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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 721 records · Page 40
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Direct Measurements of DT Fuel Preheat from Hot Electrons in Direct-Drive Inertial Confinement Fusion

Hot electrons generated by laser-plasma instabilities degrade the performance of laser-fusion implosions by preheating the DT fuel and reducing core compression. The hot-electron energy deposition in the DT fuel has been directly measured for the first time by comparing the hard x-ray signals between DT-layered and mass-equivalent ablator-only implosions. The electron energy deposition profile in the fuel is inferred through dedicated experiments using Cu-doped payloads of varying thickness. The measured preheat energy accurately explains the areal-density degradation observed in many OMEGA implosions. Furthermore, this technique can be used to assess the viability of the direct-drive approach to laser fusion with respect to the scaling of hot-electron preheat with laser energy.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Characterisation of a laser plasma betatron source for high resolution x-ray imaging

Abstract We report on the characterisation of an x-ray source, generated by a laser-driven plasma wakefield accelerator. The spectrum of the optimised source was consistent with an on-axis synchrotron spectrum with a critical energy of 13.8 − 1.9 + 2.2 keV and the number of photons per pulse generated above 1 keV was calculated to be 6 − 0.9 + 1.2 × 10 9 . The x-ray beam was used to image a resolution grid placed 37 cm from the source, which gave a measured spatial resolution of 4 µ m × 5 µ m. The inferred emission region had a radius and length of 0.5 ± 0.2 µ m and 3.2 ± 0.9 mm respectively. It was also observed that laser damage to the exit aperture of the gas cell led to a reduction in the accelerated electron beam charge and a corresponding reduction in x-ray flux due to the change in the plasma density profile.

plasma acceleration↗
DOE OSTI2021

Self-consistent core-pedestal ITER scenario modeling

The purpose of these integrated ITER simulations is to identify dependencies that can impact the performance of ITER. The dependence of fusion power production, temperature and density pedestals, and core profiles on varying magnetic-q, edge density fueling strength, neoclassical transport, magnetic field strength, and alpha heating, are examined. It is noted that ion modes usually dominate the interior, while electron modes dominate the barrier. The electron mode without flow shear is substantially stronger. The q increase tends to cause more kinetic ballooning modes at the edge and the q decrease means that the peeling is getting worse, but the ballooning is getting better. The large edge q tends to provide hollow density while small edge q gives normal density profile. This is consistent with the observation that the density of particles is inversely proportional to the density of the plasma current. The rise in the source of the edge particle increases the density of the edge and the reaction rate close to the edge increases temperature fluxes, resulting in weak pedestal barriers. When neoclassical transport is turned off or the strength of B-field is increased, the pronounced edge barriers are identified. In addition, a distinct effect on the magnetohydrodynamic (MHD) modes is observed due to the increased B-field. The interesting aspect is that the barrier collapses about q = 2 as the stability of MHD has decreased to replace the barrier with a continuous slope but with roughly the same fusion power. This would actually be good for a reactor. The slope of the H-mode pedestal is found to be reduced due to the alpha heating. It is expected that the problem of edge-localized modes causing damage to the first wall will be eased. The effects of circular, elongated, and general geometry on plasma profiles are also compared and contrasted. The circular geometry has a hollow density profile and no edge or internal thermal transport barrier (ETB or ITB). However, both ETBs and ITBs can be found in the elongated geometry. In general geometry, there is a weaker ETB, comparable ITBs, but a higher edge particle transport barrier than in elongated geometry. Higher density near the edge, on the other hand, causes more wall erosion, so elongated geometry might be the best option.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1990

Hot plasma parameters in Neptune's magnetosphere

This paper presents values of particle spectral parameters and estimates of plasma densities, temperatures, and beta parameters, obtained with the Low Energy Charged Particle instrument during the Voyager 2 encounter with Neptune on August 24-25, 1989. In addition, trapped electron intensities are compared with the whistler mode stably trapped limits. The results revealed a very good inbound-outbound symmetry for both the proton and the electron profiles, suggesting that there was little dynamical activity in Neptune's magnetosphere during the Voyager encounter. The similarities and differences observed between Neptune and Uranus in the values of plasma density, pressure, and beta are discussed.

