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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 739 records · Page 41
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Parton distributions and lattice-QCD calculations: Toward 3D structure

The strong force which binds hadrons is described by the theory of quantum chromodynamics (QCD). Determining the character and manifestations of QCD is one of the most important and challenging outstanding issues necessary for a comprehensive understanding of the structure of hadrons. Within the context of the QCD parton picture, the parton distribution functions (PDFs) have been remarkably successful in describing a wide variety of processes. However, these PDFs have generally been confined to the description of collinear partons within the hadron. New experiments and facilities provide the opportunity to additionally explore the transverse structure of hadrons which is described by generalized parton distributions (GPDs) and transverse-momentum-dependent parton distribution functions (TMD PDFs). In our previous report Lin et al. (2018), we compared and contrasted the two main approaches used to determine the collinear PDFs: the first based on perturbative QCD factorization theorems, and the second based on lattice-QCD calculations. In the present report, we provide an update of recent progress on the collinear PDFs, and also expand the scope to encompass the generalized PDFs (GPDs and TMD PDFs). We review the current state of the various calculations, and consider what new data might be available in the near future. We also examine how a shared effort can foster dialog between the PDF and lattice-QCD communities, and yield improvements for these generalized PDFs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Observation of Coherent 𝜙⁡(1020) Meson Photoproduction in Ultraperipheral PbPb Collisions at $\sqrt{𝑠_{NN}}$ = 5.36 TeV

The first observation of coherent 𝜙⁡(1020) meson photoproduction off heavy nuclei is presented using ultraperipheral lead-lead collisions at a center-of-mass energy per nucleon pair of 5.36 TeV. The data were collected by the CMS experiment and correspond to an integrated luminosity of 1.62 μ⁢𝑏 −1 . The 𝜙⁡(1020) meson signals are reconstructed via the 𝐾 + ⁢𝐾 − decay channel. The production cross section is presented as a function of the 𝜙⁡(1020) meson rapidity in the range 0.3 < |𝑦| < 1.0, probing gluons that carry a fraction of the nucleon momentum (𝑥) around 10 −4 . The observed cross section exhibits little dependence on rapidity and is significantly suppressed, by a factor of ∼5, compared to a baseline model that treats a nucleus as a collection of free nucleons. Theoretical models that incorporate the nuclear shadowing effect generally provide a better description of the 𝜙⁡(1020) data than those incorporating gluon saturation. This study establishes a powerful new tool for exploring nuclear effects and nuclear gluonic structure in the small-𝑥 regime at a unique energy scale bridging the perturbative and nonperturbative quantum chromodynamics domains.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Molten Flux Synthesis of Plutonium (IV) Silicates K 2 PuSi 2 O 7 and Rb 2 PuSi 6 O 15

Few plutonium containing silicates have been reported in the literature and only one other tetravalent plutonium silicate structure has been reported using the flux growth method. With the goal of understanding actinide incorporation into silicates, we describe herein two new plutonium (IV) silicates, Rb 2 PuSi 6 O 15 and K 2 PuSi 2 O 7 , synthesized using a mixed alkali chloride/alkali fluoride flux growth. Both structures crystallize in the C2/c space group with lattice parameters a=24.2980(10) Å, b=7.1466(3) Å, c=17.2025(8) Å and $\blacksquare$96.6560(10)° for Rb 2 PuSi 6 O 15 , and a=9.9478(2) Å, b=5.59820 (10) Å, c=13.1848(2) Å, and $\blacksquare$105.7400(10)° for K 2 PuSi 2 O 7 . Comparisons to the synthesis of other reported alkali actinide silicates (Ce, U, and Th) are made. Raman spectra and DFT calculations of formation enthalpies and vibrational modes provide confirmation of structure refinements and enhanced product characterization for comparison with other materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Chiral Effective Field Theory’s Impact on Advancing Quantum Monte Carlo Methods

