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NASA NTRS1978

Stratospheric aerosols and climatic change

Stratospht1ic sulfuric acid particles scatter and absorb sunlight and they scatter, absorb and emit terrestrial thermal radiation. These interactions play a role in the earth's radiation balance and therefore affect climate. The stratospheric aerosols are perturbed by volcanic injection of SO2 and ash, by aircraft injection of SO2, by rocket exhaust of Al2O3 and by tropospheric mixing of particles and pollutant SO2 and COS. In order to assess the effects of these perturbations on climate, the effects of the aerosols on the radiation balance must be understood and in order to understand the radiation effects the properties of the aerosols must be known. The discussion covers the aerosols' effect on the radiation balance. It is shown that the aerosol size distribution controls whether the aerosols will tend to warm or cool the earth's surface. Calculations of aerosol properties, including size distribution, for various perturbation sources are carried out on the basis of an aerosol model. Calculations are also presented of the climatic impact of perturbed aerosols due to volcanic eruptions and Space Shuttle flights.

Toon, O. B.↗

NASA NTRS1982

Stratospheric aerosols - Observation and theory

Important chemical and physical roles of aerosols are discussed, and properties of stratospheric aerosols as revealed by experimental data are described. In situ measurements obtained by mechanical collection and scattered-light detection yield the overall size distribution of the aerosols, and analyses of preserved aerosol precursor gases by wet chemical, cryogenic and spectroscopic techniques indicate the photochemical sources of particle mass. Aerosol chemical reactions including those of gaseous precursors, those in aqueous solution, and those on particle surfaces are discussed, in addition to aerosol microphysical processes such as nucleation, condensation/evaporation, coagulation and sedimentation. Models of aerosols incorporating such chemical and physical processes are presented, and simulations are shown to agree with measurements. Estimates are presented for the potential aerosol changes due to emission of particles and gases by aerospace operations and industrial consumption of fossil fuels, and it is demonstrated that although the climatic effects of existing levels of stratospheric aerosol pollution are negligible, potential increases in those levels might pose a future threat.

Turco, R. P.↗

NASA NTRS1992

Raman lidar measurements of Pinatubo aerosols over southeastern Kansas during November-December 1991

Raman lidar measurements over southeastern Kansas of stratospheric aerosols produced by the June 1991 eruptions of Mt. Pinatubo were made on 10 nights during November and December 1991. Both aerosol backscattering and extinction profiles were derived simultaneously from the lidar data since this system detects Raman scattering from nitrogen and oxygen as well as the backscattered light from aerosols and molecules. Aerosols scattering ratios greater than 3(at 351 nm) were measured on several nights. Peak aerosol concentrations were located between 19-22 km and varied significantly from night to night. Aerosol extinction/backscatter ratios computed from the lidar data and averaged over the altitude region of enhanced aerosol scattering between 15-25 km varied between 18-28 sr. Mie computations show these values to be consistent with scattering by aerosol particles with mode radii between 0.3 to 0.5 micron and that the ratios would increase to 40-65 sr at 694 nm. Aerosol optical thicknesses derived from the lidar extinction measurements at 351 nm varied between 0.04 and 0.06.

Ferrare, R. A.↗

NASA NTRS1992

Climate forcing by stratospheric aerosols

It is illustrated how climate forcing by stratospheric aerosols depends on aerosol properties. The climate forcing is a function of aerosols size distribution, but the size dependence can be described well by a single parameter: the area-weighted mean radius, r(eff). If r(eff) is greater than about 2 microns, the global average greenhouse effect of the aerosols exceeds the albedo effect, causing a surface heating. The aerosol climate forcing is less sensitive to other characteristics of the size distribution, the aerosol composition, and the altitude of the aerosols. Thus stratospheric aerosol forcing can be defined accurately from measurements of aerosol extinction over a broad wavelength range.

Lacis, Andrew↗

NASA NTRS1993

Review of recent research on the climatic effect of aerosols

A review of recent research on the climatic effects of aerosols is presented. A representative aerosol and climate models were used to study the generation, growth transport, and removal of aerosols. The structure of the radiative-convective models and general circulation models used is described. Large-scale temperature effects, effects on clouds, and local urban effects of trophospheric aerosols are examined. The effects of volcanic eruptions and stratospheric aerosols are also considered. Results indicate that solar radiation backscatter by aerosols increases the planetary albedo. Solar radiation absorption may offset cooling caused by aerosol backscatter but the absorption and emission of terrestrial radiation by aerosols produces a warming effect. It appears that the role of aerosols as cloud condensation nuclei is probably the most significant cause of the radiative effects observed.