Krimigis, S. M.↗
DOE OSTI2026

Metal–bicarbonate ion pairing in alkaline aqueous solutions from multilevel embedded correlated wavefunction theory and molecular dynamics

In this work, we examine ion-pairing mechanisms of bicarbonates in alkaline aqueous solutions with the divalent metal ions most abundantly present in seawater, namely, Ca 2+ and Mg 2+ . We employ a rare-event enhanced sampling approach within first-principles molecular dynamics to explore regions of phase space spanning solvent-shared to contact ion pairs. Second-order Møller–Plesset perturbation theory (MP2) corrections are subsequently applied in an embedding framework (EMB) to refine the electronic structure of stationary states and associated reaction barriers along the free-energy profiles while retaining the extended solvent effects at the density functional theory (DFT) level. Ca 2+ –HCO 3 − was previously hypothesized to exist in a solvent-shared ion pair (SSHIP) by DFT studies with an endergonic contact ion pair (CIP) formation; however, our EMB-MP2 refinement of the DFT ion-pairing pathways reveals that Ca 2+ and HCO 3 − form a virtually barrier-free CIP in alkaline solutions, with even more energetic ease than the widely studied Ca–CO 3 ion pair. We find qualitative agreement between DFT and EMB-MP2 for Mg 2+ —unlike Ca 2+ , Mg 2+ refuses to shed its strong hydration shell, thereby preferring a SSHIP state with a significant activation barrier to crossover to the CIP forms—a trait reminiscent of ion pairing in Mg–CO 3 and closely related to the kinetic limitations underlying the famous subject of the dolomite problem. Our study highlights the importance of improved electronic structure descriptions of liquids, modeled as a condensed phase of matter lacking in long-range crystalline order. It also strongly suggests that Ca 2+ –HCO 3 − CIPs are likely precursors involved in prenucleation of CaCO 3 mineral formation in seawater.

Sharma, Vidushi [Princeton Plasma Physics Laborato↗
DOE OSTI2021

New understanding of inter-ELM pedestal turbulence, transport, and gradient behavior in the DIII-D tokamak

New observations of pedestal localized turbulence in the inter-ELM period of H-mode plasmas in DIII-D show that ion temperature gradient mode scale (ITG-scale) density fluctuation (ñ) increases immediately after each ELM crash and is quickly suppressed during the increase in local E × B shear. This excitation and subsequent suppression of ITG-scale ñ can explain the previously reported anomalous ion heat flux, Qi during the ELM (Viezzer et al 2017 Nucl. Fusion 57 022020). Shorter wavelength trapped electron mode scale (TEM-scale) ñ starts to increase at a critical pedestal temperature gradient (∇Te,ped) and saturates as local E × B shear, ${T}_{\mathrm{i}}^{\mathrm{C}\mathrm{6}+}/{T}_{\mathrm{e}}$ ratio, and ∇Te,ped saturate. This TEM-scale ñ, which has the potential to cause electron (and also ion) heat transport, is consistent with driving an anomalous electron heat flux Qe, where Qe is estimated between ELMs using experimental profiles and power balance. Both ITG- and TEM-scale ñ amplitude variations with background Ti/Te and ∇ne,ped are found to be consistent with theoretical predictions of these measured density fluctuations being ITG and TEM instabilities respectively. Furthermore, these new and unique observations on the nature of turbulence and their potential contributions to electron and ion heat fluxes at different ELM periods (i.e. collapse, recovery, and saturation phases of pedestal gradients) can significantly test and improve our pedestal predictive capabilities for ITER and other future fusion devices.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Plasma pressure profiles in a sheared-flow-stabilized Z-pinch

We report the plasma pressure reached inside the central plasma column of a sheared-flow-stabilized Z-pinch using Thomson scattering measurements. Building on previously reported experimental results and the analysis methods established for the high temperature and moderate density plasmas generated on the FuZE device, we show evidence of a central plasma region with higher electron temperature and density, which is consistent with a pinch behavior. Elevated electron temperatures up to 2.25 ± 0.8 keV and densities up to (4.9±0.2)×1017 cm−3 are observed to temporally coincide with the fusion neutron production from the plasma. Reconstructed plasma pressure profiles highlight the presence of a several millimeter-wide column with elevated pressure whose location varies shot-to-shot. The plasma pressure rises as neutron production from the deuterium plasma increases, reaching a peak value of 2.6 kBar. This peak value is consistent with a radially force-balanced pinch equilibrium model based on the measured ∼320 kA pinch current. Complete datasets were obtained at two axial locations, 10 and 20 cm axial position from the tip of the central electrode, which corroborate the estimated neutron source axial lengths.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Parameter development and characterization of laser powder directed energy deposition of Nb – Alloy C103 for thin wall geometries

