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At least 721 records · Page 40

Radioactivities of Long Duration Exposure Facility (LDEF) materials: Baggage and bonanzas

Radioactivities in materials onboard the returned Long Duration Exposure Facility (LDEF) satellite were studied by a variety of techniques. Among the most powerful is low background Ge semiconductor detector gamma ray spectrometry. The observed radioactivities are of two origins: those radionuclides produced by nuclear reactions with the radiation field in orbit and radionuclides present initially as contaminants in materials used for construction of the spacecraft and experimental assemblies. In the first category are experiment related monitor foils and tomato seeds, and such spacecraft materials as Al, stainless steel, and Ti. In the second category are Al, Be, Ti, Va, and some special glasses. Consider that measured peak-area count rates from both categories range from a high value of about 1 count per minute down to less than 0.001 count per minute. Successful measurement of count rates toward the low end of this range can be achieved only through low background techniques, such as used to obtain the results presented here.

Smith, Alan R.↗

Induced radioactivity in LDEF components

The systematics of induced radioactivity on the Long Duration Exposure Facility (LDEF) were studied in a wide range of materials using low level background facilities for detection of gamma rays. Approx. 400 samples of materials processed from structural parts of the spacecraft, as well as materials from onboard experiments, were analyzed at national facilities. These measurements show the variety of radioisotopes that are produced with half-lives greater than 2 wks, most of which are characteristic of proton induced reactions above 20 MeV. For the higher activity, long lived isotopes, it was possible to map the depth and directional dependences of the activity. Due to the stabilized configuration of the LDEF, the induced radioactivity data clearly show contributions from the anisotropic trapped proton flux in the South Atlantic Anomaly. This effect is discussed, along with evidence for activation by galactic protons and thermal neutrons. The discovery of Be-7 was made on leading side parts of the spacecraft, although this was though not to be related to the in situ production of radioisotopes from external particle fluxes.

Harmon, B. A.↗

Radioactivities of Long Duration Exposure Facility (LDEF) materials: Baggage and bonanzas

Radioactivities in materials onboard the returned Long Duration Exposure Facility (LDEF) satellite were studied by a variety of techniques. Among the most powerful is low-background Ge-semiconductor detector gamma-ray spectrometry, illustrated here by results obtained at the Lawrence Berkeley Laboratory's (LBL) Low Background Facilities. The observed radioactivities are of two origins: those radionuclides produced by nuclear reactions with the radiation field in orbit, and radionuclides present initially as 'contaminants' in materials used for construction of the spacecraft and experimental assemblies. In the first category are experiment-related monitor foils and tomato seeds, and such spacecraft materials as aluminum, stainless steel, and titanium. In the second category are aluminum, beryllium, titanium, vanadium, and some special glasses.

Smith, Alan R.↗

Induced radioactivity in LDEF components

A systematic study of the induced radioactivity of the Long Duration Exposure Facility (LDEF) is being carried out in order to gather information about the low earth orbit radiation environment and its effects on materials. The large mass of the LDEF spacecraft, its stabilized configuration, and long mission duration have presented an opportunity to determine space radiation-induced radioactivities with a precision not possible before. Data presented include preliminary activities for steel and aluminum structural samples, and activation subexperiment foils. Effects seen in the data show a clear indication of the trapped proton anisotropy in the South Atlantic Anomaly and suggest contributions from different sources of external radiation fluxes.

Harmon, B. A.↗

Radioactive dating of the elements

The extent to which an accurate determination of the age of the Galaxy, and thus a lower bound on the age of the universe, can be obtained from radioactive dating is discussed. Emphasis is given to the use of the long-lived radioactive nuclei Re-187, Th-232, U-238, and U-235. The nature of the production sites of these and other potential Galactic chronometers is examined along with their production ratios. Age determinations from models of nucleocosmochronology are reviewed and compared with age determination from stellar sources and age constraints form cosmological considerations.