Charlock, Thomas P.↗

NASA NTRS1993

Transport and residence times of tropospheric aerosols inferred from a global three-dimensional simulation of Pb-210

A global three-dimensional model is used to investigate the transport and tropospheric residence time of Pb-210, an aerosol tracer produced in the atmosphere by radioactive decay of Rn-222 emitted from soils. The model uses meteorological input with 4 deg x 5 deg horizontal resolution and 4-hour temporal resolution from the Goddard Institute for Space Studies general circulation model (GCM). It computes aerosol scavenging by convective precipitation as part of the wet convective mass transport operator in order to capture the coupling between vertical transport and rainout. Scavenging in convective precipitation accounts for 74% of the global Pb-210 sink in the model; scavenging in large-scale precipitation accounts for 12%, and scavenging in dry deposition accounts for 14%. The model captures 63% of the variance of yearly mean Pb-210 concentrations measured at 85 sites around the world with negligible mean bias, lending support to the computation of aerosol scavenging. There are, however, a number of regional and seasonal discrepancies that reflect in part anomalies in GCM precipitation. Computed residence times with respect to deposition for Pb-210 aerosol in the tropospheric column are about 5 days at southern midlatitudes and 10-15 days in the tropics; values at northern midlatitudes vary from about 5 days in winter to 10 days in summer. The residence time of Pb-210 produced in the lowest 0.5 km of atmosphere is on average four times shorter than that of Pb-210 produced in the upper atmosphere. Both model and observations indicate a weaker decrease of Pb-210 concentrations between the continental mixed layer and the free troposphere than is observed for total aerosol concentrations; an explanation is that Rn-222 is transported to high altitudes in wet convective updrafts, while aerosols and soluble precursors of aerosols are scavenged by precipitation in the updrafts. Thus Pb-210 is not simply a tracer of aerosols produced in the continental boundary layer, but also of aerosols derived from insoluble precursors emitted from the surface of continents. One may draw an analogy between Pb-210 and nitrate, whose precursor NO(sub x) is sparingly soluble, and explain in this manner the strong correlation observed between nitrate and Pb-210 concentrations over the oceans.

Balkanski, Yves J.↗

NASA NTRS1993

The impact of the eruptions of Mount Pinatubo and Cerro Hudson on antarctic aerosol levels during the 1991 austral spring

At the beginning of the 1991 Austral spring, volcanic aerosols from Mt. Pinatubo and Cerro Hudson were present in the polar stratosphere of the Southern Hemisphere. Satellite observations of aerosol extinction were used to identify and track the movement of these aerosols in the vicinity of the Antarctic vortex during August through November 1991. A layer of mature Mt. Pinatubo aerosols was identified near 21 km and a layer of fresh Cerro Hudson aerosols was identified near 12 km. This altitude separation of the Mt. Pinatubo and Cerro Hudson aerosols was observed throughout the period. Below 15 km, the polar stratosphere was subject to episodes of strong wave activity which transported the Cerro Hudson aerosols poleward and, after the middle of September, they became a persistent feature beneath the vortex. Above 15 km, signatures of Mt. Pinatubo aerosols were observed near the vortex boundary, but significant portions of the vortex interior remained free of any detectable intrusions of Mt. Pinatubo aerosols until the final warming in mid-November.