Thirty years ago, Steven Weinberg published his seminal paper on “Nuclear Forces from chiral Lagrangians” which has revolutionized the field of theoretical nuclear physics. Nowadays, interactions derived from chiral effective field theory are routinely used to describe nuclear systems ranging from atomic nuclei to the dense matter explored in the core of neutron stars with theoretical uncertainty estimates. Here, in our contribution to the special issue “Celebrating 30 years of Steven Weinberg’s paper Nuclear Forces from Chiral Lagrangians”, we focus on the impact that chiral effective field theory interactions have played in advancing microscopic studies of atomic nuclei and the nuclear-matter equation of state using quantum Monte Carlo methods.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Electroweak Currents from Chiral Effective Field Theory

Since the pioneering work of Weinberg, Chiral Effective Field Theory (EFT) has been widely and successfully utilized in nuclear physics to study many-nucleon interactions and associated electroweak currents. Here, nuclear EFT has now developed into an intense field of research and is applied to study light to medium mass nuclei. In this contribution, we focus on the development of electroweak currents from EFT and present applications to selected nuclear electroweak observables.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Structural and thermodynamic evolution of an amorphous SiOC ceramic after swift heavy ion irradiation

Radiation induced structural and energetic changes have been widely studied in crystalline materials, but studied to a much lesser extent in amorphous solids. Using a combination of neutron pair distribution function (PDF) analysis and high temperature oxide melt solution calorimetry, we obtained critical insights into the structural and energetic evolution in a swift heavy ion irradiated amorphous SiOC polymer-derived ceramic. The radiation modified SiOC structure becomes energetically less stable by 24.0±1.6 kJ/mol compared to the unirradiated structure. This destabilization is related to decreased connectivity of the Si-O-C network and destruction of free carbon. In comparison with unirradiated SiOC, the irradiated structure is more likely to become phase separated during subsequent thermal annealing. Here, our study has important implications for evaluating amorphous SiOC ceramic as a possible radiation resistant structure for nuclear applications.

36 MATERIALS SCIENCE↗
DOE OSTI2021

The LISE package: solvers for static and time-dependent superfluid local density approximation equations in three dimensions

Nuclear implementation of the density functional theory (DFT) is at present the only microscopic framework applicable to the whole nuclear landscape. The extension of DFT to superfluid systems in the spirit of the Kohn-Sham approach, the superfluid local density approximation (SLDA) and its extension to time-dependent situations, time-dependent superfluid local density ap- proximation (TDSLDA), have been extensively used to describe various static and dynamical problems in nuclear physics, neutron star crust, and cold atom systems. In this paper, we present the codes that solve the static and time-dependent SLDA equations in three-dimensional coordinate space without any symmetry restriction. These codes are fully parallelized with the message passing interface (MPI) library and take advantage of graphic processing units (GPU) for accelerating execution. The dynamic codes have checkpoint/restart capabilities and for initial conditions one can use any generalized Slater determinant type of wave function. The code can describe a large number of physical problems: nuclear fission, collisions of heavy ions, the interaction of quantized vor- tices with nuclei in the nuclear star crust, excitation of superfluid fermion systems by time dependent external fields, quantum shock waves, domain wall generation and propagation, the dynamics of the Anderson-Bogoliubov-Higgs mode, dynamics of fragmented condensates, vortex rings dynamics, generation and dynamics of quantized vortices, their crossing and recombinations and the incipient phases of quantum turbulence.

Jin, Shi↗
DOE OSTI2026

Multi-material additive manufacturing of aluminum 6061-T6 alloy with stainless steel 304: Suppression of intermetallic compounds and interface growth mechanism

Fabricating integrated aluminum-steel structures is difficult because of metallurgical incompatibilities that promote intermetallic compound (IMC) formation at their interfaces. This work introduces a practical route for additively manufacturing 6061-T6 aluminum alloy (AA6061-T6) directly onto 304 stainless steel (SS304) using a high shear strain rate-assisted interfacial bonding mechanism. Through the friction extrusion deposition-based additive manufacturing method, both single- and multi-layer deposits of AA6061-T6 were successfully fabricated on SS304, yielding a robust hybrid multi-material structure. Comprehensive analyses of deposition quality, interface porosity, and bonding performance showed that the interface achieved a tensile strength exceeding 154 MPa under quasi-static loading. Microstructural observations revealed that the deposited aluminum layers experienced severe plastic deformation, resulting in pronounced grain refinement. Importantly, the interfacial zone was found to be free of brittle IMCs, instead containing a thin amorphous layer that evolved through a non-linear reaction-zone growth law. This solid-state additive strategy establishes a promising pathway for lightweight structural systems, nuclear energy component cladding, and multifunctional engineering components, redefining how dissimilar metals can be integrated for advanced applications.

