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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 721 records · Page 40
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Low-field-actuated giant magnetocaloric effect and excellent mechanical properties in a NiMn-based multiferroic alloy

Multiferroic magnetic shape memory alloys with first-order magntostructural transformation exhibit much enhanced magnetocaloric effect which incorporates the latent heat associated with the phase transformation itself, but they suffer from the drawbacks of large hysteresis and transformation interval and consequently too high critical field to actuate the magnetocaloric effect, greatly impeding their applications. Here, by generating a kind of specific stacking-mediated structure of martensite through minor Al substitution to improve the geometric compatibility between martensite and austenite in the Ni 40 Co 10 Mn 40 Sn 9 Al 1 alloy, we greatly reduced the thermal hysteresis and transformation temperature interval while conserving the large magnetization difference between the two phases. Consequently, a low-field-actuated giant magnetocaloric effect with isothermal entropy change of 23 J kg –1 K –1 for a field change from 0 to 2 T, which is among the highest values reported heretofore for all magnetocaloric materials, was successfully achieved. Meanwhile, with minor Al substitution, the present single-phase multiferroic alloy that is intermetallic in nature exhibits superior mechanical properties, including excellent compressive properties over a wide temperature range and a relatively high fracture toughness, which are quite beneficial for practical applications. Lastly, by incorporating the advantages of low cost, environment friendliness and easy fabrication, this alloy shows great potential for magnetocaloric applications.

36 MATERIALS SCIENCE↗
DOE OSTI2023

On a fully-implicit VMS-stabilized FE formulation for low Mach number compressible resistive MHD with application to MCF

This study presents the development and evaluation of a fully-implicit variational multiscale (VMS) stabilized unstructured finite element (FE) formulation for compressible magnetohydrodynamics (MHD) model, at low Mach number regime. The model describes the dynamics of a compressible conducting fluid in the low Mach number limit in the presence of electromagnetic fields and can be used to study aspects of astrophysical phenomena, important science and technology applications, and basic plasma physics phenomena. The specific applications that motivate this study are macroscopic simulations of the longer time-scale stability and disruptions of magnetic confinement fusion (MCF) devices, specifically the ITER tokamak. The discussion considers the development of the VMS FE representation, the structure of the stabilizing terms that deal with significant convective flows, the stabilization of the nearly incompressible response of the fluid flow, and the stabilization of the constraint that enforces the solenoidal involution on the magnetic field. The nonlinear discretized system is solved with scalable preconditioned Newton–Krylov iterative methods, which employs a multiphysics block preconditioning method based on approximate block factorizations and Schur complements. The study presents an evaluation of the VMS method on a 2D cartesian tearing mode instability, and illustrates the scalability of the solvers on MCF relevant problems. A set of results are also presented for longer time-scale stability and disruptions for the ITER tokamak. These include a vertical displacement event (VDE), and a (1,1) internal kink mode. Here, the formulation is demonstrated to be scalable and also reasonably robust with respect to the Lundquist number scaling.

42 ENGINEERING↗
DOE OSTI2022

The Impact of Structural Distortions on the Magnetism of Double Perovskites Containing 5d 1 Transition-Metal Ions