Pitts, M. C.↗

NASA NTRS1994

Mid-infrared extinction by sulfate aerosols from the Mt. Pinatubo eruption

Quantitative measurements of the wavelength dependence of aerosol extinction in the 750-3400/cm spectral region have been derived from 0.01/cm resolution stratospheric solar occultation spectra recorded by the ATMOS (Atmospheric Trace Molecule Spectroscopy) Fourier transform spectrometer about 9 1/2 months after the Mt Pinatubo volcanic eruption. Strong, broad aerosol features have been identified near 900, 1060, 1190, 1720, and 2900/cm below a tangent height of approximately 30 km. Aerosol extinction measurements derived from approximately 0.05/cm wide microwindows nearly free of telluric line absorption in the ATMOS spectra are compared with transmission calculations derived from aerosol size distribution profiles retrieved from correlative SAGE (Stratospheric Aerosol and Gas Experiment) II visible and near i.r. extinction measurements, seasonal and zonally averaged H2SO4 aerosol weight percentage profiles, and published sulfuric acid optical constants derived from room temperature laboratory measurements. The calculated shapes and positions of the aerosol features are generally consistent with the observations, thereby confirming that the aerosols are predominantly concentrated H2SO4-H2O droplets, but there are significant differences between the measured and calculated wavelength dependences of the aerosol extinction. We attribute these differences as primarily the result of errors in the calculated low temperature H2SO4-H2O optical constants. Errors in both the published room temperature optical constants and the limitations of the Lorentz-Lorenz relation are likely to be important.

Rinsland, C. P.↗

NASA NTRS1997

Simultaneous Retrieval of Multiple Aerosol Parameters Using a Multi-Angular Approach

Atmospheric aerosol particles, both natural and anthropogenic, are important to the earth's radiative balance through their direct and indirect effects. They scatter the incoming solar radiation (direct effect) and modify the shortwave reflective properties of clouds by acting as cloud condensation nuclei (indirect effect). Although it has been suggested that aerosols exert a net cooling influence on climate, this effect has received less attention than the radiative forcing due to clouds and greenhouse gases. In order to understand the role that aerosols play in a changing climate, detailed and accurate observations are a prerequisite. The retrieval of aerosol optical properties by satellite remote sensing has proven to be a difficult task. The difficulty results mainly from the tenuous nature and variable composition of aerosols. To date, with single-angle satellite observations, we can only retrieve reliably against dark backgrounds, such as over oceans and dense vegetation. Even then, assumptions must be made concerning the chemical composition of aerosols. The best hope we have for aerosol retrievals over bright backgrounds are observations from multiple angles, such as those provided by the MISR and POLDER instruments. In this investigation we examine the feasibility of simultaneous retrieval of multiple aerosol optical parameters using reflectances from a typical set of twelve angles observed by the French POLDER instrument. The retrieved aerosol optical parameters consist of asymmetry factor, single scattering albedo, surface albedo, and optical thickness.

Kuo, K. S.↗

NASA NTRS1997

A Modified Linear-Mixing Method for Calculating Atmospheric Path Radiances of Aerosol Mixtures

The top-of-atmosphere (TOA) path radiance generated by an aerosol mixture can be synthesized by linearly adding the contributions of the individual aerosol components, weighted by their fractional optical depths. The method, known as linear mixing, is exact in the single-scattering limit. When multiple scattering is significant, the method reproduces the atmospheric path radiance of the mixture with less than 3% errors for weakly absorbing aerosols up to optical thickness of 0.5. However, when strongly absorbing aerosols are included in the mixture, the errors are much larger. This is due to neglecting the effect of multiple interactions between the aerosol components, especially when the values of the single-scattering albedos of these components are so different that the parameter epsilon = (Sigma)f(sub i) absolute value of bar omega(sub i) - bar omega(sub mix)/bar omega(sub i), is larger than approx. 0.1, where bar omega(sub i) and f(sub i) are the single-scattering albedo and the fractional abundance of the i th component, and bar omega(sub i) is the effective single-scattering albedo of the mixture. We describe an empirical, modified linear-mixing method which effectively accounts for the multiple interactions between aerosol components. The modified and standard methods are identical when epsilon = 0.0 and give similar results when epsilon less than or equal to 0.05. For optical depths larger than approx. 0.5, or when epsilon greater than 0.05, only the modified method can reproduce the radiances within 5% error for common aerosol types up to optical thickness of 2.0. Because this method facilitates efficient and accurate atmospheric path radiance calculations for mixtures of a wide variety of aerosol types, it will be used as part of the aerosol retrieval methodology for the Earth Observing System (EOS) multiangle imaging spectroradiometer (MISR), scheduled for launch into polar orbit in 1998.

