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Lecture Notes on Criticality Safety Validation Using MCNP & Whisper

Training classes for nuclear criticality safety, MCNP documentation. The need for, and problems surrounding, validation of computer codes and data area considered first. Then some background for MCNP & Whisper is given--best practices for Monte Carlo criticality calculations, neutron spectra, S(α,β) thermal neutron scattering data, nuclear data sensitivities, covariance data, and correlation coefficients. Whisper is computational software designed to assist the nuclear criticality safety analyst with validation studies with the Monte Carlo radiation transport package MCNP. Whisper's methodology (benchmark selection – C k 's, weights; extreme value theory – bias, bias uncertainty; MOS for nuclear data uncertainty – GLLS) and usage are discussed.

42 ENGINEERING↗

Measurement of the prompt fission neutron spectrum from 800 keV to 10 MeV for 240 Pu(sf) and for the 240 Pu($n,f$) reaction induced by neutrons of energy from 1–20 MeV

Here, the presence of 240 Pu in nuclear fuels for reactors has resulted in high uncertainties in the results of reactor and nuclear transmutation calculations because of deficiencies in 240 Pu-related nuclear data. Specifically for the prompt fission neutron spectrum (PFNS) of 240 Pu, there is only one neutron-induced, (n,f), measurement at 0.85 MeV incident neutron energy and only one complete spontaneous fission, (sf), measurement. This limited availability of data does not sufficiently guide nuclear data evaluations of these quantities. Here we report on a measurement of both the 240 Pu(sf) and the 240 Pu(n,f) PFNS, both over the emitted neutron energy range of 0.79–10.0 MeV, and from incident neutron energies of 1.0–20.0 MeV for the (n,f) reaction. Measurements were made with a hemispherical array of liquid scintillators at the high-energy Los Alamos Neutron Science Center white neutron source at the Weapons Neutron Research facility as part of the joint LANL-LLNL Chi-Nu experimental campaign to measure actinide fission neutron spectra. These measurements are the first of their kind, and provide clear experimental evidence for second-chance fission, third chance fission, and pre-equilibrium neutron emission processes in neutron-induced fission of 240 Pu, and are the first ever measurements above 1 MeV incident neutron energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measurement of the Prompt Fission Neutron Spectrum from 800 keV to 10 MeV for 240 Pu($sf$) and for the 240 Pu($n,f$) Reaction Induced by Neutrons of Energy from 1-20 MeV

The presence of 240 Pu in nuclear fuels for reactors has resulted in high uncertainties in the results of reactor and nuclear transmutation calculations because of deficiencies in 240 Pu-related nuclear data. Specifically for the prompt fission neutron spectrum (PFNS) of 240 Pu, there is only one neutron-induced, ($n,f$), measurement at 0.85 MeV incident neutron energy and only one complete spontaneous fission, ($sf$), measurement. This limited availability of data does not sufficiently guide nuclear data evaluations of these quantities. Here we report on a measurement of both the 240 Pu($sf$) and the 240 Pu($n,f$) PFNS, both over the emitted neutron energy range of 0.79–10.0 MeV, and from incident neutron energies of 1.0–20.0 MeV for the ($n,f$) reaction. Measurements were made with a hemispherical array of liquid scintillators at the high-energy Los Alamos Neutron Science Center white neutron source at the Weapons Neutron Research facility as part of the joint LANL-LLNL Chi-Nu experimental campaign to measure actinide fission neutron spectra. These measurements are the first of their kind, and provide clear experimental evidence for second-chance fission, third-chance fission, and pre-equilibrium neutron emission processes in neutron-induced fission of 240 Pu, and are the first ever measurements above 1 MeV incident neutron energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Implementation and Validation of Reference Sensitivity Profile Calculations in TRIPOLI 4 - 14247

