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At least 721 records · Page 40
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Unravelling the radiation-induced redox chemistry of plutonium ions in aqueous solution

Plutonium plays a critical role in nuclear fuel cycle technologies, but our understanding of its fundamental radiation-induced redox chemistry is limited. Changes in oxidation states affect the speciation and transport of plutonium ions in solution. For example, solvent extraction techniques used to separate and recover plutonium from used nuclear fuel rely on the selective formation, maintenance, and complexation of specific plutonium oxidation states. However, radiolytically generated radicals, ions, and molecules can drive the oxidation state distribution of plutonium ions far from equilibrium, ultimately changing the physical and chemical properties of the bulk system. These radiation-induced processes are inevitable due to the ionizing radiation fields generated by the radioactive decay of plutonium and its daughter nuclides. Therefore, mechanistically understanding how plutonium's various oxidation states respond to ionizing radiation is essential for predicting its behavior in solution. Here, we present significant advances in our understanding of radiation-induced plutonium redox chemistry by using time-resolved (electron pulse) and dose accumulation (alpha and gamma) irradiation techniques, along with quantitative multiscale modeling methods.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2020

Dark matter through the quark vector current portal

We consider models of light dark matter coupled to quarks through a vector current interaction. For low energies, these models must be treated through the effective couplings to mesons, which are implemented here through the chiral Lagrangian. We find the rates of dark matter annihilation and decay to the light mesons, and find the expected photon spectrum from the decay of the hadrons. We compare to current and future observations, and show that there is a significant discovery reach for these models.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

TlSr 2 I 5 :Eu 2+ - A new high density scintillator for gamma-ray detection

In this paper we report on the scintillation properties of TlSr 2 I 5 doped with Eu 2+ , a novel thallium-containing high-resolution scintillator for gamma-ray spectroscopy. Here, small diameter, good quality crystals of TlSr 2 I 5 :Eu (TSI) with different Eu 2+ concentrations were grown by the vertical Bridgman method. X-ray diffraction measurements show that single crystals of TSI belong to the monoclinic system with space group P2 1 /c. TlSr 2 I 5 has a density of 5.32 g/cm 3 and effective Z of 60. The X-ray excited emission of Eu 2+ doped TlSr 2 I 5 features a broad emission band peaking between 460–470 nm. The light yield of TlSr 2 I 5 crystal doped with 1% Eu 2+ is measured to be ~72,000 ph/MeV with an energy resolution of 2.8% at 662 keV. The scintillation decay time which is characteristic of Eu 2+ shows two components, with 90% of the light in a ~500 ns component and the rest in a longer component of ~3 μs.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1979

Extraterrestrial high energy neutrino fluxes

Using the most recent cosmic ray spectra up to 2x10 to the 20th power eV, production spectra of high energy neutrinos from cosmic ray interactions with interstellar gas and extragalactic interactions of ultrahigh energy cosmic rays with 3K universal background photons are presented and discussed. Estimates of the fluxes from cosmic diffuse sources and the nearby quasar 3C273 are made using the generic relationship between secondary neutrinos and gammas and using recent gamma ray satellite data. These gamma ray data provide important upper limits on cosmological neutrinos. Quantitative estimates of the observability of high energy neutrinos from the inner galaxy and 3C273 above atmospheric background for a DUMAND type detector are discussed in the context of the Weinberg-Salam model with sq sin theta omega = 0.2 and including the atmospheric background from the decay of charmed mesons. Constraints on cosmological high energy neutrino production models are also discussed. It appears that important high energy neutrino astronomy may be possible with DUMAND, but very long observing times are required.

Stecker, F. W.↗
NASA NTRS2010

Statistical Properties of SGR J1550-5418 Bursts

Magnetars are slowly rotating neutron stars with extreme magnetic fields, over 10(exp 15) Gauss. Only few have been discovered in the last 30 years. These sources are dormant most of their lifetimes and become randomly active emitting multiple soft gamma-ray bursts. We present here our results on the temporal analysis of ~300 bursts from Soft Gamma Repeater SGR J1550-5418 recorded with the Gamma-ray Burst Monitor (GBM) onboard the Fermi Observatory during its activation on January 22-29, 2009. We employed an un-triggered burst search in the energy range 8-100keV to collect all events from the source, besides the ones that triggered GBM. For the entire sample of bursts we determined their durations, rise and decay times. We study here the statistical properties of these characteristics and discuss how these may help us better understand the physical characteristics of the magnetar model.

