quantify both the accuracy of the FFA emulator and the effectiveness of the different measurement-stage mitigation techniques. This complements the studies conducted in a parallel paper for the model-stage techniques, namely the θ-cut approach. We find that pairwise inverse probability (PIP) weights with angular upweighting recover the “true” clustering in all the cases considered, in both Fourier and configuration space. Notably, we present the first ever power spectrum measurement with PIP weights from real data.

cosmological simulations↗
DOE OSTI2022

A Novel Trichothecene Toxin Phenotype Associated with Horizontal Gene Transfer and a Change in Gene Function in Fusarium

Fusarium trichothecenes are among the mycotoxins of most concern to food and feed safety. Production of these mycotoxins and presence of the trichothecene biosynthetic gene (TRI) cluster have been confirmed in only two multispecies lineages of Fusarium: the Fusarium incarnatum-equiseti (Incarnatum) and F. sambucinum (Sambucinum) species complexes. Here, we identified and characterized a TRI cluster in a species that has not been formally described and is represented by Fusarium sp. NRRL 66739. This fungus is reported to be a member of a third Fusarium lineage: the F. buharicum species complex. Cultures of NRRL 66739 accumulated only two trichothecenes, 7-hydroxyisotrichodermin and 7-hydroxyisotrichodermol. Although these are not novel trichothecenes, the production profile of NRRL 66739 is novel, because in previous reports 7-hydroxyisotrichodermin and 7-hydroxyisotrichodermol were components of mixtures of 6–8 trichothecenes produced by several Fusarium species in Sambucinum. Heterologous expression analysis indicated that the TRI13 gene in NRRL 66739 confers trichothecene 7-hydroxylation. This contrasts the trichothecene 4-hydroxylation function of TRI13 in other Fusarium species. Phylogenetic analyses suggest that NRRL 66739 acquired the TRI cluster via horizontal gene transfer from a close relative of Incarnatum and Sambucinum. These findings provide insights into evolutionary processes that have shaped the distribution of trichothecene production among Fusarium species and the structural diversity of the toxins.

Food Science & Technology↗
NASA NTRS1995

Spectroscopy of candidate young globular clusters in NGC 1275

We present spectra of the brightest member of the population of compact blue objects discovered in the peculiar galaxy NGC 1275 by Holtzman et al. (1992) using Hubble Space Telescope images. These spectra show strong Balmer absorption lines like those observed in A-type stars, as expected if the object is a young globular cluster. The age estimated from the strength of the Balmer lines is about 0.5 Gyr, although ages ranging from 0.1 Gyr to 0.9 Gyr cannot be confidently excluded given current models of stellar populations. If these estimated ages are adopted for the young cluster population of NGC 1275 as a whole, the fading predicted by stellar populations models gives a luminosity function which is consistent with that of the Galactic globular cluster system convolved with the observational selection function for the NGC 1275 system. We also use the equivalent widths of the Mg b and Fe 5270 features to constrain the metallicity of the young cluster. Combining these absorption-line widths with the age estimates from the Balmer lines and stellar population models, we find a metallicity of roughly solar, based on the Mg b index, and somewhat higher for the Fe 5270 index. The radial velocity of the absorption lines of the cluster spectrum is offset from the emission lines of the galaxy spectrum at the same position by - 130 km/s, providing further evidence for the identification of the object as a global cluster and opening up the future possibility of studying the kinematics of young cluster systems. The discovery of objects with the characteristics of young globular clusters in NGC 1275, which shows evidence of a recent interaction or merger, supports the hypothesis that galaxy interactions and mergers are favorable sites for the formation of globular clusters.

Zepf, Stephen E.↗
DOE OSTI2024

Precision Loading and Delivery of Molecular Cargo by Size-Controlled Coacervation of Gold Nanoparticles Functionalized with Elastin-like Peptides

Thermoresponsive elastin-like peptides (ELPs) have been extensively investigated in biotechnology and medicine, but little attention has been paid to the process by which coacervation causes ELP-decorated particles to aggregate. Here, using gold nanoparticles (AuNPs) functionalized with a cysteine-terminated 96-repeat of the VPGVG sequence (V96-Cys), we show that the size of the clusters that reversibly form above the ELP transition temperature can be finely controlled in the 250 to 930 nm range by specifying the concentration of free V96-Cys in solution and using AuNPs of different sizes. We further find that the localized surface plasmon resonance peak of the embedded AuNPs progressively red-shifts with cluster size, likely due to an increase in particle–particle contacts. We exploit this fine control over size to homogeneously load precise amounts of the dye Nile Red and the antibiotic Tetracycline into clusters of different hydrodynamic diameters and deliver cargos near-quantitatively by deconstructing the aggregates below the ELP transition temperature. Beyond establishing a key role for free ELPs in the agglomeration of ELP-functionalized particles, our results provide a path for the thermally controlled delivery of precise quantities of molecular cargo. This capability might prove useful in combination photothermal therapies and theranostic applications, and to trigger spatially and temporally uniform responses from biological, electronic, or optical systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