This work focuses on the parameter development and microstructural characterization of Nb-based alloy C103 for thin wall structures produced via laser powder – directed energy deposition (LP – DED). Laser power and scanning speeds were varied as part of a design of experiments to identify adequate print parameters. Combinations were evaluated for relative density, porosity, and geometrical accuracy. A combination of a laser power of 1420 W and scanning speed of 14 mm/s resulted in a relative density >99%, exhibited a consistent weld bead profile and was used for further microstructural evaluation. A mix of optical and scanning electron microscopy (SEM) revealed small, slightly elongated grains along the edges and large epitaxial grains in the central region along the Build – Transverse view. Scanning electron microscopy (SEM) and energy dispersive spectroscopy (EDS) analysis revealed Hf rich columnar cells in the center that transition into an evenly spaced cellular structure towards the edges of the built sample. Electron backscatter diffraction (EBSD) scans show a sharp [001] texture when looking at the cross section of the sample along the build direction. The Build – Scan view revealed a zig – zag pattern that follows the back – and – forth deposition strategy that was used. Finally, microhardness measurements were taken in the as – built (AB) and stress relieved (SR) conditions to baseline preliminary mechanical properties. The AB condition exhibited a large amount of scatter in the data and averages up to 11% larger than the SR condition. The reduction in scatter upon applying the SR cycle are indicative of a large concertation of dislocations present in the AB condition.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Investigating the role of edge neutrals in exciting tearing mode activity and achieving flat temperature profiles in LTX-β

Abstract We present observations, numerical simulations, and analysis from experiments in the Lithium Tokamak Experiment-Beta (LTX- β ) in which the electron temperature profile ( T e ( r )) shifts from flat to peaked and a tearing mode is also destabilized when the average density ( n e ave ) exceeds ∼10 19 m −3 . Flat T e ( r ) is obtained routinely in LTX- β , with a lithium coated, low-recycling first wall, once the external fueling is stopped and density decays [Boyle et al 2023 Nucl. Fusion 63 056020]. In the present experiment, flat T e profiles can be sustained while maintaining constant n e ave below a line averaged density threshold ( n e ave th ) of ∼10 19 m −3 . Above n e ave th , T e ( r ) shifts from flat to peaked and a tearing mode is destabilized. Due to low recycling, the achieved n e ave can be controlled precisely by external fueling and hence, a certain threshold of the edge neutral inventory from the external fueling is experimentally manifested through n e ave th . The goal of the present work is to investigate the role of edge neutrals in determining T e ( r ) and MHD stability in the unique low-recycling regime of LTX- β . Our hypothesis is that the peaking of T e ( r ) beyond n e ave th is due ultimately to the edge cooling by the cold neutrals beyond a critical fueling flux. At lower fueling flux, flat T e ( r ) results in broader pressure profile and lower resistivity, which in turn stabilizes the tearing mode. This hypothesis is supported by edge neutral density estimation by DEGAS 2 code. Mode analysis by singular value decomposition confirms the tearing mode structure to be m / n = 2/1 ( m and n being the poloidal and toroidal mode numbers). Linear tearing stability analysis with M3D-C1 predicts that plasmas with n e ave > 10 19 are highly susceptible to a n = 1 tearing mode. ORBIT simulations, however, confirmed that the tearing modes do not contribute to the loss of fast ions from neutral beam injection. This study shows for the first time that the neutral inventory at the edge could be one of the deciding factors for the achievability of the unique operation regime of flat T e ( r ) and the excitation of tearing activity that could be disruptive for the plasmas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS2013

Eliminating Obliquity Error from the Estimation of Ionospheric Delay in a Satellite-Based Augmentation System

Current satellite-based augmentation systems estimate ionospheric delay using algorithms that assume the electron density of the ionosphere is non-negligible only in a thin shell located near the peak of the actual profile. In its initial operating capability, for example, the Wide Area Augmentation System incorporated the thin shell model into an estimation algorithm that calculates vertical delay using a planar fit. Under disturbed conditions or at low latitude where ionospheric structure is complex, however, the thin shell approximation can serve as a significant source of estimation error. A recent upgrade of the system replaced the planar fit algorithm with an algorithm based upon kriging. The upgrade owes its success, in part, to the ability of kriging to mitigate the error due to this approximation. Previously, alternative delay estimation algorithms have been proposed that eliminate the need for invoking the thin shell model altogether. Prior analyses have compared the accuracy achieved by these methods to the accuracy achieved by the planar fit algorithm. This paper extends these analyses to include a comparison with the accuracy achieved by kriging. It concludes by examining how a satellite-based augmentation system might be implemented without recourse to the thin shell approximation.

delay estimation↗
NASA NTRS2021

A theoretical assessment of the feasibility of potential Lunar Reconnaissance Orbiter radio occultation observations of the lunar ionosphere