Gorgone, Nicholas M.↗
DOE OSTI2021

Neutron detection efficiency of the Neutron dEtector with Xn Tracking (NEXT)

An efficient neutron detection system with good energy resolution is required to correctly characterize decays of neutron-rich nuclei where β-delayed neutron emission is a dominant decay mode. The Neutron dEtector with Xn Tracking (NEXT) has been designed to measure β-delayed neutron emitters. By segmenting the detector along the neutron flight path, NEXT reduces the associated uncertainties in neutron time-of-flight measurements, improving energy resolution while maintaining detection efficiency. Detector prototypes are comprised of optically separated segments of a neutron-gamma discriminating plastic scintillator coupled to position-sensitive photomultiplier tubes. In this work we discuss how the first performance studies of this detector showed that high intrinsic neutron detection efficiency could be achieved while retaining good energy resolution. The results from the efficiency measurements using neutrons from direct reactions are presented

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Complete set of bound negative-parity states in the neutron-rich nucleus 18 N

High-resolution γ -ray spectroscopy of N 18 is performed with the Advanced GAmma Tracking Array, following deep-inelastic processes induced by an O 18 beam on a Ta 181 target. Six states are newly identified, which together with the three known excitations exhaust all negative-parity excited states expected in N 18 below the neutron threshold. Spin and parities are proposed for all located states on the basis of decay branchings and comparison with large-scale shell-model calculations performed in the p-sd space, with the YSOX interaction. Of particular interest is the location of the 0 1 - and 1 2 - excitations, which provide strong constrains for cross-shell p-sd matrix elements based on realistic interactions and help to simultaneously reproduce the ground and first-excited states in N 16 and N 18 , for the first time. Overall, understanding the N 18 structure may also have significant impact on neutron-capture cross-section calculations in r-process modeling including light neutron-rich nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Search for exclusive Higgs and Z boson decays to ωγ and Higgs boson decays to K*γ with the ATLAS detector

Searches for the exclusive decays of the Higgs boson to an ω meson and a photon or a Κ * meson and a photon can probe flavour-conserving and flavour-violating Higgs boson couplings to light quarks, respectively. Searches for these decays, along with the analogous Z boson decay to an ω meson and a photon, are performed with a pp collision data sample corresponding to integrated luminosities of up to 134 fb -1 collected at $\sqrt{s}$ = 13 TeV with the ATLAS detector at the CERN Large Hadron Collider. The obtained 95% confidence-level upper limits on the respective branching fractions are $\mathscr{B}$(H → ω$\gamma$) < 5.5 x 10 -4 , $\mathscr{B}$(H → Κ *$\gamma$) < 2.2 x 10 -4 and $\mathscr{B}$(Z → ω$\gamma$) 3.9 x 10 -6 . The limits for H → ω$\gamma$ and Z → ω$\gamma$ are 370 times and 140 times the Standard Model expected values, respectively. The result for Z → ω$\gamma$ corresponds to a two-orders-of-magnitude improvement over the limit obtained by the DELPHI experiment at LEP.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1984

Beta decay and the origin of biologial chirality - New experimental results

The hypothetical connection developed by Vester and Ulbricht (1959), between the handedness of beta particles in radioactive decay and the (L) sign of biologial chirality is investigated in a radiolysis experiment. The experiment measured the predicted asymmetry in the formation triplet or 'ortho-' positronium (oPs) in amino acid enantiomers by low energy positrons under conditions of helicity reversal. The positrons were focused on amino acid powder samples. By measuring the time between positron arrival and emission of gamma rays, long-lived oPs were separated from other species. It is found that the asymmetry in leucine (0.8 x 10 to the -4th) is consistent with the theoretical prediction of 10 to the -6th. Neither the experimental limits nor the theoretical estimates are found to rule out a mechanism like that described by Vester and Ulbricht as the cause of the sign of the observed chiral polarization.