Aluminum alloy↗
DOE OSTI2022

Development of the multi-purpose Cologne Compact Differential Plunger (CoCoDiff) for the measurement of nuclear level lifetimes with the Recoil Distance Doppler-shift method

Here, a new 3-foil plunger device, the Cologne Compact Differential (CoCoDiff) plunger has been built and commissioned. Due to its compact size, it can be used together with many different spectrometers and auxiliary detectors. As a commissioning experiment, level lifetimes of the $2^{+}_{1}$ and the $4^{+}_{1}$ excited states of 50 Cr have been measured, using the Differential Decay Curve method (DDCM). A derivation is given on how this method can be applied to a differential plunger measurement, in order to measure distances for lifetimes from two different regions of sensitivity at the same time. The commissioning experiment took place at the Cologne FN tandem accelerator, using the reaction 24 Mg( 32 S,4p2n) 50 Cr. Lifetimes, deduced from this measurement, agree well with literature values from earlier measurements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Ultracentral Collisions of Small and Deformed Systems at RHIC

We study a range of collision systems involving deformed ions and compare the elliptic and triangular flow harmonics produced in a hydrodynamics scenario versus a color glass condensate (CGC) scenario. For the hydrodynamics scenario, we generate initial conditions using TRENTO and work within a linear response approximation to obtain the final flow harmonics. For the CGC scenario, we use the explicit calculation of two-gluon correlations taken in the high-p T “(semi)dilute-(semi)dilute” regime to express the flow harmonics in terms of the density profile of the collision. Here, we consider ultracentral collisions of deformed ions as a testbed for these comparisons because the difference between tip-on-tip and side-on-side collisions modifies the multiplicity dependence in both scenarios, even at zero impact parameter. We find significant qualitative differences in the multiplicity dependence obtained in the initial conditions+hydrodynamics scenario and the CGC scenario, allowing these collisions of deformed ions to be used as a powerful discriminator between models. We also find that sub-nucleonic fluctuations have a systematic effect on the elliptic and triangular flow harmonics which are most discriminating in 0–1% ultracentral symmetric collisions of small deformed ions and in 0–10% d197Au collisions. The collision systems we consider are 238 U 238 U, d 197 Au, 9 Be 197 Au, 9 Be 9 Be, 3 He 3 He, and 3 He 197 Au.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

QCD hidden-color hexadiquark in the core of nuclei

Hidden-color configurations are a key prediction of QCD with important physical consequences. In this work we examine a QCD color-singlet configuration in nuclei formed by combining six scalar [ud] diquarks in a strongly bound SU (3) C channel. The resulting hexadiquark state is a charge-2, spin-0, baryon number-4, isospin-0, color-singlet state. It contributes to alpha clustering in light nuclei and to the additional binding energy not saturated by ordinary nuclear forces in as well as the alpha-nuclei sequence of interest for nuclear astrophysics. We show that the strongly bound combination of six scalar isospin-0 [ud] diquarks within the nuclear wave function - relative to free nucleons - provides a natural explanation of the EMC effect measured by the CLAS collaboration's comparison of nuclear parton distribution function ratios for a large range of nuclei. Overall, these experiments confirmed that the EMC effect; i.e., the distortion of quark distributions within nuclei, is dominantly identified with the dynamics of neutron-proton (“isophobic”) short-range correlations within the nuclear wave function rather than proton-proton or neutron-neutron correlations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Improved high-precision mass measurements of mid-shell neon isotopes