The existence of a “dense” lunar ionosphere has been controversial for decades. Positive ions produced from the lunar surface and exosphere are inferred to have densities that are.106– 107m−3near the surface and smaller at higher altitudes, yet electron densities derived from radio occultation measurements occasionally exceed these values by orders of magnitude. For example, about 4% of the single-spacecraft radio occultation measurements from Kaguya/SELENE were consistent with peak electron densities of∼3×108m−3. Space plasmas should be neutral on macroscopic scales, so this represents a substantial discrepancy. Additional observations of electron densities in the lunar ionosphere are critical to resolving this long standing paradox. Here we theoretically assess whether radio occultation observations using two-way coherent S-band radio signals from the Lunar Reconnaissance Orbiter (LRO) spacecraft could provide useful measurements of electron densities in the lunar ionosphere. We predict the uncertainty in a single LRO radio occultation measurement of electron density to be∼3×108m−3, comparable to occasional observations by Kaguya/SELENE of a dense lunar ionosphere. Thus an individual profile from LRO is unlikely to reliably detect the lunar ionosphere; however, averages of multiple (∼10) LRO profiles acquired under similar geophysical and viewing conditions should be able to make reliable detections. An observing rate of six ingress occultations per day (∼2000 per year) could be achieved with mini-mal impact on current LRO operations. This rate compares favorably with the 378observations reported from the single-spacecraft experiment on Kaguya/SELENE between November 2007 and June 2009. The large number of observations possible for LRO would be sufficient to permit wide-ranging investigations of spatial and temporal variations in the poorly understood lunar ionosphere. These findings strengthen efforts to conduct such observations with LRO.

Paul Withers↗
DOE OSTI2023

Molten Sodium Penetration in NaSICON Electrolytes at 0.1 A cm –2

High-conductivity solid electrolytes, such as the Na superionic conductor, NaSICON, are poised to play an increasingly important role in safe, reliable battery-based energy storage, enabling advanced sodium-based batteries. Coupled demands of increased current density (≥0.1 A cm –2 ) and low-temperature (<200 °C) operation, combined with increased discharge times for long-duration storage (>12 h), challenge the limitations of solid electrolytes. Here, we explore the penetration of molten sodium into NaSICON at high current densities. Previous studies of β"-alumina proposed that Poiseuille pressure-driven cracking (mode I) and recombination of ions and electrons within the solid electrolyte (mode II) are the two main mechanisms for Na penetration, but a comprehensive study of Na penetration in NaSICON is necessary, particularly at high current density. To further understand these modes, this work employs unidirectional galvanostatic testing of Na|NaSICON|Na symmetric cells at 0.1 A cm –2 over 23 h at 110 °C. Further, while galvanostatic testing shows a relatively constant yet increasingly noisy voltage profile, electrochemical impedance spectroscopy (EIS) reveals a significant decrease in cell impedance correlated with significant sodium penetration, as observed in scanning electron microscopy (SEM). Further SEM analysis of sodium accumulation within NaSICON suggests that mode II failure may be far more prevalent than previously considered. Further, these findings suggest that total (dis)charge density (mAh cm –2 ), as opposed to current density (mA cm –2 ), may be a more critical parameter when examining solid electrolyte failure, highlighting the challenge of achieving long discharge times in batteries using solid electrolytes. Together, these results provide a better understanding of the limitations of NaSICON solid electrolytes under high current and emphasize the need for improved electrode–electrolyte interfaces.

25 ENERGY STORAGE↗
DOE OSTI2024

Natural formation of linear defect structures in MoS 2

Near surface defects can significantly impact the quality of metallic interconnects and other interfaces necessary to create device structures incorporating two-dimensional materials. Furthermore, the impact of such defects can strongly depend on their organization. In this study, we present scanning tunneling microscopy images and tunneling spectroscopy of point and linear defects near the surface of natural MoS 2 . The point defects share similar structural and electronic characteristics and occur with comparable frequency as subsurface sulfur vacancies observed previously on natural MoS 2 . The linear defects observed here occur less frequently than the point defects but share the same depth profile and electronic structure. These data indicate that the linear defects are actually a one-dimensional organization of subsurface sulfur vacancies. Our density functional calculations agree with this assessment in that, for sufficient local defect concentrations, it is energetically more favorable for the defects to be organized in a linear fashion rather than as clusters or even isolated single point defects. Given these measurements were taken from naturally formed MoS 2 , this organization likely occurs during crystal formation. Considering the impact of one-dimensional organization on the local properties of layered materials, and the potential for them to be introduced purposefully during crystal formation, research into the formation mechanism and properties of these defects could enable new paths for defect engineering in MoS 2 -based systems.