Five double perovskites, each containing a transition-metal ion with a 5d 1 configuration, have been studied to better understand the surprising diversity of magnetic ground states seen in these isoelectronic compounds. Ba 2 ZnReO 6 adopts the cubic double perovskite structure and magnetically orders below 16 K, with a canted ferromagnetic structure and a saturated magnetization of ~0.24 μ B /Re. X-ray magnetic circular dichroism indicates a substantial orbital moment of approximately 0.4 μ B /Re that opposes the spin moment. The structures of Ba 2 NaOsO 6 (canted ferromagnet, T C = 7 K) and Ba 2 LiOsO 6 (antiferromagnet, T N = 8 K) are reinvestigated using time-of-flight neutron powder diffraction and found to crystallize with the cubic double perovskite structure. No evidence for a structural distortion can be found in either compound down to 10 K. Ba 2 CdReO 6 is also cubic at room temperature but undergoes a structural transition upon cooling below ~180 K to a tetragonal structure with I4/m symmetry that involves compression of the Re–O bonds that are parallel to the c-axis. Sr 2 LiOsO 6 shows a similar tetragonal distortion at room temperature and maintains that structure down to 10 K. Surprisingly, the Os-centered octahedron in Sr 2 LiOsO 6 is distorted in the opposite direction, exhibiting an elongation of the Os–O bonds along the c-axis. Differences in the distortions of the octahedra lead to different magnetic ground states, antiferromagnetic (T N = 4 K) for Ba 2 CdReO 6 and spin glass (T g = 30 K) for Sr 2 LiOsO 6 . Theoretical modeling shows that the varied magnetic behaviors of double perovskites containing 5d 1 ions are closely tied to crystallographic distortions. Furthermore, these distortions remove the degeneracy of the 5d t 2g orbitals, leading to changes in orbital occupation that ultimately determine which of the several competing magnetic ground states is favored.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2016

Response of complex networks to compression: Ca, La, and Y aluminoborosilicate glasses formed from liquids at 1 to 3 GPa pressures

Aluminoborosilicate glasses containing relatively high field strength modifiers (Ca, La, and Y) have been compressed at pressures up to 3 GPa and near the glass transition temperature (T{sub g}) and quenched to room temperature at high pressure followed by decompression. Structural changes were quantified with high-resolution {sup 27}Al and {sup 11}B MAS nuclear magnetic resonance at 14.1–18.8 T. The changes with pressure in Al and B coordinations in the recovered samples are quite large with more than 50% decreases in tetrahedral aluminum ({sup IV}Al) and 200%-300% increases in tetrahedral boron ({sup IV}B). Glasses with higher field strength modifiers (La and Y) contain more high coordinated aluminum ({sup V,V} {sup I}Al) at all pressures studied. More high coordinated boron also correlates with higher field strength modifier if all three compositions are compared on an isothermal basis. Although lowering fictive temperature and increasing pressure both increase Al and B coordinations, our study shows that the actual mechanisms for structural changes are most probably different for temperature and pressure effects. Using a rough thermodynamic model to extrapolate to higher pressures, it appears that a simple non-bridging oxygen (NBO) consumption mechanism is not sufficient to convert all the aluminum to octahedral and boron to tetrahedral coordination, suggesting other mechanisms for structural changes could occur at high pressure as NBO becomes depleted.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Chemical pressure tuning of URu 2 Si 2 via isoelectronic substitution of Ru with Fe

We have used specific heat and neutron diffraction measurements on single crystals of URu 2–x Fe x Si₂ for Fe concentrations x ≤ 0.7 to establish that chemical substitution of Ru with Fe acts as “chemical pressure” P ch as previously proposed by Kanchanavatee et al. [Phys. Rev. B 84 , 245122 (2011)] based on bulk measurements on polycrystalline samples. Neutron diffraction reveals a sharp increase of the uranium magnetic moment at x = 0.1, reminiscent of the behavior at the “hidden order” to large moment antiferromagnetic (LMAFM) phase transition observed at a pressure P x ≈ 0.5-0.7 GPa in URu₂Si₂. Using the unit cell volume determined from our measurements and an isothermal compressibility κ T = 5.2×10⁻³ GPa⁻¹ for URu₂Si₂, we determine the chemical pressure P ch in URu 2-x Fe x Si₂ as a function of x. The resulting temperature T-chemical pressure P ch phase diagram for URu 2-x Fe x Si₂ is in agreement with the established temperature T-external pressure P phase diagram of URu₂Si₂.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Relativistic gas accretion onto supermassive black hole binaries from inspiral through merger