Cowan, John J.↗

Radioactive satellites - Intact reentry and breakup by debris impact

There is a substantial mass of radioactive material in nuclear reactors or radioisotope thermal generators (RTGs) in orbit about the earth. This paper examines the reentry of intact nuclear fuel cores and RTGs and the fragmentation and subsequent radioactive debris cloud deposition and evolution resulting from the impact of orbital debris upon an orbiting reactor, fuel core, or RTG. To assess the intact reentry, decay rates and a predicted decay date using historical and projected orbital decay data, are estimated. The current NASA debris environment model is utilized to estimate impact rates and debris cloud evolution of a fragmentation event. Results of these analyses are compared and concepts are tendered which would tend to minimize the radiological debris hazard to personnel and structures both on the earth's surface and in low earth orbit.

Anz-Meador, P. D.↗

Radioactivities induced in some LDEF samples

Radioactivities induced in several Long Duration Exposure Facilities (LDEF) samples were measured by low-level counting at Los Alamos and elsewhere. These radionuclides have activities similar to those observed in meteorites and lunar samples. Some trends were observed in these measurements in terms of profiles in trunnion layers and as a function of radionuclide half-life. Several existing computer codes were used to model the production by the protons trapped in the Earth's radiation belts and by the galactic cosmic rays of some of these radionuclides, Mn-54 and Co-57 in steel, Sc-46 in titanium, and Na-22 in alloys of titanium and aluminum. Production rates were also calculated for radionuclides possibly implanted in LDEF, Be-7, Be-10, and C-14. Enhanced concentrations of induced isotopes in the surfaces of trunnion sections relative to their concentrations in the center are caused by the lower-energy protons in the trapped radiation. Secondary neutrons made by high-energy trapped protons and by galactic cosmic rays produce much of the observed radioactivities, especially deep in an object. Comparisons of the observed to calculated activities of several radionuclides with different half-lives indicate that the flux of trapped protons at LDEF decreased significantly at the end of the mission.

Reedy, Robert C.↗

Nucleosynthesis of Short-lived Radioactivities in Massive Stars

A leading model for the source of many of the short-lived radioactivities in the early solar nebula is direct incorporation from a massive star [1]. A recent and promising incarnation of this model includes an injection mass cut, which is a boundary between the stellar ejecta that become incorporated into the solar cloud and those ejecta that do not [2-4]. This model also includes a delay time between ejection from the star and incorporation into early solar system solid bodies. While largely successful, this model requires further validation and comparison against data. Such evaluation becomes easier if we have a better sense of the nature of the synthesis of the various radioactivities in the star. That is the goal of this brief abstract.

Meyer, B. S.↗

Worswick Hot Springs: A Radioactive Hydrothermal Field Site

We report on a systematic characterization of the radiation environment and water temperatures of Worswick Hot Springs, which is in support of companion biochemical and microbial investigations of iron respiration in the ‘extreme’ microbial systems found at the field site. We have discovered localized areas of elevated radioactivity that are approximately four to five times greater than background radiation. Additionally, we have observed that both the radiation environment and the temperature of the spring waters vary over time. Because localized “hot spots” of elevated radiation and biofilms are easily accessible, various biological studies of radiation resistance and biosignature formation are possible, making this field site relevant for analog field studies that consider microbiology, geochemistry, and ionizing radiation. In addition to Worswick being a natural radiation biology laboratory that may also be relevant for space biology applications, we assert that these unusual environmental conditions may inform us about locations on Mars that are also enriched in radioactive elements and their potential for hosting biosignatures.

