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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 721 records · Page 40
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Local structure, bonding, and asymmetry of $\mathrm{((NH_2)_2CH)PbBr_3}$, $\mathrm{CsPbBr_3}$, and $\mathrm{(CH_3MH_3)PbBr_3}$

Here we report local structure measurements for CsPbBr 3 and ((NH 2 ) 2 CH)PbBr 3 (FAPbBr 3 ) and compare them with recent results for (CH 3 NH 3 )PbBr 3 (MAPbBr 3 ). The Pb-Br bonding is similar for all three systems; the effective spring constants, κ, are comparable (ranging from 1.20 to 1.95 eV/Å 2 ), but small in magnitude indicating very soft materials. However, there are also important differences between the three systems. Static disorder is very small for CsPbBr3 but increases somewhat with the size of the organic molecular ions MA + and FA + . At room temperature, dynamic disorder dominates in all compounds. The thermal disorder of the Pb-Br pair distribution function (PDF), i.e., the Debye-Waller factor σ 2 follows a correlated Debye or Einstein model up to 300 K in CsPbBr 3 (orthorhombic phase), but for FAPbBr 3 and MAPbBr 3 , there is a break in the σ 2 (T) curve at the orthorhombic-tetragonal transition (o-t) near 150 K, indicating a small change in the spring constant κ. κ increases for MAPbBr 3 but decreases in FAPbBr 3 at this transition. These changes are attributed to changes in the H-bonding between Br - and MA + or FA + at this transition, as a result of librations or rotations of these molecular cations. In addition, the Pb-Br PDF becomes asymmetric at a relatively low temperature for FAPbBr 3 and MAPbBr 3 , while this effect is significantly smaller for CsPbBr 3 . Finally, we address the question of a model to explain the asymmetric PDF. Two main models are discussed in the literature, an anharmonic pair potential and a split-pair distribution, possibly driven by the presence of a lone pair on the Pb ion. We show that the fourth cumulant C 4 can differentiate between these two models and other possible models. Experimentally C 4 is positive at 250 K and above, for all three systems and that is inconsistent with a split-peak model, for which C 4 is negative for splittings larger than 0.12 Å.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Complications in the interpretation of the charge-asymmetry-dependent π flow for the chiral magnetic wave

The charge asymmetry ($A_ch$) dependence of the $π^₋$ and $π^+$ elliptic flow difference, $Δv_2(A_{\text{ch}})$, has been regarded as a sensitive observable for the possible chiral magnetic wave (CMW) in relativistic heavy ion collisions. In this work, we first demonstrate that, due to nonflow backgrounds, the flow measurements by the Q-cumulant method using all charged particles as reference introduce a trivial linear term to $Δv_2(A_{\text{ch}})$. The trivial contribution to the slope of triangle flow difference $Δv_3( A_{\text{ch}})$ can be negative if the nonflow is dominated by back-to-back pairs. After eliminating the trivial term, we find that the nonflow between like-sign pairs gives rise to an additional positive slope to $Δv_2(A_{\text{ch}})$ because of the larger multiplicity dilution to $π^+$ ($π^₋$) at positive (negative) $A_{\text{ch}}$. We further find that the competition between different π sources can introduce another nontrivial linear-$A_{\text{ch}}$ term due to their different multiplicity fluctuations and anisotropic flows. We then study the effect of neutral cluster (resonance) decays as a mechanism for local charge conservation on the slope parameter of $Δv_2(A_{\text{ch}})$. We find that the slope parameter is sensitive to the kinematics of those neutral clusters. Light resonances give positive slopes while heavy resonances give negative slopes. Local charge conservation from continuum cluster mass distribution can give a positive slope parameter comparable to experimental data. Our studies indicate that many non-CMW physics mechanisms can give rise to a $A_{\text{ch}}$-dependent $Δv_2(A_{\text{ch}})$ and the interpretation of $Δv_2(A_{\text{ch}})$ in terms of the CMW is delicate.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Bayesian calibration of a hybrid nuclear collision model using $\textit{p}$₋Pb and Pb-Pb data at energies available at the CERN Large Hadron Collider

