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At least 721 records · Page 40
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Impact of organic solutes on capillary phenomena in water-CO2-quartz systems

Hypothesis: The migration of supercritical CO2 (scCO2) injected into underground reservoirs as part of carbon capture and storage is influenced by organic contamination affecting mineral wettability. Molecular dynamics (MD) simulations of relevant systems that incorporate representative organic solutes allow detailed investigation of changes in fundamental interfacial and capillary properties. Experiments: We use MD simulations to explore the effects of four organic solutes (quinoline, decanoic acid, coronene, sorgoleone) on the wettability of quartz by water in the presence of scCO2. We examine the impacts of polar, alkyl, and aromatic moieties as well as fluid flow velocity at elevated temperatures and pressures. Findings: Organic molecules accumulate at the water-CO2 interface, where they distribute according to their size and functional groups. Certain organics penetrate the adsorbed water film at the quartz-CO2 interface, revealing two modes of hydrogen bonding between polar organic functional group, water, and quartz surface –OH groups. Interfacial energies and contact angles are minimally impacted by organic adsorption at the water-CO2 interface, possibly due to simultaneous CO2 desorption. Non- equilibrium MD simulations reveal that flow-induced redistribution of organic compounds modulates the radii of curvature of the advancing and receding water-CO2 interfaces. Our results indicate that organic adsorption on water surfaces is likely ubiquitous during multi-phase flow in soils and sedimen- tary rocks, with implications for the mobilization and transport of organic compounds.

36 MATERIALS SCIENCE↗
NASA NTRS1976

Table and Charts of Equilibrium Normal-shock Properties for Pure Hydrogen with Velocities to 70 km/sec. Revised.

Errors found in the original edition are corrected. Refinement was made in procedures for solving the conservation relations for an incident (moving), standing, and reflected normal shock, as well as in computational methods for determining thermochemical-equilibrium hydrogen properties. A six-species hydrogen model replaces the original four-species model, and the heat of formation and spectroscopic constants used in this six-species model are listed in appendix A. In appendix B, comparisons are made between a number of methods for determining equilibrium thermodynamic properties for hydrogen for several values of pressure and temperatures to 50000 K. A comparison is also performed between the present method and a second method for determining thermodynamic properties and flow velocity behind an incident shock into pure hydrogen and behind a reflected shock.

Miller, C. G., III↗
NASA NTRS1998

Laser-Induced Fluorescence Measurements of Translational Temperature and Relative Cycle Number by use of Optically Pumped Trace-Sodium Vapor

Sodium fluorescence induced by a narrow bandwidth tunable laser has been used to measure temperature, pressure, axial velocity and species concentrations in wind tunnels, rocket engine exhausts and the upper atmosphere. Optical pumping of the ground states of the sodium, however, can radically alter the shape of the laser induced fluorescence excitation spectrum, complicating such measurements. Here a straightforward extension of rate equations originally proposed to account for the features of the pumped spectrum is to make temperature measurements from spectra taken in pumped vapor. Also determined from the spectrum is the relative fluorescence cycle number, which has application to measurement of diffusion rate and transverse flow velocity. The accuracy of both the temperature and cycle-number measurements is comparable with that of temperature measurements made in the absence of pumping.

Dobson, Chris C.↗
NASA NTRS1993

Aerothermodynamic heating due to shock wave/laminar boundary-layer interactions in high-enthalpy hypersonic flow

The interaction between a swept shock wave and a laminar boundary layer was investigated experimentally in high-enthalpy hypersonic flow. The effect of high-temperature, real gas physics on the interaction was examined by conducting tests in air and helium. Heat transfer measurements were made on the surface of a flat plate and a shock-generating fin using thin-film resistance sensors for fin incidence angles of 0, 5, and 10 deg at Mach numbers of 6.9 in air and 7.2 in helium. The experiments were conducted in the NASA HYPULSE expansion tube, an impulse-type facility capable of generating high-enthalpy, high-velocity flow with freestream levels of dissociated species that are particularly low. The measurements indicate that the swept shock wave creates high local heat transfer levels in the interaction region, with the highest heating found in the strongest interaction. The maximum measured heating rates in the interaction are order of magnitude greater than laminar flat plate boundary layer heating levels at the same location.

