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At least 721 records · Page 40

Qualification of Digitized Legacy Fast Reactor Data

The Integral Fast Reactor (IFR) fuel compatibility test program (1984-1994) included a variety of fuel pin examinations conducted at the Hot Fuel Examination Facility (HFEF) and the Alpha-Gamma Hot Cell Facility (AGHCF). Hard copy data records of these examinations have been recovered, scanned, and preserved in PDF format. Many hard copy records are now qualified in accordance with an NRC-approved Quality Assurance Program Plan (QAPP), and there is an ongoing effort to qualify additional legacy records. This legacy fuel performance data is vital to support design and licensing of fast reactors with validation of state-of-the-art codes and advanced methods for design and analysis. Stakeholders can most easily utilize this data when the PDF scans have been converted into digital data tables. However, qualification of the scanned hard copy data does not qualify the digital data file resulting from the digitization of the data contained in the record; the subject matter expert (SME) must make a review of the digitized data table as well before it can be designated as qualified. This report outlines a peer review process to qualify the digital data file(s), typically in CSV format, corresponding to hard copy records in accordance with the existing QAPP.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Testing of uranium nitride fuel in T-111 cladding at 1200 K cladding temperature

Two groups of six fuel pins each were assembled, encapsulated, and irradiated in the Plum Brook Reactor. The fuel pins employed uranium mononitride (UN) in a tantalum alloy clad. The first group of fuel pins was irradiated for 1500 hours to a maximum burnup of 0.7-atom-percent uranium. The second group of fuel pins was irradiated for about 3000 hours to a maximum burnup of 1.0-atom-percent uranium. The average clad surface temperature during irradiation of both groups of fuel pins was approximately 1200 K. The postirradiation examination revealed the following: no clad failures or fuel swelling occurred; less than 1 percent of the fission gases escaped from the fuel; and the clad of the first group of fuel pins experienced clad embrittlement whereas the second group, which had modified assembly and fabrication procedures to minimize contamination, had a ductile clad after irradiation.

Rohal, R. G.↗

Non-equilibrium radiation nuclear reactor

An externally moderated thermal nuclear reactor is disclosed which is designed to provide output power in the form of electromagnetic radiation. The reactor is a gaseous fueled nuclear cavity reactor device which can operate over wide ranges of temperature and pressure, and which includes the capability of processing and recycling waste products such as long-lived transuranium actinides. The primary output of the device may be in the form of coherent radiation, so that the reactor may be utilized as a self-critical nuclear pumped laser.

Thom, K.↗

Grooved Fuel Rings for Nuclear Thermal Rocket Engines

An alternative design concept for nuclear thermal rocket engines for interplanetary spacecraft calls for the use of grooved-ring fuel elements. Beyond spacecraft rocket engines, this concept also has potential for the design of terrestrial and spacecraft nuclear electric-power plants. The grooved ring fuel design attempts to retain the best features of the particle bed fuel element while eliminating most of its design deficiencies. In the grooved ring design, the hydrogen propellant enters the fuel element in a manner similar to that of the Particle Bed Reactor (PBR) fuel element.

Emrich, William↗

Heat transfer systems for nuclear reactor cores, and related systems

A system for transferring heat from a nuclear reactor comprises a nuclear reactor comprising a nuclear fuel and a reactor vessel surrounding the nuclear reactor and a heat transfer system surrounding the nuclear reactor. The heat transfer system comprises an inner wall surrounding the nuclear reactor vessel, first fins coupled to an outer surface of inner wall, an outer wall between the inner wall and a surrounding environment, and second fins coupled to an inner surface of the outer wall and extending in a volume between the outer surface of the inner wall and the inner surface of the outer wall, the outer surface of the inner wall and the first fins configured to transfer heat from the nuclear reactor core to the second fins and the inner surface of the outer wall by thermal radiation. The heat transfer system may be directly coupled to the nuclear reactor vessel, or may be coupled to an external reflector surrounding the nuclear reactor vessel. Related heat transfer systems and systems for selectively removing heat from a nuclear reactor are disclosed.

