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Competing atomic processes in Ba and Sr injection critical velocity experiments

The critical ionization velocity effect requires a superthermal electron population to ionize through collisional impact. Such superthermal electrons can however lose energy to competing atomic processes, as well as to ionization, thus limiting the efficiency of the effect. Considering Ba and Sr magnetospheric injection experiments designed to test the CIV theory, it is found that in both cases roughly 60 percent of the superthermal electron energy is lost on exciting line radiation. Moreover, energy loss to background neutral oxygen places a strict limit on the injected cloud densities for which critical velocity effects are possible; a finding which explains the consistently negative results in radial injection experiments.

Newell, P. T.↗

Use of Collocated KWAJEX Satellite, Aircraft, and Ground Measurements for Understanding Ambiguities in TRMM Radiometer Rain Profile Algorithm

Coordinated ground, aircraft, and satellite observations are analyzed from the 1999 TRMM Kwajalein Atoll field experiment (KWAJEX) to better understand the relationships between cloud microphysical processes and microwave radiation intensities in the context of physical evaluation of the Level 2 TRMM radiometer rain profile algorithm and uncertainties with its assumed microphysics-radiation relationships. This talk focuses on the results of a multi-dataset analysis based on measurements from KWAJEX surface, air, and satellite platforms to test the hypothesis that uncertainties in the passive microwave radiometer algorithm (TMI 2a12 in the nomenclature of TRMM) are systematically coupled and correlated with the magnitudes of deviation of the assumed 3-dimensional microphysical properties from observed microphysical properties. Re-stated, this study focuses on identifying the weaknesses in the operational TRMM 2a12 radiometer algorithm based on observed microphysics and radiation data in terms of over-simplifications used in its theoretical microphysical underpinnings. The analysis makes use of a common transform coordinate system derived from the measuring capabilities of the aircraft radiometer used to survey the experimental study area, i.e., the 4-channel AMPR radiometer flown on the NASA DC-8 aircraft. Normalized emission and scattering indices derived from radiometer brightness temperatures at the four measuring frequencies enable a 2-dimensional coordinate system that facilities compositing of Kwajalein S-band ground radar reflectivities, ARMAR Ku-band aircraft radar reflectivities, TMI spacecraft radiometer brightness temperatures, PR Ku-band spacecraft radar reflectivities, bulk microphysical parameters derived from the aircraft-mounted cloud microphysics laser probes (including liquid/ice water contents, effective liquid/ice hydrometeor radii, and effective liquid/ice hydrometeor variances), and rainrates derived from any of the individual ground, aircraft, or satellite algorithms applied to the radar or radiometer measurements, or their combination. The results support the study's underlying hypothesis, particularly in context of ice phase processes, in that the cloud regions where the 2a12 algorithm's microphysical database most misrepresents the microphysical conditions as determined by the laser probes, are where retrieved surface rainrates are most erroneous relative to other reference rainrates as determined by ground and aircraft radar. In reaching these conclusions, TMI and PR brightness temperatures and reflectivities have been synthesized from the aircraft AMPR and ARMAR measurements with the analysis conducted in a composite framework to eliminate measurement noise associated with the case study approach and single element volumes obfuscated by heterogeneous beam filling effects. In diagnosing the performance of the 2a12 algorithm, weaknesses have been found in the cloud-radiation database used to provide microphysical guidance to the algorithm for upper cloud ice microphysics. It is also necessary to adjust a fractional convective rainfall factor within the algorithm somewhat arbitrarily to achieve satisfactory algorithm accuracy.

Smith, Eric A.↗

A satellite passive 37-GHz scattering-based method for measuring oceanic rain rates

A combination of theory and measurement is used to develop a scattering-based method for quantitatively measuring rainfall over the ocean from Nimbus-7 Scanning Multichannel Microwave Radiometer (SMMR) 37-GHz observations. This technique takes the observed scattering effects of precipitation on 37-GHz brightness temperatures and applies it to the oceanic environment. It requires an estimate of the effective radiating temperature of the cloudy portion of the atmosphere, and a brightness temperature measurement of the cloud-free ocean surface. These two measurements bound all possible combinations of clear and cloudy conditions within a footprint in terms of bipolarized brightness temperatures. Any satellite-observed brightness temperature T(B) lower than these values is assumed to reflect scattering, which at 37 GHz is only due to precipitation-size hydrometeors. Because the technique involves linear transformation between dual polarized brightness temperature and rain rate, there are no nonlinear 'footprint filling' effects and a unique footprint-averaged rain rate results. It is shown that these SMMR-derived rain rates for five cases of convection over the Gulf of Mexico are closely related to simultaneously derived radar rain rates, having a correlation of 0.90. This technique is then applied to a massive squall line over the Gulf of Mexico, and the resulting rain rate distribution reflects features found in cloud top heights and texture inferred from GOES infrared and visible imagery.