Hackett, Charles M.↗
NASA NTRS1952

The effect of high viscosity on the flow around a cylinder and around a sphere

For the determination of the flow velocity one is accustomed to measure the impact pressure, i.e., the pressure intensity in front of an obstacle. In incompressible fluids the impact pressure is yv(sup 2)/2g if the influence of viscosity can be neglected. Such an influence is appreciable, however, when the Reynolds number corresponding to impact tube radius is under about 100, and must consequently be considered, if the velocity determination is not to be faulty. The first investigation of this influence are included in the work of Miss M. Barker. In the following pages, experiments will be reported which determine the intensity of impact pressure on cylinders and spheres; furthermore a theory of the phenomenon will be developed which is in good agreement with the measurements.

FLOW - PLATES, FLAT - VISCOUS↗
DOE OSTI2022

Temporal evolution of scalar modes in Richtmyer–Meshkov instability of inclined interface using high-speed PIV and PLIF measurements at 60 kHz

Abstract The current work presents simultaneous, high-speed measurements at 60,000 fields per second of velocity and mole fraction using particle image velocimetry (PIV) and planar laser induced acetone-fluorescence in a Richtmyer–Meshkov instability of an inclined interface (Atwood number, At = 0.22). Specifically, around 2 ms of temporal evolution of the vortex structures and their associated scalar modes immediately following the interface-reshock interaction is presented. Two initial interface conditions are discussed—(a) a sharp, inclined ‘single mode’ interface and (b) a ‘multi-mode’ interface where small perturbations are imposed on the single mode case. A 2D wavelet decomposition of the scalar flow field shows a highly intermittent distribution of small-scale variance throughout the interface even at late times. These are correlated strongly with the vortex structures and local turbulence intensity, where each small-scale scalar mode is sandwiched between two co-rotating vortex structures. This indicates that the interstitial regions between the vortices are significant hotspots of entrainment, which is then dispersed by the induced, counter-flow velocity fields. The multimode case demonstrates similar organization at large scales, while the scalar field is much more homogeneous at smaller scales. These observations highlight the importance of capturing the early time vortex evolution to accurately estimate any late time intermittency, especially where deposition of intense vorticity on sharp interfaces is present.

Engineering↗
NASA NTRS1985

Solar wind-magnetosphere coupling and the distant magnetotail: ISEE-3 observations

ISEE-3 Geotail observations are used to investigate the relationship between the interplanetary magnetic field, substorm activity, and the distant magnetotail. Magnetic field and plasma observations are used to present evidence for the existence of a quasi-permanent, curved reconnection neutral line in the distant tail. The distance to the neutral line varies from absolute value of X = 120 to 140 R/sub e near the center of the tail to beyond absolute value of X = 200 R/sub e at the flanks. Downstream of the neutral line the plasma sheet magnetic field is shown to be negative and directly proportional to negative B/sub z in the solar wind as observed by IMP-8. V/sub x in the distant plasma sheet is also found to be proportional to IMF B/sub z with southward IMF producing the highest anti-solar flow velocities. A global dayside reconnection efficiency of 20 +- 5% is derived from the ISEE-3/IMP-8 magnetic field comparisons. Substorm activity, as measured by the AL index, produces enhanced negative B/sub z and tailward V/sub x in the distant plasma sheet in agreement with the basic predictions of the reconnection-based models of substorms. The rate of magnetic flux transfer out of the tail as a function of AL is found to be consistent with previous near-Earth studies. Similarly, the mass and energy fluxes carried by plasma sheet flow down the tail are consistent with theoretical mass and energy budgets for an open magnetosphere. In summary, the ISEE-3 Geotail observations appear to provide good support for reconnection models of solar wind-magnetosphere coupling and substorm energy rates.

Slavin, J. A.↗
NASA NTRS1999

Laser-Induced Fluorescence Measurements of Translational Temperature and Relative Cycle Number by use of Optically Pumped Trace-Sodium Vapor

Sodium fluorescence induced by a narrow-bandwidth tunable laser has been used to measure temperature, pressure, axial velocity, and species concentrations in wind tunnels, rocket engine exhausts, and the upper atmosphere. Optical pumping of the ground states of the sodium, however, can radically alter the shape of the laser-induced fluorescence excitation spectrum, complicating such measurements. Here a straightforward extension of rate equations originally proposed to account for the features of the pumped spectrum is used to make temperature measurements from spectra taken in pumped vapor. Also determined from the spectrum is the relative fluorescence cycle number, which has application to measurement of diffusion rate and transverse flow velocity, The accuracy of both the temperature and the cycle-number measurements is comparable with that of temperature measurements made in the absence of pumping.