In current neutron transport calculations, particularly on continuous-energy Monte-Carlo codes, the major source of uncertainty is coming from nuclear data. In order to improve nuclear data evaluations, integral experiments are used. Feedback is then precisely obtained by re-estimating cross-section levels and correlations according to their sensitivity. k{sub eff}-sensitivity coefficients are traditionally obtained using deterministic codes since hands-on methods were not yet implemented in continuous energy Monte Carlo codes. In this paper, an Iterated-Fission-Probability-based method newly developed in the continuous energy Monte Carlo code TRIPOLI-4 will be used to calculate sensitivity coefficient breakdown on isotopes and reactions and results will be compared to those of ERANOS deterministic code. Objective is twofold: to show the reliability of the new TRIPOLI-4 method and to identify where and why profiles are slightly different. Sensitivity profiles, forward and adjoint fluxes are thus meticulously compared using a fine 1968-group energy structure. An OECD international benchmark (Uncertainty Analysis for Criticality Safety Assessment - UACSA - Phase III) is taken as working example to enforce validation and to compare to independent results (e.g. MCNP-6). This benchmark is constituted of two bare spheres filled with homogeneous mixture of uranium and polyethylene (respectively 2% and 50% U-235 enrichments) and gives an overview of issues encountered in thermal reactor cores. Several energy-group structures (1968G, 172G, 33G) are also tested in ERANOS to identify multi-group and implicit effects. Lessons learnt are that continuous Monte Carlo methods seem to be mature and compare well with deterministic codes. Only damper the U-238 elastic - and on certain conditions the U-238 capture - sensitivity coefficient for which difference can reach 30% between TRIPOLI-4 and ERANOS. Indeed concerning U-238, implicit effects are emphasized and multi-group theory remains limited by hypothesis; even a 1968-group structure is not refined enough to properly calculate U-238 elastic scattering k{sub eff}-sensitivity. This reference 3D continuous-energy sensitivity capability in TRIPOLI4-IFP will be extensively used in the uncertainty automated tool RIB of the French Criticality-Safety package CRISTAL. (authors)

42 ENGINEERING↗

Quasi-differential neutron induced neutron emissions from 235 U, and 239 Pu

Uncertainty in nuclear reaction cross sections, angular distributions, and other nuclear data directly impact how well simulations of nuclear systems represent physical observations. Here, to determine how well the nuclear data in ENDF/B-VIII.0, JEFF-3.3, and JENDL-4.0 evaluations describe the physical behaviour of 235 U, and 239 Pu when subjected to a neutron flux, the neutron emission spectrum was measured for carbon, 93.0% 235 U, and 93.9% 239 Pu samples, and compared against detailed MCNP6 simulations. The measurements were performed at the Los Alamos Neutron Science Center using a quasi-differential method previously developed at Rensselaer Polytechnic Institute. The measurement spanned 0.82–20 MeV and 30–150 degrees. The measurements show there are a significant number of discrepancies between library predictions of the neutron yield and physical observation. A few of the main discrepancies found are described in this paper. Based on these results a new evaluation utilizing these results for carbon, 235 U, and 239 Pu is recommended.

235U↗

Preliminary Designs for Criticality Safety Benchmarks—Iron/Steel/Chromium Series

The nuclear criticality safety community uses critical benchmarks extensively when analyzing nuclear systems. Having benchmarks sensitive to important materials of interest helps to ensure safety and constrain results. Critical benchmarks are also invaluable to the nuclear data community, which uses these benchmarks as a check and measure of quality of nuclear data libraries. Additionally, integral benchmarks are often used to validate the performance of computational tools for simulating nuclear systems. Many integral benchmarks have been documented in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook, the International Reactor Physics Experiment Evaluation Project (IRPhEP) handbook, and the Shielding Integral Benchmark Archive Database (SINBAD). The National Criticality Experiments Research Center (NCERC), operated by Los Alamos National Laboratory, is the only general purpose critical experiments facility in the United States of America. NCERC regularly designs and executes critical experiments and other measurements useful to a wide variety of fields including nuclear criticality safety, commercial nuclear energy, nonproliferation, and nuclear data. NCERC has recently developed tools to visualize gaps and deficiencies in existing criticality benchmarks – this work is still ongoing. Through this work and other reviews, some high priority deficiencies have been identified. This paper aims to highlight three areas where additional critical benchmarks would be useful to the nuclear criticality safety community and various other groups. Additionally, NCERC is seeking feedback in regard to these proposed measurements to make sure they are as useful to as many communities as possible.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Magnetic Microcalorimeter Gamma-Detectors for High-Accuracy Nuclear Decay Data