Spencer, R. W.↗

Optically thin cirrus clouds over oceans and possible impact on sea surface temperature of warm pool in western Pacific

Over the convectively active tropical ocean regions, the measurement made from space in the IR and visible spectrum have revealed the presence of optically thin cirrus clouds, which are quite transparent in the visible and nearly opaque in the IR. The Nimbus-4 IR Interferometer Spectrometer (IRIS), which has a field of view (FOV) of approximately 100 km, was utilized to examine the IR optical characteristics of these cirrus clouds. From the IRIS data, it was observed that these optically thin cirrus clouds prevail extensively over the warm pool region of the equatorial western Pacific, surrounding Indonesia. It is found that the seasonal cloud cover caused by these thin cirrus clouds exceeds 50 percent near the central regions of the warm pool. For most of these clouds, the optical thickness in the IR is less than or = 2. It is deduced that the dense cold anvil clouds associated with deep convection spread extensively and are responsible for the formation of the thin cirrus clouds. This is supported by the observation that the coverage of the dense anvil clouds is an order of magnitude less than that of the thin cirrus clouds. From these observations, together with a simple radiative-convective model, it is inferred that the optically thin cirrus can provide a greenhouse effect, which can be a significant factor in maintaining the warm pool. In the absence of fluid transports, it is found that these cirrus clouds could lead to a runaway greenhouse effect. The presence of fluid transport processes, however, act to moderate this effect. Thus, if a modest 20 W/sq m energy input is considered to be available to warm the ocean, then it is found that the ocean mixed-layer of a 50-m depth will be heated by approximately 1 C in 100 days.

Prabhakara, C.↗

An Overview of CMIP5 and CMIP6 Simulated Cloud Ice, Radiation Fields, Surface Wind Stress, Sea Surface Temperatures and Precipitation over Tropical and Subtropical Oceans

The potential links between ice water path (IWP), radiation, circulation, sea surface temperature (SST) and precipitation over the Pacific and Atlantic Oceans resulting from the falling ice radiative effects (FIREs) are examined from present day model outputs of CMIP5 and CMIP6. The latter is divided into two subsets with (SON6) and without FIREs (NOS6) as more models with FIREs are included in CMIP6 than in CMIP5. Improvement in floating cloud ice (~20 g m-2) is noticeable over convective regions in CMIP6 relative to CMIP5. The inclusion of FIREs in SON6 subset may contribute to reduce biases of overestimated outgoing longwave radiation and downward surface shortwave and overestimated reflected shortwave at the top of the atmosphere (TOA) by magnitudes of 4?8 W m-2 over convective regions against CERES, compared to NOS6 subset. The reduced biases in radiative fluxes in convective regions stabilize the atmosphere and lead to circulation, SST, cloud and precipitation changes over the trade-wind regions, as seen from improved radiative fluxes (4?15 W m-2), surface wind stress biases, SST (0.2?0.8 K) and precipitation (1 mm day-1) biases. The significant improvement from NOS6 to SON6 leads to improved multi-model means for CMIP6 relative to CMIP5 for radiation fields over the trade wind regions but the degradation over convective zones is attributed to NOS6 subset. The results suggest that other sources of uncertainty and deficiencies in climate models may play significant roles for reducing discrepancies although FIREs, via radiation-circulation coupling, may be one of the factors that help to reduce regional biases.

Jui-Lin F Li↗

Effects of cirrus composition on atmospheric radiation budgets

A radiative transfer model that can be used to determine the change in solar and infrared fluxes caused by variations in the composition of cirrus clouds was used to investigate the importance of particle size and shape on the radiation budget of the Earth-atmosphere system. Even though the cloud optical thickness dominates the radiative properties of ice clouds, the particle size and nonsphericity of ice crystals are also important in calculations of the transfer of near-IR solar wavelengths. Results show that, for a given optical thickness, ice clouds composed of larger particles would produce larger greenhouse effects than those composed of smaller particles. Moreover, spherical particles with equivalent surface areas, frequently used for ice crystal clouds, would lead to an overestimation of the greenhouse effect.