Dobson, Chris C.↗
DOE OSTI2022

Emergent Behavior at the Calcite–Water Interface during Reactive Transport in a Simple Microfluidic Channel

Geochemical reactive transport processes in natural mineral-fluid systems may produce a wide array of emergent phenomena that are difficult to predict from basic principles and to reproduce in model systems. In this study, we present experimental results obtained from a simple microfluidic system with which we explored the consequences of reacting the calcite (104) cleavage surface with an acidic Pb-bearing solution (pH = 3.5, [Pb] total = 5 mM) as a function of flow rate. This system is relevant to passive remediation systems for Pb-rich acid mine drainage. We observed periodic banding in the amounts of Pb sorption at flow velocities ≥ 926 μm s -1 , where the band spacing was spatially correlated with the amount of calcite dissolution and the development of micropyramidal topography on the calcite (104) surface. The equivalent coverage of Pb deposited in these Pb-rich bands was at least several monolayers per unit cell, yet there was no evidence for precipitation of any secondary Pb phase implying incorporation of Pb within the near-surface calcite lattice. We also observed spatial variations in nucleation and growth of euhedral secondary Pb-carbonate minerals hydrocerusite and cerussite at flow rates ≤ 278 μm s -1 ,. These findings demonstrate potential for exploiting the rich phenomenology afforded by the interplay among transport phenomena and chemical kinetics in experimental systems designed to yield deeper insights into geochemical self-organization.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1990

A survey of upwelling ion event characteristics

Quasi-static electric field data collected by the DE-1 spacecraft were used to study ionospheric ion upwelling events observed in the vicinity of the dayside cleft. Bulk plasma parameters such as ion-species density and field-aligned bulk velocity and flux were derived at points within several upwelling ion events for the H(+), He(+), O(+), and O(2+), and the ion-species bulk parameters near the source altitude were compared. It was found that O(+) ions comprise about 90 percent of the upwelling particle density, followed by H(+) at less than 10 percent; He(+) and O(2+) contribute about 1 percent each. The upwelling O(+) flux is also dominant, followed by upward H(+) flux, which is relatively more significant than the fractional H(+) density, due to its high upward flow velocity.

Pollock, C. J.↗
NASA NTRS1986

Solar wind-magnetosphere coupling and the distant magnetotail - ISEE-3 observations

ISEE-3 Geotail observations are used to investigate the relationship between the interplanetary magnetic field, substorm activity, and the distant magnetotail. Magnetic field and plasma observations are used to present evidence for the existence of a quasi-permanent, curved reconnection neutral line in the distant tail. The distance to the neutral line varies from absolute value of X = 120 to 140 R/sub e near the center of the tail to beyond absolute value of X = 200 R/sub e at the flanks. Downstream of the neutral line the plasma sheet magnetic field is shown to be negative and directly proportional to negative B/sub z in the solar wind as observed by IMP-8. V/sub x in the distant plasma sheet is also found to be proportional to IMF B/sub z with southward IMF producing the highest anti-solar flow velocities. A global dayside reconnection efficiency of 20 + or - 5 percent is derived from the ISEE-3/IMP-8 magnetic field comparisons. Substorm activity, as measured by the AL index, produces enhanced negative B/sub z and tailward V/sub x in the distant plasma sheet in agreement with the basic predictions of the reconnection-based models of substorms. The rate of magnetic flux transfer out of the tail as a function of AL is found to be consistent with previous near-earth studies. Similarly, the mass and energy fluxes carried by plasma sheet flow down the tail are consistent with theoretical mass and energy budgets for an open magnetosphere. In summary, the ISEE-3 Geotail observations appear to provide good support for reconnection models of solar wind-magnetosphere coupling and substorm energy rates.