Abdou, W. A.↗

NASA NTRS1997

A Modified Linear-Mixing Method for Calculating Atmospheric Path Radiances of Aerosol Mixtures

The top-of-atmosphere (TOA) path radiance generated by an aerosol mixture can be synthesized by linearly adding the contributions of the individual aerosol components, weighted by their fractional optical depths. The method, known as linear mixing, is exact in the single-scattering limit. When multiple scattering is significant, the method reproduces the atmospheric path radiance of the mixture with less than 3% errors for weakly absorbing aerosols up to optical thickness of 0.5. However, when strongly absorbing aerosols are included in the mixture, the errors are much larger. This is due to neglecting the effect of multiple interactions between the aerosol components, especially when the values of the single-scattering albedos of these components are so different that the parameter e = the sum of f(sub i)[(bar)omega(sub i) - (bar)omega(sub mix)]/(bar)omega(sub i) is larger than approximately 0.1, where (bar)omega(sub i)and f(sub i) are the single-scattering albedo and the fractional abundance of the ith component, and (bar)omega(sub mix) is the effective single-scattering albedo of the Mixture. We describe an empirical, modified linear-mixing method which effectively accounts for the multiple interactions between aerosol components. The modified and standard methods are identical when epsilon = 0.0 and give similar results when epsilon is less than or equal to 0.05. For optical depths larger than approximately 0.5, or when epsilon is greater than 0.05, only the modified method can reproduce the radiances within 5% error for common aerosol types up to optical thickness of 2.0. Because this method facilitates efficient and accurate atmospheric path radiance calculations for mixtures of a wide variety of aerosol types, it will be used as part of the aerosol retrieval methodology for the Earth Observing System (EOS) multiangle imaging spectroradiometer (MISR), scheduled for launch into polar orbit in 1998.

Abdou, W. A.↗

NASA NTRS1998

A Multi-Instrument Approach for Characterizing the Vertical Structure of Aerosol Properties: Case Studies in the Pacific Basin Troposphere

During February/March 1994, a series of aircraft-based aerosol measurements were carried out in the Pacific Basin troposphere using a differential absorption lidar system deployed by NASA Langley, and optical spectrometer probes and a wire-impactor system operated by NASA Ames. A modified Klett inversion algorithm was applied to extract altitude profiles of aerosol backscattering from the IR lidar signal. The algorithm that we have designed for this purpose utilizes the in situ aerosol measurements to normalize the lidar profile at the aircraft altitude and to supply the lidar ratio as a function of height. The lidar-derived aerosol backscattering coefficients were then compared to the backscattering coefficients calculated from the in situ measurements. During several local aircraft descents, we found good agreement between the remote lidar and in situ results for the absolute value of the aerosol backscattering coefficient and its altitude variation only when we allowed for several layers with different aerosol refractive indices. The agreement validates our lidar calibration method and provides an indication of the variation in aerosol refractive index as a function of altitude. Two of the three case studies performed in this paper reveal layers of anthropogenic aerosols transported long distances into the Pacific Basin troposphere. A third case implies the existence of a layer of dustlike aerosol particles in the lower troposphere, most likely of Asian origin.

Redemann, J.↗

NASA NTRS1999

Global Observations of Aerosols and Clouds from Combined Lidar and Passive Instruments to Improve Radiation Budget and Climate Studies

Current uncertainties in the effects of clouds and aerosols on the Earth radiation budget limit our understanding of the climate system and the potential for global climate change. Pathfinder Instruments for Cloud and Aerosol Spaceborne Observations - Climatologie Etendue des Nuages et des Aerosols (PICASSO-CENA) is a recently approved satellite mission within NASA's Earth System Science Pathfinder (ESSP) program which will address these uncertainties with a unique suite of active and passive instruments. The Lidar In-space Technology Experiment (LITE) demonstrated the potential benefits of space lidar for studies of clouds and aerosols. PICASSO-CENA builds on this experience with a payload consisting of a two-wavelength polarization-sensitive lidar, an oxygen A-band spectrometer (ABS), an imaging infrared radiometer (IIR), and a wide field camera (WFC). Data from these instruments will be used to measure the vertical distributions of aerosols and clouds in the atmosphere, as well as optical and physical properties of aerosols and clouds which influence the Earth radiation budget. PICASSO-CENA will be flown in formation with the PM satellite of the NASA Earth Observing System (EOS) to provide a comprehensive suite of coincident measurements of atmospheric state, aerosol and cloud optical properties, and radiative fluxes. The mission will address critical uncertainties iin the direct radiative forcing of aerosols and clouds as well as aerosol influences on cloud radiative properties and cloud-climate radiation feedbacks. PICASSO-CENA is planned for a three year mission, with a launch in early 2003. PICASSO-CENA is being developed within the framework of a collaboration between NASA and CNES.