Ougouag, Abderrafi Mohammed El-Amine↗

A Plan to Qualify New Fuel for the High Flux Isotope Reactor for Material Minimization

The High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL) is one of five high power research reactors the Office of Material Management and Minimization (M3) Program, Office of Conversion is working to convert from using highly enriched uranium (HEU) fuel to using low-enriched uranium (LEU) fuel. This effort stems from the primary objective within the U.S. Department of Energy (DOE) National Nuclear Security Administration (NNSA) to achieve permanent threat reduction by minimizing, and when possible, eliminating weapon-usable nuclear material around the world. Under M3’s Office of Conversion, the U.S. High Performance Research Reactor (USHPRR) Project is pursuing fuel qualification and licensing of LEU fuels to support the high-performance reactors. All high-performance reactors except HFIR will be converted to LEU monolithic uranium-molybdenum alloy fuel. HFIR will be evaluated for conversion to LEU using a uranium silicide fuel, namely, U3Si2-Al dispersion fuel. The mission of the USHPRR Project is to develop the technology needed to reduce, and eventually eliminate, worldwide use of HEU in civilian applications. The goal is to develop the technical means needed to use low enriched uranium (LEU) instead of HEU fuel in research and test reactors without significant penalties in performance, economics, or safety of the reactors. The USHPRR Project has four major elements, called Pillars: Fuel Qualification (FQ) managed at Idaho National Laboratory (INL), Fuel Fabrication (FF) managed at Pacific Northwest National Laboratory (PNNL), Reactor Conversion (RC) managed at Argonne National Laboratory (Argonne), and Cross-Cutting (CC) managed at Savannah River National Laboratory (SRNL). FQ is responsible for the qualification of the fuel type. RC is responsible for supporting reactor conversion analysis and overseeing licensing submittals leading to conversions of domestic reactors to LEU fuel. For the FQ effort, FQ (INL) worked in collaboration with RC (Argonne) and ORNL to develop the plan for the uranium silicide fuel qualification for HFIR. The resulting HFIR Fuel Qualification Plan provides the general approach for the USHPRR team to move the selected uranium silicide fuel design for HFIR conversion through qualification. Authorization and use in HFIR will be approved through the DOE’s Office of Science. Uranium silicide fuel was previously qualified in NUREG-1313 at an approximate maximum heat flux of 1.4 MW/m2 and a maximum fuel section temperature of about 130°C. In addition to the different regulator process utilized by DOE, these upper limits will be exceeded in HFIR; therefore, further testing will be necessary to ensure the fuel can meet HFIR qualification requirements. The HFIR fuel loading may exceed 4.8 gU/cm3 which was determined in the NUREG-1313 safety evaluation to be acceptable for use in non-power NRC-licensed reactors provided there exist no other safety considerations. In addition, the uranium silicide fuel will need to be qualified in a HFIR-specific design. This plan includes the currently available information from the USHPRR Project Functions and Requirements document and expands these requirements to ensure that planned tests have traceable results providing evidence that the requirements have been met. Data collection methods are discussed as well as the process to show that the requirements have been met. This document is designed to provide a pathway for researchers to obtain data necessary and at the appropriate quality level for HFIR fuel qualification

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Coolant Enclosure Solutions for Micro Gas Cooled Reactors with Enhanced Efficiency and Safety

Argonne’s advanced high-pressure, high-temperature gas enclosures solutions were developed and tested for Light Water Reactor (LWR) fuel applications wherein pressure, temperature, fuel and working fluid are substantially different when compared to the operating conditions typical of gas cooled reactors (GCR). For LWR applications the coolant sleeve pressure exerted on the inner and outer walls of the sleeve may be equalized by pressurizing the fuel rod (e.g., with helium gas) to compensate for the coolant high pressure exerted on the outer walls of the sleeve. This results in a lower differential pressure. Micro-GCRs are reactor systems operated at elevated temperatures and pressure with gas as a working fluid. HolosGen’s Holos-Quad represent a type of Micro-GCR wherein the core is sleeved to segregate the fuel and other components from the working fluid.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

High Flux Isotope Reactor Low-Enriched Uranium Low Density Silicide Fuel Design Parameters

