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At least 73 records · Page 4

TA-54 Flanged Tritium Waste Container Operations, Radioactive Air Emissions Summary Volume 1: Stack Emissions & Off-Site Dose Consequence

In September 2025, pressure mitigation operations began on the four Flanged Tritium Waste Containers (FTWCs) that had been in storage at Los Alamos National Laboratory (LANL), Technical Area (TA-) 54, Area G, Building 1028. Each FTWC was opened at TA-54 and put into a stable configuration, then containers were moved to LANL’s Weapons Engineering Tritium Facility (WETF) for further processing in preparation for shipment off-site. Over the course of 13 operational days, the project had air emissions of 123 curies of tritium (hydrogen-3). The radiological dose to the hypothetical maximally exposed individual (MEI) member of the public from these emissions was 0.012 millirem. This is well within the limits established by the Environmental Protection Agency (EPA), which allows 10 millirem per year to any member of the public. Naturally occurring background radiation in Northern New Mexico averages about 300-400 millirem per year to residents. This report is intended to briefly summarize operations that took place in September and October 2025, provide documentation of the radionuclide air emissions from these operations, and summarize the off-site dose consequence to the public that resulted from these air emissions. Informal notifications addressing these areas were made via email to the EPA and NMED throughout the project, and summaries of these data were also posted on the LANL external web site 1 for FTWC operations.

54 ENVIRONMENTAL SCIENCES↗

The ground state properties of spin-aligned atomic hydrogen, deuterium, and tritium

The internal energy, pressure, and compressibility of ground-state, spin-aligned atomic hydrogen, deuterium, and tritium are calculated assuming that all pair interactions occur via the atomic triplet (spin-aligned) potential. The conditions required to obtain atomic hydrogen and its isotopes in bulk are discussed; such a development would be of value in propulsion systems because of the light mass and energetic recombination of atomic hydrogen. Results show that atomic triplet hydrogen and deuterium remain gaseous at 0 K, and that tritium forms a liquid with a binding energy of approximately -0.75 K per atom at a molar volume of 130 cu cm per mole. The pair distribution function for these systems is calculated, and the predicted superfluid behavior of atomic triplet hydrogen and tritium is briefly discussed.

Etters, R. D.↗

Constraining the North Atlantic circulation with tritium data

The North Atlantic circulation derived from an inverse calculation by singular-value decomposition is tested against the historical record of tritium. A forward calculation of the tritium transient is performed using the circulation model, published estimates of atmospheric injection rates, and plausible estimates of the tracer history at the open boundaries of the model. The results do not agree with observations of the interior distributions of tritium. Consideration is given to the possibility of improving the agreement by modifying the atmospheric injection rates and the initial estimates of open boundary time histories, treating the boundary conditions as control variables.

Memery, Laurent↗

Environmental Testing of Tritium-Phosphor Glass Vials for Use in Long-Life Radioisotope Power Conversion Units

Power generation in extreme environments, such as the outer solar system, the night side of planets, or other low-illumination environments, currently presents a technology gap that challenges NASA's ambitious scientific goals. We are developing a radioisotope power cell (RPC) that utilizes commercially available tritium light sources and standard 1.85 eV InGaP2 photovoltaic cells to convert beta particle energy to electric energy. In the test program described here, we perform environmental tests on commercially available borosilicate glass vials internally coated with a ZnS luminescent phosphor that are designed to contain gaseous tritium in our proposed power source. Such testing is necessary to ensure that the glass containing the radioactive tritium is capable of withstanding the extreme environments of launch and space for extended periods of time.