Kinne, Stefan↗

Investigation of Cloud Feedback in the GLAS Model

The theoretical and observational studies of cirrus clouds were reviewed to provide information for more realistic treatments of cirrus in the general circulation models. Based on the review, one time-step and ten-day model simulations were conducted to investigate the differences in the longwave radiation flux between the black and transparent cirrus treatment in the infrared. For both experiments substantial difference in the outgoing longwave flux at the top of the atmosphere is found. For the ten-day simulations, the differences in the convective, supersaturation and total cloudiness, temperature, and sensible and latent heat fluxes are also examined on various temporal and spatial scales. Although the cause-and-effect is difficult to identify, the results clearly suggest that on the time scale of a few days and longer cloud-radiation interactions play an important role. Sensitivity study of the longwave radiation flux to different longwave radiation parameterizations was performed by comparing the calculated fluxes between the Wu-Kaplan's scheme used in the present GLAS model and the Wang's schemes for climate studies.

Wang, W. C.↗

Early-time plasma expansion characteristics of ionized clouds in the ionosphere

A series of Vlasov-Poisson simulations were conducted with barium and lithium gas mixtures expanding into an O(+) background plasma, with the values for the Ba(+)/Li(+) composition ratios and the cloud/background density ratios based on anticipated release values in the upcoming Combined Release and Radiation Effects Satellite (CRRES) experiment. The results obtained on the early-time expansion of high-density Ba(+), Li(+), and Ba(+)-Li(+) plasma clouds into low-density O(+) background plasma complement the H(+)-O(+) expansions of Gurevich et al. (1973) and Singh and Schunk (1982, 1983), and the characteristic features observed apply to the very-early-time expansion phase of the CRRES releases.

Schunk, R. W.↗

Coupling the Mars Dust and Water Cycles: Investigating the Role of Clouds in Controlling the Vertical Distribution of Dust During N. H. Summer

The dust cycle is critically important for the current climate of Mars. The radiative effects of dust impact the thermal and dynamical state of the atmosphere (Gierasch and Goody, 1968; Haberle et al., 1982; Zurek et al., 1992). Although dust is present in the Martian atmosphere throughout the year, the level of dustiness varies with season. The atmosphere is generally the dustiest during northern fall and winter and the least dusty during northern spring and summer (Smith, 2004). Dust particles are lifted into the atmosphere by dust storms that range in size from meters to thousands of kilometers across (Cantor et al., 2001). During some years, regional storms combine to produce hemispheric or planet encircling dust clouds that obscure the surface and raise atmospheric temperatures by as much as 40 K (Smith et al., 2002). Key recent observations of the vertical distribution of dust indicate that elevated layers of dust exist in the tropics and sub-tropics throughout much of the year (Heavens et al., 2011). These observations have brought particular focus on the processes that control the vertical distribution of dust in the Martian atmosphere. The goal of this work is to further our understanding of how clouds in particular control the vertical distribution of dust, particularly during N. H. spring and summer

Mars dust↗

Cloud-Scale Numerical Modeling of the Arctic Boundary Layer

The interactions between sea ice, open ocean, atmospheric radiation, and clouds over the Arctic Ocean exert a strong influence on global climate. Uncertainties in the formulation of interactive air-sea-ice processes in global climate models (GCMs) result in large differences between the Arctic, and global, climates simulated by different models. Arctic stratus clouds are not well-simulated by GCMs, yet exert a strong influence on the surface energy budget of the Arctic. Leads (channels of open water in sea ice) have significant impacts on the large-scale budgets during the Arctic winter, when they contribute about 50 percent of the surface fluxes over the Arctic Ocean, but cover only 1 to 2 percent of its area. Convective plumes generated by wide leads may penetrate the surface inversion and produce condensate that spreads up to 250 km downwind of the lead, and may significantly affect the longwave radiative fluxes at the surface and thereby the sea ice thickness. The effects of leads and boundary layer clouds must be accurately represented in climate models to allow possible feedbacks between them and the sea ice thickness. The FIRE III Arctic boundary layer clouds field program, in conjunction with the SHEBA ice camp and the ARM North Slope of Alaska and Adjacent Arctic Ocean site, will offer an unprecedented opportunity to greatly improve our ability to parameterize the important effects of leads and boundary layer clouds in GCMs.