High Flux Isotope Reactor (HFIR) highly enriched uranium (HEU) to low-enriched uranium (LEU) conversion activities are ongoing as part of the Department of Energy (DOE) National Nuclear Security Administration (NNSA)’s nuclear nonproliferation mission. Design activities studying the conversion of HFIR from HEU to LEU fuel explored different fuel design features and shapes with a low density uranium-silicide dispersion (U 3 Si 2 -Al) fuel, which has a uranium density of 4.8 gU/cm 3 . The goal of these studies is to generate several HFIR LEU fuel designs of varying fuel fabrication complexity that meet the current HEU performance metrics and safety requirements. The documented designs will serve as references for fuel fabrication and qualification activities. Recent advancements in modeling and simulation tools enable quick prototyping of fuel designs. Shift, a Monte Carlo neutron transport and depletion tool optimized for high-performance computing (HPC) architectures, is used for efficient fuel cycle and performance metrics calculations. The HFIR Steady State Heat Transfer Code (HSSHTC) is used to vet the thermal safety margin. Also, a new automation tool that connects all fuel design analysis steps, named Python HFIR Analysis and Measurement Engine (PHAME), has been developed to expedite the design study in an efficient and reproducible manner. Leveraging these tools, several candidate fuel designs were selected for varying fabrication complexity. This report provides design feature details for four selected HFIR LEU low density U 3 Si 2 -Al fuel designs and their corresponding performance and safety metrics. Nominal, best-estimate design parameters and irradiation conditions, including fission rate densities, power densities, heat fluxes, and cumulative fission densities are provided for candidate fuel designs relevant to framing irradiation experiments to support fuel qualification efforts. Simulations show that the low density U 3 Si 2 -Al, with design features to enhance safety, can meet HEU core performance metrics and safety requirements if the reactor power is increased from 85 MW (HEU) to 95 MW (LEU) and if the active fuel length is increased from 50.80 cm (HEU) to 55.88 cm (LEU).

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Involute Working Group – Validation of CFD Turbulence Models for Steady-State Safety Analysis of Corner Geometry

Worldwide, three research reactors have fuel plates curved as a circle-involute (a spiral generated around a circle): Oak Ridge National Laboratory High Flux Isotope Reactor located in Tennessee, U.S.A. [1], Institut Laue-Langevin High Flux Reactor located in Grenoble, France [2], and Technical University of Munich Research Neutron Source Heinz Maier-Leibnitz located in Garching, Germany [3]. All three reactors are currently using highly enriched uranium ( 235 U/U ≥ 20 wt%) as fuel, and all three are actively engaged in activities to convert to low-enriched uranium ( 235 U/U < 20 wt%) fuel.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A review of cladding failure thresholds in RIA conditions based on transient reactor test data and the need for continued testing

Transient reactor experiments on light water reactor (LWR) fuel pins had been conducted since the beginning of the nuclear era to help determine core coolability and cladding failure thresholds. During one such test in November of 1993 at the CABRI transient test reactor on a test involving a high burnup fuel rod with a corroded Zircaloy-4 cladding it was first observed that cladding failures could occur prior to a departure from nucleate boiling (pre-DNB) at lower-than-expected peak radial average enthalpies. This paper will present an independent review of the publicly available transient reactor test database on higher burnup LWR pins conducted at the CABRI and NSRR reactors as well as review of a selection of published out of pile mechanical testing methods. The purpose of the review is to determine how well the new regulatory limits are supported by experimental data. The review will identify if additional transient reactor tests could provide additional support for the NRC guidance or identify the need for revisions. The evaluation will consider how far the existing database can be extrapolated when considering low hydrogen zirconium alloy claddings (with and without protective coatings) containing very high burnup (> 70 MWd/kgU) UO2 fuel pellets. Finally, the authors will suggest how out of pile mechanical tests can be used in conjunction with a limited number of transient reactor tests to develop cladding specific failure thresholds in RIA type transients.

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BISON Capability to Account for Dopant Sensitivity in Relevant UO 2 Material Models

The U.S. Department of Energy’s Nuclear Energy Advanced Modeling and Simulation program aims to develop predictive capabilities using computational methods for the analysis and design of advanced reactor and fuel cycle systems. This program has been supporting the development of BISON, a high-fidelity and high-resolution fuel performance tool at the engineering scale. Incorporation of more physics-based models in BISON for the accident tolerant fuel applications motivated this study. This document details integration of new modeling capabilities in BISON, including: a tensile strength model for uranium dioxide (UO 2 ) fuel to incorporate the microstructural effects (e.g., grain size, fabrication pore size, and porosity), and atomistic-informed creep model for UO 2 fuel that is developed by Los Alamos National Laboratory. Sensitivity analyses are conducted on these models separately as well as a two-dimensional full rod application under normal operating conditions. Lastly, these new modeling capabilities in BISON are exercised in Halden IFA-677.1 and IFA-716.1 assessment cases.