Accreting supermassive black hole binaries are powerful multimessenger sources emitting both gravitational and electromagnetic (EM) radiation. Understanding the accretion dynamics of these systems and predicting their distinctive EM signals is crucial to informing and guiding upcoming efforts aimed at detecting gravitational waves produced by these binaries. To this end, accurate numerical modeling is required to describe both the spacetime and the magnetized gas around the black holes. In this paper, we present two key advances in this field of research. First, we have developed a novel 3D general relativistic magnetohydrodynamics (GRMHD) framework that combines multiple numerical codes to simulate the inspiral and merger of supermassive black hole binaries starting from realistic initial data and running all the way through merger. Throughout the evolution, we adopt a simple but functional prescription to account for gas cooling through photon emission. Next, we have applied our new computational method to follow the time evolution of a circular, equal-mass, nonspinning black hole binary for ∼200 orbits, starting from a separation of 20⁢𝑟 𝑔 and reaching the postmerger evolutionary stage of the system. We have shown how mass continues to flow toward the binary even after the binary “decouples” from its surrounding disk, but the accretion rate onto the black holes diminishes. We have identified how the minidisks orbiting each black hole are slowly drained and eventually dissolve as the binary compresses. We confirm previous findings that the system’s luminosity decreases by a factor of a few during inspiral; however, we observe an abrupt increase by ∼50% in this quantity at the time of merger, likely accompanied by an equally abrupt change in spectrum. Lastly, we have demonstrated that during the inspiral, fluid ram pressure regulates the fraction of the magnetic flux transported to the binary that attaches to the black holes’ horizons.

Accretion disk & black-hole plasma↗
DOE OSTI2018

Development of tearing instability in a current sheet forming by sheared incompressible flow

Sweet–Parker current sheets in high Lundquist number plasmas are unstable to tearing, suggesting they will not form in physical systems. Understanding magnetic reconnection thus requires study of the stability of a current sheet as it forms. Formation can occur due to sheared, sub-Alfvénic incompressible flows which narrow the sheet. Standard tearing theory is not immediately applicable to such forming sheets for two reasons: first, because the flow introduces terms not present in the standard calculation; second, because the changing equilibrium introduces time dependence to terms which are constant in the standard calculation, complicating the formulation of an eigenvalue problem. This paper adapts standard tearing mode analysis to confront these challenges. In an initial phase when any perturbations are primarily governed by ideal magnetohydrodynamics, a coordinate transformation reveals that the flow compresses and stretches perturbations. Here, a multiple scale formulation describes how linear tearing mode theory can be applied to an equilibrium changing under flow, showing that the flow affects the separable exponential growth only implicitly, by making the standard scalings time dependent. In the nonlinear Rutherford stage, the coordinate transformation shows that standard theory can be adapted by adding to the stationary rates time dependence and an additional term due to the strengthening equilibrium magnetic field. Overall, this understanding supports the use of flow-free scalings with slight modifications to study tearing in a forming sheet.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

HEATING AND ACCELERATION OF THE FAST SOLAR WIND BY ALFVÉN WAVE TURBULENCE

We present numerical simulations of reduced magnetohydrodynamic (RMHD) turbulence in a magnetic flux tube at the center of a polar coronal hole. The model for the background atmosphere is a solution of the momentum equation and includes the effects of wave pressure on the solar wind outflow. Alfvén waves are launched at the coronal base and reflect at various heights owing to variations in Alfvén speed and outflow velocity. The turbulence is driven by nonlinear interactions between the counterpropagating Alfvén waves. Results are presented for two models of the background atmosphere. In the first model the plasma density and Alfvén speed vary smoothly with height, resulting in minimal wave reflections and low-energy dissipation rates. We find that the dissipation rate is insufficient to maintain the temperature of the background atmosphere. The standard phenomenological formula for the dissipation rate significantly overestimates the rate derived from our RMHD simulations, and a revised formula is proposed. In the second model we introduce additional density variations along the flux tube with a correlation length of 0.04 R {sub ⊙} and with relative amplitude of 10%. These density variations simulate the effects of compressive MHD waves on the Alfvén waves. We find that such variations significantly enhance the wave reflection and thereby the turbulent dissipation rates, producing enough heat to maintain the background atmosphere. We conclude that interactions between Alfvén and compressive waves may play an important role in the turbulent heating of the fast solar wind.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Hofstadter states and re-entrant charge order in a semiconductor moiré lattice