Krueger, Steven K.↗

Separating Real and Apparent Effects of Cloud, Humidity, and Dynamics on Aerosol Optical Thickness near Cloud Edges

Aerosol optical thickness (AOT) is one of aerosol parameters that can be measured on a routine basis with reasonable accuracy from Sun-photometric observations at the surface. However, AOT-derived near clouds is fraught with various real effects and artifacts, posing a big challenge for studying aerosol and cloud interactions. Recently, several studies have reported correlations between AOT and cloud cover, pointing to potential cloud contamination and the aerosol humidification effect; however, not many quantitative assessments have been made. In this study, various potential causes of apparent correlations are investigated in order to separate the real effects from the artifacts, using well-maintained observations from the Aerosol Robotic Network, Total Sky Imager, airborne nephelometer, etc., over the Southern Great Plains site operated by the U.S. Department of Energy's Atmospheric Radiation Measurement Program. It was found that aerosol humidification effects can explain about one fourth of the correlation between the cloud cover and AOT. New particle genesis, cloud-processed particles, atmospheric dynamics, and aerosol indirect effects are likely to be contributing to as much as the remaining three fourth of the relationship between cloud cover and AOT.

Jeong, Myeong-Jae↗

Theoretical development of Monte Carlo codes for modeling cumulus cloud fields

Reflected fluxes are calculated for stratocumulus cloud fields as a function of skycover, cloud aspect ratio, and cloud shape. Cloud liquid water volume is held invariant as cloud shape is varied so that the results can be utilized more effectively by general circulation models and climate models. On the basis of required accuracy in the Earth Radiation Budget Experiment program, an order of magnitude value of 10 W/sq m is used to estimate significant differences between plane parallel and broken cloudiness. This limit is exceeded for cloud covers between 10% and 90%, indicating that plane paralel calculations are not satisfactory at most values of cloud cover. The choice of cloud shape also leads to large differences in reflected fluxes. These differences are traced to the anisotropic intensity pattern out the cloud sides, to the size and shape of the holes between clouds, and to variations in cloud area as viewed from the solar direction. An empirical relationship for effective cloud cover is given at solar zenith angle of theta = 60 deg. This relationship allows for the relatively accurate (delta F = 10 - 15 W/sq m.) computation of broken cloud field reflected fluxes from plane parallel calculations.

Welch, R. M.↗

A Comparison of Cloud Microphysical and Optical Properties during TOGA-COARE

The impact of cirrus clouds on climate is an issue of research interest currently. Whether cirrus clouds heat or cool the Earth-atmosphere system depends on the cloud shortwave albedo and infrared reflectance and absorptance. These in turn are determined by the size distribution, phase, and composition of particles in the clouds. The TOGA-COARE campaign presented an excellent opportunity to study cirrus clouds and their influence on climate. In this campaign, a microphysics instrument package was flown aboard the DC-8 aircraft at medium altitudes in cirrus clouds. This package included a 2D Greyscale Cloud Particle Probe, a Forward Scattering Spectrometer Aerosol Probe, and an ice crystal replicator. At the same time the ER-2 equipped with a radiation measurement system flew coordinated flight tracks above the DC-8 at very high altitude. The radiation measurement made were short and long wave fluxes, as well as narrowband fluxes, both upwelling and downwelling. In addition LIDAR data is available. The existence of these data sets allows for a the comparison of radiation measurement with microphysical measurements. For example, the optical depth and effective radius retrieved from the ER-2 radiation measurements can be compared to the microphysical data. Conversely, the optical properties and fluxes produced by the clouds can be calculated from the microphysical measurements and compared to those measured aboard the ER-2. The assumptions required to make these comparisons are discussed. Typical microphysical results show a prevalence of micron-sized particles, in addition to the cloud particles that exceed 100 mm. The large number of small particles or "haze" cause the effective cloud radii to shift to smaller sizes, leading to changes in optical parameters.

Strawa, A. W.↗

Radiative Heating Rate Profiles over the Southeast Atlantic Ocean during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. Further uncertainties in the cloud structure arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean where biomass burning aerosol is transported from the African continent. As the aerosol plume progresses across the southeast Atlantic Ocean, radiative heating within the aerosol layer has the potential to alter the thermodynamic environment and therefore the cloud structure; however, limited work has been done to quantify this along the trajectory of the aerosol plume in the region. The deployment of the First Atmospheric Radiation Measurement Mobile Facility in support of the Layered Atlantic Smoke Interactions with Clouds field campaign provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 °S, 14.35 °W). Using observed profiles of temperature, humidity, and clouds from the field campaign, alongside aerosol optical properties from MERRA-2 as input for the Rapid Radiation Transfer Model, profiles of the radiative heating rate due to aerosols and clouds were computed. Radiative heating is also assessed across the southeast Atlantic Ocean using an ensemble of back trajectories from the Hybrid Single Particle Lagrangian Integrated Trajectory Model. Idealized experiments using the Rapid Radiation Transfer Model with and without aerosols and a range of values for the single scattering albedo demonstrate that shortwave heating within the aerosol layer above Ascension Island can locally range between 2 and 8 K per day depending on the aerosol optical properties, though impacts of the aerosol can be felt elsewhere in the atmospheric column. When considered under clear conditions, the aerosol has a cooling effect at the TOA and based on the observed cloud properties at Ascension Island, the cloud albedo is not large enough to overcome this. Shortwave radiative heating due to biomass burning aerosol is not balanced by additional longwave cooling, and the net radiative impact results in a stabilization of the lower troposphere. However, these results are extremely sensitive to the single scattering albedo assumptions in models.