Van House, J.↗
NASA NTRS2006

Gamma-ray Observations with Swift and their Impact on the TeV Community

The Swift gamma-ray burst explorer was launched on Nov. 20, 2004 from Cape Canaveral, Florida. The first instrument onboard became fully operational less than a month later. Since that time the Burst Alert Telescope (BAT) on Swift has detected more than 150 gamma-ray bursts (GRBs), most of which have also been observed within two minutes by the Swift narrow-field instruments: the X-Ray Telescope (XRT) and the Ultra-Violet and Optical Telescope (UVOT). Swift trigger notices are distributed worldwide within seconds of the trigger through the Gamma-ray burst Coordinates Network (GCN) and a substantial fraction of GRBs have been followed up by ground and space-based telescopes, ranging in wavelength from radio to TeV. Results have included the first rapid localization of a short GRB and further validation of the theory that short and long bursts have different origins; detailed observations of the power-law decay of burst afterglows leading to an improved understanding of the fireball and afterglow models; and detection of the most distant GRB ever found. Swift is also a sensitive X-ray observatory with capabilities to monitor galactic and extragalactic transients on a daily basis, carry out the first all-sky hard X-ray survey since HEAO-1, and study in detail the spectra of X-ray transients. The talk will emphasize the connection between Swift/BAT GRB observations and source monitoring and TeV observations.

Krimm, Hans↗
NASA NTRS2019

The Afterglow and Kilonova of the Short GRB 160821B

GRB 160821B is a short duration gamma-ray burst (GRB) detected and localized by the Neil Gehrels Swift Observatory in the outskirts of a spiral galaxy at z = 0.1613, at a projected physical offset of 16 kpc from the galaxy’s center. We present X-ray, optical/nIR, and radio observations of its counterpart and model them with two distinct components of emission: a standard afterglow, arising from the interaction of the relativistic jet with the surrounding medium, and a kilonova, powered by the radioactive decay of the sub-relativistic ejecta. Broadband modelling of the afterglow data reveals a weak reverse shock propagating backward into the jet, and a likely jet-break at 3.5 d. This is consistent with a structured jet seen slightly off-axis (θview ∼ θcore) while expanding into a low-density medium (n ≈ 10−3 cm−3). Analysis of the kilonova properties suggests a rapid evolution towards red colours, similar toAT2017gfo, and a low-nIR luminosity, possibly due to the presence of a long-lived neutron star. The global properties of the environment, the inferred low mass (Mej <~ 0.006 Msun) and velocities (vej >~ 0.05c) of lanthanide-rich ejecta are consistent with a binary neutron star merger progenitor.

Gravitational waves↗
DOE OSTI2022

A dispersive analysis of $$\varvec{\eta '\rightarrow \pi ^+\pi ^-\gamma }$$ and $$\varvec{\eta '\rightarrow \ell ^+\ell ^-\gamma }$$

Abstract We present a dispersive representation of the $$\eta '$$ η ′ transition form factor that allows one to account, in a consistent way, for the effects of $$\rho $$ ρ – $$\omega $$ ω mixing in both the isoscalar and the isovector contributions. Using this formalism, we analyze recent data on $$\eta '\rightarrow \pi ^+\pi ^-\gamma $$ η ′ → π + π - γ to constrain the isovector part of the form factor, individually and in combination with data for the pion vector form factor, which suggests a tension in the $$\rho $$ ρ – $$\omega $$ ω mixing parameter. As a first application, we use our results, in combination with the most recent input for the isoscalar part of the form factor, to predict the corresponding spectrum of $$\eta '\rightarrow \ell ^+\ell ^-\gamma $$ η ′ → ℓ + ℓ - γ , in particular we find the slope parameter $$b_{\eta '}=1.455(24)\,\text {GeV}^{-2}$$ b η ′ = 1.455 ( 24 ) GeV - 2 . With forthcoming data on the latter process, our results establish the necessary framework to improve the evaluation of the $$\eta '$$ η ′ -pole contribution to the anomalous magnetic moment of the muon using experimental input from both $$\eta '$$ η ′ decay channels.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1985

An internally consistent gamma ray burst time history phenomenology

A phenomenology for gamma ray burst time histories is outlined. Order of their generally chaotic appearance is attempted, based on the speculation that any one burst event can be represented above 150 keV as a superposition of similarly shaped increases of varying intensity. The increases can generally overlap, however, confusing the picture, but a given event must at least exhibit its own limiting characteristic rise and decay times if the measurements are made with instruments having adequate temporal resolution. Most catalogued observations may be of doubtful or marginal utility to test this hypothesis, but some time histories from Helios-2, Pioneer Venus Orbiter and other instruments having one-to several-millisecond capabilities appear to provide consistency. Also, recent studies of temporally resolved Solar Maximum Mission burst energy spectra are entirely compatible with this picture. The phenomenology suggested here, if correct, may assist as an analytic tool for modelling of burst processes and possibly in the definition of burst source populations.