The emergence of moiré materials with flat bands provides a platform to systematically investigate and precisely control correlated electronic phases. Here, we report local electronic compressibility measurements of a twisted WSe2/MoSe2 heterobilayer which reveal a rich phase diagram of interpenetrating Hofstadter states and electron solids. We show that this reflects the presence of both flat and dispersive moiré bands whose relative energies, and therefore occupations, are tuned by density and magnetic field. At low densities, competition between moiré bands leads to a transition from commensurate arrangements of singlets at doubly occupied sites to triplet configurations at high fields. Hofstadter states (i.e., Chern insulators) are generally favored at high densities as dispersive bands are populated, but are suppressed by an intervening region of reentrant charge-ordered states in which holes originating from multiple bands cooperatively crystallize. Our results reveal the key microscopic ingredients that favor distinct correlated ground states in semiconductor moiré systems, and they demonstrate an emergent lattice model system in which both interactions and band dispersion can be experimentally controlled.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Terahertz spin-orbital excitations in the paramagnetic state of multiferroic Sr 2 FeSi 2 O 7

Here, we studied the novel multiferroic material Sr 2 FeSi 2 O 7 and found three absorption modes above the magnetic ordering transition temperature using time-domain terahertz spectroscopy. These absorption modes can be explained as the optical transitions between the spin-orbit coupling and crystal-field split 3d 6 Fe 2+ ground-state term in this material. Consideration of the compressed tetrahedral environment of the Fe 2+ site is crucial to understand the excitations. We point out, however, discrepancies between the single-site atomic picture and the experimental results.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Dynamical Modulation of Solar Flare Electron Acceleration due to Plasmoid-shock Interactions in the Looptop Region

A fast-mode shock can form in the front of reconnection outflows and has been suggested as a promising site for particle acceleration in solar flares. Recent developments in the study of magnetic reconnection have shown that numerous plasmoids can be produced in a large-scale current layer. Here we investigate the dynamical modulation of electron acceleration in the looptop region when plasmoids intermittently arrive at the shock by combining magnetohydrodynamics simulations with a particle kinetic model. As plasmoids interact with the shock, the looptop region exhibits various compressible structures that modulate the production of energetic electrons. The energetic electron population varies rapidly in both time and space. The number of 5–10 keV electrons correlates well with the compression area, while that of >50 keV electrons shows good correlation with the strong compression area but only moderate correlation with shock parameters. We further examine the impacts of the first plasmoid, which marks the transition from a quasi-steady shock front to a distorted and dynamical shock. The number of energetic electrons is reduced by ~20% at 15–25 keV and nearly 40% for 25–50 keV, while the number of 5–10 keV electrons increases. In addition, the electron energy spectrum above 10 keV evolves softer with time. We also find that double or even multiple distinct sources can develop in the looptop region when the plasmoids move across the shock. Our simulations have strong implications to the interpretation of nonthermal looptop sources, as well as the commonly observed fast temporal variations in flare emissions, including the quasi-periodic pulsations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Comparison of measured and computed radial trajectories of plasma focus devices UMDPF1 and UMDPF0

In published literature, there has been scant data on radial trajectory of the plasma focus and no comparison of computed with measured radial trajectory. This paper provides the first such comparative study. We compute the trajectories of the inward-moving radial shock and magnetic piston of UMDPF1 plasma focus and compare these with measured data taken from a streak photograph. The comparison shows agreement with the measured radial trajectory in terms of average speeds and general shape of trajectory. This paper also presents the measured trajectory of the radially compressing piston in another machine, the UMDPF0 plasma focus, confirming that the computed radial trajectory also shows similar general agreement. Features of divergence between the computed and measured trajectories, towards the end of the radial compression, are discussed. From the measured radial trajectories, an inference is made that the neutron yield mechanism could not be thermonuclear. A second inference is made regarding the speeds of axial post-pinch shocks, which are recently considered as a useful tool for damage testing of fusion-related wall materials.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Evolution and sign control of square-wave-like anisotropic magneto-resistance in spatially confined La{sub 0.3}Pr{sub 0.4}Ca{sub 0.3}MnO{sub 3}/LaAlO{sub 3}(001) manganite thin films