Zemcov, Michael↗

Design and Commissioning of a Deuterium-Tritium Gas Delivery System for Muon Catalyzed Fusion in a Diamond Anvil Cell

We report the design, commissioning, and operation of deuterium-deuterium (DD) and deuterium-tritium (DT) gas delivery systems developed to load a diamond anvil cell (DAC) beam target for muon-catalyzed fusion (muCF). The DAC approach enables DT fuel to be compressed to GPa pressures at more than twice the liquid density and heated from cryogenic temperatures through 500 K, opening access to a substantially expanded parameter range for muCF kinetics and yield measurements. In this approach, DT is cryo-condensed to a liquid in a minichamber and then compressed in the DAC using a helium-driven pneumatic membrane, achieving high pressures in a millimeter-scale DT sample volume. A DD gas delivery system was designed and used to validate the experimental apparatus, measure the gas quantities needed for filling, develop operational experience, and collect kinetics and yield data with DD targets. The DT gas delivery system adds tritium-specific capabilities for inventory minimization, secondary containment, and activity monitoring. The DT system integrates depleted uranium storage beds and a liquid helium cryogenic condenser used for pressure building and cryopumping. High-purity delivery is provided by a rapid-response palladium permeator. The system is housed in a helium-atmosphere glovebox held at negative pressure with continuous cleanup. We present the process and instrumentation design, a failure modes and effects analysis (FMEA), and data from the experiment's in situ Raman spectrometer, which provides direct confirmation of target loading and composition through the optically clear diamond anvils. The 2024 and 2025 DT campaigns achieved repeatable target fills and operation with no measurable tritium releases to the stack, demonstrating safe, high-purity DT loading at novel density-temperature conditions for muCF studies.

Koukina, Elena [Acceleron Fusion]↗

Stellarators with enhanced tritium confinement and edge radiation control

A stellarator design is described with the purpose of achieving three goals: (1) enhance the confinement time of tritium. (2) Have a sufficient density of high-Z impurities to radiate the thermal power escaping from the core while having an extremely low impurity density in the core. (3) Maintain a large fraction of the plasma in a burning plasma state with an optimal tritium fraction. Some features of this design could be used in tokamaks. Although having three confinement zones is natural for stellarators, it is not for tokamaks.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A potential emerging issue concerning repair welding of out-of-core PWR components involving tritium exposure and 3 He retention

This paper identifies a potential but previously unrecognized risk of helium-induced embrittlement and cracking during repair welding of out-of-core pressurized water reactor (PWR) components exposed to tritium-contaminated coolant. While previous weldability concerns centered on 4 He accumulation in neutron-irradiated alloys located within the in-core or near-core regions, new measurements show that 3 He generated by tritium decay can accumulate in out-of-core components. Because hydrogen isotopes readily diffuse to grain boundaries and become trapped there, significant 3 He generation at grain boundaries may lead to cracking during weld repairs. Initial data from far-below-core PWR flux thimble tubes confirm the presence of 3 He levels above known cracking thresholds for repair welds. In conclusion, these findings indicate that out-of-core regions should be considered when defining safe weld repair windows in reactors operating for 60–100 years.

Extended PWR lifetimes↗

Diagnosing up-scattered deuterium–tritium fusion neutrons produced in burning plasmas at the National Ignition Facility (invited)

In the push to higher performance fusion plasmas, two critical quantities to diagnose are α-heat deposition that can improve and impurities mixed into the plasma that can limit performance. In high-density, highly collisional inertial confinement fusion burning plasmas, there is a significant probability that deuterium–tritium (DT) fusion products, 14.1 MeV neutrons and 3.5 MeV α-particles, will collide with and deposit energy onto (“up-scatter”) surrounding deuterium and tritium fuel ions. These up-scattered D and T ions can then undergo fusion while in-flight and produce an up-scattered neutron (15–30 MeV). These reaction-in-flight (RIF) neutrons can then be uniquely identified in the measured neutron energy spectrum. Further, the magnitude, shape, and relative size of this spectral feature can inform models of stopping-power in the DT plasma and hence is directly proportional to α-heat deposition. In addition, the RIF spectrum can be related to mix into the burning fuel, particularly relevant for high-Z shell and other emerging National Ignition Facility platforms. The neutron time-of-flight diagnostic upgrades needed to obtain this small signal, ~10 –5 times the primary DT neutron peak, will be discussed. Results from several gain > 1 implosions will be shown and compared to previous RIF spectra. Finally, comparisons of experimental data to a simplified computational model will be made.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Feasibility of main thermal ion heating by ICRF waves using a top launcher in a tokamak with deuterium–tritium plasmas