Here, we posit a unified hydrodynamic and microscopic description of the quark-gluon plasma (QGP) produced in ultrarelativistic p₋Pb and Pb-Pb collisions at $\sqrt{s}_\text{NN}$ = 5.02 TeV and evaluate our assertion using Bayesian inference. Specifically, we model the dynamics of both collision systems using initial conditions with parametric nucleon substructure, a preequilibrium free streaming stage, event-by-event viscous hydrodynamics, and a microscopic hadronic afterburner. Free parameters of the model, which describe the initial state and QGP medium are then simultaneously calibrated to fit charged-particle yields, mean $p_T$, and flow cumulants. We argue that the global agreement of the calibrated model with the experimental data strongly supports the existence of hydrodynamic flow in small collision systems at ultrarelativistic energies, and that the flow produced develops at length scales smaller than a single proton. Posterior estimates for the model's input parameters are obtained, and new insights into the temperature dependence of the QGP transport coefficients and event-by-event structure of the proton are discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Sensitivity study with a $\textit{D}$ and $\textit{B}$ mesons modular simulation code of heavy flavor $R_{AA}$ and azimuthal anisotropies based on beam energy, initial conditions, hadronization, and suppression mechanisms

Heavy flavor probes provide important information about the in-medium properties of the quark-gluon plasma produced in heavy-ion collisions. In this work, we investigate the effects of 2D + 1 event-by-event fluctuating hydrodynamic backgrounds on the nuclear suppression factor and momentum anisotropies of heavy flavor mesons and nonphotonic electrons. Using the state-of-the-art $\textit{D}$ and $\textit{B}$ mesons modular simulation code (called “DAB-MOD”), we perform a systematic comparison of different transport equations in the same background, including a few energy-loss models—with and without energy-loss fluctuations—and a relativistic Langevin model with different drag parametrizations. We present the resulting $\textit{D}$ and $\textit{B}$ mesons $R_{A A}, v_2, v_3,$ and $v_4$ as well as multiparticle cumulants, in AuAu collisions at $\sqrt{s_{NN}}$ = 200 GeV and PbPb collisions at $\sqrt{s_{NN}}$ = 2.76 TeV and $\sqrt{s_{NN}}$ = 5.02 TeV , and compare them to the available experimental data. The $v_2${4}/$v_2${2} ratio, which is known to be a powerful probe of the initial conditions and flow fluctuations in the soft sector, is also studied in the context of heavy flavor. We also investigate the correlations between the transverse anisotropies of heavy mesons and all charged particles to better understand how heavy quarks couple to the hydrodynamically expanding quark-gluon plasma. Finally, we study the influence that different initial conditions and the implementation of heavy-light quark coalescence has on our results.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Probing the structure of the initial state of heavy-ion collisions with p T -dependent flow fluctuations

The connection between initial-state geometry and anisotropic flow can be quantified through a well-established mapping between p T -integrated flow harmonics and cumulants of the initial transverse energy distribution. In this paper we successfully extend this mapping to also include p T -differential flow. In doing so, we find that subleading principal components of anisotropic flow can reveal previously unobserved details of the hydrodynamic response, in both the linear and the nonlinear regimes. Most importantly, we show that they provide novel information on the small-scale structures present in the initial stage of relativistic heavy-ion collisions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Extension of the Hauser-Feshbach fission fragment decay model to multichance fission

The Hauser-Feshbach fission fragment decay model, HF 3 D, which calculates the statistical decay of fission fragments, has been expanded to include multichance fission, up to neutron incident energies of 20 MeV. The deterministic decay takes as input prescission quantities—fission probabilities and the average energy causing fission—and postscission quantities—yields in mass, charge, total kinetic energy, spin, and parity. From these fission fragment initial conditions, the full decay is followed through both prompt and delayed particle emissions, allowing for the calculation of prompt neutron and γ properties, such as multiplicity and energy distributions, both independent and cumulative fission yields, and delayed neutron observables. Here, we describe the implementation of multichance fission in the HF 3 D model, and show an example of prompt and delayed quantities beyond first-chance fission, using the example of neutron-induced fission on 235 U. This expansion represents significant progress in consistently modeling the emission of prompt and delayed particles from fissile systems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Phase transitions and critical behavior in hadronic transport with a relativistic density functional equation of state

We develop a flexible, relativistically covariant parametrization of the dense nuclear matter equation of state suited for inclusion in computationally demanding hadronic transport simulations. Within an implementation in the hadronic transport code smash, we show that effects due to bulk thermodynamic behavior are reproduced in dynamic hadronic systems, demonstrating that hadronic transport can be used to study critical behavior in dense nuclear matter, both at and away from equilibrium. We also show that two-particle correlations calculated from hadronic transport simulation data follow theoretical expectations based on the second-order cumulant ratio, and constitute a clear signature of the crossover region above the critical point.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Higher-order transverse momentum fluctuations in heavy-ion collisions