Cline, T. L.↗
NASA NTRS1987

Shepherding of the Uranian rings. I - Kinematics. II - Dynamics

The possible kinematical relationships between the Uranian rings and all ten newly discovered satellites of Uranus are examined. Observational evidence is presented for interactions between 1986U7 and 1986U8 and the epsilon, delta, and gamma rings. The likelihood that these two satellites are shepherding the epsilon ring and are responsible for some of its internal structure is assessed, and the results are used to propose a reduction in the ring radius scale. It is also proposed that 1986U7 and 1986U8 are the inner and outer shepherds for the epsilon ring, that 1986U7 is the outer shepherd for the delta ring, and that 1986U8 is an outer shepherd for the gamma ring. The results of theoretical investigations of planetary ring dynamics are then applied to these associations, and their dynamical significance is evaluated. The resonant torques which the satellites exert on each ring are calculated and compared to the viscous torque which transports angular momentum outward through the ring and to the atmospheric-drag torque which causes the ring's orbit to decay.

Porco, Carolyn C.↗
NASA NTRS2018

Interplanetary Type II Radio Bursts from Wind/WAVES and Sustained Gamma-Ray Emission from Fermi/LAT: Evidence for Shock Source

We present quantitative evidence that interplanetary type II radio bursts and sustained gamma-ray emission (SGRE) events from the Sun are closely related. Out of about 30 SGRE events reported in Share et al. we consider 13 events that had a duration exceeding 5 hr to exclude any are-impulsive phase gamma-rays. The SGRE duration also has a linear relation with the ending frequency of the bursts. The synchronism between the ending times of SGRE and the type II emission strongly supports the idea that the same shock accelerates electrons to produce type II bursts and protons (>300 MeV) that propagate from the shock to the solar surface to produce SGRE via pion decay. The acceleration of high-energy particles is confirmed by the associated solar energetic particle (SEP) events detected at Earth and/or at the Solar Terrestrial Relations Observatory spacecraft. Furthermore, the presence of >300 MeV protons is corroborated by the fact that the underlying coronal mass ejections (CMEs) had properties identical to those associated with ground-level enhancement events: they had speeds of >2000 km s1 and all were full-halo CMEs. Many SEP events did not have detectable flux at Earth in the >300 MeV energy channels, presumably because of poor magnetic connectivity.

Gopalswamy, Nat↗
DOE OSTI2025

Extraction of the non-spin- and spin-transfer isovector responses via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B reaction

The isovector response in 12 B was investigated via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B* reaction at 100⁢𝐴MeV. By utilizing the 𝛾-decay properties of the 1.74 MeV 0 + and 0.718 MeV 1 + states in 10 B, the separate extraction of the non-spin-transfer (Δ⁢𝑆 = 0) and spin-transfer (Δ⁢𝑆 = 1) isovector responses up to an excitation energy of 50 MeV in 12 B in a single measurement is demonstrated. The experimental setup employed the S800 spectrometer to detect and analyze the 10 B ejectiles and the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA) for obtaining the Doppler-reconstructed spectrum for 𝛾 rays emitted in flight by 10 B. A 12 C foil was placed at the pivot point of the spectrograph. Here, the 12 B reaction product was not detected. Contributions from transitions associated with the transfer of different units of angular momentum in the non-spin- and spin-transfer responses were analyzed using a multipole decomposition analysis. The extracted non-spin-dipole (Δ⁢𝑆 = 0, Δ⁢𝐿 = 1) and spin-dipole (Δ⁢𝑆 = 1, Δ⁢𝐿 = 1) responses were found to be consistent with available data from other charge-exchange probes, validating the non-spin- and spin-transfer filters used. While statistical uncertainties and experimental resolutions were relatively large due to the modest intensity of the 10 Be secondary beam, the results show that, with the much higher intensities that will be available at new rare-isotope beam facilities, the ( 10 Be, 10 B + 𝛾) reaction and its Δ⁢𝑇 𝑧 = −1 partner, the ( 10 C, 10 B + 𝛾) reaction, are powerful tools for elucidating the isovector non-spin- and spin-transfer responses in nuclei.

