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At least 721 records · Page 40

Report on Preliminary Detailed Experimental Plan for Neutron Irradiation of A709 at ATR and HFIR

Advanced nuclear power technologies will use higher temperatures as a means to extract energy at a higher efficiency than current plants and therefore put a larger demand on the structural materials. Improved performance of structural materials could enable greater safety margins, longer plant lifetimes, and reduce maintenance costs. Alloy 709 is championed as the next generation of austenitic alloys for advanced nuclear reactors. In parallel to the ASME code case pursued, the AMMT program is initiating a neutron irradiation campaign to provide first-of-a-kind engineering data to establish operational design parameters and how the mechanical response is modified by environmental factors. This document refines the AMMT neutron irradiation campaign to a 4 year program to support the generation of creep knockdown factors for Alloy 709 and welded Alloy 709. The campaign is divided among two national laboratories, Oak Ridge National Laboratory and Idaho National Laboratory, to use the strengths of each laboratory. Through a cooperative plan, time-independent properties and time-dependent properties will be obtained across a large temperature window, nominally 300°C to 800°C, damage levels up to 10 dpa, and with and without the impacts of transmutation produced helium.

99 GENERAL AND MISCELLANEOUS↗

Report on Preliminary Detailed Experimental Plan for Neutron Irradiation of A709 at ATR and HFIR

Advanced nuclear power technologies will use higher temperatures as a means to extract energy at a higher efficiency than current plants and therefore put a larger demand on the structural materials. Improved performance of structural materials could enable greater safety margins, longer plant lifetimes, and reduce maintenance costs. Alloy 709 is championed as the next generation of austenitic alloys for advanced nuclear reactors. In parallel to the ASME code case pursued, the AMMT program is initiating a neutron irradiation campaign to provide first-of-a-kind engineering data to establish operational design parameters and how the mechanical response is modified by environmental factors. This document refines the AMMT neutron irradiation campaign to a 4 year program to support the generation of creep knockdown factors for Alloy 709 and welded Alloy 709. The campaign is divided among two national laboratories, Oak Ridge National Laboratory and Idaho National Laboratory, to use the strengths of each laboratory. Through a cooperative plan, time-independent properties and time-dependent properties will be obtained across a large temperature window, nominally 300°C to 800°C, damage levels up to 10 dpa, and with and without the impacts of transmutation produced helium.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

KJRR FUEL (U-7MO) QUALIFICATION PLAN AND ITS STATUS

In order to cope with global shortage of Mo-99 supplies and with growing demand of neutron transmutation doping, KJRR construction plan has been launched since April 2012 to provide self-sufficiency of domestic RI demand, and to extend Si doping capacity for power device market growth. Through comprehensive surveillance of the fuel’s in-reactor behavior, KAERI has selected the fuel meat of U-7%Mo/Al-5%Si since Molybdenum contents in fuel more than 6% showed a stable and good irradiation behavior in-reactor. As part of efforts for fuel qualification of the KJRR fuel, 16 mini-plates irradiation program and PIE designated as HAMPs (HAnaro Mini-Plate Irradiations) are planned to supplement the irradiation and PIE data to be obtained from an LTA irradiation and PIE at the ATR. This paper focuses on the plan and current on-going status of KJRR U-Mo fuel qualification.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Post-irradiation Examination Plan for ORNL and University of California Santa Barbara Assessment of UCSB ATR-2 Irradiation Experiment

New and existing databases will be combined to support development of physically based models of transition temperature shifts (TTS) for high fluence-low flux (φ < 10 11 n/cm 2 -s) conditions, beyond the existing surveillance database, to neutron fluences of at least 1×10 20 n/cm 2 (>1 MeV). All references to neutron flux and fluence in this report are for fast neutrons (>1 MeV). The reactor pressure vessel (RPV) task of the Light Water Reactor Sustainability (LWRS) Program is working with various organizations to obtain archival surveillance materials from commercial nuclear power plants to allow for comparisons of the irradiation-induced microstructural features from reactor surveillance materials with those from similar materials irradiated under high flux conditions in test reactors

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Effects of fuel thickness on thermal and mechanical performance of U10-Mo monolithic fuel plates