Slavin, J. A.↗
NASA NTRS2011

Comparisons of Supergranule Characteristics During the Solar Minima of Cycles 22/23 and 23/24

Supergranulation is a component of solar convection that manifests itself on the photosphere as a cellular network of around 35 Mm across, with a turnover lifetime of 1 2 days. It is strongly linked to the structure of the magnetic field. The horizontal, divergent flows within supergranule cells carry local field lines to the cell boundaries, while the rotational properties of supergranule upflows may contribute to the restoration of the poloidal field as part of the dynamo mechanism, which controls the solar cycle. The solar minimum at the transition from cycle 23 to 24 was notable for its low level of activity and its extended length. It is of interest to study whether the convective phenomena that influence the solar magnetic field during this time differed in character from periods of previous minima. This study investigates three characteristics (velocity components, sizes and lifetimes) of solar supergranulation. Comparisons of these characteristics are made between the minima of cycles 22/23 and 23/24 using MDI Doppler data from 1996 and 2008, respectively. It is found that whereas the lifetimes are equal during both epochs (around 18 h), the sizes are larger in 1996 (35.9 plus or minus 0.3 Mm) than in 2008 (35.0 plus or minus 0.3 Mm), while the dominant horizontal velocity flows are weaker (139 plus or minus m per second in 1996; 141 plus or minus 1 m per second in 2008). Although numerical differences are seen, they are not conclusive proof of the most recent minimum being inherently unusual.

Williams, Peter E.↗
NASA NTRS1984

The collisionless macroscopic Kelvin-Helmholtz instabiity. I Transverse electrostatic mode

The electrostatic limit of the Kelvin-Helmholtz instability in a collisionless plasma is investigated for a magnetic field perpendicular to the velocity flow. A two-fluid eigenvalue analysis of the transverse electrostatic Kelvin-Helmholtz instability is performed using the Chew-Goldberger-Low hydromagnetic equations with first-order finite Larmer radius corrections, establishing that the transverse electrostatic mode reduces to the incompressible transverse MHD mode in the limit of zero ion gyroradius. The linear growth rates are determined and a strong stabilization of the instability for (k-perpendicular) (rho sub i) of 0.2 or greater is observed. The nonlinear stage of the instability displays large vortices whose size is many times the initial velocity shear length. At saturation the simulation is dominated by the longest-wavelength mode permitted in the system. The simulation results can be understood in terms of a simple model which assumes that saturation occurs when the angular frequency of the vortex motion reaches the linear growth rate of the instability.

Prichett, P. L.↗
NASA NTRS1994

Location and characteristics of the reconnection X-line deduced from low-altitude satellite and radar observations

We present an analysis of a cusp ion step observed between two poleward-moving events of enhanced ionospheric electron temperature. From the computed variation of the reconnection rate and the onset times of the associated ionospheric events, the distance between the satellite and the X-line can be estimated, but with a large uncertainty due to that in the determination of the low-energy cut-off of the ion velocity distribution function, f(E). Nevertheless, analysis of the time series f(t) shows the reconnection site to be on the dayside magnetopause, consistent with the pulsating cusp model, and the best estimate of the X-line location is 13 R(E) from the satellite. The ion precipitation is used to reconstruct the field-parallel part of the Cowley-D ion distribution function injected into the open low latitude boundary layer (LLBL) in the vicinity of the X-line. From this the Alfven speed, plasma density, magnetic field, parallel ion temperature, and flow velocity of the magnetosheath near the X-line can be derived.

Lockwood, M.↗
NASA NTRS1995

Magnetohydrodynamic simulations of outflows from accretion disks

Magnetohydrodynamic simulations have been made of the formation of outflows from a Keplerian disk threaded by a magnetic field. The disk is treated as a boundary condition, where matter is ejected with Keplerian azimuthal speed and poloidal speed less than the slow magnetosonic velocity, and where boundary conditions on the magnetic field correspond to a highly conducting disk. Initially, the space above the disk, the corona, is filled with high specific entropy plasma in thermal equilibrium in the gravitational potential of the central object. The initial magnetic field is poloidal and is represented by a superposition of monopoles located below the plane of the disk. The rotation of the disk twists the initial poloidal magnetic field, and this twist propagates into the corona pushing and collimating matter into jetlike outflow in a cylindrical region. Matter outflowing from the disk flows and accelerates in the z-direction owing to both the magnetic and pressure gradient forces. The flow accelerates through the slow magnetosonic and Alfven surfaces and at larger distances through the fast magnetosonic surface. The flow velocity of the jet is approximately parallel to the z-axis, and the collimation results from the pinching force of the toroidal magnetic field. For a nonrotating disk no collimation is observed.