Magnetic microcalorimeters (MMCs) are low-energy gamma-ray detectors with ultra-high energy resolution that are operated at temperatures below 50 mK. They use metallic Au absorbers and paramagnetic Ag:Er sensors to measure gamma-ray energies from an increase in detector temperature. Ultra-low temperatures are made accessible to non-expert users with “dry” dilution refrigerators that replace the traditional liquid N 2 and He pre-cooling with a mechanically cooled pulse-tube refrigerator. Our MMC gamma detectors have achieved an energy resolution below 40 eV FWHM at 60 keV, and they have a uniform and reproducible response function that allows adding spectra from different detector pixels without loss in energy resolution. These properties make MMCs well-suited to re-measure nuclear decay data with increased precision and smaller systematic errors to increase the accuracy of non-destructive assays (NDA). We present recent MMC gamma-ray spectra of Th-234 to show how MMCs can resolve lines that are relevant for NDA analysis and that overlap in Ge spectra. We also discuss the accuracy that MMCs can achieve for nuclear decay data with an emphasis on gamma-ray energies and intensity ratios that current NDA codes are based on.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Optimization Algorithm for Criticality Experiment Design Using Whisper

Many criticality experiments performed to aid in nuclear data evaluation are designed to maximize the sensitivity of the system’s effective neutron multiplication factor to a certain nuclide reaction pair over an energy region of interest. This is typically done by evaluating possible designs in a transport code such as MCNP and selecting the one with the highest desired sensitivity. A designer has many tools to try to maximize this sensitivity such as different moderators, reflectors, fuels, and geometries. This balancing act of identifying a critical and maximally sensitive system become very computationally expensive as more variables are added and higher precisions are desired. In order to identify these optimal configurations more efficiently a Particle Swarm Optimization (PSO) algorithm coupled with MCNP has been developed by Los Alamos National Laboratory (LANL). This algorithm has been used to design two upcoming criticality experiments that will be performed at the National Criticality Experiments Research Center (NCERC), located at the Nevada National Security Site, and operated by LANL, the only general-purpose critical experiments laboratory in the United States. PSO uses a population (swarm) of candidate solutions (particles) on a search space of dimensions such as moderator and reflector thicknesses or enrichments and concentrations. These particles move around the search space from generation to generation according to simple rules. Eventually, the swarm converges on the configuration that is both critical and maximally sensitive to a piece of nuclear data. PSO is well suited for criticality experiments as the algorithm is agnostic to the underlying physics, meaning it is effective on many different experimental setups. This algorithm has been modified to maximize the nuclear data similarity coefficient between an application case and an experiment aimed at replicating the application case using WHISPER, a nuclear criticality safety analysis tool. This allows for the efficient design of critical experiments informed by nuclear data sensitives.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Update of the Cesium-136 Cumulative Fission Yields at Multiple Neutron Energies

Nuclear data is foundational to several fields, including nuclear forensics. Nuclear forensics investigations of fission events, relies heavily on the cumulative fission yields, however several highly useful fission products suffer from very poor nuclear data including cumulative fission yields or associated uncertainties in that value. Cesium-136 is a highly relevant example of this issue, where the cumulative fission yield may be accurate but its uncertainty high enough to preclude its usefulness. In this work we evaluate and calculate an updated cumulative fission yield for 136 Cs for 235 U, 238 U, and 239 Pu at multiple neutron energies or sources using data obtained from irradiation campaigns. In all cases these newly determined cumulative fission yields provided small changes to the actual fission yields but had dramatic improvements to the uncertainty in those yields. These improvements in uncertainty will enable nuclear forensics end users to use 136 Cs data with more confidence.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Integral Experiment Final Design for Thermal/Epithermal eXperiments (TEX) using Highly Enriched Uranium with Polyethylene at Low Temperature (IER-479 CED-2 Report)

The goal of IER-479 is to design uranium critical experiments that can be used to validate low temperature cross sections and criticality safety analyses over multiple neutron energy regimes. Currently, there are no benchmarks in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook at temperatures lower than room temperature (International Criticality Safety Benchmark Evaluation Project Handbook, 2019). However, there are many needs for validation of criticality safety analysis at lower temperatures, including meeting transportation requirements and operations conducted outside or in unheated facilities. Additionally, NCSP has funded North Carolina State (NCSU) to generate new thermal scattering laws, including at lower temperatures, and the lack of integral benchmarks impedes data testing of these new cross sections. To address these needs, this report will present a critical experiment design covering various fission energy regimes with a goal temperature of -40°C (-40°F), which is based on the lower bound of expected non-cryogenic operational temperatures. The goal of the U.S. Nuclear Criticality Safety Program’s (NCSP) Thermal/Epithermal eXperiments (TEX) is to design and conduct new critical experiments to address high priority nuclear data needs from the nuclear criticality safety and nuclear data communities. The TEX program includes two series of baseline experimental configurations, one based on plutonium fuel (plutonium-aluminum Zero Power Physics Reactor (ZPPR) plates) and the other based on uranium fuel (highly enriched uranium (HEU) plates), that are moderated with varying thickness of polyethylene to create assemblies which span the thermal, intermediate, and fast fission energy regimes. The configurations are designed to be easily modified (for example, to add diluent materials of interest) to allow for efficient generation of additional benchmark configurations and allow for added nuclear data testing utility when comparing modified configurations to baseline configurations. The goal of IER-479 is to use the TEX-HEU concept (stack of HEU plates and polyethylene moderators) to design a critical experiment that can be used to validate low temperature cross sections and criticality safety analyses.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Benchmarking GEANT4 and PHITS for 14.8-MeV neutron transport in polyethylene and graphite materials