Winker, David M.↗

NASA NTRS1998

Global Distribution of Dust, Smoke, Volcanic Ash, and Pollutant Aerosols Seen from Space

New technique for observing aerosols from space, using ultraviolet (UV) wavelengths, have been developed during the past three years. The chief benefit from observing aerosols in the UV is that they are easily visible over both land and water. While there is presently more than one satellite that can observe aerosols in the UV, only Total Ozone Mapping Spectrometer (TOMS) has a long-term record (since 1979) and adequate spatial resolutions (50 to 100 km) to observe the seasonal and interannual variations, and to locate some of the land sources of dust, smoke, volcanic ash and sulfate pollutants. The data has been assembled into daily images of the atmospheric aerosol loading in terms of optical depth and UV transmittance. For the major sources of aerosols, it is common for at least 50% of the total UV to be absorbed underneath aerosol plumes. This is particularly true for the spectacular smoke plumes originating from the recent Indonesian and Mexican fires, as well as under the huge African dust plumes. The sulfate pollutants are mostly present in the Northern Hemisphere and are associated with regions of high industrial activity. The location and seasonal dependence of these aerosol plumes over Europe and North America will be contrasted with the relatively clean Southern Hemisphere. Because of the success of this technique, it has formed the basis for a new generation of space-borne aerosol detection instruments. These new instruments combine the UV observations with the more traditional visible-wavelength data to obtain a more comprehensive characterization of aerosols that is possible with either UV or visible techniques by themselves.

Herman, Jay R.↗

NASA NTRS1999

Towards a Strategy of Remote Sensing of Aerosol Direct and Indirect Radiative Forcing

The role of aerosol forcing remains one of the largest uncertainties in estimating man's impact on the global climate system. One school of thought suggests that remote sensing by satellite sensors will provide the data necessary to narrow these uncertainties. Much effort has gone into the development of new satellite sensors specifically designed to retrieve aerosol loading and some information about the sizes of the aerosols. These next generation remote sensing instruments (EOS-MODIS, EOS-MISR, POLDER, ATSR) will provide unprecedented accuracy in the retrieval of aerosol loading. Although the new generation of sensors has excellent accuracy compared to the heritage instruments of the past, they still have measurement limitations. In clean, pristine regions the absolute magnitude of the uncertainty in the aerosol retrieval becomes comparable in magnitude to the signal itself. If much of the aerosol forcing is occurring at very low magnitudes of aerosol concentrations, satellite remote sensing will miss it. This study attempts to quantify remote sensing limitations due to the accuracy limits of the retrieval algorithms. We use a combination of numerical aerosol transport models, ground-based AERONET data and ISCCP cloud climatology to determine how much of the forcing occurs in regions too clean to determine from satellite retrievals. This study is not an intercomparison of global transport models. It is not an estimation of global aerosol forcing. This study is an exercise to determine whether satellite remote sensing can live up to our high expectations. The results show that while remote sensing will be able to measure a majority of the direct forcing, it will miss roughly half of the indirect forcing.

Remer, L. A.↗

NASA NTRS2000

In Situ Aerosol Size Distributions and Clear Column Radiative Closure During ACE-2

As part of the second Aerosol Characterization Experiment (ACE-2) during June and July of 1997, aerosol size distributions were measured on board the CIRPAS Pelican aircraft through the use of a DMA and two OPCS. During the campaign, the boundary layer aerosol typically possessed characteristics representative of a background marine aerosol or a continentally influenced aerosol, while the free tropospheric aerosol was characterized by the presence or absence of a Saharan dust layer. A range of radiative closure comparisons were made using the data obtained during vertical profiles flown on four missions. Of particular interest here are the comparisons made between the optical properties as determined through the use of measured aerosol size distributions and those measured directly by an airborne 14-wavelength sunphotometer and three nephelometers. Variations in the relative humidity associated with each of the direct measurements required consideration of the hygroscopic properties of the aerosol for size distribution based calculations. Simultaneous comparison with such a wide range of directly measured optical parameters not only offers evidence of the validity of the physicochemical description of the aerosol when closure is achieved, but also provides insight into potential sources of error when some or all of the comparisons result in disagreement. Agreement between the derived and directly measured optical properties varied for different measurements and for different cases. Averaged over the four case studies, the derived extinction coefficient at 525 nm exceeded that measured by the sunphotomoter by 2.5% in the clean boundary later, but underestimated measurements by 13% during pollution events. For measurements within the free troposphere, the mean derived extinction coefficient was 3.3% and 17% less than that measured by the sunphotometer during dusty and nondusty conditions, respectively. Likewise, averaged discrepancies between the derived and measured scattering coefficient were -9.6%, +4.7%, +17%, and -41% for measurements within the clean boundary layer, polluted boundary layer, free troposphere with a dust layer, and free troposphere without a dust layer, respectively. Each of these quantities, as well as the majority of the > 100 individual comparisons from which they were averaged, were within estimated uncertainties.