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Quantitative Voltammetry Measurements of High-Concentration Actinides in Molten Chloride Fuel Salts

Molten chloride mixtures containing high concentrations of UCl 3 (i.e., >70 wt%) are candidates for next-generation molten salt reactor (MSR) fuel salts that enable new plant optimization and fuel cycle strategies. MSR licensing, however, is contingent on the development of effective material control and accounting (MC&A) practices for these salts. To close this gap, we have developed an electroanalytical approach that enables accurate in situ measurements of uranium concentrations in these highly loaded fuel salts. This methodology uses a multielectrode array voltammetry sensor combined with digital simulations that account for non-idealities such as uncompensated resistance effects. The theory-based numerical simulations of voltammetry responses yielded correction factors that are agnostic of electrochemical cell geometry and produced consistent voltammetry peak current results when correcting for varying amounts of ohmic resistance. In doing so, we have demonstrated accurate concentration measurements for UCl 3 in LiCl-KCl-UCl 3 across a range of mass fractions between 55 and 72.3 wt% at 550 °C.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BISON Fuel Fragmentation Relocation and Dispersal (FFRD) Assessment Database for Eventual Use in Bayesian Calibration

Existing light-water reactor (LWR) fuel vendors have been interested in seeking increased discharge burnups of nuclear fuel rods for improved economics for quite a few years. With increased burnups come additional challenges that must be addressed. It has been experimentally observed that average burnups higher than the current regulatory limit of 62 MWd/kgU may undergo fuel fragmentation, relocation, and dispersal (FFRD) during a loss-of-coolant accident (LOCA). Industry must demonstrate approaches to mitigate FFRD. In an effort to support industry, the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program within the U.S. Department of Energy (DOE) has for several years invested in developing multiscale models and creating a validation/assessment database for these models to study the mechanisms driving FFRD. This report provides an update on changes made to the assessment database and new models added to BISON to support the study of fuel rod behavior during FFRD. An effort has been initiated this year to begin adding dedicated inputs to the publicly available Virtual Test Bed (VTB) repository for industry use. A section of this report details the efforts made in this area. NEAMS has recently developed new capabilities in the Multiphysics Object-Oriented Simulation Environment (MOOSE) framework’s stochastic tools module for calibration using Bayesian inference. The goal in the future is to use these capabilities to calibrate and identify weaknesses in the existing BISON models for FFRD. The report concludes with a discussion on the models most likely to benefit the most from such calibration.

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Fuel Storage Requirements

2023 No fuel storage plan had been developed 2024 The shipping & receiving requirements are understood A storage location has been selected and designated The storage limitations are known and incorporated The INL coordination & approval groups have been determined

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Atomistic and cluster dynamics modeling of fission gas (Xe) diffusivity in TRISO fuel kernels

TRISO fuel particles are candidates for use in next generation reactors including gas reactors, fluoride salt-cooled high temperature reactors, and micro-reactors. The UCO fuel kernel consists of a uranium dioxide (UO) and uranium carbide mixture. The addition of UC helps suppress the formation of carbon monoxide gas, which led to failures during initial TRISO development. The addition of uranium carbide alters the chemistry of the UO kernel, which is known to influence performance parameters such as fission gas diffusivity, although the impact has not been quantified and no models exist that take the change in chemistry into account. Therefore, better understanding and more accurate models of the impact of chemistry on fuel performance are of high priority. In this paper, a first-principles density functional theory (DFT) and empirical potential based multi-scale study has been carried out to model the diffusivity of fission gas xenon (Xe) in UCO TRISO fuel kernels. The focus is on the UO component in the UCO fuel kernels, as that represents the largest volume fraction of the fuel kernels. The study relies on DFT and empirical potential calculations to determine Xe and point defect properties, which are then used in thermodynamic and kinetic models to predict diffusion for intrinsic conditions. In addition, the information is utilized in cluster dynamics simulations using the Centipede code to estimate the impact of irradiation on defect transport. Additionally, the presence of UC or UC in the UCO fuel kernels is shown to have a substantial impact on the UO non-stoichiometry by inducing oxygen vacancies and driving UO sub-stoichiometric, which causes much slower Xe diffusion in UCO compared to light water reactor UO fuel. The application of this model in fuel performance simulations using the Bison code is also demonstrated.

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