In relativistic heavy-ion collisions, the event-by-event mean transverse momentum fluctuations are sensitive to overlap area and energy density fluctuations in the initial state. We present a framework to calculate p T fluctuations up to fourth order using standard and subevent methods, which is validated using the HIJING model. We observe a power-law dependence for cumulants of all orders as a function of charged particle multiplicity N ch , consistent with a simple independent source picture. The fluctuation in pp collisions is observed to be larger than for p+Pb, Pb + Pb, and Xe + Xe collisions at the same N ch due to bias in the number of contributing sources. The short-range correlations are greatly suppressed in the subevent method in comparison to calculations based on the standard method. This paper provides a baseline for transverse momentum fluctuations without the presence of final-state effects.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Determination of β -decay feeding patterns of 88 Rb and 88 Kr using the Modular Total Absorption Spectrometer at ORNL HRIBF

We report precise determination of ground-state feeding in the β decay of fission products is an important but challenging component in modeling reactor antineutrino flux and reactor decay heat. The Modular Total Absorption Spectrometer (MTAS) is a versatile NaI(Tl) detector array that determines the true β-decay pattern free from the pandemonium effect, including precise ground-state feeding intensities. In this paper, we report MTAS results of the β feeding intensities of 88 Rb and 88 Kr, fission products with large cumulative yields in nuclear reactors. By comparing MTAS results with previous measurements, 88 Rb provides a validation of MTAS's ability to determine ground-state feedings in β decays, while the precision of 88 Kr ground-state feeding is improved when compared with the Evaluated Nuclear Structure Data File (ENSDF). The investigation of sources that contribute to β feeding branching uncertainties in MTAS experiments is discussed in detail. Lastly, the deconvolution of 88 Rb decay spectra suggests that MTAS can distinguish an allowed β spectral shape from a first forbidden unique β spectral shape.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Deciphering Nb 98 β decay with the Modular Total Absorption Spectrometer at ORNL

An assessment done under the auspices of the Organization for Economic Co-operation and Developement Nuclear Energy Agency (OECD-NEA) in 2007 suggested that the β decays of many abundantly produced fission products in nuclear reactors may be incomplete. In this assessment, the fission product 98 Nb was assigned the highest priority for study by total absorption spectroscopy due to its large cumulative fission branching fraction and because the β-decay data from several experiments are discrepant. To obtain the complete β-decay feeding pattern of 98 Nb and determine the impact on the average γ energy per 98 Nb β decay and v¯e emission calculations. The complete 98 Nb β-decay feeding pattern includes ground-state to ground-state β feeding and direct β feeding to the 0 + first-excited state (both have no associated γ rays), and the ground-state to excited-state β transitions followed by γ transitions to the ground state of the daughter nucleus, 98 Mo. The complete β-decay intensities of 98 Nb were measured with the Modular Total Absorption Spectrometer at Oak Ridge National Laboratory (ORNL). Here, the 98 Nb was produced by the β decay of mass 98 fission fragments at ORNL's On-Line Test Facility (OLTF) using proton-induced fission of 238 U. We find that changes to the current ENSDF assessment of 98 Nb β-decay intensity are required. We report improved uncertainties for the β-decay feeding values and report new β feedings to high-energy levels in 98 Mo. A more complete 98 Nb β-feeding pattern with improved accuracy and precision is offered. The impacts of the measured changes to the 98 Nb β-feeding pattern on both reactor decay heat calculations and predicted detection rates of reactor v¯e are presented. The Modular Total Absorption Spectrometer measurements of 98 Nb demonstrate the importance of reexamining and remeasuring complex β-decaying fission products with total absorption spectroscopy, including nuclei very near β stability.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Probing the high-density nuclear symmetry energy with the Ξ – / Ξ 0 ratio in heavy-ion collisions at s N N ≈ 3 GeV