We investigated magneto-transport properties of a compressively strained spatially confined La{sub 0.3}Pr{sub 0.4}Ca{sub 0.3}MnO{sub 3} (LPCMO) thin film micro-bridge deposited on LaAlO{sub 3}. Angular dependence of the magneto-resistance R(θ) of this bridge, where θ is the angle between the magnetic field and the current directions in the film plane, exhibits sharp positive and negative percolation jumps near T{sub MIT}. The sign and the magnitude of these jumps can be tuned using the magnetic field. Such behavior has not been observed in LPCMO micro-bridges subjected to tensile strain, indicating a correlation between the type of the lattice strain, the distribution of electronic domains, and the anisotropic magneto-resistance in spatially confined manganite systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Fast-timing microchannel plate photodetectors: design, fabrication and characterization

We report a detailed design, fabrication, and characterization of 6 x 6 cm(2) fast timing photodetectors based on next-generation microchannel plates (MCPs). The whole assembly is made of low-cost borosilicate glass materials and hermetically sealed with a bialkali photocathode in a vacuum. The flexible photodetector design provides the potential of modifying individual components as well as the entire configuration to fit for different applications. A series of prototype MCP-photodetectors were fabricated following a step-by-step process including functionalization of glass capillary array through atomic layer deposition, MCP baking and scrubbing, photocathode deposition, and hermetic thermo-compression sealing. The prototype MCP-photodetectors exhibit electron gains well beyond 107 level with good relative uniformity. An excellent rise time of 439 ps, timing distribution root-mean-square at a single photoelectron mode of 105 ps, a timing resolution of 20 ps, and magnetic field tolerance up to 1.3 T were achieved for a photodetector with 10 mu m pore size MCPs, comparing to that of 536 ps, 205 ps, 63 ps, and 0.7 T for the one with 20 mu m pore size MCPs. Published under license by AIP Publishing.

fast timing↗
DOE OSTI2017

Collimated Propagation of Fast Electron Beams Accelerated by High-Contrast Laser Pulses in Highly Resistive Shocked Carbon

In this study, collimated transport of ultrahigh intensity electron current was observed in cold and in laser-shocked vitreous carbon, in agreement with simulation predictions. The fast electron beams were created by coupling high-intensity and high-contrast laser pulses onto copper-coated cones drilled into the carbon samples. The guiding mechanism—observed only for times before the shock breakout at the inner cone tip—is due to self-generated resistive magnetic fields of ~ 0.5–1 kT arising from the intense currents of fast electrons in vitreous carbon, by virtue of its specific high resistivity over the range of explored background temperatures. The spatial distribution of the electron beams, injected through the samples at different stages of compression, was characterized by side-on imaging of hard x-ray fluorescence.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Comparison of algorithms for determination of rotation measure and Faraday structure. I. 1100–1400 MHz