Charge-exchange reactions↗
DOE OSTI2023

The 100-month Swift catalogue of supergiant fast X–ray transients

Supergiant fast X-ray transients (SFXTs) are high mass X-ray binaries (HMXBs) displaying X-ray outbursts that can reach peak luminosities up to 10 38 erg s -1 and spend most of their lives in more quiescent states with luminosities as low as 10 32 -10 33 erg s -1 . During the quiescent states, less luminous flares are also frequently observed with luminosities of 10 34 -10 35 erg s -1 . The main goal of the comprehensive and uniform analysis of the SFXT Swift triggers presented in this paper is to provide tools to predict whether a transient that has no known X-ray counterpart may be an SFXT candidate. These tools can be exploited for the development of future missions exploring the variable X-ray sky through large field-of-view instruments. We examined all available data on outbursts of SFXTs that triggered the Swift/Burst Alert Telescope (BAT) collected between 2005 August 30 and 2014 December 31, in particular those for which broad-band data, including the Swift/X-ray Telescope (XRT) data, are also available. This work complements and extends our previous catalogue of SFXT flares detected by BAT from 2005 February 12 to 2013 May 31, since we now include the additional BAT triggers recorded until the end of 2014 (i.e. beyond the formal first 100 months of the Swift mission). Due to a change in the mission’s observational strategy, virtually no SFXT triggers obtained a broad-band response after 2014. We processed all BAT and XRT data uniformly by using the Swift Burst Analyser to produce spectral evolution dependent flux light curves for each outburst in the sample. The BAT data allowed us to infer useful diagnostics to set SFXT triggers apart from the general γ-ray burst population, showing that SFXTs uniquely give rise to image triggers and are simultaneously very long, faint, and ‘soft’ hard-X-ray transients. We find that the BAT data alone can discriminate very well the SFXTs from other classes of fast transients, such as anomalous X-ray pulsars and soft gamma repeaters. On the contrary, the XRT data collected around the time of the BAT triggers are shown to be decisive for distinguishing SFXTs from, for instance, accreting millisecond X-ray pulsars and jetted tidal disruption events. The XRT observations of 35 (out of 52 in total) SFXT BAT triggers show that in the soft X-ray energy band, SFXTs display a decay in flux from the peak of the outburst of at least three orders of magnitude within a day and rarely undergo large re-brightening episodes, favouring in most cases a rapid decay down to the quiescent level within three to five days (at most).

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1985

Evidence for long-term variability in the ultra high energy photon flux from Cygnus X-3

A time-correlation analysis of atmospheric Cerenkov pulses by a wide-angle photomultiplier system was previously shown to have present in it a nonrandom component which seemed associated with the Right Ascension (RA) range approx. 20+or-04h. A recent examination of multi-muon events recorded by a photon-decay detector shows a similar time-dependent effect, closely matching the previous results, supporting the suggestion that the effect is of cosmic origin. However, even though Cyg. X-3 lies well inside the region of peak intensity, it does not seem possible to ascribe to it the whole effect, for the implied photon flux appears too large to be reconciled to various gamma-ray measurements of Cyg. X-3. The original data were subjected to a phase-histogram analysis and it as found that only 2.5% of overall recorded data are compatible with a phase-dependent emission from Cyg. X-3. Assuming these events to be gamma rays yields a detected flux of (2.6 + or - 0.3) x 10 to the minus 12th power gamma cm -2s-1 above 5 x 10 to the 14th power eV. Comparing this value with more recent ultra high energy (UHE) photon data from the same source, it is suggested that the available data generally favor a long-term reduction in the Cyg. X-3 inferred luminosity ( 10 to the 13th power eV) by a factor of (1.8 + or - 0.3) per year.

Bhat, C. L.↗