Recent beam energy scan experiments at the BNL Relativistic Heavy Ion Collider by the STAR Collaboration found that hadronic interactions dominate the collective flow and the proton cumulant ratios are driven by baryon number conservation in a region of high baryon density in √ s NN = 3 GeV Au + Au reactions, indicating that the dense medium formed in such collisions is likely hadronic matter. Within an updated a relativistic transport model with momentum dependent isoscalar and isovector single-nucleon mean-field potentials corresponding to different symmetry energies at suprasaturation densities, the n/p, π – /π + , $K$ $^{0}_{s}$/K + , Σ – /Σ + , and Ξ – /Ξ 0 ratios are studied for central Au + Au collisions at √ s NN = 3 GeV, where the maximum central density reaches about (3.6–4.0) ρ 0 . The doubly strange Ξ – /Ξ 0 ratio is found to have the strongest sensitivity to the variation of high-density nuclear symmetry energy. Furthermore, the Ξ – /Ξ 0 ratio in relativistic heavy-ion reactions at √ s NN~3 GeV may help probe sensitively the poorly known symmetry energy of dense neutron-rich matter critically important for understanding various properties of neutron stars.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Measuring differential flow angle fluctuations in relativistic nuclear collisions

Recently studies of the differential nature of the flow angle fluctuations, known as event plane angular decorrelation, indicated that measurements that assume a common symmetry plane may need to consider the flow angle fluctuations effect. Using the HIJING and AMPT models, it is shown that the flow angle fluctuations measurements, obtained with the two- and three-subevents correlation method, could have significant nonflow effects associated with long- and short-range nonflow correlations. The current study demonstrates the four-subevents cumulant methods' ability to reduce the nonflow effects. Finally, it is further argued that the measurements using the four-subevents correlation method can be used to provide accurate quantification of the differential flow angle fluctuations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Consideration of memory of spin and parity in the fissioning compound nucleus by applying the Hauser-Feshbach fission fragment decay model to photonuclear reactions

Prompt and β-delayed fission observables, such as the average number of prompt and delayed neutrons, the independent and cumulative fission product yields, and the prompt γ-ray energy spectra for the photonuclear reactions on 235,238 U and 239 Pu, are calculated with the Hauser-Feshbach fission fragment decay (HF 3 ⁢D) model and compared with available experimental data. Further, in the analysis of neutron-induced fission reactions to the case of photo-induced fission, an excellent reproduction of the delayed neutron yields supports a traditional assumption that the photo fission might be similar to the neutron-induced fission at the same excitation energies regardless of the spin and parity of the fissioning systems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Correlations between flow and transverse momentum in Xe + Xe and Pb + Pb collisions at the LHC with the ATLAS detector: A probe of the heavy-ion initial state and nuclear deformation

The correlations between flow harmonics v n for n = 2, 3, and 4 and mean transverse momentum [p T ] in 129 Xe + 129 Xe and 208 Pb + 208 Pb collisions at $\sqrt{s}$ = 5.44 and 5.02 TeV, respectively, are measured using charged particles with the ATLAS detector. The correlations are potentially sensitive to the shape and size of the initial geometry, nuclear deformation, and initial momentum anisotropy. The effects from nonflow and centrality fluctuations are minimized, respectively, via a subevent cumulant method and an event-activity selection based on particle production at very forward rapidity. The v n -[p T ] correlations show strong dependencies on centrality, harmonic number n, p T , and pseudorapidity range. Current models qualitatively describe the overall centralityand system-dependent trends but fail to quantitatively reproduce all features of the data. In central collisions, where models generally show good agreement, the v 2 -[p T ] correlations are sensitive to the triaxiality of the quadruple deformation. Comparison of the model with the Pb + Pb and Xe + Xe data confirms that the 129 Xe nucleus is a highly deformed triaxial ellipsoid that has neither a prolate nor oblate shape. This provides strong evidence for a triaxial deformation of the 129 Xe nucleus from high-energy heavy-ion collisions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Initial energy-momentum to final flow: A general framework for heavy-ion collisions