Jon C. Rask↗

SAVANNAH RIVER SITE INCIPIENT SLUDGE MIXING IN RADIOACTIVE LIQUID WASTE STORAGE TANKS DURING SALT SOLUTION BLENDING

This paper is the second in a series of four publications to document ongoing pilot scale testing and computational fluid dynamics (CFD) modeling of mixing processes in 85 foot diameter, 1.3 million gallon, radioactive liquid waste, storage tanks at Savannah River Site (SRS). Homogeneous blending of salt solutions is required in waste tanks. Settled solids (i.e., sludge) are required to remain undisturbed on the bottom of waste tanks during blending. Suspension of sludge during blending may potentially release radiolytically generated hydrogen trapped in the sludge, which is a safety concern. The first paper (Leishear, et. al. [1]) presented pilot scale blending experiments of miscible fluids to provide initial design requirements for a full scale blending pump. Scaling techniques for an 8 foot diameter pilot scale tank were also justified in that work. This second paper describes the overall reasons to perform tests, and documents pilot scale experiments performed to investigate disturbance of sludge, using non-radioactive sludge simulants. A third paper will document pilot scale CFD modeling for comparison to experimental pilot scale test results for both blending tests and sludge disturbance tests. That paper will also describe full scale CFD results. The final paper will document additional blending test results for stratified layers in salt solutions, scale up techniques, final full scale pump design recommendations, and operational recommendations. Specifically, this paper documents a series of pilot scale tests, where sludge simulant disturbance due to a blending pump or transfer pump are investigated. A principle design requirement for a blending pump is UoD, where Uo is the pump discharge nozzle velocity, and D is the nozzle diameter. Pilot scale test results showed that sludge was undisturbed below UoD = 0.47 ft{sup 2}/s, and that below UoD = 0.58 ft{sup 2}/s minimal sludge disturbance was observed. If sludge is minimally disturbed, hydrogen will not be released. Installation requirements were also determined for a transfer pump which will remove tank contents, and which is also required to not disturb sludge. Testing techniques and test results for both types of pumps are presented.

08 HYDROGEN↗

Dynamic radioactive particle source

A method and apparatus for providing a timed, synchronized dynamic alpha or beta particle source for testing the response of continuous air monitors (CAMs) for airborne alpha or beta emitters is provided. The method includes providing a radioactive source; placing the radioactive source inside the detection volume of a CAM; and introducing an alpha or beta-emitting isotope while the CAM is in a normal functioning mode.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

RECERTIFICATION OF THE MODEL 9977 RADIOACTIVE MATERIAL PACKAGING

The Model 9977 Packaging was initially issued a Certificate of Compliance (CoC) by the Department of Energy’s Office of Environmental Management (DOE-EM) for the transportation of radioactive material (RAM) in the Fall of 2007. This first CoC was for a single radioactive material and two packing configurations. In the five years since that time, seven Addendums have been written to the Safety Analysis Report for Packaging (SARP) and five Letter Amendments have been written that have authorized either new RAM contents or packing configurations, or both. This paper will discuss the process of updating the 9977 SARP to include all the contents and configurations, including the addition of a new content, and its submittal for recertification.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Containers and systems for the measurement of radioactive gases and related methods

Containers for a fluid sample containing a radionuclide for measurement of radiation from the radionuclide include an outer shell having one or more ports between an interior and an exterior of the outer shell, and an inner shell secured to the outer shell. The inner shell includes a detector receptacle sized for at least partial insertion into the outer shell. The inner shell and outer shell together at least partially define a fluid sample space. The outer shell and inner shell are configured for maintaining an operating pressure within the fluid sample space of at least about 1000 psi. Systems for measuring radioactivity in a fluid include such a container and a radiation detector received at least partially within the detector receptacle. Methods of measuring radioactivity in a fluid sample include maintaining a pressure of a fluid sample within a Marinelli-type container at least at about 1000 psi.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Chemical, biological, and radioactive contamination remediation with lasers

A laser is used to clean surfaces contaminated with chemical, biological, or radioactive substances. The laser directs a laser beam onto the surfaces and the ejecta is collected by a getter which can be a version of vacuum cleaner. A mobile system includes a laser transporting arm and collection system used in cleanup of metal and concrete surfaces contaminated with chemical, biological, or radioactive substances.