Monolithic fuels are being considered for conversion of high performance research and test reactors. These plate-type fuels are comprised of a low enrichment, high density U-Mo alloy fuels within an aluminum cladding. Although the plates have demonstrated satisfactory performance; still, use of a high density fuel in a foil form retains technical challenges that could affect the overall performance. To understand performance of this new design during fabrication and irradiation, the plates have been evaluated for various geometrical and operational variables. As a part of these set of parametric sensitivity studies, effects of foil thickness on performance were studied. Because high performance research reactors will utilize different fuel thicknesses, it is necessary to evaluate possible effects for a range of thicknesses that are being considered for various designs. Based on the preliminary design specifications, the fuel thicknesses were varied between the limiting cases. The bounding fuel thicknesses were 0.203 mm as minimum that is projected for ATR, and 0.635 mm as maximum that is projected for MITR. To study possible effects, a behavioral model was developed for a selected plate from RERTR-12 experiments and the plate was simulated with as run irradiation history. The simulations were repeated for a range of fuel thicknesses, while keeping the cladding thickness and the operational parameters the same. The results have indicated that the plates with thicker fuels would have higher temperatures, deformations and shutdown stresses. To investigate the effects of fuel thickness exclusively, operational parameters were scaled. In particular, a second set of simulations with prorated volumetric heat generation rates were performed. The results indicated that the fabrication stresses in the fuel foil decrease with an increasing fuel thickness. On contrary, irradiation stresses of the fuel at shutdown are higher for the plates with thicker fuels. Greater peak deformations occurred in plates with thicker fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Drawing 445754 rev5

Drawing 445754 contains the details for fabricating plastic flux wands used in ATR and ATRC. The flux wands are used to position flux wires in fuel elements. The flux wands are basically a tool to position the flux wires. The flux wires are later removed from the flux wands and counted to determine the amount of flux they received. The flux wands come in contact with reactor primary coolant, but do not control the primary coolant (this is in reference to 10 CFR Part 810). Additional wands need to be fabricated. This drawing needs to be sent to a vendor or vendors for procurement of new flux wands as done in the past. LWP-11201 rev 11 (pg. 27) indicates providing information to a vender is not a public release. This drawing does not need to be released to all of the public if that is an option. It just needs to go to a vendors or vendors. A vendor will likely need to see the drawing to determine if they can build the flux wands.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Cable aging and condition monitoring of radiation resistant nano-dielectrics in advanced reactor applications

Cross-linked polyethylene (XLPE) nanocomposites have been developed in an effort to improve cable insulation lifetime to serve in both instrument cables and auxiliary power systems in advanced reactor applications as well as to provide an alternative for new or retro-fit cable insulation installations. Nano-dielectrics composed of different weight percentages of MgO & SiO 2 have been subjected to radiation at accumulated doses approaching 20 MRad and thermal aging temperatures exceeding 100 C. Depending on the composition, the performance of the nanodielectric insulation was influenced, both positively and negatively, when quantified with respect to its electrical and mechanical properties. For virgin unradiated or thermally aged samples, XLPE nanocomposites with 1wt.% SiO 2 showed improvement in breakdown strength and reduction in its dissipation factor when compared to pure undoped XLPE, while XLPE 3wt.% SiO 2 resulted in lower breakdown strength. When aged in air at 120 C, retention of electrical breakdown strength and dissipation factor was observed for XLPE 3wt.% MgO nanocomposites. Irrespective of the nanoparticle species, XLPE nanocomposites that were gamma irradiated up to the accumulated dose of 18 MRad showed a significant drop in breakdown strength especially for particle concentrations greater than 3 wt.%. Additional attenuated total reflectance Fourier transform infrared (ATR-FTIR) spectroscopy measurements suggest changes in the structure of the XLPE SiO 2 nanocomposites associated with the interaction of silicon and oxygen. Discussion on the relevance of property changes with respect to cable aging and condition monitoring is presented.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Modeling of SRS Aluminum-clad Spent Nuclear Fuel in Standard DOE Sealed Canisters

At the Savannah River Site (SRS), approximately 7 MTHM of aluminum-clad spent nuclear fuel is currently in wet storage at L-basin. A significant portion of this fuel is slated to be dried and sealed in DOE standard canisters for long-term storage. This report will focus on a few fuel types, which should bound all other fuel stored at SRS. These consist of the reference fuel assembly, the MURR fuel and the HFIR fuel. These bound a hypothetical maximum scenario for MTR box fuel, a maximum for decay heat in an assembly, and a maximum for the aluminum surface area, respectively. The geometry for the packages were created from DOE specifications for storage of each of the fuels. As long as the minimum time from reactor discharge to sealed storage is 3 years, then the highest temperatures which occur within the sealed canisters do not exceed 100° C for all scenarios considered here. In the geometry considered, while the HFIR fuel has a large surface area, the packaging configuration leaves large void areas, such that the aluminum surface to free volume ratio is about 30% less than an ATR or MURR packaging configuration.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The effect of phosphorus on precipitation in irradiated reactor pressure vessel (RPV) steels

Embrittlement of light water reactor pressure vessels (RPV) steels by fast neutron irradiation may limit extended nuclear plant life. Embrittlement, which is manifested as increases in various indexes of a ductile to brittle transition temperatures (ΔT), is primarily due to hardening by nanoscale precipitates containing Cu, Ni, Mn, and Si, which form under irradiation. In addition to these elements, P has also been found to play a role in embrittlement. While only slightly enriched in the precipitates, hardening and embrittlement increase with trace P concentrations in low-Cu steels. Here, we characterize the individual and synergistic irradiation precipitation and hardening mechanisms in a series of RPV steels containing no to low-Cu and with systematic variations in Ni and P. In this study, the steels were irradiated to a fluence of ~ 1.38 x 10 20 n/cm 2 at ~ 292 °C in the UCSB ATR-2 experiment. In Cu-free medium and high-Ni RPV steels, atom probe tomography shows that P and Ni promotes precipitation of P-Mn-Si-Ni and Mn-Si-Ni precipitates, respectively. The precipitate microstructure correlates with the observed irradiation hardening.