2D materials↗
DOE OSTI2024

Extracting the electronic structure of light elements in bulk materials through a Compton scattering method in the readily accessible hard x-ray regime

Here, our Compton profile measurements of Ti and TiH 2 using readily available hard X-ray radiation at 27.5 keV, detected by both a Hitachi Vortex silicon-drift detector and a high-resolution superconducting transition-edge sensor array, are found to be in excellent accord with state-of-the-art density functional theory based calculations. The spherically averaged difference between the Compton profiles of TiH 2 and Ti is well described by an inverted parabola, supporting an itinerant behavior of the electron gas screening the protons in the Ti matrix. Our experimental approach, validated by two different detectors, extends the applicability of Compton scattering technique to the readily accessible hard x-ray regime (below 30 keV). Our study suggests possibilities for experiments at low-flux bending magnet synchrotron beamlines and paves the way for the development of tabletop Compton experiments with x-ray tubes.

36 MATERIALS SCIENCE↗
NASA NTRS1982

Direct measurements of plasma characteristics in space-simulation beam-plasma interactions

Recent laboratory investigations of space-simulated electron-beam-plasma interactions are discussed. The plasma has been characterized with respect to its spatial distributions in density, temperature, and density fluctuation power spectra. The latter results have been further classified in terms of amplitude and spectral distributions. The overall results include: (1) detailed radial profiles of plasma density as a function of beam parameters; (2) the association of low-frequency large amplitude fluctuations with ion acoustic, ion cyclotron, and drift-wave modes; (3) the identification and spatial mapping of suprathermal electrons in the beam core; and (4) the experimental definition of a density-dependent criterion for the ignition of the beam-plasma-discharge.

Szuszczewicz, E. P.↗
NASA NTRS1999

Piezoelectric Field Enhanced Second-Order Nonlinear Optical Susceptibilities in Wurtzite GaN/AlGaN Quantum Wells

Second-order nonlinear optical processes including second-harmonic generation, optical rectification, and difference-frequency generation associated with intersubband transitions in wurtzite GaN/AlGaN quantum well (QW) are investigated theoretically. Taking into account the strain-induced piezoelectric (PZ) effects, we solve the electronic structure of the QW from coupled effective-mass Schrodinger equation and Poisson equation including the exchange-correlation effect under the local-density approximation. We show that the large PZ field in the QW breaks the symmetry of the confinement potential profile and leads to large second-order susceptibilities. We also show that the interband optical pump-induced electron-hole plasma results in an enhancement in the maximum value of the nonlinear coefficients and a redshift of the peak position in the nonlinear optical spectrum. By use of the difference-frequency generation, THz radiation can be generated from a GaN/Al(0.75)Ga(0.25)N with a pump laser of 1.55 micron.

Liu, Ansheng↗
NASA NTRS1976

The nighttime ionosphere of Mars from Mars-4 and Mars-5 radio occultation dual-frequency measurements

Dual frequency radio sounding of the Martian nighttime ionosphere was carried out during the exits from behind the planet of the Mars-4 spacecraft on February 2, 1974 and the Mars-5 spacecraft on February 18, 1974. In these experiments, the spacecraft transmitter emitted two coherent monochromatic signals in decimeter and centimeter wavelength ranges. At the Earth receiving station, the reduced phase difference (or frequencies) of these signals was measured. The nighttime ionosphere of Mars measured in both cases had a peak electron density of approximately 5 X 1,000/cu cm at an altitude of 110 to 130 km. At the times of spacecraft exit, the solar zenith angles at the point of occultation were 127 deg and 106 deg, respectively. The height profiles of electron concentration were obtained assuming spherical symmetry of the Martian ionosphere.

Savich, N. A.↗
NASA NTRS1971

Thin electrostatically self-focusing electron streams.

Study of 30 to 380 microampere, 50 to 550 V, 1 to 2 mm, electrostatically self-focusing electron streams (50 cm long) drifting through mercury vapor (at 50 microtorr to 2 millitorr) in a tube with a radius of 6.6 cm. The inside surface of the tube is coated with a transparent layer whose resistivity is 50 ohm-cm per centimeter. In order to determine the charged-particle densities and the potential profile in and around the beam without disturbing the system, a multigrid electrostatic charged particle energy analyzer was used to study separately the energy distributions of both ions and electrons ejected radially from the beam. The results show two energy groupings for electrons. The energy distribution of the high-energy group is produced by ionizing collisions between beam electrons and neutral gas atoms; a group of flow-energy electrons becomes trapped in the potential well within and around the beam, subsequently escaping by collisional mechanisms.

Mccorkle, R. A.↗