A scenario of ion cyclotron range of frequency (ICRF) wave injection from a top launcher is proposed as an efficient and direct heating method for thermal deuterium ions in deuterium–tritium tokamak plasmas. Positioned between the tritium cyclotron layer and ion–ion hybrid layer, the top launcher allows effective wave penetration to the ion–ion hybrid layer and enables significant power transfer to thermal deuterium. This is achieved through favorable wave polarization for fundamental cyclotron damping. There is a Doppler broadening around the cyclotron resonance and this overlaps with the ion–ion hybrid layer. Low toroidal mode numbers and ion temperature in the range of 5–20 keV are favorable for enhancing the main ion damping relative to electron damping. In contrast to the neutral beam injection, which penetration strongly depends on machine size and plasma density, the proposed ICRF-based direct ion heating scenario is shown to be scalable and applicable to both larger and smaller tokamak devices within practical constraints.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Renewable low-Z wall for fusion reactors with built-in tritium recovery (Final Technical Report)

This project pursued development of a novel renewable plasma-facing wall technology for fusion reactors. The technology is based on a slurry which can be easily delivered by delivery tubes to the reactor wall. The slurry dries at the hot reactor wall into pebble rods which are extruded out into the hot plasma, where the pebbles break off and fall along the reactor wall and can be recovered by gravity and re-used. The falling pebbles carry away heat and tritium and also protect the wall against large scale erosion or redeposition of material. The research focused on carbon-based pebble rods and demonstrated that pebble rods could be produced from slurry with tolerable levels of outgassing on a reactor-relevant timescale (< 5 minutes). Steady-state handling of reactor relevant (up to 50 MW/m 2 ) normal-incidence heat loads was demonstrated. Pebble release velocities were found to be sufficiently small (< 1 m/s) to allow recovery below the vacuum chamber. Tunability of the pebble rod breaking rate was demonstrated by changing the fill fraction of the interpebble matrix which binds the pebbles together. This work could benefit the public by helping move forward the design of commercially viable fusion energy reactors. Designing a first wall for magnetic fusion reactors which can handle the huge heat loads present and also avoid buildup of tritium-containing deposits is extremely challenging and requires novel approaches like the one being investigated here.

36 MATERIALS SCIENCE↗

Project 8 apparatus for cyclotron radiation emission spectroscopy with 83m Kr and tritium

Cyclotron Radiation Emission Spectroscopy (CRES) is a novel technique for the precise measurement of relativistic electron energy. This technique is being employed by the Project 8 collaboration for measuring a high-precision tritium beta decay spectrum to perform a frequency-based measurement of the neutrino mass. In this work, we describe the Project 8 Phase II apparatus, used for the detection of the CRES signal from the conversion electrons of 83m Kr and the first CRES measurement of the beta-decay spectrum of molecular tritium.

Neutrino detectors↗

EMC Effect of Tritium and Helium-3 from the JLab MARATHON Experiment

Measurements of the EMC effect in the tritium and helium-3 mirror nuclei are reported. The data were obtained by the MARATHON Jefferson Lab experiment, which performed deep inelastic electron scattering from deuterium and the three-body nuclei, using a cryogenic gas target system and the high resolution spectrometers of the Hall A Facility of the Lab. The data cover the Bjorken 𝑥 range from 0.20 to 0.83, corresponding to a squared four-momentum transfer 𝑄 2 range from 2.7 to 11.9 (GeV/𝑐) 2 , and to an invariant mass 𝑊 of the final hadronic state greater than 1.84 GeV/𝑐 2 . The tritium EMC effect measurement is the first of its kind. The MARATHON experimental results are compared to results from previous measurements by DESY-HERMES and JLab–Hall C experiments, as well as with few-body theoretical predictions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Tritium β decay and proton-proton fusion in pionless effective field theory