36 MATERIALS SCIENCE↗

Conceptual Design Report for the I2 Instrumentation Experiment in ATRC

The US Department of Energy In-Pile Instrumentation (I2) program is tasked with developing advanced sensors for in-pile service as well as supporting the engineering required to implement existing nuclear sensor technologies in US high-power test reactors. The ATRC instrumentation test has been conceived to address both of these missions, specifically with respect to neutron flux measurements. Space has been allocated in the test for Self-Powered Neutron Detectors (SPNDs), fission chambers, and Micro-Pocket Fission Detectors (MPFDs). The real-time flux readings obtained from these instruments will be compared with time integrated data obtained from passive neutron dosimetry (i.e., “flux” wires). This work will be complementary to data obtained from the TREAT MIMIC-N experiment. This experiment is expected to support instrumentation efforts related to the proposed Medium-I loop and to instrumenting loop experiments conducted in the ATR center flux trap. While the MIMIC-N experiment was conducted in a dry environment, the ATRC I-19 experiment will be conducted in an aqueous environment, similar to the center flux trap loop experiments but will take place at ambient temperature and pressure, and at a much lower neutron flux. One of the challenges of the ATRC I-19 experiment will be low amplitude signals produced by the sensors in the low neutron fluxes of ATRC. However, related work conducted several years ago in ATRC was able to reliably detect signals using a similar instrument set.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Probabilistic Analysis of Uncertainty in ATRC Flux Profiles

ATRC is a replica of the larger ATR design and is used to conduct research and obtain data such as flux measurements, excess reactivity, and loading requirements before being loaded into ATR. One method for determining the impact an experiment will have at ATR is by looking at the axial flux profile along the fuel rod in the corresponding ATRC experiment; however, flux wand measurements includes large amounts of variation which makes drawing conclusions from the data difficult. This poster describes a definitive method to propagate the uncertainty from ATRC measurements using Python code.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Advanced Test Reactor Long-Term Asset Management Accomplishments 2016 to 2022

Advanced Test Reactor Long-Term Asset Management Accomplishments report contains photographs and information on completed projects or completed phase of a project for 2022. This book will be presented for the year-end report in Washington, D.C. as well as delivered to our clients at the Navy Nuclear Laboratory.

99 GENERAL AND MISCELLANEOUS↗

2013 Radiological Monitoring Results Associated with the Advanced Test Reactor Complex Cold Waste Pond

This report summarizes radiological monitoring performed of the Idaho National Laboratory Site’s Advanced Test Reactor Complex Cold Waste wastewater prior to discharge into the Cold Waste Pond and of specific groundwater monitoring wells associated with the Industrial Wastewater Reuse Permit (#LA-000161-01, Modification B). All radiological monitoring is performed to fulfill Department of Energy requirements under the Atomic Energy Act.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

AGC-4 As-Run Uncertainty Analysis

The concept of measuring neutron flux (or fluence rate) with activation foils has existed since the late 1940s and is a well-used methodology. Activation foils are selected for their unique isotopic cross sections that create reaction products with desirable properties: relatively simple radioactive decay scheme, measurable quantities of gamma-rays or betas, and half-lives appropriate for the irradiation and decay durations of the experiment. The activation materials, deemed flux wires, fluence wires, dosimeters, or flux foils, are fabricated to have a mass appropriate for the irradiation as well so the measurement using a radiation detector following the irradiation is sufficient but not overwhelming in terms of total activity. Activation measurement results are expressed in terms of reaction rate, which can then be used to “adjust” the neutron spectrum. The Advanced Graphite Creep (AGC)-4 experiment contained 26 flux wire packages, each containing an iron and a niobium wire inside a vanadium capsule. For all stackup positions, the value of fast to thermal neutrons is higher than expected, but the total neutron fluence is near the predicted value of ~2 x 1022 n/cm2. As compared to the predicted neutron spectrum, there are four takeaways in the results as compared to the predicted ATR irradiation: 1) Additional fast (fission) neutrons present, 2) Spectrum hardening due to temperature, 3) Spectrum hardening due to container attenuation, 4) Total neutron fluence is close to predicted values. Since the neutron energy spectrum is a key parameter when attributing neutron damage in materials, the adjusted energy-dependent spectrum and the total neutron fluence results from the dosimeters can be incorporated for future calculations.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