Collins, D. R.↗

NASA NTRS2000

Case Studies of the Vertical Structure of the Direct Shortwave Aerosol Radiative Forcing During TARFOX

The vertical structure of aerosol-induced radiative flux changes in the Earth's troposphere affects local heating rates and thereby convective processes, the formation and lifetime of clouds, and hence the distribution of chemical constituents. We present observationally-based estimates of the vertical structure of direct shortwave aerosol radiative forcing for two case studies from the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) which took place on the US East coast in July 1996. The aerosol radiative forcings are computed using the Fu-Liou broadband radiative transfer model. The aerosol optical properties used in the radiative transfer simulations are calculated from independent vertically-resolved estimates of the complex aerosol indices of refraction in two to three distinct vertical layers, using profiles of in situ particle size distributions measured aboard the University of Washington research aircraft. Aerosol single-scattering albedos at 450 nm thus determined range from 0.9 to 0.985, while the asymmetry factor varies from 0.6 to 0.8. The instantaneous shortwave aerosol radiative forcings derived from the optical profiles of the aerosols are of the order of -36 W/sq m at the top of the atmosphere and about -56 W/sq m at the surface for both case studies.

Redemann, J.↗

NASA NTRS2000

Clear-Sky Closure Studies of Tropospheric Aerosol and Water Vapor During ACE-2 Using Airborne Sunphotometer, Airborne In-Situ, Space-Borne, and Ground-Based Measurements

We report on clear-sky column closure experiments (CLEARCOLUMN) performed in the Canary Islands during the second Aerosol Characterization Experiment (ACE-2) in June/July 1997. We present CLEARCOLUMN results obtained by combining airborne sunphotometer and in-situ (a differential mobility analyzer, three optical particle counters, three nephelometers, and one absorption photometer) measurements taken aboard the Pelican aircraft, space-borne NOAA/AVHRR data and ground-based lidars. A wide range of aerosol types was encountered throughout the ACE-2 area, including background Atlantic marine, European pollution-derived, and (although less frequently than expected) African mineral dust. During the two days discussed here, vertical profiles flown in cloud free air masses revealed three distinctly different layers: a marine boundary layer (MBL) with varying pollution levels, an elevated dust layer, and a very clean layer between the MBL and the dust layer. Based on size-resolved composition information we have established an aerosol model that allows us to compute optical properties of the ambient aerosol using the optical particle counter results. In the dust, the agreement in layer AOD (lambda=380-1060 nm) is 3-8%. In the MBL there is a tendency for the in-situ results to be slightly lower than the sunphotometer measurements (10-17% at lambda=525 nm), but these differences are within the combined error bars of the measurements and computations. Aerosol size-distribudon closure based on in-situ size distributions and inverted sunphotometer extinction spectra has been achieved in the MBL (total surface area and volume agree within 0.2, and 7%, respectively) but not in the dust layer. The fact that the three nephelometers operated at three different relative humidities (RH) allowed to parameterize hygroscopic growth and to therefore estimate optical properties at ambient RH. The parameters derived for different aerosol types are themselves useful for the aerosol modeling community. The fact that the nephelometers and the absorption photometer sampled the aerosol through a cyclone make those measurements less useful for thee closure study carried out here. Large corrections (especially in the dust) had to be applied. Therefore, it is not surprising that closure with the sunphotometer was not always achieved. Agreement within 0.02 in AOD was achieved in the dust layer when the airorne sunphotometer extinction or AOD was compared to ground-based lidar measurements. We found that the presence of the elevated dust layers removes the good agreement between satellite and sunphotometer AOD usually found in the absence of the dust layer. We still compare the scattering phase functions used in the satellite retrieval with those obtained from the aerosol or the sunphotometer measurements.

Schmid, Beat↗