The Gamow-Teller and Fermi matrix elements, 〈 GT 〉 and 〈 F 〉 , respectively, for tritium β decay are calculated to next-to-leading order (NLO) in pionless effective field theory in the absence of Coulomb interactions and isospin violation giving the leading order predictions 〈 GT 〉 0 = 0.9807 and 〈 F 〉 0 = 1 . Using an experimentally determined value for the tritium β decay GT matrix element, the two-body axial current low energy constant is fixed at NLO yielding L 1 , A = 6.01 ± 2.08 fm 3 at the renormalization scale of the physical pion mass, which agrees with predictions based on naive dimensional analysis. The impact of L 1 , A on proton-proton fusion is also discussed. Finally, the consequences of Wigner-SU(4) spin-isospin symmetry are considered for the Gamow-Teller matrix element. Published by the American Physical Society 2024

Physics↗

Forward Modeling of Gamma Reaction History Signatures From Anticipated Deuterium-Tritium Filled MagLIF Implosions on Sandia’s Z-Machine

Nuclear reaction history measurements provide a bang time and burn width of Inertial Confinement Fusion (ICF) implosions and are essential for understanding implosion performance to constrain ICF capsule design. When fusion fuel contains Deuterium (D) and Tritium (T) gas, reaction history is informed by measuring the 16.75 MeV gamma rays generated from the D(T,γ) 5 He reaction. Such DT based reaction history measurements have not been made on the Magnetized Laser Inertial Fusion (MagLIF) platform on Sandia’s Z-Machine due to the lack of Tritium being used. The recent development of ICF implosions with tritiated fuel will open the possibility of measuring the gamma reaction history on the Z-Machine. A forward model of the Gamma Reaction History diagnostic on Z (GRH-Z) has been developed using the MCNP6.3 (Monte-Carlo N-Particle) radiation transport code. The model included the Z-Machine geometry of interest to characterize the impact of neutron induced gamma rays on the DT reaction history measurements. In addition, the impulse response functions of the GRH-Z diagnostic to understand the temporal response of the detector, and the minimum yields required to make a reaction history measurement were calculated. This approach also predicted that with T 2 gas doping of MagLIF implosions a reaction history may be made for high performance shots >8e12-2.4e13 depending on the chosen threshold for the detector, with a maximum signal to background ratio of 25%. It was found that for long duration ICF implosions that additional collimation will be needed to prevent the neutron induced gamma rays from modifying the shape of the measured DT reaction history curve.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Custom ORIGEN Libraries for Tritium Production in Discrete Burnable Absorbers

The ORIGEN module in SCALE is a common method of performing quick depletion and irradiation calculations of various materials in light-water reactors. However, these analyses depend on the neutron spectra in the ARP libraries being accurate for the situation presented. When using insertable burnable absorbers in a LWR with Li-6 in order to produce tritium, the neutron spectrum is highly different than those in the default libraries in ORIGEN, which leads to significant mispredictions in tritium production. Therefore, custom libraries are required, and when comparing to lattice physics codes (CASMO5 and WIMS10) with ORIGEN, using custom libraries is much more accurate than using the default libraries.

Ivanusa, Pavlo↗

A kinetic study of fusion burn waves in compressed deuterium–tritium and proton–boron plasmas

We present particle-in-cell simulations with Monte Carlo collisions of fusion burn waves in compressed deuterium–tritium and proton–boron plasmas. We study the energy balance in the one-dimensional expansion of a hot-spot by simulating Coulomb collisions, fusion reactions, and bremsstrahlung emission with a Monte Carlo model and inverse bremsstrahlung absorption using a new PIC model. This allows us to self-consistently capture the alpha particle heating and radiative losses in the expanding hot-spot and surrounding cold fuel. After verifying our model in a code-to-code comparison with both kinetic and fluid codes for the case of a deuterium–tritium hot-spot, we simulate the expansion of a proton–boron hot-spot initialized at 200 keV and 1,000 g/cm 3 . Our model predicts that energy radiated by the hot-spot is recaptured by the surrounding high-density opaque fuel reducing the expansion work done by the propagating burn wave. As a result, we find the net fusion energy produced over the course of $20$~ps is twice the initial hot-spot energy independent of whether radiation physics is included.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