Allison B. Marquardt Collow↗

Marine stratocumulus cloud characteristics from multichannel satellite measurements

Understanding the effects of aerosols on the microphysical characteristics of marine stratocumulus clouds, and the resulting influence on cloud radiative properties, is a primary goal of FIRE. The potential for observing variations of cloud characteristics that might be related to variations of available aerosols is studied. Some results from theoretical estimates of cloud reflectance are presented. Also presented are the results of comparisons between aircraft measured microphysical characteristics and satellite detected radiative properties of marine stratocumulus clouds. These results are extracted from Mineart where the analysis procedures and a full discussion of the observations are presented. Only a brief description of the procedures and the composite results are presented.

Durkee, Philip A.↗

Theoretical studies of volatile processes in the outer solar system

Four studies of volatile processes in the outer solar system are discussed. Researchers suggest that the convective and conductive regions of Triton's atmosphere join at the tropopause near 10 km. A model of volatile transport on Triton's surface was constructed that predicts that Triton's surface north of 15 degrees north latitude is experiencing deposition of nitrogen frosts, as are the bright portions of the south polar cap near the equator. Also discussed are numerical models of the evolution of Titan's surface and atmosphere. Results of a study of the rheology of ammonia-water liquids were applied to the icy satellites of the outer solar system. Finally, the researchers examined the frictional heating, sublimation, and re-condensation of grains free-falling into the solar nebula from a surrounding interstellar cloud. The sublimation model includes the effect of various volatile species and accounts for the poor radiating properties of small grains using Mie theory.

Lunine, Jonathan I.↗

Diffusion model for lightning radiative transfer

A one-speed Boltzmann transport theory, with diffusion approximations, is applied to study the radiative transfer properties of lightning in optically thick thunderclouds. Near-infrared (lambda = 0.7774 micrometers) photons associated with a prominent oxygen emission triplet in the lightning spectrum are considered. Transient and spatially complex lightning radiation sources are placed inside a rectangular parallelepiped thundercloud geometry and the effects of multiple scattering are studied. The cloud is assumed to be composed of a homogeneous collection of identical spherical water droplets, each droplet a nearly conservative, anisotropic scatterer. Conceptually, we treat the thundercloud like a nuclear reactor, with photons replaced by neutrons, and utilize standard one-speed neutron diffusion techniques common in nuclear reactor analyses. Valid analytic results for the intensity distribution (expanded in spherical harmonics) are obtained for regions sufficiently far from sources. Model estimates of the arrival-time delay and pulse width broadening of lightning signals radiated from within the cloud are determined and the results are in good agreement with both experimental data and previous Monte Carlo estimates. Additional model studies of this kind will be used to study the general information content of cloud top lightning radiation signatures.

Koshak, William J.↗

Monitoring Aerosols from Space: What We can Say, and What We Can't

Aerosols are understood to play a significant role is the global energy balance, and especially on atmospheric as well as surface energy balances regionally. A combination of direct radiative cooling of the surface, atmospheric warming through diabatic heating, and indirect effects of aerosol on clouds are all thought to contribute to the net aerosol effect, though the magnitudes of each are both highly variable in space and time, and highly uncertain. Passive space-based remote sensing is a key tool for constraining these effects, due to the frequent, global coverage satellites can provide. However, information from such observations about total-column aerosol amount (i.e., aerosol optical depth or AOD), and especially about aerosol type, is limited. The current generation of passive aerosol remote-sensing instruments, including the Multi-angle Imaging SpectroRadiometer (MISR) and the MODerate resolution Imaging Spectroradiometer (MODIS) offer vast improvements over previous instruments, including AOD over water and much of the land surface, fine vs. coarse particle type over ocean from MODIS, and discrimination of about a dozen aerosol types from MISR under good retrieval conditions, based on particle size, shape, and single-scattering albedo (SSA) constraints. This presentation will summarize the capabilities and expected improvements in the currently available aerosol products, in light of required energy budget constraints. Ways of addressing the need for detailed information about particle microphysical properties, especially SSA, unobtainable from MISR or MODIS, will be discussed.

Kahn, Ralph A.↗