The feasibility of GEANT4 and PHITS with ENDF/B-VIII.0, JEFF-3.3 and JENDL-4.0 evaluated nuclear data libraries in 14.8-MeV neutron transport simulation are verified by comparing with the MCNP calculations and the experimental data. Here the measured data are from neutron integral experiments including graphite and polyethylene samples. For 6 cm-thick polyethylene and 20 cm-thick graphite samples, the results from GEANT4 and PHITS with three evaluated nuclear data libraries agree well with the MCNP calculations. For a 2 cm-thick graphite sample, the simulated results from GEANT4 and PHITS agree with the MCNP calculations, and they all underestimate the experiment data in below 3 MeV and overestimate them in the energy range of 5–7 MeV. The difference between the simulation results and the experimental data depends on the evaluated nuclear data libraries. In overall, GEANT4 and PHITS are performing reasonable jobs for 14.8-MeV neutron transport simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Accelerating nuclear-integrated data center pursuits in the USA: SWOT analysis, power-thermal management strategies and demonstration plan

Here, this study explores the increasing interest in leveraging nuclear power to meet the escalating energy demands of data centers in the United States (U.S.) by focusing on key factors that contribute to accelerated deployment. The study highlights the importance of N+1/N+2 power supplies (where N is the required number of units), outlines research and innovations in nuclear-integrated data center thermal management and demonstration plan. It also provides updates about status and costing of various reactor system designs. A summarized strengths, weaknesses, opportunities, and threats (SWOT) analysis shows the potential options for grid connectivity, reactors, and site selection. Suitable site discussions consider land and water availability, grid access, and optical fiber connectivity, and the study presents graded prospects for Department of Energy (DOE) sites with a specific example. Community engagement and partnerships are emphasized, particularly the roles of local government, federal agencies, utilities, and data center industry partners, which are crucial for accelerating deployment, business outreach, and approvals. The study provides actionable insights for stakeholders to accelerate the deployment of nuclear-powered data centers.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Issue Summary of INL Phase IV Transient Results for IAEA CRP on HTGR UAM Benchmark

This report details the Parallel and Highly Innovative Simulation for Idaho National Laboratory (INL) Code System (PHISICS)/Reactor Excursions and Leak Analysis Program (RELAP5)-3D results obtained for the transient core exercises defined for Phase IV of the International Atomic Energy Agency (IAEA) Coordinated Research Project (CRP) on high-temperature gas cooled reactor (HTGR) uncertainty analysis in modeling (UAM). The Phase III models and results are linked to the earlier Standardized Computer Analyses for Licensing Evaluation (SCALE)/Sampler/New ESC-based Weighting Transport (NEWT) data generated for the lattice physics (lattice) stage Phase I of the CRP. The focus of this report is the Uncertainty/Sensitivity Assessment (U/SA) of the prismatic modular high-temperature gas cooled reactor (MHTGR)-350 design, and specifically for Exercises IV-1 and IV-2 of the benchmark: the Control Rod Withdrawal (CRW) and Pressurised Loss of Cooling (PLOFC) events. The statistical U/SA methodology is implemented and demonstrated using the RAVEN code, based on perturbed cross-section libraries obtained from the SCALE/Sampler sequence. Uncertainties in nuclear data (cross-sections and the average number of neutrons produced per fission, 235U[¯v ]) lead to standard deviations (uncertainties of one s) of approximately 0.5% in the core eigenvalues of the MHTGR-350 and core models. For the coupled neutronics/thermal fluid model, local power density uncertainties up to 3.6% were observed in the colder regions of the core, while the local maximum fuel temperature uncertainties reached 1.5% for the models that included thermal fluid uncertainties. The addition of thermal fluid uncertainties dominated the impacts of nuclear data uncertainties in all cases. The main contributors to uncertainties in the power density and fuel temperatures during the transients were uncertainties in the reactor operating conditions (total power, inlet mass flow rate and inlet gas temperature). Variations in the bypass flows did not have significant impact on any of the output variables. For the nuclear data uncertainties it was found that the 235U(¯v ) / 235U(¯v ) covariance produced the largest sensitivities in terms of its impact on the eigenvalue and peak reactor power. It was also observed that the impact of any nuclear data uncertainties on the maximum fuel temperature was much less significant that the impact on eigenvalue and power. Another important finding was that although the use of eight or more energy groups is recommended for best-estimate HTGR simulation, two-group models produced acceptable uncertainty and sensitivity results for most FOMs. Since the statistical U/SA methodology is computationally expensive, and most transient solver requirements will scale directly with the number of energy groups, two energy groups could be used by HTGR developers during the early stages of design when larger uncertainty margins can be tolerated.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Activation analysis of the concrete in the Fleurus cyclotron facility - 25604