The evolution of a relativistic heavy-ion collision is typically understood as a process that transmutes the initial geometry of the system into the final momentum distribution of observed hadrons, which can be described via a cumulant expansion of the initial distribution of energy density and is represented at leading order as the well-known eccentricity scaling of anisotropic flow. We extend this framework to include the contribution from initial momentum-space properties, as encoded in other components of the energy-momentum tensor. Furthermore, we confirm the validity of the framework in state-of-the-art hydrodynamic simulations of large and small systems. With this framework, it is possible to separate the effects of early time dynamics from those of final-state evolution, even in the case when the distribution of energy does not fully determine subsequent evolution, as for example, in small systems. Specifically, we answer the question of when and how azimuthal correlations from the initial state survive to the final state. In very small systems such as 𝑝−𝑝, for example, initial momentum degrees of freedom dominate over energy. Thus, even if the system forms a quark-gluon plasma that is well described by hydrodynamics, the usual hydrodynamic picture of the transmutation of initial geometry to final momentum anisotropy is broken. Nevertheless, we show that the hydrodynamic response to the full energy-momentum tensor can be well understood in a similar manner as larger systems. Additionally, this framework elucidates the generic features of the system's evolution that are responsible for the impressive success of hydrodynamic simulations, but which may still hold even in cases where hydrodynamics is not applicable.

Relativistic heavy-ion collisions↗
DOE OSTI2024

Decay studies of the 𝛽-delayed neutron emitters 87 Br and 88 Br measured by means of the Modular Total Absorption Spectrometer at ORNL HRIBF

The β decays of 87 Br, 88 Br, and 87 Kr were measured with the Modular Total Absorption Spectrometer (MTAS) at Oak Ridge National Laboratory’s Holifield Radioactive Ion Beam Facility (HRIBF). Both bromine isotopes are β-delayed neutron emitters that have large cumulative fission yields and were identified as top-priority cases for total absorption study by the Nuclear Energy Agency in 2007. Our investigations corroborate that the decay schemes of 87 Br and 88 Br suffer from the so-called pandemonium effect. Unique MTAS properties enable direct neutron measurements. Here, we present MTAS-derived β-delayed neutron spectra, β-delayed neutron emission probabilities of P n ( 87 Br) = 2.36(24)%, and P n ( 88 Br) = 6.4(6)%, and the β-delayed neutron transitions intensity of 4(2)% to the first excited 87 Kr state, populated in the β-neutron decay of 88Br. Incorporating new data into calculations of the electromagnetic decay heat component emitted during thermal neutron fission of 235 U and 239 Pu improves agreement with experimental data up to approximately 80 s after fission. The estimation of the nuclear reactor $\bar{ν}_e$ flux results in changes of up to 1% in the expected $\bar{ν}_e$ interactions with the detector material for 235 U, 238 U, 239Pu, and 241 Pu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Bayesian reconstruction of anisotropic flow fluctuations at fixed impact parameter

The cumulants of the distribution of anisotropic flow are measured accurately in Pb+Pb collisions at the LHC as a function of centrality classifiers (charged multiplicity and/or transverse energy). Using Bayesian inference, we reconstruct from these measurements the probability distribution of anisotropic flow in the ``theorists' frame'' where the impact parameter has a fixed magnitude and orientation, up to ∼70% centrality. The variation of flow fluctuations with impact parameter displays direct evidence of viscous damping, which is larger for higher Fourier harmonics, in line with expectations from hydrodynamics. We use intensive measures of non-Gaussian flow fluctuations, which have reduced dependence on centrality. Here, we infer from ATLAS data the magnitude of these intensive non-Gaussianities in each Fourier harmonic. They provide data-driven estimates of response coefficients to initial anisotropies, without resorting to any specific microscopic model of initial conditions. These estimates agree with viscous hydrodynamic calculations.

Bayesian methods↗
DOE OSTI2020

Blinded challenge for precision cosmology with large-scale structure: Results from effective field theory for the redshift-space galaxy power spectrum

An accurate theoretical template for the galaxy power spectrum is key for the success of ongoing and future spectroscopic surveys. We examine to what extent the effective field theory (EFT) of large-scale structure is able to provide such a template and correctly estimate cosmological parameters. To that end, we initiate a blinded challenge to infer cosmological parameters from the redshift-space power spectrum of high-resolution mock catalogs mimicking the BOSS galaxy sample but covering a 100 times larger cumulative volume. This gigantic simulation volume allows us to separate systematic bias due to theoretical modeling from the statistical error due to sample variance. The challenge is to measure three unknown input parameters used in the simulation: the Hubble constant, the matter density fraction, and the clustering amplitude. We present analyses done by two independent teams, who have fitted the mock simulation data generated by yet another independent group. This allows us to avoid any confirmation bias by analyzers and to pin down possible tuning of the specific EFT implementations. Both independent teams have recovered the true values of the input parameters within subpercent statistical errors corresponding to the total simulation volume.

79 ASTRONOMY AND ASTROPHYSICS↗