Faraday rotation measures (RMs) and more general Faraday structures are key parameters for studying cosmic magnetism and are also sensitive probes of faint ionized thermal gas. A definition of which derived quantities are required for various scientific studies is needed, as well as addressing the challenges in determining Faraday structures. A wide variety of algorithms has been proposed to reconstruct these structures. In preparation for the Polarization Sky Survey of the Universe's Magnetism (POSSUM) to be conducted with the Australian Square Kilometre Array Pathfinder and the ongoing Galactic Arecibo L-band Feeds Array Continuum Transit Survey (GALFACTS), we run a Faraday structure determination data challenge to benchmark the currently available algorithms, including Faraday synthesis (previously called RM synthesis in the literature), wavelet, compressive sampling, and QU-fitting. The input models include sources with one Faraday thin component, two Faraday thin components, and one Faraday thick component. The frequency set is similar to POSSUM/GALFACTS with a 300 MHz bandwidth from 1.1 to 1.4 GHz. We define three figures of merit motivated by the underlying science: (1) an average RM weighted by polarized intensity, RM{sub wtd}, (2) the separation Δϕ of two Faraday components, and (3) the reduced chi-squared χ{sub r}{sup 2}. Based on the current test data with a signal-to-noise ratio of about 32, we find the following. (1) When only one Faraday thin component is present, most methods perform as expected, with occasional failures where two components are incorrectly found. (2) For two Faraday thin components, QU-fitting routines perform the best, with errors close to the theoretical ones for RM{sub wtd} but with significantly higher errors for Δϕ. All other methods, including standard Faraday synthesis, frequently identify only one component when Δϕ is below or near the width of the Faraday point-spread function. (3) No methods as currently implemented work well for Faraday thick components due to the narrow bandwidth. (4) There exist combinations of two Faraday components that produce a large range of acceptable fits and hence large uncertainties in the derived single RMs; in these cases, different RMs lead to the same Q, U behavior, so no method can recover a unique input model. Further exploration of all these issues is required before upcoming surveys will be able to provide reliable results on Faraday structures.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

The Acceleration of Energetic Particles at Coronal Shocks and Emergence of a Double Power-law Feature in Particle Energy Spectra

We present numerical modeling of particle acceleration at coronal shocks propagating through a streamer-like magnetic field by solving the Parker transport equation with spatial diffusion both along and across the magnetic field. We show that the location on the shock where the high-energy particle intensity is the largest, depends on the energy of the particles and on time. The acceleration of particles to more than 100 MeV mainly occurs in the shock-streamer interaction region, due to perpendicular shock geometry and the trapping effect of closed magnetic fields. A comparison of the particle spectra to that in a radial magnetic field shows that the intensity at 100 MeV (200 MeV) is enhanced by more than one order (two orders) of magnitude. This indicates that the streamer-like magnetic field can be an important factor in producing large solar energetic particle events. We also show that the energy spectrum integrated over the simulation domain consists of two different power laws. Further analysis suggests that it may be a mixture of two distinct populations accelerated in the streamer and open field regions, where the acceleration rate differs substantially. Our calculations also show that the particle spectra are affected considerably by a number of parameters, such as the streamer tilt angle, particle spatial diffusion coefficient, and shock compression ratio. While the low-energy spectra agree well with standard diffusive shock acceleration theory, the break energy ranges from ~1 MeV to ~90 MeV and the high-energy spectra can extend to ~1 GeV with a slope of ~2–3.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2024

Thermodynamic properties and enhancement of diamagnetism in nitrogen doped lutetium hydride synthesized at high pressure

Nitrogen doped lutetium hydride has drawn global attention in the pursuit of room-temperature superconductivity near ambient pressure and temperature. However, variable synthesis techniques and uncertainty surrounding nitrogen concentration have contributed to extensive debate within the scientific community about this material and its properties. We used a solid-state approach to synthesize nitrogen doped lutetium hydride at high pressure and temperature (HPT) and analyzed the residual starting materials to determine its nitrogen content. High temperature oxide melt solution calorimetry determined the formation enthalpy of LuH 1.96 N 0.02 (LHN) from LuH 2 and LuN to be −28.4 ± 11.4 kJ/mol. Magnetic measurements indicated diamagnetism which increased with nitrogen content. Ambient pressure conductivity measurements observed metallic behavior from 5 to 350 K, and the constant and parabolic magnetoresistance changed with increasing temperature. High pressure conductivity measurements revealed that LHN does not exhibit superconductivity up to 26.6 GPa. We compressed LHN in a diamond anvil cell to 13.7 GPa and measured the Raman signal at each step, with no evidence of any phase transition. Despite the absence of superconductivity, a color change from blue to purple to red was observed with increasing pressure. Thus, our findings confirm the thermodynamic stability of LHN, do not support superconductivity, and provide insights into the origins of its diamagnetism.

Science & Technology - Other Topics↗