Ustyugova, G. V.↗
NASA NTRS2021

Burning and Suppression of Solids–II (BASS-II) Summary Report

The Burning and Suppression of Solids (BASS) experiment hardware is a small flow duct that provides containment for small scale burning of solid samples within the Microgravity Science Glovebox (MSG) aboard the International Space Station (ISS). A video camera with a data overlay and a 35-mm still camera record the combustion events. The controls (ignition, fan speed, etc.) are operated by an astronaut while the principal investigator team monitors the experiment from the ground and communicates directly with the astronaut. For the first time on ISS, BASS–II utilized MSG working volume dilution with gaseous N2. We developed a perfectly stirred reactor model to determine the N2 flow time and flow rate to obtain the desired reduced O2 concentration in the working volume for each test. We calibrated the model with the Compound Specific Analyzer-Combustion Products (CSA-CP) O2 readings offset using the Major Constituents Analyzer reading of the ISS ambient atmosphere data for that day. This worked out extremely well for operations, and added a new vital variable, ambient O2 level, to our test matrices. The main variables tested in BASS–II were ambient O2 concentration, ventilation flow velocity, and fuel type, thickness, and geometry. BASS–II also utilized the onboard CSA-CP for O2 and CO readings, and the Carbon Dioxide Monitor for CO2 readings before and after each test. Readings from these sensors allow us to evaluate the completeness of the combustion. The O2 and CO2 readings before and after each test were analyzed and compared very well to stoichiometric ratios for a one-step gas-phase reaction. The CO versus CO2 followed a linear trend for some datasets, but not for all the different geometries of fuel and flow tested. We calculated the heat release rates during each test from the O2 consumption and burn times, using the constant 13.1 kJ of heat released per gram of O2 consumed. The results showed that most of the tests had heat release rates well below 100 W. Lastly, the global equivalence ratio for the tests is estimated to be fuel rich, 1.3 on average using mass loss and O2 consumption data.

Microgravity↗
NASA NTRS1975

Comparison of techniques for measuring +Gz tolerance in man

Two objective methods and one subjective method for measuring +Gz tolerance (inertial vector in a head-to-foot direction) were compared on the human centrifuge. Direct eye-level blood pressure (Pa), blood flow velocity in the superficial temporal artery (Qta), and subjective visual symptoms were used to determine tolerance to rapid-onset acceleration (1 G/s) on the USAFSAM human centrifuge. Seven 'relaxed' subjects with extensive centrifuge experience were exposed to gradually increasing +Gz plateaus until the subject reported 100% loss of peripheral centrifuge gondola lights (PLL) and 50% loss of central light (CLD); viz., blackout. Zero forward Qta occurred 6 s (range 4-9 s) before subjective blackout and when mean eye-level blood pressure had reached 20 + or - 1 mm Hg (SE). The results of this study indicate that flow changes in the superficial temporal artery reflect flow changes in the retinal circulation during +Gz stress.

Krutz, R. W., Jr.↗
NASA NTRS2015

Results from On-Board CSA-CP and CDM Sensor Readings During the Burning and Suppression of Solids II (BASS-II) Experiment in the Microgravity Science Glovebox (MSG)

For the first time on ISS, BASS-II utilized MSG working volume dilution with gaseous nitrogen (N2). We developed a perfectly stirred reactor model to determine the N2 flow time and flow rate to obtain the desired reduced oxygen concentration in the working volume for each test. We calibrated the model with CSA-CP oxygen readings offset using the Mass Constituents Analyzer reading of the ISS ambient atmosphere data for that day. This worked out extremely well for operations, and added a new vital variable, ambient oxygen level, to our test matrices. The main variables tested in BASS-II were ambient oxygen concentration, ventilation flow velocity, and fuel type, thickness, and geometry. BASS-II also utilized the on-board CSA-CP for oxygen and carbon monoxide readings, and the CDM for carbon dioxide readings before and after each test. Readings from these sensors allow us to evaluate the completeness of the combustion. The oxygen and carbon dioxide readings before and after each test were analyzed and compared very well to stoichiometric ratios for a one step gas-phase reaction. The CO versus CO2 followed a linear trend for some datasets, but not for all the different geometries of fuel and flow tested. Lastly, we calculated the heat release rates during each test from the oxygen consumption and burn times, using the constant 13.1 kJ of heat released per gram of oxygen consumed. The results showed that the majority of the tests had heat release rates well below 100 Watts.

combustion products↗