The purpose of this paper is to discuss the approach and the results of a recent activation analysis concerning a cyclotron facility located in Fleurus, Belgium, where isotopes of medical applications were produced by irradiating either solid (Tl) or gaseous targets (Xe) with 20-30 MeV proton beams. This paper discusses the choice of the intra-nuclear cascade model implemented in MCNP/X to correctly simulate the spallation reactions of the protons in the target, since no nuclear data are available for the isotopes of interest. TENDL nuclear data library, which is based on the models of the nuclear code system TALYS, plays a key role in the selection of the model. The neutron flux distribution throughout the installation and the activation rates in the concrete walls are then calculated with the help of a comprehensive MCNPX model of the facility. The estimated activities are in good agreement with the measurements taken in 2017 in the frame of the ongoing decommissioning of this facility. (authors)

43 PARTICLE ACCELERATORS↗

Nondestructive Assay Technical Infrastructure Program Mission and Vision

The Nondestructive Assay Program (NDAP) mission and vision is achieved by identifying and accomplishing a set of programmatic goals that correspond with eight broad technical program elements. The NDAP was created as a result of Defense Nuclear Facility Safety Board Recommendation 2007-1, entitled “Safety-Related In Situ Nondestructive Assay of Radioactive Materials,” which emphasized the need to improve in situ measurements of radioactive material at US Department of Energy (DOE) defense nuclear facilities. An NDAP five-year plan will define tasks to accomplish specific goals identified in the NDAP mission and vision. This mission and vision is applicable for eight technical program elements: Hardware/Software Development, Algorithm Development and Nuclear Data, Uncertainty Quantification, Nuclear Materials, Staffing, Personnel, And Training, Data Management, Requirement and Standards, and Information Preservation and Dissemination. An additional program element is technical support, which provides daily execution management support for the NDAP, site scope, and deliverable tracking via site task managers, along with technical advisement and support from the technical support group. The NDAP mission and vision provides attributes with specific goals for each program element, and some goals benefit multiple program elements. The goals and attributes defined herein are implemented via an NDAP five-year execution plan that defines site work scope, budget, and deliverables, all of which are updated annually. The NDAP is designed to benefit nondestructive assay (NDA) needs to support DOE nuclear criticality safety programs, ensuring that NDA technology is sufficiently capable of guaranteeing the safety of those who handle, store, process, or transport fissionable materials in the complex. Especially important for the NDAP is to maximize capabilities to identify, characterize, and manage in situ fissile material deposits in process equipment to ensure nuclear criticality safety at processing facilities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