New mass values measured with the TITAN MR-TOF-MS are reported for the short-lived isotopes 24-26 Ne, produced at TRIUMF's ISAC facility using a uranium carbide target and cold FEBIAD ion source. A least-squares adjustment within the framework of the Atomic Mass Evaluation was performed and the improved precision of the new mass values is highlighted. The improved mass accuracy in this N = 14mid-shell region can also point to the refinement in values of the charge radii. By reducing the mass uncertainty of isotopes, their contribution of the mass shift uncertainty in laser spectroscopy can be negated. The work is part of developments for reaching the N = 20 Island of Inversion, where high molecular contamination hinders mass measurements of the neon isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Systematic many-fermion Hamiltonian input scheme and spectral calculations on quantum computers

We present a novel input scheme for general second-quantized Hamiltonians of relativistic or non-relativistic many-fermion systems. This input scheme incorporates the fermionic anticommutation relations, particle number variations, and respects the symmetries of the Hamiltonian. Based on our input scheme, we propose a hybrid quantum-classical framework for spectral calculations on future quantum hardwares. We provide explicit circuit designs and the associated gate cost. We demonstrate our hybrid framework by solving the low-lying spectra of 42 Ca and 46 Ca. Our input scheme provides new pathways to solving the spectra and dynamics of the relativistic and nonrelativistic many-fermion systems via first-principles approaches.

Hybrid spectral calculation framework↗
DOE OSTI2022

An Aluminum-Based Metal–Organic Cage for Cesium Capture

Metal–organic cages are a class of supramolecular structures that often require the careful selection of organic linkers and metal nodes. Of this class, few examples of metal–organic cages exist where the nodes are composed of main group metals. Herein, we have prepared an aluminum-based metal–organic cage, H 8 [Al 8 (pdc) 8 (OAc) 8 O 4 ] (Al-pdc-AA), using inexpensive and commercially available materials. The cage formation was achieved via solvothermal self-assembly of solvated aluminum and pyridine-dicarboxylic linkers in the presence of a capping agent, acetic acid. The obtained supramolecular structure was characterized by single-crystal X-ray diffraction (SCXRD), thermogravimetric analysis, and NMR spectroscopy. Based on crystal structure and computational analyses, the cage has a 3.7 Å diameter electron-rich cavity suitable for the binding of cations such as cesium (ionic radius of 1.69 Å). Here, the host–guest interactions were probed with 1 H and 133 Cs NMR spectroscopy in DMSO, where at low concentrations, Cs + binds to Al-pdc-AA in a 1:1 ratio. The binding site was identified from the crystal structure of CsH 7 [Al 8 (pdc) 8 (OAc) 8 O 4 ] (Cs + Al-pdc-AA), and a binding affinity of ~10 6 –10 7 M –1 was determined from NMR titration experiments. The Al-pdc-AA showed improved selectivity for cesium binding over alkali metal cations (Cs + > Rb + > K + >> Na + ~ Li + ). Collectively, the study reports a novel aluminum cage that can serve as a promising host for efficient and selective cesium removal.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Doubly Stereogenic Sandwich Frameworks: Diastereomeric Metallobiscorroles

A number of Group 6 metallobiscorrole sandwich compounds with square-antiprismatic coordination were separated into diastereomers by means of careful preparative thin-layer chromatography. The diastereomers differ with respect to the relative orientation of the corrole macrocycles, which are rotated approximately ± 45° or ± 135° relative to each other. The most clear-cut results were obtained for two tungsten corroles, W[TBCF 3 PC] 2 {TBCF 3 PC = meso-tris[3,5-bis(trifluoromethyl)phenyl]corrolato} and W[TDOMePC] 2 [TDOMePC = meso-tris(3,5-dimethoxyphenyl)corrolato], for which single-crystal X-ray structures were obtained for the 135° diastereomer; the existence of the 45° diastereomer was inferred by elimination and with support from DFT calculations. For Mo[TBCF 3 PC] 2 and W[TBCF 3 PC] 2 , both diastereomers were also fully characterized spectroscopically and their 1 H NMR spectra were essentially fully assigned. The fact that each diastereomer is chiral and exists as two enantiomers (which was previously demonstrated for the 135° form of a tungsten biscorrole) establishes the doubly stereogenic nature of the metallobiscorrole framework – to our knowledge, the first such demonstration for a sandwich compound.

Aromatic compounds↗