47 OTHER INSTRUMENTATION↗

Radioactive Material Inventory Optimization Using the Plutonium-239 Equivalent Curie Methodology

ABSTRACT The purpose of this paper is to provide the technical basis for application of the Plutonium 239 equivalent curies (PEC) concept used to optimize and limit the material-at-risk (MAR) in the Irradiated Materials Characterization Laboratory (IMCL) located at the Materials and Fuels Complex (MFC). The PEC concept offers a method to normalize all radionuclides to a common radiotoxic hazard index that can be summed to a single value. This paper describes the technical approach to applying the PEC concept, documents the weighting factors and specific activities to be utilized in the calculation, and provides an example of the application of the concept to a radionuclide distribution that is representative of materials encountered in the IMCL. The IMCL is operated to provide a dynamic, re-configurable capability to analyze and characterize irradiated or non-irradiated radioactive material samples. The operations unique to the IMCL include sample storage, preparation, and analysis using experiment-specific instrumentation such as, Electron probe micro-analyzer (EPMA), Focused ion beam (FIB), Transmission electron microscope (TEM), and Scanning electron microscope (SEM). The methodology used to characterize the radioactive material inventory enables the IMCL to operate in such a way that complements their capability and program goals without compromising the safety of the worker, co-located worker, or the general public. The PEC concept offers a method in which all radionuclide inventory is normalized to a common radiotoxic hazard index that can be summed to a single value. The PEC concept is useful in the comparison of various material types for hazard categorization and for identifying worst-case and bounding inventory.

07 ISOTOPE AND RADIATION SOURCES↗

Miniaturized pulsed discharge ionization detector, non-radioactive ionization sources, and methods thereof

The present application relates to pulsed discharge ionization detectors (PDIDs) and non-radioactive ionization sources, including miniaturized forms thereof. In some examples, the PDID includes annular electrodes, where each electrode is disposed between annular insulators. Also provided herein are methods of making and using such PDIDs, such as for detecting one or more volatile organic compounds, as well as non-radioactive ionization sources.

47 OTHER INSTRUMENTATION↗

Perspectives on Regulatory Design and Development for Transport Security of Nuclear and other Radioactive Materials

The responsibility for nuclear security rests entirely with the State but the International Atomic Energy Agency (IAEA) recognizes that a cornerstone in the development of a nuclear security regime is the development of regulations that address security of nuclear material and other radioactive material in transport. While the IAEA provides recommendations and guidance for security of materials in transport through Nuclear Security Series (NSS) documents, the challenge of integrating those recommendations into a Member State’s national legal framework is significant. Specifically, the development of transport security regulations requires coordination between both legal and technical experts within the country’s competent authority and multiple governmental agencies, as well as input from transport operators and other stakeholders. In addition to these interactions, the regulations must reflect the legal traditions of the Member State to fit within its overall national legal framework. Recognizing the challenge, the IAEA has requested input from international legal and technical experts to develop a methodology for drafting regulations on transport security of nuclear material and other radioactive material. This paper discusses the progress made so far in developing the methodology and provides a perspective on the need for transport security regulations and the challenges associated with their development. Ultimately, the goal of this paper is to introduce the IAEA-proposed methodology and to facilitate the discussion of this methodology with Member States that need support in developing their transport security regulations.

Ladsous, David↗

Miniaturized pulsed discharge ionization detector, non-radioactive ionization sources, and methods thereof

The present application relates to pulsed discharge ionization detectors (PDIDs) and non-radioactive ionization sources, including miniaturized forms thereof. In some examples, the PDID includes annular electrodes, where each electrode is disposed between annular insulators. Also provided herein are methods of making and using such PDIDs, such as for detecting one or more volatile organic compounds, as well as non-radioactive ionization sources.

42 ENGINEERING↗