MONK10: A Monte Carlo Code for Criticality Analysis - 14574

The MONK{sup R} code, if we include its predecessor GEM, has now been in use for 50 years. It is a Monte Carlo code for nuclear criticality and reactor physics analyses which is used extensively in the UK nuclear industry and worldwide. In 2014 a major new version of the code, MONK10A, was released introducing many new features; these are described with example applications presented where appropriate. Experience with MONK9A models indicates that MONK10A has increased run-time performance for all cases and on average runs 2.4 times faster. New geometry options include the direct import of CAD generated models using the new IGES body, POLY body, TETMESH Hole and TETMESH Zone features. Example calculations for a selection of CAD import options are presented and compared with the intrinsic MONK geometry representation, with relative merits discussed. New Features are included to assist with the modeling of distributed parameters; such features include Unified Tally (UT), Action Tallies (AT) in UT and Shannon entropy. The latter is useful in assessing the convergence of distributed parameters, such as scalar neutron flux. As such it is an important tool in determining the appropriate point to stop settling and begin scoring stages in a Monte Carlo simulation. The utility of UT, AT-in-UT and Shannon entropy is demonstrated using calculations employing the new CAD import geometry options. Runtime Doppler broadening is included to allow accurate representation of temperature distributions within models. Example calculations which further demonstrate UT and AT-in-UT are presented for different bodies at different temperatures to evaluate the effects of temperature differences on k-effective and reaction rates. The MONK10A code was issued with a new set of continuous energy and group nuclear data libraries. These include JEFF3.1, JEFF3.1.1, JEFF 3.1.2, ENDF/B-VII.0 and CENDL 3.1 libraries. The inclusion of a range of libraries allows the user to evaluate the impact of different international nuclear data evaluations on their results and an example is provided to illustrate the differences that can arise from the use of different nuclear data evaluations. The code was also issued with a new version of the VisualWorkshop IDE to allow easy construction and editing of input decks, running of calculations and display of geometry and results. Examples are provided of the geometry and results display and showing how results can be superimposed upon the geometry. (authors)

42 ENGINEERING↗

RPI LINAC refurbishment and upgrade project

The Electron Linear Accelerator at Rensselaer Polytechnic Institute (RPI) was constructed in the late 1950s and started operation in 1961 [1]. The facility was designed and used primarily for measurements of Nuclear Data (ND) with emphasis on the resonance energy region. As such it was designed to produce short pulses of neutrons (5-5000 ns) and equipped with detection stations at different neutron flight path distances from the source (15 m-250 m). When the LINAC started operation it was one of the most powerful accelerators in the world for high energy-resolution measurements in the resonance region. The original LINAC with some upgrades is still in operation but no longer provides world class capabilities for measurements with short pulses. In 2011 discussions between the RPI ND group, Naval Reactors, and the Nuclear Criticality Safety Program about the future of the LINAC concluded that maintaining the capability to perform world-class nuclear data measurements at RPI was desirable. To that end, it was decided to refurbish the facility and upgrade the accelerator capabilities to enable high accuracy measurement in the resonance region with narrow neutron pulse and high electron beam power. Located at a major US technical university, this project provides a needed US nuclear data capability for both research and education, and also includes external users and industrial applications.

43 PARTICLE ACCELERATORS↗

Development and Testing of Neutron Cross Section Covariance Data for SCALE 6.2

Neutron cross-section covariance data are essential for many sensitivity/uncertainty and uncertainty quantification assessments performed both within the TSUNAMI suite and more broadly throughout the SCALE code system. The release of ENDF/B-VII.1 included a more complete set of neutron cross-section covariance data: these data form the basis for a new cross-section covariance library to be released in SCALE 6.2. A range of testing is conducted to investigate the properties of these covariance data and ensure that the data are reasonable. These tests include examination of the uncertainty in critical experiment benchmark model k eff values due to nuclear data uncertainties, as well as similarity assessments of irradiated pressurized water reactor (PWR) and boiling water reactor (BWR) fuel with suites of critical experiments. The contents of the new covariance library, the testing performed, and the behavior of the new covariance data are described in this paper. The neutron cross-section covariances can be combined with a sensitivity data file generated using the TSUNAMI suite of codes within SCALE to determine the uncertainty in system k eff caused by nuclear data uncertainties. The Verified, Archived Library of Inputs and Data (VALID) maintained at Oak Ridge National Laboratory (ORNL) contains over 400 critical experiment benchmark models, and sensitivity data are generated for each of these models. The nuclear data uncertainty in k eff is generated for each experiment, and the resulting uncertainties are tabulated and compared to the differences in measured and calculated results. The magnitude of the uncertainty for categories of nuclides (such as actinides, fission products, and structural materials) is calculated for irradiated PWR and BWR fuel to quantify the effect of covariance library changes between the SCALE 6.1 and 6.2 libraries. One of the primary applications of sensitivity/uncertainty methods within SCALE is the assessment of similarities between benchmark experiments and safety applications. This is described by a c k value for each experiment with each application. Several studies have analyzed typical c k values for a range of critical experiments compared with hypothetical irradiated fuel applications. The c k value is sensitive to the cross-section covariance data because the contribution of each nuclide is influenced by its uncertainty; large uncertainties indicate more likely bias sources and are thus given more weight. Changes in c k values resulting from different covariance data can be used to examine and assess underlying data changes. These comparisons are performed for PWR and BWR fuel in storage and transportation systems.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